arXiv subjects

James L. Webb

Publications and source records attributed to James L. Webb.

8 recordsLinked to original sources

arXiv2026

Simulation of Axion-Induced Electromagnetic Signal Detection Using Plasmonic Metasurfaces and Diamond NV Centers

The axion represents a strong candidate for weakly interacting dark matter. To date, high sensitivity lab based experiments and astrophysical observations have ruled out a substantial part of the axion mass and photon coupling parameter space. However, a challenge remains in searching for the presence of the axion in the higher mass range 0.01-1eV corresponding approximately to axion field oscillation at THz frequencies. This work investigates via numerical simulation the feasibility of a high sensitivity, lab-based axion sensor operating in this range, based on plasmonic electric field enhancement by a nanostructured metasurface, combined with heterodyne detection and quantum sensing via nitrogen-vacancy (NV) centers in diamond. Estimates of the sensor response to anomalous electromagnetic fields resulting from axion coupling are given using Ti/Au nanopillars on LiNb at axion mass corresponding to telecommunications wavelength ($\approx$0.8eV, 196 THz). Finally, the possibility of sensing in the lower axion mass $<$10$^{-2}$ to 10$^{-1}$eV range is explored using alternative materials, with CdTe as an example.

hep-ph↗

arXiv2026

Millisecond-Scale Calibration and Benchmarking of Superconducting Qubits

Superconducting qubit parameters drift on sub-second timescales, motivating calibration and benchmarking techniques that can be executed on millisecond timescales. We demonstrate an on-FPGA workflow that co-locates pulse generation, data acquisition, analysis, and feed-forward, eliminating CPU round trips. Within this workflow, we introduce sparse-sampling and on-FPGA inference tools, including computationally efficient methods for estimation of exponential and sine-like response functions, as well as on-FPGA implementations of Nelder-Mead optimization and golden-section search. These methods enable low-latency primitives for readout calibration, spectroscopy, pulse-amplitude calibration, coherence estimation, and benchmarking. We deploy this toolset to estimate $T_1$ in 10 ms, optimize readout parameters in 100 ms, optimize pulse amplitudes in 1 ms, and perform Clifford randomized gate benchmarking in 107 ms on a flux-tunable superconducting transmon qubit. Running a closed-loop on-FPGA recalibration protocol continuously for 6 hours enables more than 74,000 consecutive recalibrations and yields gate errors that consistently retain better performance than the baseline initial calibration. Correlation analysis shows that recalibration suppresses coupling of gate error to control-parameter drift while preserving a coherence-linked performance. Finally, we quantify uncertainty versus time-to-decision under our sparse sampling approaches and identify optimal parameter regimes for efficient estimation of qubit and pulse parameters.

quant-ph↗

arXiv2021

Investigation and comparison of measurement schemes in the low frequency biosensing regime using solid-state defect centers

Ensembles of solid state defects in diamond make promising quantum sensors with high sensitivity and spatiotemporal resolution. The inhomogeneous broadening and drive amplitude variations across such ensembles have differing impacts on the sensitivity depending on the sensing scheme used, adding to the challenge of choosing the optimal sensing scheme for a particular sensing regime. In this work, we numerically investigate and compare the predicted sensitivity of schemes based on continuous-wave (CW) optically detected magnetic resonance (ODMR) spectroscopy, pi-pulse ODMR and Ramsey interferometry for sensing using nitrogen-vacancy centers in the low-frequency (<10 kHz) range typical for signals from biological sources. We show that inhomogeneous broadening has the strongest impact on the sensitivity of Ramsey interferometry, and drive amplitude variations least impact the sensitivity of CW ODMR, with all methods constrained by the Rabi frequency. Based on our results, we can identify three different regions of interest. For inhomogeneous broadening less than 0.3 MHz, typical of diamonds used in state of the art sensing experiments, Ramsey interferometry yields the highest sensitivity. In the regime where inhomogeneous broadening is greater than 0.3 MHz, such as for standard optical grade diamonds or in miniaturized integrated devices, drive amplitude variations determine the optimal protocol to use. For low to medium drive amplitude variations, the highest sensitivity is reached using pi-pulse ODMR. For high drive amplitude variations, relevant for widefield microscopic imaging, CW ODMR can yield the best sensing performance.

quant-ph↗

arXiv2021

Interplay of crystal thickness and in-plane anisotropy and evolution of quasi-one dimensional electronic character in ReSe$_{2}$

We study the valence band structure of ReSe$_{2}$ crystals with varying thickness down to a single layer using nanoscale angle-resolved photoemission spectroscopy and density functional theory. The width of the top valence band in the direction perpendicular to the rhenium chains decreases with decreasing number of layers, from 280 meV for the bulk to 61 meV for monolayer. This demonstrates increase of in-plane anisotropy induced by changes in the interlayer coupling and suggests progressively more one-dimensional character of electronic states in few-layer rhenium dichalcogenides.

