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Jan Behrends

Publications and source records attributed to Jan Behrends.

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Second-Order Bulk-Boundary Correspondence in Rotationally Symmetric Topological Superconductors from Stacked Dirac Hamiltonians

Two-dimensional second-order topological superconductors host zero-dimensional Majorana bound states at their boundaries. In this work, focusing on rotation-invariant crystalline topological superconductors, we establish a bulk-boundary correspondence linking the presence of such Majorana bound states to bulk topological invariants introduced by Benalcazar et al. We thus establish when a topological crystalline superconductor protected by rotational symmetry displays second-order topological superconductivity. Our approach is based on stacked Dirac Hamiltonians, using which we relate transitions between topological phases to the transformation properties between adjacent gapped boundaries. We find that in addition to the bulk rotational invariants, the presence of Majorana boundary bound states in a given geometry depends on the interplay between weak topological invariants and the location of the rotation center relative to the lattice. We provide numerical examples for our predictions and discuss possible extensions of our approach.

cond-mat.mes-hall

Symmetry classes, many-body zero modes, and supersymmetry in the complex Sachdev-Ye-Kitaev model

The complex Sachdev-Ye-Kitaev (cSYK) model is a charge-conserving model of randomly interacting fermions. The interaction term can be chosen such that the model exhibits chiral symmetry. Then, depending on the charge sector and the number of interacting fermions, level spacing statistics suggests a fourfold categorization of the model into the three Wigner-Dyson symmetry classes. In this work, inspired by previous findings for the Majorana Sachdev-Ye-Kitaev model, we embed the symmetry classes of the cSYK model in the Altland-Zirnbauer framework and identify consequences of chiral symmetry originating from correlations across different charge sectors. In particular, we show that for an odd number of fermions, the model hosts exact many-body zero modes that can be combined into a generalized fermion that does not affect the system's energy. This fermion directly leads to quantum-mechanical supersymmetry that, unlike explicitly supersymmetric cSYK constructions, does not require fine-tuned couplings, but only chiral symmetry. Signatures of the generalized fermion, and thus supersymmetry, include the long-time plateau in time-dependent correlation functions of fermion-parity-odd observables: The plateau may take nonzero value only for certain combinations of the fermion structure of the observable and the system's symmetry class. We illustrate our findings through exact diagonalization simulations of the system's dynamics.

hep-th

Anomalous conductance scaling in strained Weyl semimetals

Magnetotransport provides key experimental signatures in Weyl semimetals. The longitudinal magnetoresistance is linked to the chiral anomaly and the transversal magnetoresistance to the dominant charge relaxation mechanism. Axial magnetic fields that act with opposite sign on opposite chiralities facilitate new transport experiments that probe the low-energy Weyl nodes. As recently realized, these axial fields can be achieved by straining samples or adding inhomogeneities to them. Here, we identify a robust signature of axial magnetic fields: an anomalous scaling of the conductance in the diffusive ultraquantum regime. In particular, we demonstrate that the longitudinal conductivity in the ultraquantum regime of a disordered Weyl semimetal subjected to an axial magnetic field increases with both the field strength and sample width due to a spatial separation of charge carriers. We contrast axial magnetic with real magnetic fields to clearly distinguish the different behavior of the conductance. Our results rely on numerical tight-binding simulations and are supported by analytical arguments. We argue that the spatial separation of charge carriers can be used for directed currents in microstructured electronic devices.

