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Jason W. A. Robinson

Publications and source records attributed to Jason W. A. Robinson.

At least 19 recordsLinked to original sources

Competing magnetic states in a non-coplanar Kagome magnet

Non-collinear Kagome antiferromagnets (AFMs) Mn3X (X = Sn, Ga, Ge, Ir, Pt) can generate an anomalous Hall effect (AHE) despite vanishing net magnetization, enabled by broken time-reversal and inversion symmetries. However, strong in-plane anisotropy has limited studies of the AFM-AHE and electronic applications to coplanar spin configurations. Non-coplanar spin textures in these systems have been realized only in low temperature spin-glass states or at interfaces with heavy metals. Here, we report an intrinsic non-coplanar spin configuration persisting up to 400 K in cubic-phase Mn3Ge, originating from coexisting symmetric and antisymmetric exchange interactions. Competing magnetic states associated with this non-coplanar spin configuration give rise to an unconventional AHE with a magnetic-field-induced sign reversal and a hump-like feature. Our findings establish a platform for non-coplanar magnetism in AFM spintronics.

cond-mat.mtrl-sci↗

Weak-anti-localization-to-spin-dependent scattering at a proximity-magnetized heavy metal interface

A change in a materials electrical resistance with magnetic field (magnetoresistance) results from quantum interference effects and, or spin-dependent transport, depending on materials properties and dimensionality. In disordered conductors, electron interference leads to weak localization or anti-localization; in contrast, ferromagnetic conductors support spin-dependent scattering, leading to giant magnetoresistance (GMR). By varying the thickness of Au between 4 and 28 nm in a EuS/Au/EuS spin-switches, we observe a crossover from weak anti-localization to interfacial GMR. The crossover is related to a magnetic proximity effect in Au due to electron scattering at the insulating EuS interface. The proximity-induced exchange field in Au suppresses weak anti-localization, consistent with Maekawa-Fukuyama theory. With increasing Au thickness, GMR emerges along with spin Hall magnetoresistance. These findings demonstrate spin transport governed by interfacial exchange fields, building a framework for spintronic functionality without metallic magnetism.

cond-mat.mtrl-sci↗

Interfacial spin-orbit-coupling-induced strong spin-to-charge conversion at an all-oxide ferromagnetic /quasi-two-dimensional electron gas interface

Functional oxides and hybrid structures with interfacial spin orbit coupling and the Rashba-Edelsterin effect (REE) are promising materials systems for thermal tolerance spintronic device applications. Here, we demonstrate efficient spin-to-charge conversion through enhanced interfacial spin orbit coupling at the all-oxide interface of La1-xCaxMnO3 with quasi-two-dimensional (quasi-2D) SrTiO3 (LCMO/STO). The quasi-2D interface is generated via oxygen vacancies at the STO surface. We obtain a spin-to-charge conversion efficiency of ~ 2.32 +- 1.3 nm, most likely originating from the inverse REE, which is relatively large versus all-metallic spin-to-charge conversion materials systems. The results highlight that the LCMO/STO 2D electron gas is a potential platform for spin-based memory and transistor applications.

cond-mat.mes-hall↗

Colloquium: Spin-orbit effects in superconducting hybrid structures

Spin-orbit coupling (SOC) relates to the interaction between an electron's motion and its spin, and is ubiquitous in solid-state systems. Although the effect of SOC in normal-state phenomena has been extensively studied, its role in superconducting hybrid structures and devices opens many unexplored questions. In conjunction with broken symmetries and material inhomogeneities within superconducting hybrid structures, SOC may have additional contributions, beyond its effects in homogenous materials. Remarkably, even with well-established magnetic or nonmagnetic materials and conventional s-wave spin-singlet superconductors, SOC leads to emergent phenomena including equal-spin triplet pairing and topological superconductivity (hosting Majorana states), a modified current-phase relationship in Josephson junctions, and nonreciprocal transport. SOC is also responsible for transforming quasiparticles in superconducting structures which enhances the spin Hall effect and changes spin dynamics. Taken together, SOC in superconducting hybrid structures and the potential for electric tuning of the SOC strength, creates fascinating possibilities to advance superconducting spintronic devices for energy-efficient computing, and enable topological fault-tolerant quantum computing. By providing a description of experimental techniques and theoretical methods to study SOC, this Colloquium describes the current understanding of resulting phenomena in superconducting structures and offers a framework to select and design a growing class of materials systems where SOC plays an important role.

cond-mat.supr-con↗

Realisation of de Gennes$'$ Absolute Superconducting Switch with a Heavy Metal Interface

