arXiv subjects

Jean-François Lampin

Publications and source records attributed to Jean-François Lampin.

5 recordsLinked to original sources

arXiv2026

Fully optoelectronic coherent THz spectroscopy

Coherent terahertz spectroscopy of molecular transients has so far relied on electronic sources whose bandwidth is limited to a fraction of their center frequency. Photoconductive devices offer a complementary approach, combining intrinsically broadband operation with coherent optoelectronic generation and detection. We report free-induction-decay spectroscopy of carbonyl sulfide at 0.29 THz in which, to our knowledge for the first time, both the pulsed emitter and the coherent heterodyne receiver are LT-GaAs photoconductors simultaneously pumped by a single free-running dual-frequency Ti:Sa laser. The receiver operates within 15 dB of the thermal noise limit, and the shared optical reference maintains phase coherence over more than 1000 averaged acquisitions. The measured transients agree with a time-domain Maxwell-Bloch model based on HITRAN parameters. These results demonstrate the feasibility of fully optoelectronic coherent THz spectroscopy and establish photoconductive optoelectronic mixing as a practical route toward frequency-agile, high-resolution coherent THz spectrometers over broad spectral ranges.

physics.app-ph↗

arXiv2024

Maximizing the electromagnetic efficiency of spintronic terahertz emitters

Spintronic Terahertz Emitters (STE) represent a significant advancement in source technology, exploiting the ultrafast demagnetization process of spin-electrons to unveil a 30THz wide, gapless spectrum, accessible through femtosecond lasers across the full VIS-IR range. This innovation not only positions STEs as a pivotal advancement in THz source technology but also underscores their role as a cost-effective, high-performance solution, thereby redefining standards within the field. However, the inherent spintronic nature of these devices introduces a challenge: a lower optical-to-terahertz conversion efficiency, which positions them at a notable disadvantage relative to other sources. In response, this work aims to substantially improve the electromagnetic efficiency of these emitters. This is accomplished by maximizing the energy conversion from the pumping laser for spin-electron generation. Our design integrates STEs with an optimized 1D trapping cavity, specifically engineered to fulfill critical aspects of ultrafast excitation and THz extraction. As a result, we have realized a 245% enhancement in emission and an increase of 8dB in overall intensity, positions our results among the most substantial improvements documented in this field. Furthermore, we delineate the optimal geometry for the deployment of STEs and explore the strategic selection of substrates in depth. Such enhanced emitters advance spintronic emitters towards broader applications in time-domain spectroscopy, ellipsometry, and nonlinear THz-pump spectroscopy. Enhancing spintronic emitter efficiency, combined with rapid magnetic field modulation, indicates the potential for dynamic ranges that rival traditional sources. Our predictions of STE's efficiencies, made through an electromagnetic approach, highlight its capability to uncover overlooked aspects from an optical standpoint, leading to subsequent improvements.

physics.optics↗

arXiv2021

360° polarization control of terahertz spintronic emitters using uniaxial FeCo/TbCo2/FeCo trilayers

Polarization control of THz light is of paramount interest for the numerous applications offered in this frequency range. Recent developments in THz spintronic emitters allow for a very efficient broadband emission, and especially unique is their ability of THz polarization switching through magnetization control of the ferromagnetic layer. Here we present an improved scheme to achieve full 360° nearly coherent polarization rotation that does not require multipolar or rotating external magnetic bias nor complex cascaded emitters. By replacing the FM layer of the spintronic emitter with a carefully designed FeCo/TbCo2/FeCo anisotropic heterostructure, we experimentally demonstrate Stoner-Wohlfarth-like coherent rotation of the THz polarization over a full 2pi azimuth only by a bipolar variation of the strength of the hard axis field, and with only a negligible decrease in the emission efficiency as compared to standard Pt/CoFeB/W inverse spin Hall emitters. THz measurements are in agreement with our model of the non-perfect Stoner-Wohlfarth behaviour. These emitters are well adapted for the implementation of polarimetric characterization not requiring any mechanically rotating polarizing elements. An example is given with the characterization of the birefringence in a quartz plate.

physics.optics↗

arXiv2021

Broadband super-resolution Terahertz Time domain spectroscopy applied to Gas analysis

Terahertz (THz) Time domain spectroscopy (THz-TDS) is a broadband spectroscopic technique spreading its uses in multiple fields: in science from material science to biology, in industry where it measures the thickness of a paint layer during the painting operation. Using such practical commercial apparatus with broad spectrum for gas spectroscopy could be a major asset for air quality monitoring and tracking of atmospheric composition. However, gas spectroscopy needs high resolution and the usual approach in THz-TDS, where the recorded time trace is Fourier transform, suffers from resolution limitation due to the size of the delay line in the system. In this letter, we introduce the concept of constraint reconstruction for super-resolution spectroscopy based on the modeling of the spectroscopic lines in a sparse spectrum. Light molecule gas typically shows sparse and narrow lines on a broad spectrum and we propose an algorithm reconstructing these lines with a resolution improvement of 10 the ultimate resolution reachable by the apparatus. We envision the proposed technique to lead to broadband, selective, rapid and cheap gas monitoring applications.

physics.app-ph↗

arXiv2016

Magneto-optical properties of InSb for terahertz applications

Magneto-optical permittivity tensor spectra of undoped InSb, n-doped and p-doped InSb crystals were determined using the terahertz time-domain spectroscopy (THz-TDS) and the Fourier transform far-infrared spectroscopy (far-FTIR). A Huge polar magneto-optical (MO) Kerr-effect (up to 20 degrees in rotation) and a simultaneous plasmonic behavior observed at low magnetic field (0.4 T) and room temperature are promising for terahertz nonreciprocal applications. We demonstrate the possibility of adjusting the the spectral rage with huge MO by increase in n-doping of InSb. Spectral response is modeled using generalized magneto-optical Drude-Lorentz theory, giving us precise values of free carrier mobility, density and effective mass consistent with electric Hall effect measurement.

physics.optics↗