Searcharxiv⌕ Search

arXiv subjects

James P. Sethna

Publications and source records attributed to James P. Sethna.

At least 145 records · Page 8Linked to original sources
arXiv1997

Rate theory for correlated processes: Double-jumps in adatom diffusion

We study the rate of activated motion over multiple barriers, in particular the correlated double-jump of an adatom diffusing on a missing-row reconstructed Platinum (110) surface. We develop a Transition Path Theory, showing that the activation energy is given by the minimum-energy trajectory which succeeds in the double-jump. We explicitly calculate this trajectory within an effective-medium molecular dynamics simulation. A cusp in the acceptance region leads to a sqrt{T} prefactor for the activated rate of double-jumps. Theory and numerical results agree.

cond-mat.mtrl-sci↗
arXiv1997

Multicanonical Methods vs. Molecular Dynamics vs. Monte Carlo: Comparison for Lennard-Jones Glasses

We applied a multicanonical algorithm (entropic sampling) to a two-dimensional and a three-dimensional Lennard-Jones system with quasicrystalline and glassy ground states. Focusing on the ability of the algorithm to locate low lying energy states, we compared the results of the multicanonical simulations with standard Monte Carlo simulated annealing and molecular dynamics methods. We find slight benefits to using entropic sampling in small systems (less than 80 particles), which disappear with larger systems. This is disappointing as the multicanonical methods are designed to surmount energy barriers to relaxation. We analyze this failure theoretically, and show (1) the multicanonical method is reduced in the thermodynamic limit (large systems) to an effective Monte Carlo simulated annealing with a random temperature vs. time, and (2) the multicanonical method gets trapped by unphysical entropy barriers in the same metastable states whose energy barriers trap the traditional quenches. The performance of Monte Carlo and molecular dynamics quenches were remarkably similar.

cond-mat.stat-mech↗
arXiv1997

Hysteresis, Avalanches, and Barkhausen Noise

Hysteresis, the lag between the force and the response, is often associated with noisy, jerky motion which have recently been called ``avalanches''. The interesting question is why the avalanches come in such a variety of sizes: naively one would expect either all small events or one large one. Power-law distributions are often seen near transitions, or critical points. We study the zero temperature random field Ising model as a model for noise and avalanches in hysteretic systems. Tuning the amount of disorder in the system, we find an ordinary critical point with avalanches on all length scales. We study this critical point in 6-epsilon dimensions, and with simulations in 2, 3, 4, 5, 7, and 9 dimensions with systems as large as 1000^3. The power-law distributions in principle only occur for a special value of the randomness (the critical point), but many decades of scaling occur quite far from this special value: three decades of scaling (a publishable experiment) are obtained a factor of two away from the critical value. Perhaps many of the power laws observed in nature are just systems near their critical points?

cond-mat.stat-mech↗
arXiv1997

Zero-temperature Hysteresis in Random-field Ising Model on a Bethe Lattice

We consider the single-spin-flip dynamics of the random-field Ising model on a Bethe lattice at zero temperature in the presence of a uniform external field. We determine the average magnetization as the external field is varied from minus infinity to plus infinity by setting up the self-consistent field equations, which we show are exact in this case. We find that for a 3-coordinated Bethe lattice, there is no jump discontinuity in magnetization for arbitrarily small gaussian disorder, but the discontinuity is present for larger coordination numbers. We have checked our results by Monte Carlo simulations employing a technique for simulating classical interacting systems on the Bethe lattice which avoids surface effects altogether.

cond-mat.stat-mech↗
arXiv1997

Martensitic Tweed and the Two-Way Shape-Memory Effect

We briefly introduce tweed, which is found above the martensitic transition in a variety of shape-memory, high-T_c, and other materials. Based on our previous mapping of the problem onto a spin-glass model, we conjecture that the two-way shape-memory effect is due to tweed.

cond-mat.dis-nn↗
arXiv1996

Improved Magnetic Information Storage using Return-Point Memory

The traditional magnetic storage mechanisms (both analog and digital) apply an external field signal H(t) to a hysteretic magnetic material, and read the remanent magnetization M(t), which is (roughly) proportional to H(t). We propose a new analog method of recovering the signal from the magnetic material, making use of the shape of the hysteresis loop M(H). The field H, ``stored'' in a region with N domains or particles, can be recovered with fluctuations of order 1/N using the new method - much superior to the 1/sqrt{N} fluctuations in traditional analog storage.

cond-mat.mtrl-sci↗
arXiv1996

Statistical Mechanics of Cracks: Thermodynamic Limit, Fluctuations, Breakdown, and Asymptotics of Elastic Theory