cond-mat.mtrl-sci↗

arXiv2021

High speed microcircuit and synthetic biosignal widefield imaging using nitrogen vacancies in diamond

The ability to measure the passage of electrical current with high spatial and temporal resolution is vital for applications ranging from inspection of microscopic electronic circuits to biosensing. Being able to image such signals passively and remotely at the same time is of high importance, to measure without invasive disruption of the system under study or the signal itself. A new approach to achieve this utilises point defects in solid state materials, in particular nitrogen vacancy (NV) centres in diamond. Acting as a high density array of independent sensors, addressable opto-electronically and highly sensitive to factors including temperature and magnetic field, these are ideally suited to microscopic widefield imaging. In this work we demonstrate such imaging of signals from a microscopic lithographically patterned circuit at the micrometer scale. Using a new type of lock-in amplifier camera, we demonstrate sub-millisecond (up to 3500 frames-per-second) spatially resolved recovery of AC and pulsed electrical current signals, without aliasing or undersampling. Finally, we demonstrate as a proof of principle the recovery of synthetic signals replicating the exact form of signals in a biological neural network: the hippocampus of a mouse.

quant-ph↗

arXiv2021

Optimal control of a nitrogen-vacancy spin ensemble in diamond for sensing in the pulsed domain

Defects in solid state materials provide an ideal, robust platform for quantum sensing. To deliver maximum sensitivity, a large ensemble of non-interacting defects hosting coherent quantum states are required. Control of such an ensemble is challenging due to the spatial variation in both the defect energy levels and in any control field across a macroscopic sample. In this work we experimentally demonstrate that we can overcome these challenges using Floquet theory and optimal control optimization methods to efficiently and coherently control a large defect ensemble, suitable for sensing. We apply our methods experimentally to a spin ensemble of up to 4 $\times$ 10$^9$ nitrogen vacancy (NV) centers in diamond. By considering the physics of the system and explicitly including the hyperfine interaction in the optimization, we design shaped microwave control pulses that can outperform conventional ($π$-) pulses when applied to sensing of temperature or magnetic field, with a potential sensitivity improvement between 11 and 78\%. Through dynamical modelling of the behaviour of the ensemble, we shed light on the physical behaviour of the ensemble system and propose new routes for further improvement.

quant-ph↗

arXiv2021

Laser threshold magnetometry using green light absorption by diamond nitrogen vacancies in an external cavity laser

Nitrogen vacancy (NV) centers in diamond have attracted considerable recent interest for use in quantum sensing, promising increased sensitivity for applications ranging from geophysics to biomedicine. Conventional sensing schemes involve monitoring the change in red fluorescence from the NV center under green laser and microwave illumination. Due to the strong fluorescence background from emission in the NV triplet state and low relative contrast of any change in output, sensitivity is severely restricted by a high optical shot noise level. Here, we propose a means to avoid this issue, by using the change in green pump absorption through the diamond as part of a semiconductor external cavity laser run close to lasing threshold. We show theoretical sensitivity to magnetic field on the pT/sqrt(Hz) level is possible using a diamond with an optimal density of NV centers. We discuss the physical requirements and limitations of the method, particularly the role of amplified spontaneous emission near threshold and explore realistic implementations using current technology.

quant-ph↗

arXiv2017

Electronic bandstructure of ReS2 by high resolution angle resolved photoemission spectroscopy

The rhenium-based transition metal dichalcogenides (TMDs) are atypical of the TMD family due to their highly anisotropic crystalline structure and are recognized as promising materials for two dimensional heterostructure devices. The nature of the band gap (direct or indirect) for bulk, few and single layer forms of ReS$_2$ is of particular interest, due to its comparatively weak inter-planar interaction. However, the degree of inter-layer interaction and the question of whether a transition from indirect to direct gap is observed on reducing thickness (as in other TMDs) are controversial. We present a direct determination of the valence band structure of bulk ReS$_2$ using high resolution angle resolved photoemission spectroscopy (ARPES). We find a clear in-plane anisotropy due to the presence of chains of Re atoms, with a strongly directional effective mass which is larger in the direction orthogonal to the Re chains (2.2 $m_e$) than along them (1.6 $m_e$), in good agreement with density functional theory calculations. An appreciable inter-plane interaction results in an experimentally-measured difference of ~100-200 meV between the valence band maxima at the Z point (0,0,1/2) and the $Γ$ point (0,0,0) of the three-dimensional Brillouin zone. This leads to a direct gap at Z and a close-lying but larger gap at $Γ$, implying that bulk ReS2 is marginally indirect. This may account for recent conflicting transport and photoluminescence measurements and the resulting uncertainty about the direct or indirect gap nature of this material.

cond-mat.mtrl-sci↗