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Jasper van Wezel

Publications and source records attributed to Jasper van Wezel.

At least 91 records · Page 5Linked to original sources
arXiv2012

Polar charge and orbital order in 2H-TaS2

It was recently discovered that in spite of the scalar nature of its order parameter, the charge order in 1T-TiSe2 can be chiral. This is made possible by the emergence of orbital order in conjunction with the charge density modulations. Here we show that a closely related charge and orbital ordered state arises in 2H-TaS2. In both materials, the microscopic mechanism driving the transition is based on the interaction between three differently polarized displacement waves. The relative phase shifts between these waves lead both to the formation of orbital order and to the breakdown of inversion symmetry. In contrast to 1T-TiSe2 however, the presence of a mirror plane in the lattice of 2H-TaS2 prevents the distorted structure in this material from being chiral, and a polar charge and orbital ordered state arises instead. It is stressed that bulk experiments are indispensable in differentiating between the chiral and polar phases.

cond-mat.str-el↗
arXiv2011

Resolving magnetic frustration in a pyrochlore lattice

CeFe$_2$ is a geometrically frustrated ferromagnet that lies close to an instability at which a subtle change in the lattice symmetry couples to a transition to antiferromagnetism. We use x-ray diffraction, diamond-anvil-cell techniques, and numerical simulation to identify the ground states and to quantitatively illustrate effects of competing magnetic energy scales and geometrical frustration on the magnetic phase diagram. Comparison of phase transitions under both chemical substitution and applied pressure suggests a general solution to the physics of pyrochlore rare earth inter-metallic magnets.

cond-mat.str-el↗
arXiv2011

A Nanoscale Experiment Measuring Gravity's Role in Breaking the Unitarity of Quantum Dynamics

Modern, state of the art nanomechanical devices are capable of creating spatial superpositions that are massive enough to begin to experimentally access the quantum to classical crossover, and thus force us to consider the possible ways in which the usual quantum dynamics may be affected. One recent theoretical proposal describes the crossover from unitary quantum mechanics to classical dynamics as a form of spontaneous symmetry breaking. Here, we propose a specific experimental setup capable of identifying the source of unitarity breaking in such a mechanism. The experiment is aimed specifically at clarifying the role played by gravity, and distinguishes the resulting dynamics from that suggested by alternative scenarios for the quantum to classical crossover. We give both a theoretical description of the expected dynamics, and a discussion of the involved experimental parameter values and the proposed experimental protocol.

cond-mat.mes-hall↗
arXiv2011

The Effect of Charge Order on the Plasmon Dispersion in Transition-Metal Dichalcogenides

We investigate the dispersion of the charge carrier plasmon in the three prototypical charge-density wave bearing transition-metal dichalcogenides 2H-TaSe2, 2H-TaS2 and 2H-NbSe2 employing electron energy-loss spectroscopy. For all three compounds the plasmon dispersion is found to be negative for small momentum transfers. This is in contrast to the generic behavior observed in simple metals as well as the related system 2H-NbS2, which does not exhibit charge order. We present a semiclassical Ginzburg-Landau model which accounts for these observations, and argue that the vicinity to a charge ordered state is thus reflected in the properties of the collective excitations.

cond-mat.str-el↗
arXiv2011

Chirality and Orbital Order in Charge Density Waves

We show that the recently observed chirality in the charge ordered phase of TiSe2 can be understood as a form of orbital ordering. The microscopic mechanism driving the transition between the novel chiral state and the non-chiral charge density wave is discussed, and shown to be of a general form, thus allowing for a broad class of materials to display this type of orbitally ordered chiral charge density wave.

cond-mat.str-el↗
arXiv2010

Exciton-phonon interactions and superconductivity bordering charge order in TiSe2

The strong coupling between lattice modes and charges which leads to the formation of charge density waves in materials such as the transition-metal dichalcogenides may also give rise to superconductivity in the same materials, mediated by the same exciton or phonon modes that dominate the charge ordered state. Such a superconducting phase has recently been observed for example in TiSe2, both upon intercalation with Copper and in the pristine material under pressure. Here we investigate the interplay of exciton formation and electron-phonon coupling within a simplified model description. We find that the combined exciton-phonon modes previously suggested to drive the charge density wave instability in TiSe2 are also responsible for the pairing of electrons in its superconducting regions. Based on these results, it is suggested that both of the observed domes form part of a single superconducting phase. We also study the effect of the quantum critical fluctuations emerging from the suppressed charge order on the transport properties directly above the superconducting region, and compare our finding with reported experimental results.

