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Jan Glorius

Publications and source records attributed to Jan Glorius.

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Precision masses of neutron-rich platinum and gold nuclei reveal enhanced $N=126$ shell strength below doubly-magic $^{208}$Pb

The heaviest stable nuclei in the universe owe their existence to quantum shell structure, the grouping of protons and neutrons into discrete energy levels separated by gaps. The largest known neutron shell gap in stable nuclei, at $N=126$, stabilizes doubly-magic $^{208}$Pb and is responsible for the characteristic abundance peak of heavy elements near gold and platinum produced by the rapid neutron-capture process (r-process). Whether this shell gap persists as protons are removed from lead is a question central to both nuclear structure and the modeling of heavy-element synthesis, yet it has remained unanswered due to the extraordinary difficulty of producing the relevant neutron-rich nuclei. Direct experimental knowledge in this region was essentially absent. Here we report the first precision mass measurements of $^{203,204}$Pt and $^{204,205,206}$Au, performed at GSI using a novel combination of Schottky and isochronous mass spectrometry in a heavy-ion storage ring. The $N=126$ isotones $^{204}$Pt and $^{205}$Au are more strongly bound than the extrapolated trend of the previously known mass surface by 403 and 464~keV, respectively, revealing an unexpectedly enhanced $N=126$ shell strength below doubly-magic $^{208}$Pb. Furthermore, the proton-neutron interaction strength exhibits a hitherto unobserved bifurcation at $N=126$ as protons are removed from $^{208}$Pb. Our results redefine the nuclear mass surface in the neutron-rich heavy-element region and provide direct experimental benchmarks for theoretical models whose extrapolations toward more exotic nuclei are essential for r-process nucleosynthesis calculations.

nucl-ex

Surrogate neutron-capture studies with fission detection in inverse kinematics at the ESR storage ring

The NECTAR (Nuclear rEaCTions At storage Rings) experiment at the ESR heavy-ion storage ring at GSI/FAIR Darmstadt is dedicated to surrogate reaction studies of neutron-induced reactions on heavy nuclei in inverse kinematics. In this work, we report on the implementation and performance of a newly developed fission-fragment detection system integrated into the NECTAR experimental setup. The upgraded detector configuration enables, for the first time in a surrogate experiment, the simultaneous detection ofgamma-decay residues, multi-neutron-emission residues, and fission fragments. The full setup was used for the first time in an experiment where a stored beam of bare 238U92+ ions at 17.24 MeV/u interacted with a gas-jet deuterium target, populating excited 238U and 239U nuclei via the 238U(d,d') and 238U(d,p) reactions. We describe the geometry of the used fission fragment detectors, design constraints, and simulation-based efficiency determination. The target-like particle identification and beam-like residue spectra demonstrating the performance of the complete setup are also shown.

physics.ins-det

Schottky detection techniques for ultra-rare short-lived ions in heavy ion storage rings

Non-destructive Schottky detectors are indispensable devices widely used in experiments at heavy-ion storage rings. In particular, they can be used to accurately determine the masses and lifetimes of short-lived exotic nuclear species. Single-ion sensitivity -- which enables highest sensitivity -- has been regularly achieved in the past utilizing resonant cavity detectors. Recent designs and analysis methods aim at pushing the limits of measurement accuracy by increasing the dimensionality of the acquired data, namely the position of the particle as well as the phase difference between several detectors. This work describes current methods and future perspectives of Schottky detection techniques focusing at their application for mass and lifetime measurements of the most rare and simultaneously short-lived radio nuclides.

physics.ins-det

Quantum Electrodynamics in Strong Electromagnetic Fields: Substate Resolved K$\alpha$ Transition Energies in Helium-like Uranium

Using novel metallic magnetic calorimeter detectors at the CRYRING@ESR, we recorded X-ray spectra of stored and electron cooled helium-like uranium (U$^{90+}$) with an unmatched spectral resolution of close to 90 eV. This allowed for an accurate determination of the energies of all four components of the K$\alpha$ transitions in U$^{90+}$. We find good agreement with state-of-the-art bound-state QED calculations for the strong-field regime. Our results do not support any systematic deviation between experiment and theory in helium-like systems, the presence of which was subject of intense debates in recent years.

physics.atom-ph

Towards experiments with highly charged ions at HESR

The atomic physic collaboration SPARC is a part of the APPA pillar at the future Facility for Antiproton and Ion Research. It aims for atomic-physics research across virtually the full range of atomic matter. A research area of the atomic physics experiments is the study of the collision dynamics in strong electro-magnetic fields as well as the fundamental interactions between electrons and heavy nuclei at the HESR. Here we give a short overview about the central instruments for SPARC experiments at this storage ring.

