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Jan Rothhardt

Publications and source records attributed to Jan Rothhardt.

24 records · Page 2Linked to original sources

High-precision calculations of the $1s^{2} 2s 2p$ $^1P_{1} \to 1s^{2} 2s^{2}$ $^1S_{0}$ spin-allowed $E1$ transition in C {\small III}

Large-scale relativistic calculations are performed for the transition energy and line strength of the $ 1s^{2} 2s 2p$ $^1P_{1} \,-\ 1s^{2} 2s^{2}$ $^1S_{0} $ transition in Be-like carbon. Based on the multiconfiguration Dirac-Hartree-Fock~(MCDHF) approach, different correlation models are developed to account for all major electron-electron correlation contributions. These correlation models are tested with various sets of the initial and the final state wave functions. The uncertainty of the predicted line strength due to missing correlation effects is estimated from the differences between the results obtained with those models. The finite nuclear mass effect is accurately calculated taking into account the energy, wave functions as well as operator contributions. As a result, a reliable theoretical benchmark of the $E1$ line strength is provided to support high precision lifetime measurement of the $ 1s^{2} 2s 2p$ $^1P_{1} $ state in Be-like carbon.

physics.atom-ph

Wavelength-scale ptychographic coherent diffractive imaging using a high-order harmonic source

Ptychography enables coherent diffractive imaging (CDI) of extended samples by raster scanning across the illuminating XUV/X-ray beam thereby generalizing the unique advantages of CDI techniques. Table-top realizations of this method are urgently needed for many applications in sciences and industry. Previously, it was only possible to image features much larger than the illuminating wavelength with table-top ptychography although knife-edge tests suggested sub-wavelength resolution. However, most real-world imaging applications require resolving of the smallest and closely-spaced features of a sample in an extended field of view. In this work, we resolve features as small as 2.5 λ(45 nm) by using a table-top ptychography setup and a high-order harmonic XUV source. For the first time, a Rayleigh-type criterion is used as a direct and unambiguous resolution metric for high-resolution table-top setup. This reliably qualifies this imaging system for real-world applications e.g. in biological sciences, material sciences, imaging integrated circuits and semiconductor mask inspection.

physics.optics

Table-Top Milliwatt-Class Extreme Ultraviolet High Harmonic Light Source

Extreme ultraviolet (XUV) lasers are essential for the investigation of fundamental physics. Especially high repetition rate, high photon flux sources are of major interest for reducing acquisition times and improving signal to noise ratios in a plethora of applications. Here, an XUV source based on cascaded frequency conversion is presented, which delivers due to the drastic better single atom response for short wavelength drivers, an average output power of (832 +- 204) μW at 21.7 eV. This is the highest average power produced by any HHG source in this spectral range surpassing precious demonstrations by more than a factor of four. Furthermore, a narrow-band harmonic at 26.6 eV with a relative energy bandwidth of only ΔE/E= 1.8 x 10E-3 has been generated, which is of high interest for high precision spectroscopy experiments.

physics.optics

High-repetition-rate and high-photon-flux 70 eV high-harmonic source for coincidence ion imaging of gas-phase molecules

Unraveling and controlling chemical dynamics requires techniques to image structural changes of molecules with femtosecond temporal and picometer spatial resolution. Ultrashort-pulse x-ray free-electron lasers have significantly advanced the field by enabling advanced pump-probe schemes. There is an increasing interest in using table-top photon sources enabled by high-harmonic generation of ultrashort-pulse lasers for such studies. We present a novel high-harmonic source driven by a 100 kHz fiber laser system, which delivers 10$^{11}$ photons/s in a single 1.3 eV bandwidth harmonic at 68.6 eV. The combination of record-high photon flux and high repetition rate paves the way for time-resolved studies of the dissociation dynamics of inner-shell ionized molecules in a coincidence detection scheme. First coincidence measurements on CH$_3$I are shown and it is outlined how the anticipated advancement of fiber laser technology and improved sample delivery will, in the next step, allow pump-probe studies of ultrafast molecular dynamics with table-top XUV-photon sources. These table-top sources can provide significantly higher repetition rates than the currently operating free-electron lasers and they offer very high temporal resolution due to the intrinsically small timing jitter between pump and probe pulses.

physics.atom-ph

High photon flux table-top coherent extreme ultraviolet source

High harmonic generation (HHG) enables extreme ultraviolet radiation with table-top setups. Its exceptional properties, such as coherence and (sub)-femtosecond pulse durations, have led to a diversity of applications. Some of these require a high photon flux and megahertz repetition rates, e.g. to avoid space charge effects in photoelectron spectroscopy. To date this has only been achieved with enhancement cavities. Here, we establish a novel route towards powerful HHG sources. By achieving phase-matched HHG of a megahertz fibre laser we generate a broad plateau (25 eV - 40 eV) of strong harmonics, each containing more than $10^{12}$ photons/s, which constitutes an increase by more than one order of magnitude in that wavelength range. The strongest harmonic (H25, 30 eV) has an average power of 143 $μ$W ($3\cdot10^{13}$ photons/s). This concept will greatly advance and facilitate applications in photoelectron or coincidence spectroscopy, coherent diffractive imaging or (multidimensional) surface science.

physics.optics

Enhancing narrowband high order harmonic generation by Fano resonances

Resonances in the photo-absorption spectrum of the generating medium can modify the spectrum of high order harmonics. In particular, window-type Fano resonances can reduce photo-absorption within a narrow spectral region and, consequently, lead to an enhanced emission of high-order harmonics in absorption-limited generation conditions. For high harmonic generation in argon it is shown that the 3s3p6 np 1P1 window resonances (n=4,5,6) give rise to enhanced photon yield. In particular, the 3s3p6 4p 1P1 resonance at 26.6 eV allows a relative enhancement up to a factor of 30 compared to the characteristic photon emission of the neighboring harmonic order. This enhanced, spectrally isolated and coherent photon emission line has a relative energy bandwidth of only ΔE/E=3*10-3. Therefore, it might be directly applied for precision spectroscopy or coherent diffractive imaging without the need of additional spectral filtering. The presented mechanism can be employed for tailoring and controlling the high harmonic emission of manifold target materials.

physics.optics