arXiv subjects

Javier E. Villegas

Publications and source records attributed to Javier E. Villegas.

14 recordsLinked to original sources

arXiv2026

Anomalous spin-pumping behavior of half-metallic ferromagnet/d-wave superconductor heterostructures

Spin-pumping experiments in superconductor/ferromagnet heterostructures, which probe spin-sinking by the superconductor, have revealed a variety of complex behaviors. Most studies have focused on conventional s-wave superconductors combined with metallic or insulating ferromagnets. Here, we study a d-wave superconductor paired with a half-metallic ferromagnet, in epitaxial YBa2Cu3O7-d/La0.7Sr0.3MnO3 heterostructures with two crystalline orientations: one in which YBCO is c-axis oriented, and the other in which YBCO grows along the (103) direction. Using ferromagnetic resonance (FMR), we probe the temperature-dependent Gilbert damping coefficient α. For (103) heterostructures, α(T) initially decreases below Tc, but then increases at lower temperatures, exceeding normal-state levels. This behavior can be understood in terms of the opening of the superconducting gap and spin transport via nodal quasiparticles, which dominate when the ab-plane of YBCO is exposed at the interface. In stark contrast, c-axis heterostructures exhibit a pronounced enhancement of α(T) below Tc, peaking at 0.65-0.7Tc before decaying. This anomaly suggests the dominance of interface-bound Andreev states, arising from a locally suppressed superconducting order parameter due to proximity effects with the half-metallic LSMO.

cond-mat.supr-con↗

arXiv2026

Dimensionality of vortex matter in superconducting infinite-layer nickelates

Characterizing the dimensionality of the superconducting state in infinite-layer (IL) nickelates is essential for understanding its nature. Most studies have addressed this by examining the anisotropy of the upper critical fields. However, the dominance of Pauli paramagnetic effects over orbital effects complicates the interpretation of these experiments in terms of dimensionality. Here, we approach the question from a different perspective by mapping the vortex phase diagram. We show that superconducting Pr0.8Sr0.2NiO2 thin films with low disorder exhibit a vortex liquid-to-glass transition of a quasi-two-dimensional (2D) nature. In contrast, increasing disorder drives a crossover into a pure 2D state. This demonstrates that pure bidimensionality is an extrinsic property, resulting from the decoupling of NiO2 planes due to enhanced disorder. Our findings establish disorder as a key control parameter of superconductivity in IL nickelates and suggest that it resides within the NiO2 planes, providing two fundamental insights for understanding these materials.

cond-mat.supr-con↗

arXiv2023

Disentangling photodoping, photoconductivity, and photosuperconductivity in the cuprates

The normal-state conductivity and superconducting critical temperature of oxygen-deficient YBa2Cu3O7-x can be persistently enhanced by illumination. Strongly debated for years, the origin of those effects -- termed persistent photoconductivity (PPC) and photosuperconductivity (PPS) -- has remained an unsolved critical problem, whose comprehension may provide key insights to harness the origin of high-temperature superconductivity itself. Here we make essential steps toward understanding PPS. While the models proposed so far assume that it is caused by a carrier-density increase (photodoping) observed concomitantly, our experiments contradict such conventional belief: we demonstrate that it is instead linked to a photo-induced decrease of the electronic scattering rate. Furthermore, we find that the latter effect and photodoping are completely disconnected and originate from different microscopic mechanisms since they present different wavelength and oxygen-content dependencies as well as strikingly different relaxation dynamics. Besides helping disentangle photodoping, PPC, and PPS, our results provide new evidence for the intimate relation between critical temperature and scattering rate, a key ingredient in modern theories on high-temperature superconductivity.

cond-mat.supr-con↗

arXiv2023

Memristive effects in YBa2Cu3O7-x devices with transistor-like structure

Cuprate superconductors are strongly sensitive materials to disorder and oxygen stoichiometry; even minute variations of those parameters drastically change their electronic properties. Here we exploit this characteristic to engineer a memristive device based on the high-T_C superconductor YBa2Cu3O7-x (YBCO), in which local changes of the oxygen content and induced disorder are exploited to produce memory effects. These effects are triggered electrically in a three-terminal device whose structure is reminiscent of a transistor, consisting of a YBCO channel and an Al gate. The Al/YBCO interface, which controls the gate conductance, displays a giant, bipolar, reversible switching across a continuum of non-volatile conductance states that span over two Decades. This phenomenon is controlled by the gate voltage magnitude and is caused by oxygen exchange between YBCO and Al. Concomitantly, the channel shows a gradual, irreversible superconductor-to-insulator transition that retains a memory of the power dissipated in the device, and can be explained by induced bulk disorder. The observed effects, and the understanding of the interplay between the underlying mechanisms, constitute interesting ingredients for the design and realization of novel memristors and switches for superconducting electronics.

