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Jan Rothörl

Publications and source records attributed to Jan Rothörl.

12 recordsLinked to original sources

Skyrmion Lattice Domain Formation in a Non-Flat Energy Landscape

Magnetic skyrmions are chiral spin structures with non-trivial topology that comprise two-dimensional quasi-particles and are promising information carriers for data storage and processing devices. Skyrmion lattices in magnetic thin films exhibit Kosterlitz-Thouless-Halperin-Nelson-Young (KTHNY) phase transitions and have garnered significant interest for studying emergent 2D phase behavior. In experimental skyrmion lattices, the main factor limiting the quasi-long-range order in thin films has been the non-flat energy landscape - often referred to as pinning effects. We demonstrate direct control of the skyrmion lattice order by effectively tuning the energy landscape employing magnetic field oscillations. By quantifying lattice order and dynamics, we explore how domain boundaries form and evolve due to pinning effects in Kerr microscopy experiments and in Brownian dynamics simulations, offering a pathway to control and study emergent skyrmion lattice properties and 2D phase behavior.

cond-mat.mes-hall

Skyrmion Lattice Order Controlled by Confinement Geometry

Magnetic skyrmions forming two-dimensional (2D) lattices provide a versatile platform for investigating phase transitions predicted by Kosterlitz-Thouless-Halperin-Nelson-Young (KTHNY) theory. While 2D melting in skyrmion systems has been demonstrated, achieving controlled ordering in skyrmion lattices remains challenging due to pinning effects from a non-uniform energy landscape, which often results in polycrystalline structures. Skyrmions in thin films, however, offer thermal diffusion with high tunability and can be directly imaged via Kerr microscopy, enabling real-time observation of their dynamics. To regulate lattice order in such flexible systems, we introduce geometric confinements of varying shapes. Combining Kerr microscopy experiments with Thiele model simulations, we demonstrate that confinement geometry critically influences lattice order. Specifically, hexagonal confinements commensurate with the skyrmion lattice stabilize monodomain hexagonal ordering, while incommensurate geometries induce domain formation and reduce overall order. Understanding these boundary-driven effects is essential for advancing the study of 2D phase behavior and for the design of skyrmion-based spintronic applications, ranging from memory devices to unconventional computing architectures.

cond-mat.mes-hall

Persistent Homology-Based Indicator of Orientational Ordering in Two-Dimensional Quasi-Particle Systems Applied to Skyrmion Lattices

Two-dimensional (2D) particle systems, such as magnetic skyrmions, exhibit topological phase transitions between unique 2D phases. However, a simple and computationally efficient methodology to capture lattice configurational properties and construct an appropriate, easily calculable descriptor for phase identification remains elusive. Here, we propose an indicator for topological phase transitions using persistent homology (PH). PH offers novel insights beyond conventional indicators by capturing topological features derived from the configurational properties of the lattice. The proposed persistent-homology-based indicator, which selectively counts stable features in a persistence diagram, effectively traces the lattice's ordering changes, as confirmed by comparisons with the conventionally used measure of the ordering (the magnitude of the orientational order parameter $\langle|Ψ_6|\rangle$), typically used to identify lattice phases. We demonstrate the applicability of our indicator to experimental data, showing that it yields results consistent with those of simulations. This experimental validation highlights the robustness of the proposed method for real physical systems beyond idealized simulated systems. While our method is demonstrated in the context of skyrmion lattice systems, the approach is general and can be extended to other two-dimensional systems composed of interacting particles. As a key advantage, our indicator offers lower computational complexity than the conventionally used measures.

cond-mat.stat-mech

Real-Time Modeling of Skyrmion Dynamics in Arbitrary 2D Spatially Dependent Pinning Potential Landscapes