cond-mat.mes-hall

The tenfold way and many-body zero modes in the Sachdev-Ye-Kitaev model

The Sachdev-Ye-Kitaev (SYK) model, in its simplest form, describes $k$ Majorana fermions with random all-to-all four-body interactions. We consider the SYK model in the framework of a many-body Altland-Zirnbauer classification that sees the system as belonging to one of eight (real) symmetry classes depending on the value of $k\mod 8$. We show that, depending on the symmetry class, the system may support exact many-body zero modes with the symmetries also dictating whether these may have a nonzero contribution to Majorana fermions, i.e., single-particle weight. These zero modes appear in all but two of the symmetry classes. When present, they leave clear signatures in physical observables that go beyond the threefold (Wigner-Dyson) possibilities for level spacing statistics studied earlier. Signatures we discover include a zero-energy peak or hole in the single-particle spectral function, depending on whether symmetries allow or forbid zero modes to have single-particle weight. The zero modes are also shown to influence the many-body dynamics, where signatures include a nonzero long-time limit for the out-of-time-order correlation function. Furthermore, we show that the extension of the four-body SYK model by quadratic terms can be interpreted as realizing the remaining two complex symmetry classes; we thus demonstrate how the entire tenfold Altland-Zirnbauer classification may emerge in the SYK model.

cond-mat.dis-nn

Landau levels, Bardeen polynomials and Fermi arcs in Weyl semimetals: the who's who of the chiral anomaly

Condensed matter systems realizing Weyl fermions exhibit striking phenomenology derived from their topologically protected surface states as well as chiral anomalies induced by electromagnetic fields. More recently, inhomogeneous strain or magnetization were predicted to result in chiral electric $\mathbf{E}_5$ and magnetic $\mathbf{B}_5$ fields, which modify and enrich the chiral anomaly with additional terms. In this work, we develop a lattice-based approach to describe the chiral anomaly, which involves Landau and pseudo-Landau levels and treats all anomalous terms on equal footing, while naturally incorporating Fermi arcs. We exemplify its potential by physically interpreting the largely overlooked role of Fermi arcs in the covariant (Fermi level) contribution to the anomaly and revisiting the factor of $1/3$ difference between the covariant and consistent (complete band) contributions to the $\mathbf{E}_5\cdot\mathbf{B}_5$ term in the anomaly. Our framework provides a versatile tool for the analysis of anomalies in realistic lattice models as well as a source of simple physical intuition for understanding strained and magnetized inhomogeneous Weyl semimetals.

cond-mat.mes-hall

Site-selective measurement of coupled spin pairs in an organic semiconductor

From organic electronics to biological systems, understanding the role of intermolecular interactions between spin pairs is a key challenge. Here we show how such pairs can be selectively addressed with combined spin and optical sensitivity. We demonstrate this for bound pairs of spin-triplet excitations formed by singlet fission, with direct applicability across a wide range of synthetic and biological systems. We show that the site-sensitivity of exchange coupling allows distinct triplet pairs to be resonantly addressed at different magnetic fields, tuning them between optically bright singlet (S=0) and dark triplet, quintet (S=1,2) configurations: this induces narrow holes in a broad optical emission spectrum, uncovering exchange-specific luminescence. Using fields up to 60 T, we identify three distinct triplet-pair sites, with exchange couplings varying over an order of magnitude (0.3-5 meV), each with its own luminescence spectrum, coexisting in a single material. Our results reveal how site-selectivity can be achieved for organic spin pairs in a broad range of systems.

physics.chem-ph

Transversal magnetotransport in Weyl semimetals: Exact numerical approach

Magnetotransport experiments on Weyl semimetals are essential for investigating the intriguing topological and low-energy properties of Weyl nodes. If the transport direction is perpendicular to the applied magnetic field, experiments have shown a large positive magnetoresistance. In this work, we present a theoretical scattering matrix approach to transversal magnetotransport in a Weyl node. Our numerical method confirms and goes beyond the existing perturbative analytical approach by treating disorder exactly. It is formulated in real space and is applicable to mesoscopic samples as well as in the bulk limit. In particular, we study the case of clean and strongly disordered samples.