In 1966, Pierre-Gilles de Gennes proposed a non-volatile mechanism for switching superconductivity on and off in a magnetic device. This involved a superconductor (S) sandwiched between ferromagnetic (F) insulators in which the net magnetic exchange field could be controlled through the magnetisation-orientation of the F layers. Because superconducting switches are attractive for a range of applications, extensive studies have been carried out on $F/S/F$ structures. Although these have demonstrated a sensitivity of the superconducting critical temperature ($T_{c}$) to parallel (P) and antiparallel (AP) magnetisation-orientations of the F layers, corresponding shifts in $T_c$ (i.e., $ΔT_c = T_{c,AP} - T_{c,P}$) are lower than predicted with $ΔT_c$ only a small fraction of $T_{c,AP}$, precluding the development of applications. Here, we report $EuS/Au/Nb/EuS$ structures where EuS is an insulating ferromagnet, Nb is a superconductor and Au is a heavy metal. For P magnetisations, the superconducting state in this structure is quenched down to the lowest measured temperature of 20 mK meaning that $ΔT_c/T_{c,AP}$ is practically 1. The key to this so-called absolute switching effect is a sizable spin-mixing conductance at the $EuS/Au$ interface which ensures a robust magnetic proximity effect, unlocking the potential of $F/S/F$ switches for low power electronics.

cond-mat.supr-con↗

Enhanced controllable triplet proximity effect in superconducting spin-orbit coupled spin valves with modified superconductor/ferromagnet interfaces

In a superconductor/ferromagnet hybrid, a magnetically controlled singlet-to-triplet Cooper pair conversion can modulate the superconducting critical temperature. In these triplet superconducting spin valves, such control usually requires inhomogeneous magnetism. However, in the presence of spin-orbit coupling from an interfacial heavy-metal layer, the singlet/triplet conversion rate and thus the critical temperature, can be controlled via the magnetization direction of a single homogeneous ferromagnet. Here, we report significantly enhanced controllable pair conversion to a triplet state in a Nb/Pt/Co/Pt superconducting spin valve in which Pt/Co/Pt is homogeneously magnetized and proximity-coupled to a superconducting layer of Nb. The Co/Pt interface furthest away from Nb is modified by a sub-nanometer-thick layer of Cu or Au. We argue that the enhancement is most likely associated from an improvement of the Co/Pt interface due to the insertion of Cu and Au layers. Additionally, the higher normalized orbital moments in Au measured using X-ray magnetic circular dichroism shows that increasing spin-orbit coupling enhances the triplet proximity effect - an observation supported by our theoretical calculations. Our results provide a pathway to enhancing triplet pair creation by interface engineering for device development in superspintronics.

cond-mat.supr-con↗

Unveiling unconventional magnetism at the surface of Sr$_2$RuO$_4$

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered oxide perovskite Sr$_2$RuO$_4$ is a strongly correlated electron material that has been intensively investigated since its discovery due to its unusual physical properties. Whilst recent experiments have reopened the debate on the exact symmetry of the superconducting state in Sr$_2$RuO$_4$, a deeper understanding of the Sr$_2$RuO$_4$ normal state appears crucial as this is the background in which electron pairing occurs. Here, by using low-energy muon spin spectroscopy we discover the existence of magnetism at the surface of Sr$_2$RuO$_4$ in its normal state. We detect static weak dipolar fields yet manifesting below a relatively high onset temperature larger than 50 K, which reveals the unconventional nature of the observed magnetism. We relate the origin of this phase breaking time reversal symmetry to electronic ordering in the form of orbital loop currents that originate at the reconstructed Sr$_2$RuO$_4$ surface. Our observations set a reference for the discovery of the same magnetic phase in other materials and unveil an electronic ordering mechanism that can influence unconventional electron pairing with broken time reversal symmetry in those materials where the observed magnetic phase coexists with superconductivity.

cond-mat.str-el↗

Quantized conductance in split gate superconducting quantum point contacts with InGaAs semiconducting two-dimensional electron systems

Quantum point contact or QPC -- a constriction in a semiconducting two-dimensional (2D) electron system with a quantized conductance -- has been found as the building block of novel spintronic, and topological electronic circuits. They can also be used as readout electronic, charge sensor or switch in quantum nanocircuits. A short and impurity-free constriction with superconducting contacts is a Cooper pairs QPC analogue known as superconducting quantum point contact (SQPC). The technological development of such quantum devices has been prolonged due to the challenges of maintaining their geometrical requirement and near-unity superconductor-semiconductor interface transparency. Here, we develop advanced nanofabrication, material and device engineering techniques and report on an innovative realisation of nanoscale SQPC arrays with split gate technology in semiconducting 2D electron systems, exploiting the special gate tunability of the quantum wells, and report the first experimental observation of conductance quantization in hybrid InGaAs-Nb SQPCs. We observe reproducible quantized conductance at zero magnetic fields in multiple quantum nanodevices fabricated in a single chip and systematically investigate the quantum transport of SQPCs at low and high magnetic fields for their potential applications in quantum metrology, for extremely accurate voltage standards, and fault-tolerant quantum technologies.