Non-flat energy landscapes leading to localized pinning of skyrmions pose an inherent and unavoidable challenge for studies of fundamental 2D spin structure dynamics as well as applications. Accounting for pinning is a key requirement for predictive modeling of skyrmion systems, as it impacts the systems' dynamics and introduces randomizing effects. In this article, we use magneto-optical Kerr microscopy to image skyrmions in a magnetic thin film system in real time and analyze their hopping dynamics within the non-flat energy landscape. To achieve a fully quantitative model, we utilize skyrmion diffusion and dwell times at pinning sites to extrapolate the pinning energy landscape into regions that cannot be sampled on reasonable experimental time scales. For evaluation with a coarse-grained Thiele model, we perform long-time measurements of skyrmion diffusion and then develop a two-step procedure to determine simulation parameters by comparing them to experimentally accessible behavior. This provides a direct conversion between simulation and experimental units, which is the missing key step that has previously prevented quantitative quasiparticle modeling. We demonstrate the predictive power of our approach by measuring the experimentally unexplored density dependence of skyrmion diffusion and show that it is in excellent agreement with simulation predictions. Our technique thus enables quantitative skyrmion simulations on experimental time and length scales, allowing for predictive in-silico prototyping of skyrmion devices.

cond-mat.stat-mech

Realizing Quantitative Quasiparticle Modeling of Skyrmion Dynamics in Arbitrary Potentials

We demonstrate fully quantitative Thiele model simulations of magnetic skyrmion dynamics on previously unattainable experimentally relevant large length and time scales by ascertaining the key missing parameters needed to calibrate the experimental and simulation time scales and current-induced forces. Our work allows us to determine complete spatial pinning energy landscapes that enable quantification of experimental studies of diffusion in arbitrary potentials within the Lifson-Jackson framework. Our method enables us to ascertain the time scales, and by isolating the effect of ultra-low current density (order $10^6 A/m^2$) generated torques we directly infer the total force acting on the skyrmion for a quantitative modelling.

cond-mat.stat-mech

Imaging Topological Defect Dynamics Mediating 2D Skyrmion Lattice Melting

Topological defects are the key feature mediating 2D phase transitions. However, both resolution and tunability have been lacking to access the dynamics of the transitions. With dynamic Kerr microscopy, we directly capture the melting of a confined 2D magnetic skyrmion lattice with high resolution in real-time and -space. Skyrmions in magnetic thin films are two-dimensional, topologically non-trivial quasi-particles that provide rich dynamics as well as unique tunability as an essential ingredient for controlling phase behavior: We tune the skyrmion size and effective temperature on the fly to drive the two-step melting through an intermediate hexatic regime between the solid lattice and the isotropic liquid. We quantify the characteristic occurrence of topological defects mediating the transitions and reveal the so-far inaccessible dynamics of the lattice dislocations. The full real-time and -space imaging reveals the diffusion coefficient of the dislocations, which we find to be orders of magnitudes higher than that of the skyrmions.

cond-mat.stat-mech

Skyrmion flow in periodically modulated channels

Magnetic skyrmions, topologically stabilized chiral magnetic textures with particle-like properties have so far primarily been studied statically. Here, we experimentally investigate the dynamics of skyrmion ensembles in metallic thin film conduits where they behave as quasi-particle fluids. By exploiting our access to the full trajectories of all fluid particles by means of time-resolved magneto-optical Kerr microscopy, we demonstrate that boundary conditions of skyrmion fluids can be tuned by modulation of the channel geometry. We observe as a function of channel width deviations from classical flow profiles even into the no- or partial-slip regime. Unlike conventional colloids, the skyrmion Hall effect can also introduce transversal flow-asymmetries and even local motion of single skyrmions against the driving force which we explore with particle-based simulations, demonstrating the unique properties of skyrmion liquid flow that uniquely deviates from previously known behavior of other quasi-particles.

cond-mat.mes-hall

Coarse-graining collective skyrmion dynamics in confined geometries

Magnetic skyrmions are magnetic quasi-particles with enhanced stability and different manipulation mechanisms using external fields and currents making them promising candidates for future applications for instance in neuromorphic computing. Recently, several measurements and simulations have shown that thermally activated skyrmions in confined geometries, as they are necessary for device applications, arrange themselves predominantly based on commensurability effects. In this simulational study, based on the Thiele model, we investigate the enhanced dynamics and degenerate non-equilibrium steady state of a system in which the intrinsic skyrmion-skyrmion and skyrmion-boundary interaction compete with thermal fluctuations as well as current-induced spin-orbit torques. The investigated system is a triangular-shaped confinement geometry hosting four skyrmions, where we inject spin-polarized currents between two corners of the structure. We coarse-grain the skyrmion states in the system to analyze the intricacies of skyrmion arrangements of the skyrmion ensemble. In the context of neuromorphic computing, such methods address the key challenge of optimizing read-out positions in confined geometries and form the basis to understand collective skyrmion dynamics in systems with competing interactions on different scales.