cond-mat.supr-con↗
arXiv2009

Broken Time Translation Symmetry as a model for Quantum State Reduction

The symmetries that govern the laws of nature can be spontaneously broken, enabling the occurrence of ordered states. Crystals arise from the breaking of translation symmetry, magnets from broken spin rotation symmetry and massive particles break a phase rotation symmetry. Time translation symmetry can be spontaneously broken in exactly the same way. The order associated with this form of spontaneous symmetry breaking is characterised by the emergence of quantum state reduction: systems which spontaneously break time translation symmetry act as ideal measurement machines. In this review the breaking of time translation symmetry is first compared to that of other symmetries such as spatial translations and rotations. It is then discussed how broken time translation symmetry gives rise to the process of quantum state reduction and how it generates a pointer basis, Born's rule, etc. After a comparison between this model and alternative approaches to the problem of quantum state reduction, the experimental implications and possible tests of broken time translation symmetry in realistic experimental settings are discussed.

quant-ph↗
arXiv2009

An Alternative Interpretation of Recent ARPES Measurements on TiSe2

Recently there has been a renewed interest in the charge density wave transition of TiSe2, fuelled by the possibility that this transition may be driven by the formation of an excitonic insulator or even an excitonic condensate. We show here that the recent ARPES measurements on TiSe2 can also be interpreted in terms of an alternative scenario, in which the transition is due to a combination of Jahn-Teller effects and exciton formation. The hybrid exciton-phonons which cause the CDW formation interpolate between a purely structural and a purely electronic type of transition. Above the transition temperature, the electron-phonon coupling becomes ineffective but a finite mean-field density of excitons remains and gives rise to the observed diffuse ARPES signals.

cond-mat.str-el↗
arXiv2008

Observing the Spontaneous Breakdown of Unitarity

During the past decade, the experimental development of being able to create ever larger and heavier quantum superpositions has brought the discussion of the connection between microscopic quantum mechanics and macroscopic classical physics back to the forefront of physical research. Under equilibrium conditions this connection is in fact well understood in terms of the mechanism of spontaneous symmetry breaking, while the emergence of classical dynamics can be described within an ensemble averaged description in terms of decoherence. The remaining realm of individual-state quantum dynamics in the thermodynamic limit was addressed in a recent paper proposing that the unitarity of quantum mechanical time evolution in macroscopic objects may be susceptible to a spontaneous breakdown. Here we will discuss the implications of this theory of spontaneous unitarity breaking for the modern experiments involving truly macroscopic Schrodinger cat states.

quant-ph↗
arXiv2008

Quantum Dynamics in the Thermodynamic Limit

The description of spontaneous symmetry breaking that underlies the connection between classically ordered objects in the thermodynamic limit and their individual quantum mechanical building blocks is one of the cornerstones of modern condensed matter theory and has found applications in many different areas of physics. The theory of spontaneous symmetry breaking however, is inherently an equilibrium theory, which does not address the dynamics of quantum systems in the thermodynamic limit. Here, we will use the example of a particular antiferromagnetic model system to show that the presence of a so-called thin spectrum of collective excitations with vanishing energy -one of the well-known characteristic properties shared by all symmetry-breaking objects- can allow these objects to also spontaneously break time-translation symmetry in the thermodynamic limit. As a result, that limit is found to be able, not only to reduce quantum mechanical equilibrium averages to their classical counterparts, but also to turn individual-state quantum dynamics into classical physics. In the process, we find that the dynamical description of spontaneous symmetry breaking can also be used to shed some light on the possible origins of Born's rule. We conclude by describing an experiment on a condensate of exciton polaritons which could potentially be used to experimentally test the proposed mechanism.

cond-mat.other↗
arXiv2008

Schrodinger-Newton equation as a possible generator of quantum state reduction

It has been suggested by Diosi and Penrose that the occurrence of quantum state reduction in macroscopic objects is related to a manifestation of gravitational effects in quantum mechanics. Although within Penrose's framework the dynamics of the quantum state reduction is not prescribed, it was suggested that the so called Schrodinger-Newton equation can be used to at least identify the resulting classical end states. Here we analyze the extent to which the Schrodinger-Newton equation can be used as a model to generate a full, time dependent description of the quantum state reduction process. We find that when supplied with an imaginary gravitational potential, the Schrodinger-Newton equation offers a rationalisation for some of the hitherto unexplained characteristics of quantum state reduction. The description remains incomplete however, because it is unclear how to fully recover Born's rule.