cond-mat.mes-hall

Nodal-line semimetals from Weyl superlattices

The existence and topological classification of lower-dimensional Fermi surfaces is often tied to the crystal symmetries of the underlying lattice systems. Artificially engineered lattices, such as heterostructures and other superlattices, provide promising avenues to realize desired crystal symmetries that protect lower-dimensional Fermi surface, such as nodal lines. In this work, we investigate a Weyl semimetal subjected to spatially periodic onsite potential, giving rise to several phases, including a nodal-line semimetal phase. In contrast to proposals that purely focus on lattice symmetries, the emergence of the nodal line in this setup does not require small spin-orbit coupling, but rather relies on its presence. We show that the stability of the nodal line is understood from reflection symmetry and a combination of a fractional lattice translation and charge-conjugation symmetry. Depending on the choice of parameters, this model exhibits drumhead surface states that are exponentially localized at the surface, or weakly localized surface states that decay into the bulk at all energies.

cond-mat.mes-hall

Strongly angle-dependent magnetoresistance in Weyl semimetals with long-range disorder

The chiral anomaly in Weyl semimetals states that the left- and right-handed Weyl fermions, constituting the low energy description, are not individually conserved, resulting, for example, in a negative magnetoresistance in such materials. Recent experiments see strong indications of such an anomalous resistance response; however, with a response that at strong fields is more sharply peaked for parallel magnetic and electric fields than expected from simple theoretical considerations. Here, we uncover a mechanism, arising from the interplay between the angle-dependent Landau level structure and long-range scalar disorder, that has the same phenomenology. In particular, we ana- lytically show, and numerically confirm, that the internode scattering time decreases exponentially with the angle between the magnetic field and the Weyl node separation in the large field limit, while it is insensitive to this angle at weak magnetic fields. Since, in the simplest approximation, the internode scattering time is proportional to the anomaly-related conductivity, this feature may be related to the experimental observations of a sharply peaked magnetoresistance.

cond-mat.mes-hall

Bulk-boundary correspondence from the inter-cellular Zak phase

The Zak phase $γ$, the generalization of the Berry phase to Bloch wave functions in solids, is often used to characterize inversion-symmetric 1D topological insulators; however, since its value can depend on the choice of real-space origin and unit cell, only the difference between the Zak phase of two regions is believed to be relevant. Here, we show that one can extract an origin-independent part of $γ$, the so-called inter-cellular Zak phase $γ^{\mathrm{inter}}$, which can be used as a bulk quantity to predict the number of surface modes as follows: a neutral finite 1D tight-binding system has $n_s = γ^{\mathrm{inter}}/π$ (mod 2) number of in-gap surface modes below the Fermi level if there exists a commensurate bulk unit cell that respects inversion symmetry. We demonstrate this by first verifying that $\pm eγ^{\mathrm{inter}}/2π$ (mod $e$) is equal to the extra charge accumulation in the surface region for a general translationally invariant 1D insulator, while the remnant part of $γ$, the intra-cellular Zak phase $γ^{\mathrm{intra}}$, corresponds to the electronic part of the dipole moment of the bulk's unit cell. Second, we show that the extra charge accumulation can be related to the number of surface modes when the unit cell is inversion symmetric. This bulk-boundary correspondence using $γ^{\mathrm{inter}}$ reduces to the conventional one using $γ$ when the real-space origin is at the inversion center. Our work thereby clarifies the usage of $γ$ in the bulk-boundary correspondence. We study several tight binding models to quantitatively check the relation between the extra charge accumulation and the inter-cellular Zak phase as well as the bulk-boundary correspondence using the inter-cellular Zak phase.

cond-mat.str-el

Visualizing the chiral anomaly in Dirac and Weyl semimetals with photoemission spectroscopy