cond-mat.supr-con↗

arXiv2022

Superconducting bimodal ionic photo-memristor

Memristive circuit elements constitute a cornerstone for novel electronic applications, such as neuromorphic computing, called to revolutionize information technologies. By definition, memristors are sensitive to the history of electrical stimuli, to which they respond by varying their electrical resistance across a continuum of nonvolatile states. Recently, much effort has been devoted to developing devices that present an analogous response to optical excitation. Here we realize a new class of device, a tunnelling photo-memristor, whose behaviour is bimodal: both electrical and optical stimuli can trigger the switching across resistance states in a way determined by the dual optical-electrical history. This unique behaviour is obtained in a device of ultimate simplicity: an interface between a high-temperature superconductor and a transparent semiconductor. The microscopic mechanism at play is a reversible nanoscale redox reaction between both materials, whose oxygen content determines the electron tunnelling rate across their interface. Oxygen exchange is controlled here via illumination by exploiting a competition between electrochemistry, photovoltaic effects and photo-assisted ion migration. In addition to their fundamental interest, the unveiled electro-optic memory effects have considerable technological potential. Especially in combination with high-temperature superconductivity which, beyond facilitating the high connectivity required in neuromorphic circuits, brings photo-memristive effects to the realm of superconducting electronics.

cond-mat.supr-con↗

arXiv2020

Long-Range Propagation and Interference of $d$-wave Superconducting Pairs in Graphene

Recent experiments have shown that proximity with high-temperature superconductors induces unconventional superconducting correlations in graphene. Here we demonstrate that those correlations propagate hundreds of nanometer, allowing for the unique observation of $d$-wave Andreev pair interferences in YBa$_2$Cu$_3$O$_7$-graphene devices that behave as a Fabry-Pérot cavity. The interferences show as a series of pronounced conductance oscillations analogous to those originally predicted by de Gennes--Saint-James for conventional metal-superconductor junctions. The present work is pivotal to the study of exotic directional effects expected for nodal superconductivity in Dirac materials.

cond-mat.supr-con↗

arXiv2020

Tailored flux pinning in superconductor/ferromagnet multilayers with engineered magnetic domain morphology from stripes to skyrmions

Superconductor/Ferromagnet (S/F) hybrid systems show interesting magneto-transport behaviors that result from the transfer of properties between both constituents. For instance, magnetic memory can be transferred from the F into the S through the pinning of superconducting vortices by the ferromagnetic textures. The ability to tailor this type of induced behavior is important to broaden its range of applications. Here we show that engineering the F magnetization reversal allows tuning the strength of the vortex pinning (and memory) effects, as well as the field range in which they appear. This is done by using magnetic multilayers in which Co thin films are combined with different heavy metals (Ru, Ir, Pt). By choosing the materials, thicknesses, and stacking order of the layers, we can design the characteristic domain size and morphology, from out-of-plane magnetized stripe domains to much smaller magnetic skyrmions. These changes strongly affect the magneto-transport properties. The underlying mechanisms are identified by comparing the experimental results to a magnetic pinning model.

cond-mat.supr-con↗

arXiv2019

Josephson current through a ferromagnetic bilayer: Beyond the quasiclassical approximation

Based on the Bogoliubov-de Gennes equations, we provide an exact numerical solution for the critical current of Josephson junctions with a composite ferromagnetic bilayer. We demonstrate that for the antiparallel orientation of the magnetic moments of the bilayer, the presence of a potential barrier at the bilayer interface results in large oscillations of the critical current as a function of ferromagnet thickness and/or exchange field. Because of this, and remarkably, in the range of small exchange field and thicknesses, the magnetism leads to the increase of the critical current. This effect is well pronounced at low temperature but disappears near $T_c$. If the potential barrier is replaced by a spin-active barrier at the bilayer interface the conventional 0-$π$ transition, similar to the case of an uniform ferromagnetic Josephson junction, is observed. Strikingly, for a parallel orientation of the magnetic moments of the bilayer, the presence of the spin-active barrier restores the anomalous behavior---potential barrier in the antiparallel case. These behaviors result from the resonant tunneling of Cooper pairs across the composite barrier---an effect related to the spin-dependent Fermi vector in the presence of the ferromagnets' exchange field.

cond-mat.supr-con↗

arXiv2019

Factors limiting ferroelectric field-effect doping in complex-oxide heterostructures

