arXiv subjects

Jean-Michel Hartmann

Publications and source records attributed to Jean-Michel Hartmann.

At least 19 recordsLinked to original sources

arXiv2026

New features of the sea-surface slope distribution revealed by IASI observations: Directional properties, influence of the wave height, large wave tilts

By analysis of the reflected solar contribution to mid-infrared radiance spectra collected by the IASI instrument, we investigate the influences of both the wind and significant wave height on the wave-slope probability distribution function (PDF). We show that, at equal wind speed, smaller wave heights enhance the directional (upwind-downwind and upwind-crosswind) asymmetries of the probabilities. We also point out that the sea-surface mean square slopes slightly decrease as the wave height increases (by about $5\%$ per meter for winds slower than 6 m/s), an original result for which we propose possible causes (short-scale damping by long waves and/or effect of compounding statistical processes). We also investigate the so far practically unstudied case of steep slopes and find large deviations from the quasi Gaussian behavior of the central part of the PDF, with a quite universal exponential decay of the probabilities with increasing tilt. We here observe larger probabilities in the downwind direction, but similar values in the up- and cross-wind ones. The physical mechanisms responsible for these trends are discussed. Finally, we propose refined parametrizations of the mean square slope versus wind-speed, which departs from the Cox and Munk linear relationships at moderate wind speed (5-8 m/s).

physics.ao-ph↗

arXiv2026

Andreev-enhanced conductance quantization and gate-tunable induced superconducting gap in germanium

Ge/SiGe quantum well heterostructures confining a high-mobility two-dimensional hole gas (2DHG) have emerged as a compelling platform for hybrid superconductor(S)-semiconductor(Sm) quantum devices. Here, we investigate the low-temperature transport properties of split-gate quantum point contacts (QPC) defined in one such heterostructure and positioned at different distances from an aluminum superconducting contact. We observe ballistic one-dimensional transport evidenced by conductance quantization with at least four clearly visible plateaus. Andreev reflection at the S/Sm interface induces a 40% enhancement of the conductance steps relative to the normal-state conductance staircase measured under a 100-mT out-of-plane magnetic field. This result is in excellent agreement with the theoretical expectation for an interface transparency of 0.88. By operating the QPCs in the tunneling regime, we probe the local density of states of the proximitized 2DHG. We report direct experimental evidence of an induced superconducting gap, demonstrating that its magnitude can be tuned by a gate voltage acting on the carrier density in the 2DHG.

cond-mat.mes-hall↗

arXiv2025

Laser-induced alignment of nanoparticles and macromolecules for single-particle-imaging applications

Laser-induced alignment of particles and molecules was long envisioned to support three-dimensional structure determination using "single-molecule diffraction" with x-ray free-electron lasers [PRL 92, 198102 (2004)]. However, the alignment of isolated macromolecules has not yet been demonstrated, also because quantitative modeling is very expensive. We computationally demonstrated that the alignment of nanorods and proteins is possible with standard laser technology. We performed a comprehensive analysis on the dependence of the degree of alignment on molecular properties and experimental details, e.g., particle temperature and laser-pulse energy. Considering the polarizability anisotropy of about 150,000 proteins, our analysis revealed that most of these proteins can be aligned using realistic experimental parameters.

physics.comp-ph↗

arXiv2024

Gatemon qubit on a germanium quantum-well heterostructure

Gatemons are superconducting qubits resembling transmons, with a gate-tunable semiconducting weak link as the Josephson element. Here, we report a gatemon device featuring an aluminum microwave circuit on a Ge/SiGe heterostructure embedding a Ge quantum well. Owing to the superconducting proximity effect, the high-mobility two-dimensional hole gas confined in this well provides a gate-tunable superconducting weak link between two Al contacts. We perform Rabi oscillation and Ramsey interference measurements, demonstrate the gate-voltage dependence of the qubit frequency, and measure the qubit anharmonicity. We find relaxation times T$_{1}$ up to 119 ns, and Ramsey coherence times T$^{*}_{2}$ up to 70 ns, and a qubit frequency gate-tunable over 3.5 GHz. The reported proof-of-concept reproduces the results of a very recent work [Sagi et al., Nat. Commun. 15, 6400 (2024)] using similar Ge/SiGe heterostructures thereby validating a novel platform for the development of gatemons and parity-protected cos(2$ϕ$) qubits.

cond-mat.mes-hall↗

arXiv2024

One Million Quality Factor Integrated Ring Resonators in the Mid-Infrared

We report ring resonators on a silicon germanium on silicon platform operating in the mid-infrared wavelength range around 3.5 - 4.6 μm with quality factors reaching up to one million. Advances in fabrication technology enable us to demonstrate such high Q-factors, which put silicon germanium at the forefront of mid-infrared integrated photonic platforms. The achievement of high Q is attested by the observation of degeneracy lifting between clockwise (CW) and counter-clockwise (CCW) resonances, as well as optical bistability due to an efficient power buildup in the rings.

