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Jason Boynewicz

Publications and source records attributed to Jason Boynewicz.

3 recordsLinked to original sources

Brownian motion: non-equilibrium states from equilibrium trajectories -- recovering hydrodynamic regimes from prepared displacement measurements

Owing to the Chapman-Kolmogorov equation for Markovian dynamics,any equilibrium trajectory of a Brownian particle in a solvent fluid can be viewed as the superposition of an uncountable number of non-equilibrium states. This property permits the unraveling of fine details of fluid-particle interactions at microscales defined by its non-equilibrium properties from the analysis of a single Brownian trajectory and to connect them to the hydrodynamics of the solvent fluid, simply considering the lower-order (second) moments of particle position in trapped conditions. In this way, the acceleration due to thermal-hydrodynamic fluctuational forces is isolated from the other factors and the short-time displacement statistics is completely determined by the correlation properties of the fluctuational thermal-hydrodynamic force. This approach not only confirms the $t^{5/2}$-law obtained by Boynewicz et al. (2026), related to fluid inertial effects, but indicates that this scaling may be superseded by a $t^4$-scaling at very short times once the correlated nature of the stochastic forcings is taken into account. The latter result is related to the regularity properties of particle velocity realizations.

cond-mat.stat-mech

The fractal dimension of Brownian dynamics in liquids

The classical Einstein-Langevin theory of Brownian motion assumes a memoryless thermal bath, establishing a universal fractal dimension of $d_v = 3/2$ for the velocity fluctuations of a particle. In this Letter, we demonstrate experimentally and theoretically that fluid-inertial memory effects fundamentally redefine the fractal scaling of these fluctuations. In analyzing highly resolved measurements of Brownian microspheres in liquids, we show that the non-Markovian hydrodynamic thermal noise establishes a distinct velocity fractal dimension of $d_v = 7/4$. Coupled with theoretical analysis of non-equilibrium short-time dynamics and the initial scaling of the velocity autocorrelation function, this result establishes the non-equilibrium universality class of Brownian motion in fluid media possessing a finite non-vanishing density.

cond-mat.stat-mech

Observation of Super-ballistic Brownian Motion in Liquid

Brownian motion is a foundational physical process characterized by a mean squared displacement that scales linearly in time in thermal equilibrium, known as diffusion. At short times, the mean squared displacement becomes ballistic, scaling as t^2. This effect was predicted by Einstein in 1907 and recently observed experimentally. We report that this picture is only true on average; by conditioning specific initial velocities, we predict theoretically and confirm by experiment that the mean squared displacement becomes super-ballistic, with a power scaling law of t^(5/2). This result is due to the colored noise of incompressible fluids, resulting in a non-zero first moment for the thermal force when conditioned on non-zero initial velocities. These results are a step towards the unraveling of nonequilibrium dynamics of fluids.

cond-mat.stat-mech