Jakob M. Grzesik | Searcharxiv

arXiv2026

A general framework for interactions between electron beams and quantum optical systems

We provide a theoretical framework to describe the dynamics of a free-electron beam interacting with quantized bound systems in arbitrary electromagnetic environments. This expands the quantum optics toolbox to incorporate free-electron beams for applications in highly tunable quantum control, imaging, and spectroscopy at the nanoscale. The framework recovers previously studied results and shows that electromagnetic environments can amplify the intrinsically weak coupling between a free-electron and a bound electron to reach previously inaccessible interaction regimes. We leverage this enhanced coupling for experimentally feasible protocols in coherent qubit control and towards the nondestructive readout and projective control of the electron beam's quantum-number statistics. Our framework is broadly applicable to microwave-frequency qubits, optical nanophotonics, cavity quantum electrodynamics, and emerging platforms at the interface of electron microscopy and quantum information.

quant-ph↗

arXiv2025

Quantum sensing of electron beams using solid-state spins

Scattering experiments with energetic particles, such as free electrons, have been historically used to reveal the quantum structure of matter. However, realizing coherent interactions between free-electron beams and solid-state quantum systems has remained out of reach, owing to their intrinsically weak coupling. Realizing such coherent control would open up opportunities for hybrid quantum platforms combining free electrons and solid-state qubits for coincident quantum information processing and nanoscale sensing. Here, we present a framework that employs negatively charged nitrogen-vacancy centers (NV-) in diamond as quantum sensors of a bunched electron beam. We develop a Lindblad master equation description of the magnetic free-electron--qubit interactions and identify spin relaxometry as a sensitive probe of the interaction. Experimentally, we integrate a confocal fluorescence microscopy setup into a microwave-bunched electron beam line. We monitor charge-state dynamics and assess their impact on key sensing performance metrics (such as spin readout contrast), defining safe operating parameters for quantum sensing experiments. By performing $T_1$ relaxometry under controlled electron beam exposure, we establish an upper bound on the free-electron--spin coupling strength. Our results establish NV- centers as quantitative probes of free electrons, providing a metrological benchmark for free-electron--qubit coupling under realistic conditions, and chart a route toward solid-state quantum control with electron beams.

quant-ph↗