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James P. Sethna

Publications and source records attributed to James P. Sethna.

At least 37 records · Page 2Linked to original sources

Information geometry for multiparameter models: New perspectives on the origin of simplicity

Complex models in physics, biology, economics, and engineering are often sloppy, meaning that the model parameters are not well determined by the model predictions for collective behavior. Many parameter combinations can vary over decades without significant changes in the predictions. This review uses information geometry to explore sloppiness and its deep relation to emergent theories. We introduce the model manifold of predictions, whose coordinates are the model parameters. Its hyperribbon structure explains why only a few parameter combinations matter for the behavior. We review recent rigorous results that connect the hierarchy of hyperribbon widths to approximation theory, and to the smoothness of model predictions under changes of the control variables. We discuss recent geodesic methods to find simpler models on nearby boundaries of the model manifold -- emergent theories with fewer parameters that explain the behavior equally well. We discuss a Bayesian prior which optimizes the mutual information between model parameters and experimental data, naturally favoring points on the emergent boundary theories and thus simpler models. We introduce a `projected maximum likelihood' prior that efficiently approximates this optimal prior, and contrast both to the poor behavior of the traditional Jeffreys prior. We discuss the way the renormalization group coarse-graining in statistical mechanics introduces a flow of the model manifold, and connect stiff and sloppy directions along the model manifold with relevant and irrelevant eigendirections of the renormalization group. Finally, we discuss recently developed `intensive' embedding methods, allowing one to visualize the predictions of arbitrary probabilistic models as low-dimensional projections of an isometric embedding, and illustrate our method by generating the model manifold of the Ising model.

cond-mat.stat-mech↗

Dissipation by surface states in superconducting RF cavities

Recent experiments on superconducting cavities have found that under large radio-frequency (RF) electromagnetic fields the quality factor can improve with increasing field amplitude, a so-called "anti-Q slope." Linear theories of dissipation break down under these extreme conditions and are unable to explain this behavior. We numerically solve the Bogoliubov-de Gennes equations at the surface of a superconductor in a parallel AC magnetic field, finding that at large fields there are quasiparticle surface states with energies below the bulk value of the superconducting gap. As the field oscillates, such states emerge and disappear with every cycle. We consider the dissipation resulting from inelastic quasiparticle-phonon scattering into these states and investigate the ability of this mechanism to explain features of the experimental observations, including the field dependence of the quality factor. We find that this mechanism is likely not the dominant source of dissipation and does not produce an anti-Q slope by itself; however, we demonstrate in a modified two-fluid model how these bound states can play a role in producing an anti-Q slope.

cond-mat.supr-con↗

Avalanches and deformation in glasses and disordered systems

In this chapter, we discuss avalanches in glasses and disordered systems, and the macroscopic dynamical behavior that they mediate. We briefly review three classes of systems where avalanches are observed: depinning transition of disordered interfaces, yielding of amorphous materials, and the jamming transition. Without extensive formalism, we discuss results gleaned from theoretical approaches -- mean-field theory, scaling and exponent relations, the renormalization group, and a few results from replica theory. We focus both on the remarkably sophisticated physics of avalanches and on relatively new approaches to the macroscopic flow behavior exhibited past the depinning/yielding transition.

cond-mat.dis-nn↗

Power laws in physics

Getting the most from power-law-type data can be challenging. James Sethna points out some of the pitfalls in studying power laws arising from emergent scale invariance, as well as important opportunities.

physics.data-an↗

Average Evolution and Size-Topology Relations for Coarsening 2d Dry Foams

Two-dimensional dry foams coarsen according to the von Neumann law as $dA/dt \propto (n-6)$ where $n$ is the number of sides of a bubble with area $A$. Such foams reach a self-similar scaling state where area and side-number distributions are stationary. Combining self-similarity with the von Neumann law, we derive time derivatives of moments of the bubble area distribution and a relation connecting area moments with averages of the side-number distribution that are weighted by powers of bubble area. To test these predictions, we collect and analyze high precision image data for a large number of bubbles squashed between parallel acrylic plates and allowed to coarsen into the self-similar scaling state. We find good agreement for moments ranging from two to twenty.

