arXiv subjects

Jayaprakash Sahoo

Publications and source records attributed to Jayaprakash Sahoo.

2 recordsLinked to original sources

arXiv2026

Evolution of terahertz third harmonic response across rare-earth nickelate phase-diagram

High harmonic generation (HHG) is a sensitive probe for investigating electronic structures and dynamics of materials and a source for attosecond pulses. In particular, HHG with terahertz (THz) light can enable probing of nonlinear responses in correlated materials arising from low-energy many-body interactions. However, THz HHG studies have so far largely focused on topological materials and superconductors, leaving out other potential material systems which could also become efficient THz HHG sources. Here, we report THz third harmonic generation (THG) in rare-earth nickelates -- a prototype material for exploring the Mott insulator-metal transition and related technological applications. We find that the THG amplitude is highly sensitive to the strengths of electronic and magnetic phases of nickelates. In films with sharp phase-transitions, the local maximum and minimum in the temperature-dependent THG amplitude coincide with insulator-metal and magnetic transition temperatures, respectively. While in films with weaker transitions, these features shift toward lower temperatures or even monotonous THG enhancement is observed down to low temperatures. We developed a generalized theory for THz harmonic generation in negative charge-transfer insulators and outlined strategies to enhance the THz nonlinearities further. Our study broadens the scope of THz HHG studies and related applications to strongly correlated materials.

cond-mat.str-el↗

arXiv2026

Room-Temperature Terahertz Photoconductivity Polarity Switching in High Entropy Nickelates with Implications for Photonic Synapses

High entropy oxides (HEO) hold the potential to revolutionize the conventional material paradigms by leveraging high order of chemical disorder that induces highly desirable exotic phases for advanced applications. Here, we devise a methodology to enhance the efficiency of an artificial photonic synapse using a high entropy rare earth nickelate. Combined with epitaxial strain, we show that high entropy can further manipulate the phase of these locally disordered materials. Using time-averaged and time resolved Terahertz (THz) spectroscopy as dynamic probe, for the first time we show a rare combination of i) crystal axis dependent insulator to metal THz electronic phase transition and ii) coexistence of negative and positive THz photoconductivity at room temperature. Detailed analysis within theoretical models, including density functional theory (DFT)-based band structure calculations, suggest origin of these properties as disproportionate ordering of oxygen vacancies. Based on these findings, a conceptual THz-based artificial photonic synapse is proposed. This work underlines the pivotal role of HEO in advancing diverse THz functionalities, representing a critical step toward futuristic applications like THz-based high-speed computing and communication with an emphasis in THz frequency domain.

cond-mat.mtrl-sci↗