arXiv subjects

James Le Houx

Publications and source records attributed to James Le Houx.

3 recordsLinked to original sources

arXiv2026

Benchmarking Autonomy in Scientific Experiments: A Hierarchical Taxonomy for Autonomous Large-Scale Facilities

The transition from automated data collection to fully autonomous discovery requires a shared vocabulary to benchmark progress. While the automotive industry relies on the SAE J3016 standard, current taxonomies for autonomous science presuppose an owner-operator model that is incompatible with the operational rigidities of Large-Scale User Facilities. Here, we propose the Benchmarking Autonomy in Scientific Experiments (BASE) Scale, a 6-level taxonomy (Levels 0-5) specifically adapted for these unique constraints. Unlike owner-operator models, User Facilities require zero-shot deployment where agents must operate immediately without extensive training periods. We define the specific technical requirements for each tier, identifying the Inference Barrier (Level 3) as the critical latency threshold where decisions shift from scalar feedback to semantic digital twins. Fundamentally, this level extends the decision manifold from spatial exploration to temporal gating, enabling the agent to synchronise acquisition with the onset of transient physical events. By establishing these operational definitions, the BASE Scale provides facility directors, funding bodies, and beamline scientists with a standardised metric to assess risk, define liability, and quantify the intelligence of experimental workflows.

physics.ins-det↗

arXiv2025

Autonomous battery research: Principles of heuristic operando experimentation

Unravelling the complex processes governing battery degradation is critical to the energy transition, yet the efficacy of operando characterisation is severely constrained by a lack of Reliability, Representativeness, and Reproducibility (the 3Rs). Current methods rely on bespoke hardware and passive, pre-programmed methodologies that are ill-equipped to capture stochastic failure events. Here, using the Rutherford Appleton Laboratory's multi-modal toolkit as a case study, we expose the systemic inability of conventional experiments to capture transient phenomena like dendrite initiation. To address this, we propose Heuristic Operando experiments: a framework where an AI pilot leverages physics-based digital twins to actively steer the beamline to predict and deterministically capture these rare events. Distinct from uncertainty-driven active learning, this proactive search anticipates failure precursors, redefining experimental efficiency via an entropy-based metric that prioritises scientific insight per photon, neutron, or muon. By focusing measurements only on mechanistically decisive moments, this framework simultaneously mitigates beam damage and drastically reduces data redundancy. When integrated with FAIR data principles, this approach serves as a blueprint for the trusted autonomous battery laboratories of the future.

physics.ins-det↗

arXiv2024

Three-Dimensional, Multimodal Synchrotron Data for Machine Learning Applications

Machine learning techniques are being increasingly applied in medical and physical sciences across a variety of imaging modalities; however, an important issue when developing these tools is the availability of good quality training data. Here we present a unique, multimodal synchrotron dataset of a bespoke zinc-doped Zeolite 13X sample that can be used to develop advanced deep learning and data fusion pipelines. Multi-resolution micro X-ray computed tomography was performed on a zinc-doped Zeolite 13X fragment to characterise its pores and features, before spatially resolved X-ray diffraction computed tomography was carried out to characterise the homogeneous distribution of sodium and zinc phases. Zinc absorption was controlled to create a simple, spatially isolated, two-phase material. Both raw and processed data is available as a series of Zenodo entries. Altogether we present a spatially resolved, three-dimensional, multimodal, multi-resolution dataset that can be used for the development of machine learning techniques. Such techniques include development of super-resolution, multimodal data fusion, and 3D reconstruction algorithm development.

cs.LG↗