cond-mat.soft↗

Universal scaling for disordered viscoelastic matter II: Collapses, global behavior and spatio-temporal properties

Disordered viscoelastic materials are ubiquitous and exhibit fascinating invariant scaling properties. In a companion article, we have presented comprehensive new results for the critical behavior of the dynamic susceptibility of disordered elastic systems near the onset of rigidity. Here we provide additional details of the derivation of the singular scaling forms of the longitudinal response near both jamming and rigidity percolation. We then discuss global aspects associated with these forms, and make scaling collapse plots for both undamped and overdamped dynamics in both the rigid and floppy phases. We also derive critical exponents, invariant scaling combinations and analytical formulas for universal scaling functions of several quantities such as transverse and density responses, elastic moduli, viscosities, and correlation functions. Finally, we discuss tentative experimental protocols to measure these behaviors in colloidal suspensions.

cond-mat.soft↗

Smooth and global Ising universal scaling functions

We describe a method for approximating the universal scaling functions for the Ising model in a field. By making use of parametric coordinates, the free energy scaling function has a polynomial series everywhere. Its form is taken to be a sum of the simplest functions that contain the singularities which must be present: the Langer essential singularity and the Yang--Lee edge singularity. Requiring that the function match series expansions in the low- and high-temperature zero-field limits fixes the parametric coordinate transformation. For the two-dimensional Ising model, we show that this procedure converges exponentially with the order to which the series are matched, up to seven digits of accuracy. To facilitate use, we provide Python and Mathematica implementations of the code at both lowest order (three digit) and high accuracy.

cond-mat.stat-mech↗

Reconstruction of Current Densities from Magnetic Images by Bayesian Inference

Electronic transport is at the heart of many phenomena in condensed matter physics and material science. Magnetic imaging is a non-invasive tool for detecting electric current in materials and devices. A two-dimensional current density can be reconstructed from an image of a single component of the magnetic field produced by the current. In this work, we approach the reconstruction problem in the framework of Bayesian inference, i.e. we solve for the most likely current density given an image obtained by a magnetic probe. To enforce a sensible current density priors are used to associate a cost with unphysical features such as pixel-to-pixel oscillations or current outside the device boundary. Beyond previous work, our approach does not require analytically tractable priors and therefore creates flexibility to use priors that have not been explored in the context of current reconstruction. Here, we implement several such priors that have desirable properties. A challenging aspect of imposing a prior is choosing the optimal strength. We describe an empirical way to determine the appropriate strength of the prior. We test our approach on numerically generated examples. Our code is released in an open-source \texttt{python} package called \texttt{pysquid}.

physics.data-an↗

Analysis of Magnetic Vortex Dissipation in Sn-Segregated Boundaries in Nb$_3$Sn Superconducting RF Cavities

We study mechanisms of vortex nucleation in Nb$_3$Sn Superconducting RF (SRF) cavities using a combination of experimental, theoretical, and computational methods. Scanning transmission electron microscopy (STEM) image and energy dispersive spectroscopy (EDS) of some Nb$_3$Sn cavities show Sn segregation at grain boundaries in Nb$_3$Sn with Sn concentration as high as $\sim$35 at.\% and widths $\sim$3 nm in chemical composition. Using ab initio calculations, we estimate the effect excess tin has on the local superconducting properties of the material. We model Sn segregation as a lowering of the local critical temperature. We then use time-dependent Ginzburg-Landau theory to understand the role of segregation on magnetic vortex nucleation. Our simulations indicate that the grain boundaries act as both nucleation sites for vortex penetration and pinning sites for vortices after nucleation. Depending on the magnitude of the applied field, vortices may remain pinned in the grain boundary or penetrate the grain itself. We estimate the superconducting losses due to vortices filling grain boundaries and compare with observed performance degradation with higher magnetic fields. We estimate that the quality factor may decrease by an order of magnitude ($10^{10}$ to $10^9$) at typical operating fields if 0.03\% of the grain boundaries actively nucleate vortices. We additionally estimate the volume that would need to be filled with vortices to match experimental observations of cavity heating.