quant-ph↗
arXiv2007

Towards an Experimental Test of Gravity-induced Quantum State Reduction

According to the hypothesis of Penrose and Diosi, quantum state reduction is a manifestation of the incompatibilty of general relativity and the unitary time evolution of quantum physics. Dimensional analysis suggests that Schrodinger cat type states should collapse on measurable time scales when masses and lengths of the order of bacterial scales are involved. We analyze this hypothesis in the context of modern developments in condensed matter and cold atoms physics, aimed at realizing macroscopic quantum states. We first consider 'micromechanical' quantum states, analyzing the capacity of an atomic force microscopy based single spin detector to measure the gravitational state reduction, but we conclude that it seems impossible to suppress environmental decoherence to the required degree. We subsequently discuss 'split' cold atom condensates to find out that these are at present lacking the required mass scale by many orders of magnitude. We then extent Penrose's analysis to superpositions of mass current carrying states, and we apply this to the flux quantum bits realized in superconducting circuits. We find that the flux qubits approach the scale where gravitational state reduction should become measurable, but bridging the few remaining orders of magnitude appears to be very difficult with present day technology.

cond-mat.str-el↗
arXiv2007

Spontaneous Symmetry Breaking and Decoherence in Superconductors

We show that superconductors have a thin spectrum associated with spontaneous symmetry breaking similar to that of antiferromagnets, while still being in full agreement with Elitzur's theorem, which forbids the spontaneous breaking of local (gauge) symmetries. This thin spectrum in the superconductors consists of in-gap states that are associated with the spontaneous breaking of a global phase symmetry. In qubits based on mesoscopic superconducting devices, the presence of the thin spectrum implies a maximum coherence time which is proportional to the number of Cooper pairs in the device. Here we present the detailed calculations leading up to these results and discuss the relation between spontaneous symmetry breaking in superconductors and the Meissner effect, the Anderson-Higgs mechanism and the Josephson effect. Whereas for the Meissner effect a symmetry breaking of the phase of the superconductor is not required, it is essential for the Josephson effect.

cond-mat.supr-con↗
arXiv2007

Thin Spectrum States in Superconductors

We show that finite size superconductors have a spectrum of states at extremely low energy, i.e. inside the superconducting gap. The presence of this {\it thin spectrum} is a generic feature and related to the fact that in a superconductor the global phase rotation symmetry is spontaneously broken. For a strong coupling superconductor we find the spectrum by exactly solving the Lieb-Mattis type Hamiltonian onto which the problem maps. One of the physical consequences of the presence of thin states is that they cause quantum decoherence in superconducting qubits of finite extent.

cond-mat.supr-con↗
arXiv2006

Spontaneous Symmetry Breaking in Quantum Mechanics

We present a clear and mathematically simple procedure explaining spontaneous symmetry breaking in quantum mechanical systems. The procedure is applicable to a wide range of models and can be easily used to explain the existence of a symmetry broken state in crystals, antiferromagnets and even superconductors. It has the advantage that it automatically brings to the fore the main players in spontaneous symmetry breaking: the symmetry breaking field, the thermodynamic limit, and the global excitations of the thin spectrum.

physics.class-ph↗
arXiv2006

On the relation between decoherence and spontaneous symmetry breaking

We have recently shown that there is a limit to quantum coherence in many-particle spin qubits due to spontaneous symmetry breaking. These results were derived for the Lieb-Mattis spin model. Here we will show that the underlying mechanism of decoherence in systems with spontaneous symmetry breaking is in fact more general. We present here a generic route to finding the decoherence time associated with spontaneous symmetry breaking in many particle qubits, and subsequently we apply this approach to two model systems, indicating how the continuous symmetries in these models are spontaneously broken and discussing the relation of this symmetry breaking to the thin spectrum. We then present in detail the calculations that lead to the limit to quantum coherence, which is due to energy shifts in the thin spectrum.

cond-mat.str-el↗
arXiv2005

Orbital-Peierls State in NaTiSi2O6

Does the quasi one-dimensional titanium pyroxene NaTiSi2O6 exhibit the novel {\it orbital-Peierls} state? We calculate its groundstate properties by three methods: Monte Carlo simulations, a spin-orbital decoupling scheme and a mapping onto a classical model. The results show univocally that for the spin and orbital ordering to occur at the same temperature --an experimental observation-- the crystal field needs to be small and the orbitals are active. We also find that quantum fluctuations in the spin-orbital sector drive the transition, explaining why canonical bandstructure methods fail to find it. The conclusion that NaTiSi2O6 shows an orbital-Peierls transition is therefore inevitable.

cond-mat.str-el↗