We study a class of models for brittle fracture: elastic theory models which allow for cracks but not for plastic flow. We show that these models exhibit, at all finite temperatures, a transition to fracture under applied load similar to that at a first order liquid-gas transition. We study this transition at low temperature for small tension. We discuss the appropriate thermodynamic limit of these theories: a large class of boundary conditions is identified for which the energy release for a crack becomes independent of the macroscopic shape of the material. Using the complex variable method in a two-dimensional elastic theory, we prove that the energy release in an isotropically stretched material due to the creation of an arbitrary curvy cut is the same to cubic order as the energy release for the straight cut with the same end points. We find the normal modes and the energy spectrum for crack shape fluctuations and for crack surface phonons, under a uniform isotropic tension. For small uniform isotropic tension in two dimensions we calculate the essential singularity associated with fracturing the material in a saddle point approximation including quadratic fluctuations. This singularity determines the lifetime of the material (half-life for fracture), and also determines the asymptotic divergence of the high-order corrections to the zero temperature elastic coefficients. We calculate the asymptotic ratio of the high-order elastic coefficients of the inverse bulk modulus and argue that the result is unchanged by nonlinearities --- the ratio of the high-order nonlinear terms are determined solely by the linear theory.

cond-mat.mtrl-sci↗
arXiv1996

Decay of isolated surface features driven by the Gibbs-Thomson effect in analytic model and simulation

A theory based on the thermodynamic Gibbs-Thomson relation is presented which provides the framework for understanding the time evolution of isolated nanoscale features (i.e., islands and pits) on surfaces. Two limiting cases are predicted, in which either diffusion or interface transfer is the limiting process. These cases correspond to similar regimes considered in previous works addressing the Ostwald ripening of ensembles of features. A third possible limiting case is noted for the special geometry of "stacked" islands. In these limiting cases, isolated features are predicted to decay in size with a power law scaling in time: A is proportional to (t0-t)^n, where A is the area of the feature, t0 is the time at which the feature disappears, and n=2/3 or 1. The constant of proportionality is related to parameters describing both the kinetic and equilibrium properties of the surface. A continuous time Monte Carlo simulation is used to test the application of this theory to generic surfaces with atomic scale features. A new method is described to obtain macroscopic kinetic parameters describing interfaces in such simulations. Simulation and analytic theory are compared directly, using measurements of the simulation to determine the constants of the analytic theory. Agreement between the two is very good over a range of surface parameters, suggesting that the analytic theory properly captures the necessary physics. It is anticipated that the simulation will be useful in modeling complex surface geometries often seen in experiments on physical surfaces, for which application of the analytic model is not straightforward.

cond-mat↗
arXiv1996

Disorder-Induced Critical Phenomena in Hysteresis: A Numerical Scaling Analysis

Experimental systems with a first order phase transition will often exhibit hysteresis when out of equilibrium. If defects are present, the hysteresis loop can have different shapes: with small disorder the hysteresis loop has a macroscopic jump, while for large disorder the hysteresis loop is smooth. The transition between these two shapes is critical, with diverging length scales and power laws. We simulate such a system with the zero temperature random field Ising model, in 2, 3, 4, 5, 7, and 9 dimensions, with systems of up to 1000^3 spins, and find the critical exponents from scaling collapses of several measurements. The numerical results agree well with the analytical predictions from a renormalization group calculation.

cond-mat↗
arXiv1996

Microscopic Estimates for Electromigration Velocities of Intragranular Voids in Aluminum Lines

We explore the effect of faceting on possible mechanisms for mass transport around electromigration voids in aluminum interconnects. Motivated by linear response estimates which suggest that particle flux would be much higher along steps than across terraces on a clean aluminum surface, we study step nucleation in the presence of a small driving force along a surface. We find that step nucleation, even on a nearly defect-free void surface, would be slow if the step energy is equal to that calculated for a clean aluminum surface. In the presence of a uniform electromigration force, the creation of new steps between existing ones should not occur unless the free energy cost of a step is much less than thermal energies. We conclude that voids cannot move intragranularly at $μ$m/hr rates without help from other factors such as local heating and impurities.