quant-ph↗

Direct Observation of a Superconducting Vortex Diode

The interplay between magnetism and superconductivity can lead to unconventional proximity and Josephson effects. A related phenomenon that has recently attracted considerable attention is the superconducting diode effect, in which a non-reciprocal critical current emerges. Although superconducting diodes based on superconducting/ferromagnetic (S/F) bilayers were demonstrated more than a decade ago, the precise underlying mechanism remains unclear. While not formally linked to this effect, the Fulde-Ferrell-Larkin-Ovchinikov (FFLO) state is a plausible mechanism, due to the 2-fold rotational symmetry breaking caused by the finite center-of-mass-momentum of the Cooper pairs. Here, we directly observe, for the first time, a tunable superconducting vortex diode in Nb/EuS (S/F) bilayers. Based on our nanoscale SQUID-on-tip (SOT) microscope and supported by in-situ transport measurements, we propose a theoretical model that captures our key results. Thus, we determine the origin for the vortex diode effect, which builds a foundation for new device concepts.

cond-mat.supr-con↗

Multiple Andreev reflections in two-dimensional Josephson junctions with broken time-reversal symmetry

Andreev bound states (ABS) occur in Josephson junctions when the total phase of the Andreev and normal reflections is a multiple of $2π$. In ballistic junctions with an applied voltage bias, a quasi-particle undergoes multiple Andreev reflections before entering the leads, resulting in peaks in the current-voltage $I(V)$ curve. Here we present a general model for Josephson junctions with spin-active interlayers i.e., magnetic or topological materials with broken time-reversal symmetry. We investigate how ABS change the peak positions and shape of $I(V)$, which becomes asymmetric for a single incident angle. We show how the angle-resolved $I(V)$ curve becomes a spectroscopic tool for the chirality and degeneracy of ABS.

cond-mat.supr-con↗

Nodal superconducting exchange coupling

The superconducting equivalent of giant magnetoresistance, involves placing a thin-film superconductor between two ferromagnetic layers. A change of magnetization-alignment in such a superconducting spin-valve from parallel (P) to antiparallel (AP) creates a positive shift in the superconducting transition temperature (ΔTc) due to an interplay of the magnetic exchange energy and the superconducting condensate. The magnitude of ΔTc scales inversely with the superconductor thickness (dS) and is zero when dS exceeds the superconducting coherence length (ξ) as predicted by de Gennes. Here, we report a superconducting spin-valve effect involving a different underlying mechanism that goes beyond de Gennes in which magnetization-alignment and ΔTc are determined by the nodal quasiparticle-excitation states on the Fermi surface of the d-wave superconductor YBa2Cu3O7-δ (YBCO) grown between insulating layers of ferromagnetic Pr0.8Ca0.2MnO3. We observe ΔTc values that approach 2 K with ΔTc oscillating with dS over a length scale exceeding 100 ξ and, for particular values of dS, we find that the superconducting state reinforces an antiparallel magnetization-alignment. These results pave the way for all-oxide superconducting memory in which superconductivity modulates the magnetic state.

cond-mat.supr-con↗

Quantum Dot-Based Parametric Amplifiers

Josephson parametric amplifiers (JPAs) approaching quantum-limited noise performance have been instrumental in enabling high fidelity readout of superconducting qubits and, recently, semiconductor quantum dots (QDs). We propose that the quantum capacitance arising in electronic two-level systems (the dual of Josephson inductance) can provide an alternative dissipation-less non-linear element for parametric amplification. We experimentally demonstrate phase-sensitive parametric amplification using a QD-reservoir electron transition in a CMOS nanowire split-gate transistor embedded in a 1.8~GHz superconducting lumped-element microwave cavity, achieving parametric gains of -3 to +3 dB, limited by Sisyphus dissipation. Using a semi-classical model, we find an optimised design within current technological capabilities could achieve gains and bandwidths comparable to JPAs, while providing complementary specifications with respect to integration in semiconductor platforms or operation at higher magnetic fields.