Quantum anomalies are the breaking of a classical symmetry by quantum fluctuations. They dictate how physical systems of diverse nature, ranging from fundamental particles to crystalline materials, respond topologically to external perturbations, insensitive to local details. The anomaly paradigm was triggered by the discovery of the chiral anomaly that contributes to the decay of pions into photons and influences the motion of superfluid vortices in $^3$He-A. In the solid state, it also fundamentally affects the properties of topological Weyl and Dirac semimetals, recently realized experimentally in TaAs, Na$_3$Bi, Cd$_3$As$_2$, and ZrTe$_{5}$. In this work we propose that the most identifying consequence of the chiral anomaly, the charge density imbalance between fermions of different chirality induced by non-orthogonal electric and magnetic fields, can be directly observed in these materials with the existing technology of photoemission spectroscopy. With angle resolution, the chiral anomaly is identified by a characteristic note-shaped pattern of the emission spectra, originating from the imbalanced occupation of the bulk states and a previously unreported momentum dependent energy shift of the surface state Fermi arcs. We further demonstrate that the chiral anomaly likewise leaves an imprint in angle averaged emission spectra, facilitating its experimental detection. Thereby, our work provides essential theoretical input to foster the direct visualization of the chiral anomaly in condensed matter.

cond-mat.mes-hall

The Post-Merger Magnetized Evolution of White Dwarf Binaries: The Double-Degenerate Channel of Sub-Chandrasekhar Type Ia Supernovae and the Formation of Magnetized White Dwarfs

Type Ia supernovae (SNe Ia) play a crucial role as standardizable cosmological candles, though the nature of their progenitors is a subject of active investigation. Recent observational and theoretical work has pointed to merging white dwarf binaries, referred to as the double-degenerate channel, as the possible progenitor systems for some SNe Ia. Additionally, recent theoretical work suggests that mergers which fail to detonate may produce magnetized, rapidly-rotating white dwarfs. In this paper, we present the first multidimensional simulations of the post-merger evolution of white dwarf binaries to include the effect of the magnetic field. In these systems, the two white dwarfs complete a final merger on a dynamical timescale, and are tidally disrupted, producing a rapidly-rotating white dwarf merger surrounded by a hot corona and a thick, differentially-rotating disk. The disk is strongly susceptible to the magnetorotational instability (MRI), and we demonstrate that this leads to the rapid growth of an initially dynamically weak magnetic field in the disk, the spin-down of the white dwarf merger, and to the subsequent central ignition of the white dwarf merger. Additionally, these magnetized models exhibit new features not present in prior hydrodynamic studies of white dwarf mergers, including the development of MRI turbulence in the hot disk, magnetized outflows carrying a significant fraction of the disk mass, and the magnetization of the white dwarf merger to field strengths $\sim 2 \times 10^8$ G. We discuss the impact of our findings on the origins, circumstellar media, and observed properties of SNe Ia and magnetized white dwarfs.

astro-ph.SR

Direct Detection of Photoinduced Charge Transfer Complexes in Polymer:Fullerene Blends

We report transient electron paramagnetic resonance (trEPR) measurements with sub-microsecond time resolution performed on a P3HT:PCBM blend at low temperature. The trEPR spectrum immediately following photoexcitation reveals signatures of spin-correlated polaron pairs. The pair partners (positive polarons in P3HT and negative polarons in PCBM) can be identified by their characteristic g-values. The fact that the polaron pair states exhibit strong non-Boltzmann population unambiguously shows that the constituents of each pair are geminate, i.e. originate from one exciton. We demonstrate that coupled polaron pairs are present even several microseconds after charge transfer and suggest that they embody the intermediate charge transfer complexes which form at the donor/acceptor interface and mediate the conversion from excitons into free charge carriers.

cond-mat.mtrl-sci

Lock-in detection for pulsed electrically detected magnetic resonance

We show that in pulsed electrically detected magnetic resonance (pEDMR) signal modulation in combination with a lock-in detection scheme can reduce the low-frequency noise level by one order of magnitude and in addition removes the microwave-induced non-resonant background. This is exemplarily demonstrated for spin-echo measurements in phosphorus-doped Silicon. The modulation of the signal is achieved by cycling the phase of the projection pulse used in pEDMR for the read-out of the spin state.

cond-mat.mtrl-sci