physics.optics↗

arXiv2024

Gate- and flux-tunable sin(2$φ$) Josephson element with proximitized Ge-based junctions

Hybrid superconductor-semiconductor Josephson field-effect transistors (JoFETs) function as Josephson junctions with a gate-tunable critical current. Additionally, they can feature a non-sinusoidal current-phase relation (CPR) containing multiple harmonics of the superconducting phase difference, a so-far underutilized property. In this work, we exploit this multi-harmonicity to create a Josephson circuit element with an almost perfectly $π$-periodic CPR, indicative of a largely dominant charge-4e supercurrent transport. Such a Josephson element was recently proposed as the basic building block of a protected superconducting qubit. Here, it is realized using a superconducting quantum interference device (SQUID) with low-inductance aluminum arms and two nominally identical JoFETs. The latter are fabricated from a SiGe/Ge/SiGe quantum-well heterostructure embedding a high-mobility two-dimensional hole gas. By carefully adjusting the JoFET gate voltages and finely tuning the magnetic flux through the SQUID close to half a flux quantum, we achieve a regime where the $\sin(2φ)$ component accounts for more than \SI{95}{\percent} of the total supercurrent. This result demonstrates a new promising route for the realization of superconducting qubits with enhanced coherence properties.

cond-mat.mes-hall↗

arXiv2024

Laser Annealed SiO2/Si1-xGex Scaffolds for Nanoscaled Devices, Synergy of Experiment and Computation

Ultraviolet nanosecond laser annealing (UV-NLA) proves to be an important technique, particularly when tightly controlled heating and melting are necessary. In the realm of semiconductor technologies, the significance of nanosecond laser annealing (NLA) grows in tandem with the escalating intricacy of integration schemes in nano-scaled devices. Silicon-germanium alloys have been studied for decades for their compatibility with silicon devices. Indeed, they enable the manipulation of properties like strain, carrier mobilities and bandgap. In this framework, they can for instance boost the performances of p-type MOSFETs but also enable near infra-red absorption and emission for applications in photo-detection and photonics. Laser melting on such type of layers, however results, up to now, in the development of extended defects and poor control over layer morphology and homogeneity. In our study, we investigate the laser melting of ~700 nm thick relaxed silicon-germanium samples coated with SiO2 nano-arrays, observing the resulting material to maintain an unaltered lattice. We found the geometrical parameters of the silicon oxide having an impact on the thermal budget samples see, influencing melt threshold, melt depth and germanium distribution.

cond-mat.mes-hall↗

arXiv2024

Hopping of the center-of-mass of single G centers in silicon-on-insulator

Among the wealth of single fluorescent defects recently detected in silicon, the G center catches interest for its telecom single-photon emission that could be coupled to a metastable electron spin triplet. The G center is a unique defect where the standard Born-Oppenheimer approximation breaks down as one of its atoms can move between 6 lattice sites under optical excitation. The impact of this atomic reconfiguration on the photoluminescence properties of G centers is still largely unknown, especially in silicon-on-insulator (SOI) samples. Here, we investigate the displacement of the center-of-mass of the G center in silicon. We show that single G defects in SOI exhibit a multipolar emission and zero-phonon line fine structures with splittings up to $\sim1$ meV, both indicating a motion of the defect central atom over time. Combining polarization and spectral analysis at the single-photon level, we evidence that the reconfiguration dynamics are drastically different from the one of the unperturbed G center in bulk silicon. The SOI structure freezes the delocalization of the G defect center-of-mass and as a result, enables to isolate linearly polarized optical lines. Under above-bandgap optical excitation, the central atom of G centers in SOI behaves as if it were in a 6-slot roulette wheel, randomly alternating between localized crystal sites at each optical cycle. Comparative measurements in a bulk silicon sample and ab initio calculations highlight that strain is likely the dominant perturbation impacting the G center geometry. These results shed light on the importance of the atomic reconfiguration dynamics to understand and control the photoluminescence properties of the G center in silicon. More generally, these findings emphasize the impact of strain fluctuations inherent to SOI wafers for future quantum integrated photonics applications based on color centers in silicon.

