arXiv subjects

Jason H. V. Nguyen

Publications and source records attributed to Jason H. V. Nguyen.

8 recordsLinked to original sources

arXiv2021

Optimizing Electronic Structure Simulations on a Trapped-ion Quantum Computer using Problem Decomposition

Quantum computers have the potential to advance material design and drug discovery by performing costly electronic structure calculations. A critical aspect of this application requires optimizing the limited resources of the quantum hardware. Here, we experimentally demonstrate an end-to-end pipeline that focuses on minimizing quantum resources while maintaining accuracy. Using density matrix embedding theory as a problem decomposition technique, and an ion-trap quantum computer, we simulate a ring of 10 hydrogen atoms without freezing any electrons. The originally 20-qubit system is decomposed into 10 two-qubit problems, making it amenable to currently available hardware. Combining this decomposition with a qubit coupled cluster circuit ansatz, circuit optimization, and density matrix purification, we accurately reproduce the potential energy curve in agreement with the full configuration interaction energy in the minimal basis set. Our experimental results are an early demonstration of the potential for problem decomposition to accurately simulate large molecules on quantum hardware.

quant-ph↗

arXiv2020

Generalized Hamiltonian to describe imperfections in ion-light interaction

We derive a general Hamiltonian that governs the interaction between an $N$-ion chain and an externally controlled laser field, where the ion motion is quantized and the laser field is considered beyond the plane-wave approximation. This general form not only explicitly includes terms that are used to drive ion-ion entanglement, but also a series of unwanted terms that can lead to quantum gate infidelity. We demonstrate the power of our expressivity of the general Hamiltonian by singling out the effect of axial mode heating and confirm this experimentally. We discuss pathways forward in furthering the trapped-ion quantum computational quality, guiding hardware design decisions.

quant-ph↗

arXiv2020

Creation and Characterization of Matter-Wave Breathers

We report the creation of quasi-1D excited matter-wave solitons, "breathers", by quenching the strength of the interactions in a Bose-Einstein condensate with attractive interactions. We characterize the resulting breathing dynamics and quantify the effects of the aspect ratio of the confining potential, the strength of the quench, and the proximity of the 1D-3D crossover for the 2-soliton breather. We furthermore demonstrate the complex dynamics of a 3-soliton breather created by a stronger interaction quench. Our experimental results, which compare well with numerical simulations, provide a pathway for utilizing matter-wave breathers to explore quantum effects in large many-body systems.

cond-mat.quant-gas↗

arXiv2020

Methods for Preparing Quantum Gases of Lithium

Lithium is an important element in atomic quantum gas experiments because its interactions are highly tunable, due to broad Feshbach resonances and zero-crossings, and because it has two stable isotopes, $^6$Li, a fermion, and $^7$Li, a boson. Although lithium has special value for these reasons, it also presents experimental challenges. In this article, we review some of the methods that have been developed or adapted to confront these challenges, including beam and vapor sources, Zeeman slowers, sub-Doppler laser cooling, laser sources at 671 nm, and all-optical methods for trapping and cooling. Additionally, we provide spectral diagrams of both $^6$Li and $^7$Li, and present plots of Feshbach resonances for both isotopes.

physics.atom-ph↗

arXiv2017

Formation of matter-wave soliton trains by modulational instability

Nonlinear systems can exhibit a rich set of dynamics that are inherently sensitive to their initial conditions. One such example is modulational instability, which is believed to be one of the most prevalent instabilities in nature. By exploiting a shallow zero-crossing of a Feshbach resonance, we characterize modulational instability and its role in the formation of matter-wave soliton trains from a Bose-Einstein condensate. We examine the universal scaling laws exhibited by the system, and through real-time imaging, address a long-standing question of whether the solitons in trains are created with effectively repulsive nearest neighbor interactions, or rather, evolve into such a structure.

cond-mat.quant-gas↗

arXiv2015

Broadband optical cooling of molecular rotors from room temperature to the ground state

Laser cycling of resonances can remove entropy from a system via spontaneously emitted photons, with electronic resonances providing the fastest cooling timescales because of their rapid relaxation rates. Although atoms are routinely laser cooled, even simple molecules pose two interrelated challenges for cooling: every populated rotational-vibrational state requires a different laser frequency, and electronic relaxation generally excites vibrations. Here, we cool trapped AlH+ molecules to their ground rotational-vibrational quantum state using an electronically-exciting broadband laser to simultaneously drive cooling resonances from many different rotational levels. Undesired vibrational excitation is avoided because of vibrational-electronic decoupling in AlH+. We demonstrate rotational cooling on the 140(20) ms timescale from room temperature to 3.8(+0.9/-0.3) K, with the ground state population increasing from ~3% to 95.4(+1.3/-2.0) %. This cooling technique could be applied to several other neutral and charged molecular species useful for quantum information processing, ultracold chemistry applications, and precision tests of fundamental symmetries.

physics.atom-ph↗

arXiv2014

Collisions of matter-wave solitons

Solitons are localised wave disturbances that propagate without changing shape, a result of a nonlinear interaction which compensates for wave packet dispersion. Individual solitons may collide, but a defining feature is that they pass through one another and emerge from the collision unaltered in shape, amplitude, or velocity. This remarkable property is mathematically a consequence of the underlying integrability of the one-dimensional (1D) equations, such as the nonlinear Schrödinger equation, that describe solitons in a variety of wave contexts, including matter-waves$^{1,2}$. Here we explore the nature of soliton collisions using Bose-Einstein condensates of atoms with attractive interactions confined to a quasi-one-dimensional waveguide. We show by real-time imaging that a collision between solitons is a complex event that differs markedly depending on the relative phase between the solitons. Yet, they emerge from the collision unaltered in shape or amplitude, but with a new trajectory reflecting a discontinuous jump. By controlling the strength of the nonlinearity we shed new light on these fundamental features of soliton collisional dynamics, and explore the implications of collisions that bring the wave packets out of the realm of integrability, where they may undergo catastrophic collapse. 1. Zabusky, N.J. & Kruskal, M.D. Interaction of "solitons" in a collisionless plasma and the recurrence of initial states. Phys. Rev. Lett. 15, 240 (1965). 2. Zakharov, V.E. & Shabat, A.B. Exact theory of two-dimensional self-focusing and one-dimensional self-moduation of waves in nonlinear media. Sov. Phys. JEPT. 34, 62 (1972).

cond-mat.quant-gas↗

arXiv2011

Challenges of laser-cooling molecular ions

The direct laser cooling of neutral diatomic molecules in molecular beams suggests that trapped molecular ions can also be laser cooled. The long storage time and spatial localization of trapped molecular ions provides the opportunity for multi-step cooling strategies, but also requires a careful consideration of rare molecular transitions. We briefly summarize the requirements that a diatomic molecule must meet for laser cooling, and we identify a few potential molecular ion candidates. We then perform a detailed computational study of the candidates BH+ and AlH+, including improved ab initio calculations of the electronic state potential energy surfaces and transition rates for rare dissociation events. Based on an analysis of population dynamics, we determine which transitions must be addressed for laser cooling and compare experimental schemes using continuous-wave and pulsed lasers

physics.atom-ph↗