cond-mat.supr-con↗

Reaction rates and the noisy saddle-node bifurcation: Renormalization group for barrier crossing

Barrier crossing calculations in chemical reaction-rate theory typically assume that the barrier is large compared to the temperature. When the barrier vanishes, however, there is a qualitative change in behavior. Instead of crossing a barrier, particles slide down a sloping potential. We formulate a renormalization group description of this noisy saddle-node transition. We derive the universal scaling behavior and corrections to scaling for the mean escape time in overdamped systems with arbitrary barrier height. We also develop an accurate approximation to the full distribution of barrier escape times by approximating the eigenvalues of the Fokker-Plank operator as equally spaced. This lets us derive a family of distributions that captures the barrier crossing times for arbitrary barrier height. Our critical theory draws links between barrier crossing in chemistry, the renormalization group, and bifurcation theory.

cond-mat.stat-mech↗

Visualizing probabilistic models in Minkowski space with intensive symmetrized Kullback-Leibler embedding

We show that the predicted probability distributions for any $N$-parameter statistical model taking the form of an exponential family can be explicitly and analytically embedded isometrically in a $N{+}N$-dimensional Minkowski space. That is, the model predictions can be visualized as control parameters are varied, preserving the natural distance between probability distributions. All pairwise distances between model instances are given by the symmetrized Kullback-Leibler divergence. We give formulas for these intensive symmetrized Kullback Leibler (isKL) coordinate embeddings, and illustrate the resulting visualizations with the Bernoulli (coin toss) problem, the ideal gas, $n$ sided die, the nonlinear least squares fit, and the Gaussian fit. We highlight how isKL can be used to determine the minimum number of parameters needed to describe probabilistic data, and conclude by visualizing the prediction space of the two-dimensional Ising model, where we examine the manifold behavior near its critical point.

cond-mat.stat-mech↗

The OpenKIM Processing Pipeline: A Cloud-Based Automatic Materials Property Computation Engine

The Open Knowledgebase of Interatomic Models (OpenKIM) project is a framework intended to facilitate access to standardized implementations of interatomic models for molecular simulations along with computational protocols to evaluate them. These protocols includes tests to compute materials properties predicted by models and verification checks to assess their coding integrity. While housing this content in a unified, publicly available environment constitutes a major step forward for the molecular modeling community, it further presents the opportunity to understand the range of validity of interatomic models and their suitability for specific target applications. To this end, OpenKIM includes a computational pipeline that runs tests and verification checks using all available interatomic models contained within the OpenKIM Repository at https://openkim.org. The OpenKIM Processing Pipeline is built on a set of Docker images hosted on distributed, heterogeneous hardware and utilizes open-source software to automatically run test-model and verification check-model pairs and resolve dependencies between them. The design philosophy and implementation choices made in the development of the pipeline are discussed as well as an example of its application to interatomic model selection.

physics.comp-ph↗

Weird scaling for 2-D avalanches: Curing the faceting, and scaling in the lower critical dimension

The non-equilibrium random-field Ising model is well studied, yet there are outstanding questions. In two dimensions, power law scaling approaches fail and the critical disorder is difficult to pin down. Additionally, the presence of faceting on the square lattice creates avalanches that are lattice dependent at small scales. We propose two methods which we find solve these issues. First, we perform large scale simulations on a Voronoi lattice to mitigate the effects of faceting. Secondly, the invariant arguments of the universal scaling functions necessary to perform scaling collapses can be directly determined using our recent normal form theory of the Renormalization Group. This method has proven useful in cleanly capturing the complex behavior which occurs in both the lower and upper critical dimensions of systems and here captures the 2D NE-RFIM behavior well. The obtained scaling collapses span over a range of a factor of ten in the disorder and a factor of $10^4$ in avalanche cutoff. They are consistent with a critical disorder at zero and with a lower critical dimension for the model equal to two.