cond-mat.mtrl-sci

Constructing coarse-grained skyrmion potentials from experimental data with Iterative Boltzmann Inversion

In an effort to understand skyrmion behavior on a coarse-grained level, skyrmions are often described as 2D quasi particles evolving according to the Thiele equation. Interaction potentials are the key missing parameters for predictive modeling of experiments. We apply the Iterative Boltzmann Inversion technique commonly used in soft matter simulations to construct potentials for skyrmion-skyrmion and skyrmion-magnetic material boundary interactions from a single experimental measurement without any prior assumptions of the potential form. We find that the two interactions are purely repulsive and can be described by an exponential function for experimentally relevant skyrmions. This captures the physics on experimental time and length scales that are of interest for most skyrmion applications and typically inaccessible to atomistic or micromagnetic simulations.

cond-mat.mtrl-sci

Brownian reservoir computing realized using geometrically confined skyrmions

Reservoir computing (RC) has been considered as one of the key computational principles beyond von-Neumann computing. Magnetic skyrmions, topological particle-like spin textures in magnetic films are particularly promising for implementing RC, since they respond strongly nonlinear to external stimuli and feature inherent multiscale dynamics. However, despite several theoretical proposals that exist for skyrmion reservoir computing, experimental realizations have been elusive until now. Here, we propose and experimentally demonstrate a conceptually new approach to skyrmion RC that leverages the thermally activated diffusive motion of skyrmions. By confining the electrically gated and thermal skyrmion motion, we find that already a single skyrmion in a confined geometry suffices to realize non-linearly separable functions, which we demonstrate for the XOR gate along with all other Boolean logic gate operations. Besides this universality, the reservoir computing concept ensures low training costs and ultra-low power operation with current densities orders of magnitude smaller than those used in existing spintronic reservoir computing demonstrations. Our proposed concept can be readily extended by linking multiple confined geometries and/or by including more skyrmions in the reservoir, suggesting high potential for scalable and low-energy reservoir computing.

cond-mat.mtrl-sci

Knot formation of dsDNA pushed inside a nanochannel

Recent experiments demonstrated that knots in single DNA strands can be formed by hydrodynamic compression in a nanochannel. In this letter, we further elucidate the underlying molecular mechanisms by carrying out a compression experiment in silico, where an equilibrated coarse-grained double-stranded DNA confined in a square channel is pushed by a piston. The probability of forming knots is a non-monotonic function of the persistence length and can be enhanced significantly by increasing the piston speed. Under compression, knots are abundant and delocalized due to a backfolding mechanism from which chain-spanning loops emerge, while knots are less frequent and only weakly localized in equilibrium. Our in silico study thus provides insights into the formation, origin and control of DNA knots in nanopores.

cond-mat.soft

Commensurability between element symmetry and the number of skyrmions governing skyrmion diffusion in confined geometries

Magnetic skyrmions are topological magnetic structures, which exhibit quasi-particle properties and can show enhanced stability against perturbation from thermal noise. Recently, thermal Brownian diffusion of these quasi-particles has been found in continuous films and applications in unconventional computing have received significant attention, which however require structured elements. Thus, as the next necessary step, we here study skyrmion diffusion in confined geometries and find it to be qualitatively different: The diffusion is governed by the interplay between the total number of skyrmions and the structure geometry. In particular, we ascertain the effect of circular and triangular geometrical confinement and find that for triangular geometries the behavior is drastically different for the cases when the number of skyrmions in the element is either commensurate or incommensurate with a symmetric filling of the element. This influence of commensurability is corroborated by simulations of a quasi-particle model.

cond-mat.mtrl-sci