quant-ph↗

arXiv2024

Genuine and faux single G centers in carbon-implanted silicon

Among the wide variety of single fluorescent defects investigated in silicon, numerous studies have focused on color centers with a zero-phonon line around $1.28 μ$m and identified to a common carbon-complex in silicon, namely the G center. However, inconsistent estimates regarding their quantum efficiency cast doubt on the correct identification of these individual emitters. Through a comparative analysis of their single-photon emission properties, we demonstrate that these single color centers are split in two distinct families of point defects. A first family consists of the genuine single G centers with a well-identified microscopic structure and whose photoluminescence has been investigated on ensemble measurements since the 60's. The remaining defects belong to a new color center, which we will refer to as G$^{\star}$ center, whose atomic configuration has yet to be determined. These results provide a safeguard against future defect misidentifications, which is crucial for further development of quantum technologies relying on G or G$^{\star}$ center quantum properties.

quant-ph↗

arXiv2023

From nonreciprocal to charge-4e supercurrents in Ge-based Josephson devices with tunable harmonic content

Hybrid superconductor(S)-semiconductor(Sm) devices bring a range of new functionalities into superconducting circuits. In particular, hybrid parity-protected qubits and Josephson diodes were recently proposed and experimentally demonstrated. Such devices leverage the non-sinusoidal character of the Josephson current-phase relation (CPR) in highly transparent S-Sm-S junctions. Here we report an experimental study of superconducting quantum-interference devices (SQUIDs) embedding Josephson field-effect transistors fabricated from a SiGe/Ge/SiGe heterostructure grown on a 200-mm silicon wafer. The single-junction CPR shows up to three harmonics with gate tunable amplitude. In the presence of microwave irradiation, the ratio of the first two dominant harmonics, corresponding to single and double Cooper-pair transport processes, is consistently reflected in relative weight of integer and half-integer Shapiro steps. A combination of magnetic-flux and gate-voltage control enables tuning the SQUID functionality from a nonreciprocal Josephson-diode regime with 27% asymmetry to a $π$-periodic Josephson regime suitable for the implementation of parity-protected superconducting qubits. These results illustrate the potential of Ge-based hybrid devices as versatile and scalable building blocks of novel superconducting quantum circuits.

cond-mat.mes-hall↗

arXiv2023

Revisiting the Cox and Munk wave-slope statistics using IASI observations of the sea surface

We use radiances collected from space by the Infrared Atmospheric Sounder Interferometer (IASI) when looking down at ocean surfaces during the day to remotely determine the probability distribution of wave slopes. This is achieved by using about 300 channels between 3.6 and 4.0 $μ$m and a physically-based approach which properly takes the contribution of the reflected solar radiation into account. Based on about 150 million observations, the same number of wave-slope probabilities are retrieved for wind speeds up to 15 m/s. We revisit and discuss the methodology proposed by Cox and Munk (CM) to derive their celebrated wave-slope probability distribution function (pdf) from photographs of the sun glitter. We propose an original and robust approach for accurate retrievals of the 7 parameters appearing in the Gram-Charlier representation of the pdf. Our results for the mean square slopes are fully compatible with those of CM, and with the more recent results by Bréon and Henriot, but our lower uncertainties enable us to point out departures from the linear wind-speed dependencies and a slight overestimation of the upwind MSS described by the linear fit of CM at moderate wind speed. Our skewness and kurtosis coefficients show clear influences of the wind speed, with a steady decrease of the former and the alongwind kurtosis coefficient being maximal at moderate wind speeds, features that CM could not point out due to the limitations of their measurements. We revisit the renormalization procedure employed by CM to obtain the complete variances from truncated pdf and show that it imposes stringent conditions on the kurtosis coefficients that allow us to determine them accurately, with wind-dependent values specific to the local sea state.

physics.ao-ph↗

arXiv2023

Impact of surface reflectivity on the ultra-fast laser melting of silicon-germanium alloys

Ultraviolet nanosecond laser annealing (LA) is a powerful tool where strongly confined heating and melting are desirable. In semiconductor technologies the importance of LA increases with the increasing complexity of the proposed integration schemes. Optimizing the LA process along with the experimental design is challenging, especially when complex 3D nanostructured systems with various shapes and phases are involved. Within this context, reliable simulations of laser melting are required for optimizing the process parameters while reducing the number of experimental tests. This gives rise to a virtual Design of Experiments (DoE). $Si_{1-x}Ge_{x}$ alloys are nowadays used for their compatibility with silicon devices enabling to engineer properties such as strain, carrier mobilities and bandgap. In this work, the laser melting process of relaxed and strained $Si_{1-x}Ge_{x}$ is simulated with a finite element method / phase field approach. Particularly, we calibrated the dielectric functions of the alloy for its crystalline and liquid phase using experimental data. We highlighted the importance of reproducing the exact reflectivity of the interface between air and the material in its different aggregation states, to correctly mimic the process. We indirectly discovered intriguing features on the optical behavior of melt silicon-germanium.