mtrl-th↗
arXiv1996

Elastic Theory Has Zero Radius of Convergence

Nonlinear elastic theory studies the elastic constants of a material (such as Young's modulus or bulk modulus) as a power series in the applied load. The inverse bulk modulus K, for example depends on the compression P: $ {1/ K(P)} = c_0 + c_1 P + c_2 P^2 \cdots + c_n P^n + \cdots $. Elastic materials that allow cracks are unstable at finite temperature with respect to fracture under a stretching load; as a result, the above power series has zero radius of convergence and thus can at best be an asymptotic series. Considering thermal nucleation of cracks in a two-dimensional isotropic, linear--elastic material at finite temperature we compute the asymptotic form $ { c_{n+1}/ c_n}\to C n^{1/2}$ as $n \rightarrow \infty$. We present an explicit formula for $C$ as a function of temperature and material properties.

cond-mat↗
arXiv1995

Acoustic Emission from crumpling paper

From magnetic systems to the crust of the earth, many physical systems that exibit a multiplicty of metastable states emit pulses with a broad power law distribution in energy. Digital audio recordings reveal that paper being crumpled, a system that can be easily held in hand, is such a system. Crumpling paper both using the traditional hand method and a novel cylindrical geometry uncovered a power law distribution of pulse energies spanning at least two decades: (exponent 1.3 - 1.6) Crumpling initally flat sheets into a compact ball (strong crumpling), we found little or no evidence that the energy distribution varied systematically over time or the size of the sheet. When we applied repetitive small deformations (weak crumpling) to sheets which had been previously folded along a regular grid, we found no systematic dependence on the grid spacing. Our results suggest that the pulse energy depends only weakly on the size of the paper regions responsible for sound production.

cond-mat↗
arXiv1995

A Generalization of the Theory of Normal Forms

Normal forms allow the use of a restricted class of coordinate transformations (typically homogeneous polynomials) to put the bifurcations found in nonlinear dynamical systems into a few standard forms. We investigate here the consequences of relaxing the restrictions of the form of the coordinate transformations. In the Duffing equation, a logarithmic transformation can remove the nonlinearity: in one interpretation, the nonlinearity is replaced by a branch cut leading to a Poincare section. When the linearized problem is autonomous with diagonal Jordan form, we can remove all nonlinearities order by order using these singular coordinate transformations.

chao-dyn↗
arXiv1995

Hysteresis, Avalanches, and Disorder Induced Critical Scaling: A Renormalization Group Approach

We study the zero temperature random field Ising model as a model for noise and avalanches in hysteretic systems. Tuning the amount of disorder in the system, we find an ordinary critical point with avalanches on all length scales. Using a mapping to the pure Ising model, we Borel sum the $6-ε$ expansion to $O(ε^5)$ for the correlation length exponent. We sketch a new method for directly calculating avalanche exponents, which we perform to $O(ε)$. Numerical exponents in 3, 4, and 5 dimensions are in good agreement with the analytical predictions.

cond-mat↗
arXiv1995

Avalanches, Barkhausen Noise, and Plain Old Criticality

We explain Barkhausen noise in magnetic systems in terms of avalanches near a plain old critical point in the hysteretic zero-temperature random-field Ising model. The avalanche size distribution has a universal scaling function, making non-trivial predictions of the shape of the distribution up to 50\% above the critical point, where two decades of scaling are still observed. We simulate systems with up to $1000^3$ domains, extract critical exponents in 2, 3, 4, and 5 dimensions, compare with our 2d and $6-ε$ predictions, and compare to a variety of experimental Barkhausen measurements.

cond-mat↗
arXiv1995

Defect--Defect Correlation Functions, Generic Scale Invariance, and the Complex Ginzburg--Landau Equation

Motivated by the idea of developing a ``hydrodynamic'' description of spatiotemporal chaos, we have investigated the defect--defect correlation functions in the defect turbulence regime of the two--dimensional, anisotropic complex Ginzburg--Landau equation. We compare our results with the predictions of generic scale invariance. Using the topological nature of the defects, we prove that defect--defect correlations cannot decay as slowly as predicted by generic scale invariance. We also present results on the fluctuations of the amplitude field $A$.

patt-sol↗
arXiv1994

Atomic Tunneling from a STM/AFM tip: Dissipative Quantum Effects from Phonons

We study the effects of phonons on the tunneling of an atom between two surfaces. In contrast to an atom tunneling in the bulk, the phonons couple very strongly, and qualitatively change the tunneling behavior. This is the first example of {\it ohmic} coupling from phonons for a two-state system. We propose an experiment in which an atom tunnels from the tip of an STM, and show how its behavior would be similar to the Macroscopic Quantum Coherence behavior predicted for SQUIDS. The ability to tune and calculate many parameters would lead to detailed tests of the standard theories. (For a general intro to this work on the on the World-Wide-Web: http://www.lassp.cornell.edu. Click on ``Entertaining Science Done Here'' and ``Quantum Tunneling of Atoms'')

cond-mat↗