physics.atom-ph

Behavior of a trapezoid-based data acquisition system up to 100 kHz and beyond

In this work, we investigated the ability of a high-purity germanium detector connected to a trapezoid-filter-based data acquisition system to reliably record signals in spite of high sample activities. By activating multiple Na$_{2}$CO$_{3}$ samples with different Na content, we were able to deduce efficiency, resolution and dead time of the system used as a function of the sample activity. Based on the results, we were able to find a setting which allows measurements of event rates up to 35~kHz per readout channel with an energy resolution of 0.3\% at the 2754 keV $^{24}$Na line.

physics.ins-det

Nucleosynthesis simulations for the production of the p-nuclei $^{\text{92}}$Mo and $^{\text{94}}$Mo in a Supernova type II model

We present a nucleosynthesis sensitivity study for the $\gamma$-process in a Supernova type II model within the NuGrid research platform. The simulations aimed at identifying the relevant local production and destruction rates for the p-nuclei of molybdenum and at determining the sensitivity of the final abundances to these rates. We show that local destruction rates strongly determine the abundance of $^{92}$Mo and $^{94}$Mo, and quantify the impact.

astro-ph.IM

Measurements of neutron-induced reactions in inverse kinematics and applications to nuclear astrophysics

Neutron capture cross sections of unstable isotopes are important for neutron-induced nucleosynthesis as well as for technological applications. A combination of a radioactive beam facility, an ion storage ring and a high flux reactor would allow a direct measurement of neutron induced reactions over a wide energy range on isotopes with half lives down to minutes. The idea is to measure neutron-induced reactions on radioactive ions in inverse kinematics. This means, the radioactive ions will pass through a neutron target. In order to efficiently use the rare nuclides as well as to enhance the luminosity, the exotic nuclides can be stored in an ion storage ring. The neutron target can be the core of a research reactor, where one of the central fuel elements is replaced by the evacuated beam pipe of the storage ring. Using particle detectors and Schottky spectroscopy, most of the important neutron-induced reactions, such as (n,$\gamma$), (n,p), (n,$\alpha$), (n,2n), or (n,f), could be investigated.

nucl-ex

First Measurement of the $^{96}$Ru(p,$\gamma$)$^{97}$Rh Cross Section for the p-Process with a Storage Ring

This work presents a direct measurement of the $^{96}$Ru($p, \gamma$)$^{97}$Rh cross section via a novel technique using a storage ring, which opens opportunities for reaction measurements on unstable nuclei. A proof-of-principle experiment was performed at the storage ring ESR at GSI in Darmstadt, where circulating $^{96}$Ru ions interacted repeatedly with a hydrogen target. The $^{96}$Ru($p, \gamma$)$^{97}$Rh cross section between 9 and 11 MeV has been determined using two independent normalization methods. As key ingredients in Hauser-Feshbach calculations, the $\gamma$-ray strength function as well as the level density model can be pinned down with the measured ($p, \gamma$) cross section. Furthermore, the proton optical potential can be optimized after the uncertainties from the $\gamma$-ray strength function and the level density have been removed. As a result, a constrained $^{96}$Ru($p, \gamma$)$^{97}$Rh reaction rate over a wide temperature range is recommended for $p$-process network calculations.

nucl-ex

Experimental cross sections of 165Ho(\alpha,n)168Tm and 166Er(\alpha,n)169Yb for optical potential studies relevant for the astrophysical \gamma-process

Background: Optical potentials are crucial ingredients for the prediction of nuclear reaction rates needed in simulations of the astrophysical \gamma-process. Associated uncertainties are particularly large for reactions involving \alpha-particles. This includes (\gamma,\alpha) reactions which are of special importance in the \gamma-process. Purpose: The measurement of (\alpha,n) reactions allows for an optimization of currently used \alpha-nucleus potentials. The reactions 165Ho(\alpha,n) and 166Er(\alpha,n) probe the optical model in a mass region where \gamma-process calculations exhibit an underproduction of p nuclei which is not yet understood. Method: To investigate the energy-dependent cross sections of the reactions 165Ho(\alpha,n) and 166Er(\alpha,n) close to the reaction threshold, self-supporting metallic foils were irradiated with \alpha-particles using the FN tandem Van de Graaff accelerator at University of Notre Dame. The induced activity was determined afterwards by monitoring the specific \beta-decay channels. Results: Hauser-Feshbach predictions with a widely used global \alpha-potential describe the data well at energies where the cross sections are almost exclusively sensitive to the \alpha-widths. Increasing discrepancies appear towards the reaction threshold at lower energy. Conclusions: The tested global \alpha-potential is suitable at energies above 14 MeV, while a modification seems necessary close to the reaction threshold. Since the \gamma- and neutron width show non-negligible impact on the predictions, complementary data are required to judge whether or not the discrepancies found can to be solely assigned to the \alpha-width.

nucl-ex