cond-mat.mes-hall↗

Non-reciprocal Pauli Spin Blockade in a Silicon Double Quantum Dot

Spin qubits in gate-defined silicon quantum dots are receiving increased attention thanks to their potential for large-scale quantum computing. Readout of such spin qubits is done most accurately and scalably via Pauli spin blockade (PSB), however various mechanisms may lift PSB and complicate readout. In this work, we present an experimental observation of a new, highly prevalent PSB-lifting mechanism in a silicon double quantum dot due to incoherent tunneling between different spin manifolds. Through dispersively-detected magnetospectroscopy of the double quantum dot in 16 charge configurations, we find the mechanism to be energy-level selective and non-reciprocal for neighbouring charge configurations. Additionally, using input-output theory we report a large coupling of different electron spin manifolds of 7.90 $μ$eV, the largest reported to date, indicating an enhanced spin-orbit coupling which may enable all-electrical qubit control.

cond-mat.mes-hall↗

A Review of Electronic Transport in Superconducting Sr$_2$RuO$_4$ Junctions

We review electronic transport in superconducting junctions with Sr$_2$RuO$_4$. Transport measurements provide evidence for chiral domain walls and, therefore, chiral superconductivity in superconducting Sr$_2$RuO$_4$, but so far, the symmetry of the underlying superconducting state remains inconclusive. Further studies involving density of states measurements and spin-polarised transport in local/non--local Sr$_2$RuO$_4$ junctions with magnetic materials could lead to fundamental discoveries and a better understanding of the superconducting state.

cond-mat.supr-con↗

Controllable enhancement of $p$-wave superconductivity via magnetic coupling to a conventional superconductor

Unconventional superconductors are of high interest due to their rich physics, a topical example being topological edge-states associated with $p$-wave superconductivity. A practical obstacle in studying such systems is the very low critical temperature $T_\text{c}$ that is required to realize a $p$-wave superconducting phase in a material. We predict that the $T_\text{c}$ of an intrinsic $p$-wave superconductor can be significantly enhanced by coupling it via an atomically thin ferromagnetic layer (F) to a conventional $s$-wave or a $d$-wave superconductor with a higher critical temperature. We show that this $T_\text{c}$-boost is tunable via the direction of the magnetization in F. Moreover, we show that the enhancement in $T_\text{c}$ can also be achieved using the Zeeman-effect of an external magnetic field. Our findings provide a way to increase $T_\text{c}$ in $p$-wave superconductors in a controllable way and make the exotic physics associated with such materials more easily accessible experimentally.

cond-mat.supr-con↗

Large dispersive interaction between a CMOS double quantum dot and microwave photons

We report fast charge state readout of a double quantum dot in a CMOS split-gate silicon nanowire transistor via the large dispersive interaction with microwave photons in a lumped-element resonator formed by hybrid integration with a superconducting inductor. We achieve a coupling rate $g_0/(2π) = 204 \pm 2$ MHz by exploiting the large interdot gate lever arm of an asymmetric split-gate device, $α=0.72$, and by inductively coupling to the resonator to increase its impedance, $Z_\text{r}=560~Ω$. In the dispersive regime, the large coupling strength at the double quantum dot hybridisation point produces a frequency shift comparable to the resonator linewidth, the optimal setting for maximum state visibility. We exploit this regime to demonstrate rapid dispersive readout of the charge degree of freedom, with a SNR of 3.3 in 50 ns. In the resonant regime, the fast charge decoherence rate precludes reaching the strong coupling regime, but we show a clear route to spin-photon circuit quantum electrodynamics using hybrid CMOS systems.

cond-mat.mes-hall↗

Boosting spintronics with superconductivity

Spintronics aims to utilize the spin degree of freedom for energy-efficient, non-volatile memory and logic devices. In this research update, we review state-of-the-art developments and new directions in charge- and spin-based memory/logic with a focus on spintronics and the fascinating potential for superconductivity to boost spin transmission via spin-polarized quasiparticles or triplet Cooper pairs.

cond-mat.supr-con↗

Thermal annealing enhancement of Josephson critical currents in ferromagnetic CoFeB

The electrical and structural properties of Co40Fe40B20 (CoFeB) alloy are tunable with thermal annealing. This is key in the optimization of CoFeB-based spintronic devices, where the advantageously low magnetic coercivity, high spin polarization, and controllable magnetocrystalline anisotropy are utilised. So far, there has been no report on superconducting devices based on CoFeB. Here, we report Nb/CoFeB/Nb Josephson devices and demonstrate an enhancement of the critical current by up to 700% following thermal annealing due to increased structural ordering of the CoFeB. The results demonstrate that CoFeB is a promising material for the development of superconducting spintronic devices.

cond-mat.supr-con↗