cond-mat.dis-nn↗

Yield precursor dislocation avalanches in small crystals: the irreversibility transition

The transition from elastic to plastic deformation in crystalline metals shares history dependence and scale-invariant avalanche signature with other non-equilibrium systems under external loading: dilute colloidal suspensions, plastically-deformed amorphous solids, granular materials, and dislocation-based simulations of crystals. These other systems exhibit transitions with clear analogies to work hardening and yield stress, with many typically undergoing purely elastic behavior only after 'training' through repeated cyclic loading; studies in these other systems show a power law scaling of the hysteresis loop extent and of the training time as the peak load approaches a so-called reversible-irreversible transition (RIT). We discover here that deformation of small crystals shares these key characteristics: yielding and hysteresis in uniaxial compression experiments of single-crystalline Cu nano- and micro-pillars decay under repeated cyclic loading. The amplitude and decay time of the yield precursor avalanches diverge as the peak stress approaches failure stress for each pillar, with a power law scaling virtually equivalent to RITs in other nonequilibrium systems.

cond-mat.mtrl-sci↗

Visualizing probabilistic models: Intensive Principal Component Analysis

Unsupervised learning makes manifest the underlying structure of data without curated training and specific problem definitions. However, the inference of relationships between data points is frustrated by the `curse of dimensionality' in high-dimensions. Inspired by replica theory from statistical mechanics, we consider replicas of the system to tune the dimensionality and take the limit as the number of replicas goes to zero. The result is the intensive embedding, which is not only isometric (preserving local distances) but allows global structure to be more transparently visualized. We develop the Intensive Principal Component Analysis (InPCA) and demonstrate clear improvements in visualizations of the Ising model of magnetic spins, a neural network, and the dark energy cold dark matter (ΛCDM) model as applied to the Cosmic Microwave Background.

cond-mat.stat-mech↗

Online storage ring optimization using dimension-reduction and genetic algorithms

Particle storage rings are a rich application domain for online optimization algorithms. The Cornell Electron Storage Ring (CESR) has hundreds of independently powered magnets, making it a high-dimensional test-problem for algorithmic tuning. We investigate algorithms that restrict the search space to a small number of linear combinations of parameters ("knobs") which contain most of the effect on our chosen objective (the vertical emittance), thus enabling efficient tuning. We report experimental tests at CESR that use dimension-reduction techniques to transform an 81-dimensional space to an 8-dimensional one which may be efficiently minimized using one-dimensional parameter scans. We also report an experimental test of a multi-objective genetic algorithm using these knobs that results in emittance improvements comparable to state-of-the-art algorithms, but with increased control over orbit errors.

physics.acc-ph↗

Normal form for renormalization groups

The results of the renormalization group are commonly advertised as the existence of power law singularities near critical points. The classic predictions are often violated and logarithmic and exponential corrections are treated on a case-by-case basis. We use the mathematics of normal form theory to systematically group these into universality families of seemingly unrelated systems united by common scaling variables. We recover and explain the existing literature and predict the nonlinear generalization for the universal homogeneous scaling functions. We show that this procedure leads to a better handling of the singularity even in classic cases and elaborate our framework using several examples.

cond-mat.stat-mech↗

Image registration and super resolution from first principles

Image registration is the inference of transformations relating noisy and distorted images. It is fundamental in computer vision, experimental physics, and medical imaging. Many algorithms and analyses exist for inferring shift, rotation, and nonlinear transformations between image coordinates. Even in the simplest case of translation, however, all known algorithms are biased and none have achieved the precision limit of the Cramer Rao bound (CRB). Following Bayesian inference, we prove that the standard method of shifting one image to match another cannot reach the CRB. We show that the bias can be cured and the CRB reached if, instead, we use Super Registration: learning an optimal model for the underlying image and shifting that to match the data. Our theory shows that coarse-graining oversampled images can improve registration precision of the standard method. For oversampled data, our method does not yield striking improvements as measured by eye. In these cases, however, we show our new registration method can lead to dramatic improvements in extractable information, for example, inferring $10\times$ more precise particle positions.

physics.data-an↗