Ferroelectric field-effect doping has emerged as a powerful approach to manipulate the ground state of correlated oxides, opening the door to a new class of field-effect devices. However, this potential is not fully exploited so far, since the size of the field-effect doping is generally much smaller than expected. Here we study the limiting factors through magneto-transport, scanning transmission electron and piezo-response force microscopy in ferroelectric/superconductor (YBa2Cu3O7-δ /BiFeO3) heterostructures, a model system showing very strong field-effects. Still, we find that they are limited in the first place by an incomplete ferroelectric switching. This can be explained by the existence of a preferential polarization direction set by the atomic terminations at the interface. More importantly, we also find that the field-effect carrier doping is accompanied by a strong modulation of the carrier mobility. Besides making quantification of field-effects via Hall measurements not straightforward, this finding suggests that ferroelectric poling produces structural changes (e.g. charged defects or structural distortions) in the correlated oxide channel. Those findings have important consequences for the understanding of ferroelectric field-effects and for the strategies to further enhance them.

cond-mat.mtrl-sci↗

arXiv2019

Tunable Klein-like tunneling of high-temperature superconducting pairs into graphene

Superconductivity can be induced in a normal material via the leakage of superconducting pairs of charge carriers from an adjacent superconductor. This so-called proximity effect is markedly influenced by graphene unique electronic structure, both in fundamental and technologically relevant ways. These include an unconventional form of the leakage mechanism the Andreev reflection and the potential of supercurrent modulation through electrical gating. Despite the interest of high-temperature superconductors in that context, realizations have been exclusively based on low-temperature ones. Here we demonstrate gate-tunable, high-temperature superconducting proximity effect in graphene. Notably, gating effects result from the perfect transmission of superconducting pairs across an energy barrier -a form of Klein tunneling, up to now observed only for non-superconducting carriers- and quantum interferences controlled by graphene doping. Interestingly, we find that this type of interferences become dominant without the need of ultra-clean graphene, in stark contrast to the case of low-temperature superconductors. These results pave the way to a new class of tunable, high-temperature Josephson devices based on large-scale graphene.

cond-mat.mes-hall↗

arXiv2013

Freezing and melting of vortex ice

We report on the realization of artificial ice using superconducting vortices in geometrically frustrated pinning arrays. This vortex ice shows two unique properties among artificial ice systems. The first comes from the possibility to switch the array geometric frustration on/off through temperature variations, which allows "freezing" and "melting" the vortex ice. The second is that the depinning and dynamics of the frozen vortex ice are insensitive to annealing, which implies that the ordered ground state is spontaneously approached. The major role of thermal fluctuations and the strong vortex-vortex interactions are at the origin of this unusual behavior.

cond-mat.supr-con↗

arXiv2011

Strong field-matching effects in superconducting YBa2Cu3O7-δ films with vortex energy landscapes engineered via masked ion irradiation

We have developed a masked ion irradiation technique to engineer the energy landscape for vortices in oxide superconductors. This approach associates the possibility to design the landscape geometry at the nanoscale with the unique capability to adjust depth of the energy wells for vortices. This enabled us to unveil the key role of vortex channeling in modulating the amplitude of the field matching effects with the artificial energy landscape, and to make the latter govern flux dynamics over an usually wide range of temperatures and applied fields.

cond-mat.supr-con↗

arXiv2011

Nanoscale ferroelectric manipulation of magnetic flux quanta

Using heterostructures that combine a large-polarization ferroelectric (BiFeO3) and a high-temperature superconductor (YBa2Cu3O7-δ), we demonstrate the modulation of the superconducting condensate at the nanoscale via ferroelectric field effects. Through this mechanism, a nanoscale pattern of normal regions that mimics the ferroelectric domain structure can be created in the superconductor. This yields an energy landscape for magnetic flux quanta and, in turn, couples the local ferroelectric polarization to the local magnetic induction. We show that this form of magnetoelectric coupling, together with the possibility to reversibly design the ferroelectric domain structure, allows the electrostatic manipulation of magnetic flux quanta.

cond-mat.supr-con↗

arXiv2011

Controllable manipulation of superconductivity using magnetic vortices

The magneto-transport of a superconducting/ferromagnetic hybrid structure consisting of a superconducting thin film in contact with an array of magnetic nanodots in the so-called "magnetic vortex-state" exhibits interesting properties. For certain magnetic states, the stray magnetic field from the vortex array is intense enough to drive the superconducting film into the normal state. In this fashion, the normal-to-superconducting phase transition can be controlled by the magnetic history. The strong coupling between superconducting and magnetic subsystems allows characteristically ferromagnetic properties, such as hysteresis and remanence, to be dramatically transferred into the transport properties of the superconductor.

cond-mat.supr-con↗