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Jared Z. Dans

Publications and source records attributed to Jared Z. Dans.

4 recordsLinked to original sources

Single crystal growth, structural and magnetic properties of CeZn$_{2-x}$Ga$_{2+x}$

The tetragonal BaAl$_4$ ($I4/mmm$) parent structure underpins a diverse family of materials exhibiting novel phenomena, including nematic superconductivity, topological semimetallicity, and heavy fermion behavior. The recent growth of ternary R-Zn-Ga compounds, such as the previously reported CeZn$_2$Ga$_2$, has explored some of the members exhibiting rare-earth magnetism within this family. In this paper, we report on the structural and magnetic properties of single crystals of CeZn$_{2-x}$Ga$_{2+x}$, a Ga-rich analogue of CeZn$_2$Ga$_2$. Our CeZn$_{2-x}$Ga$_{2+x}$ samples exhibit magnetic properties distinct from the paramagnetic behavior previously reported for CeZn$_2$Ga$_2$. We observe a magnetic transition around 4 K, pronounced metamagnetic states at low temperatures, and strong magnetic anisotropy. Though there are batch-to-batch variations that suggest a strong sensitivity to local structural imperfections, we consistently see the presence of magnetic transitions and metamagnetic states in our crystals. To investigate the local structural sensitivity hypothesis, we performed Reverse Monte Carlo analysis of collected powder neutron diffraction data, revealing the presence of significant local crystallographic disorder of the magnetic Ce site. Our findings demonstrate that the positional disorder drives competing ferromagnetic and antiferromagnetic correlations that lead to the observed spin glass behavior and complex anisotropic magnetism. This study illustrates that tuning the local crystallographic disorder enables engineering frustrated magnetic states in BaAl$_4$-type and similar intermetallic structures.

cond-mat.str-el

Resilient $j$=3/2 superconductivity in topological semimetal YPtBi

Cooper pairing in most of the known fermionic superfluids occurs via spin-1/2 quasiparticle interactions that lead to spin-singlet or spin-triplet pairing. In the topological semimetal YPtBi, strong spin-orbit coupling results in a band inversion between highly symmetric $s$- and $p$-like electronic bands and a degeneracy at the $Γ$ point that ensures the manifold of $j$=3/2 quasiparticle states thrive near the Fermi level, where superconducting pairing occurs. Here we study the effects of magnetic and nonmagnetic disorder and carrier density on this exotic superconducting pairing state. By varying levels of disorder and carrier densities by nearly two and three orders of magnitude, respectively, we show that the superconducting critical temperature of YPtBi has a remarkable robustness, with little variation across this span. Our results suggest that superconductivity in YPtBi may reside in a regime where phase stiffness, rather than pair formation, governs the transition temperature. The insensitivity of Cooper pairing to dramatic changes in quasiparticle environment in a $j$=3/2 superconductor highlights a new form of protection realized in topological high-spin superconductors.

cond-mat.supr-con

Non-Fermi liquid behavior in La$_3$Ni$_2$O$_7$ thin films under hydrostatic pressure

The discovery of superconductivity in bilayer nickel-oxides has revived an intense effort to understand the potential of high-temperature superconductivity in these materials and their relation to cuprate superconductors. In this work, we investigate the growth and properties of bilayer La$_3$Ni$_2$O$_7$ thin films as a function of substrate, oxygen treatment and applied pressure in order to study the evolution of transport properties. We report epitaxial growth of La$_3$Ni$_2$O$_7$ thin films on LaAlO$_3$ (LAO) (001) and SrLaAlO$_4$ (SLAO) (001) substrates, and the effects of ex-situ annealing in a high pressure furnace under an oxygen-rich environment. Transport measurements show that the La$_3$Ni$_2$O$_7$ thin films on LAO(001) exhibit Fermi liquid-like metallic behavior with a slight Kondo-like upturn at low temperatures, which evolves with the application of modest hydrostatic pressures toward non-Fermi liquid behavior with a temperature dependence of resistance approaching $\sim$ T$^{1.4}$ at 1.41 GPa. The ability to tune the normal state resistivity of La$_3$Ni$_2$O$_7$ films to display non-Fermi liquid behavior under such a modest hydrostatic pressure range - only 6 - 8 % of that typically applied via diamond anvil cell (DAC) in La$_3$Ni$_2$O$_7$ single crystals to achieve comparable effects - is both noteworthy and unexpected. These findings imply the strong tunability of La$_3$Ni$_2$O$_7$ in thin film form and the likely proximity of a strongly fluctuating ordered state leading to non-Fermi liquid behavior under even modest applied pressures.

cond-mat.str-el

Quantum Oscillations and Superconductivity in YPtBi Under Pressure

The topological semimetal YPtBi has attracted considerable attention, owing to its novel superconducting and normal state properties. A strong band inversion from spin-orbit coupling allows the existence of $j=3/2$ quasiparticles near the Fermi level, which form Cooper pairs with angular momentum potentially higher than single or triplet states. In this report, we present high-pressure magnetotransport and Shubnikov-de Haas effect measurements on high-quality YPtBi up to $P = 2.08$ GPa. As a function of pressure, we observe a trend toward more insulating resistivity at low temperatures concomitant with a suppression of quantum oscillation amplitude. Together with a decrease of the upper critical field and significant increase in the Dingle temperature, the pressure-induced changes point to a weakening of the band inversion and potential tuning of the topological nature of YPtBi, suggesting pressure as a useful tool for understanding the nature of topology in other related half-Heusler compounds.

cond-mat.supr-con