cond-mat.mes-hall↗

arXiv2023

Atomistic insights into ultrafast SiGe nanoprocessing

Controlling ultrafast material transformations with atomic precision is essential for future nanotechnology. Pulsed laser annealing (LA), inducing extremely rapid and localized phase transitions, is a powerful way to achieve this, but it requires careful optimization together with the appropriate system design. We present a multiscale LA computational framework able to simulate atom-by-atom the highly out-of-equilibrium kinetics of a material as it interacts with the laser, including effects of structural disorder. By seamlessly coupling a macroscale continuum solver to a nanoscale super-lattice Kinetic Monte Carlo code, this method overcomes the limits of state-of-the-art continuum-based tools. We exploit it to investigate nontrivial changes in composition, morphology and quality of laser-annealed SiGe alloys. Validations against experiments and phase-field simulations, as well as advanced applications to strained, defected, nanostructured and confined SiGe are presented, highlighting the importance of a multiscale atomistic-continuum approach. Current applicability and potential generalization routes are finally discussed.

physics.comp-ph↗

arXiv2022

Detection of single W-centers in silicon

Controlling the quantum properties of individual fluorescent defects in silicon is a key challenge towards advanced quantum photonic devices prone to scalability. Research efforts have so far focused on extrinsic defects based on impurities incorporated inside the silicon lattice. Here we demonstrate the detection of single intrinsic defects in silicon, which are linked to a tri-interstitial complex called W-center, with a zero-phonon line at 1.218$μ$m. Investigating their single-photon emission properties reveals new information about this common radiation damage center, such as its dipolar orientation and its photophysics. We also identify its microscopic structure and show that although this defect does not feature electronic states in the bandgap, Coulomb interactions lead to excitonic radiative recombination below the silicon bandgap. These results could set the stage for numerous quantum perspectives based on intrinsic luminescent defects in silicon, such as quantum integrated photonics, quantum communications and quantum sensing.

quant-ph↗

arXiv2022

Single G centers in silicon fabricated by co-implantation with carbon and proton

We report the fabrication of G centers in silicon with an areal density compatible with single photon emission at optical telecommunication wavelengths. Our sample is made from a silicon-on-insulator wafer which is locally implanted with carbon ions and protons at various fluences. Decreasing the implantation fluences enables to gradually switch from large ensembles to isolated single defects, reaching areal densities of G centers down to $\sim$0.2 $μ$m$^{-2}$. Single defect creation is demonstrated by photon antibunching in intensity-correlation experiments, thus establishing our approach as a reproducible procedure for generating single artificial atoms in silicon for quantum technologies.

physics.app-ph↗

arXiv2022

Single SiGe Quantum Dot Emission Deterministically Enhanced in a High-Q Photonic Crystal Resonator

We report the resonantly enhanced radiative emission from a single SiGe quantum dot (QD), which is deterministically embedded into a bichromatic photonic crystal resonator (PhCR) at the position of its largest modal electric field by a scalable method. By optimizing our molecular beam epitaxy (MBE) growth technique, we were able to reduce the amount of Ge within the whole resonator to obtain an absolute minimum of exactly one QD, accurately positioned by lithographic methods relative to the PhCR, and an otherwise flat, a few monolayer thin, Ge wetting layer (WL). With this method, record quality (Q) factors for QD-loaded PhCRs up to $Q\sim 10^5$ are achieved. A comparison with control PhCRs on samples containing a WL but no QDs is presented, as well as a detailed analysis of the dependence of the resonator-coupled emission on temperature, excitation intensity, and emission decay after pulsed excitation. Our findings undoubtedly confirm a single QD in the center of the resonator as a potentially novel photon source in the telecom spectral range.

physics.optics↗

arXiv2021

Rotation of polarization of light propagating through a gas of molecular super-rotors

We present a detailed theoretical and experimental study of the rotation of the plane of polarization of light traveling through a gas of fast-spinning molecules. This effect is similar to the polarization drag phenomenon predicted by Fermi a century ago and it is a mechanical analog of the Faraday effect. In our experiments, molecules were spun up by an optical centrifuge and brought to the super-rotor state that retains its rotation for a relatively long time. Polarizability properties of fast-rotating molecules were analyzed considering the rotational Doppler effect and Coriolis forces. We used molecular dynamics simulations to account for intermolecular collisions. We found, both experimentally and theoretically, a nontrivial nonmonotonic time dependence of the polarization rotation angle. This time dependence reflects transfer of the angular momentum from rotating molecules to the macroscopic gas flow, which may lead to the birth of gas vortices. Moreover, we show that the long-term behavior of the polarization rotation is sensitive to the details of the intermolecular potential. Thus, the polarization drag effect appears as a novel diagnostic tool for the characterization of intermolecular interaction potentials and studies of collisional processes in gases.

physics.optics↗

arXiv2020

Reduced lasing thresholds in GeSn microdisk cavities with defect management of the optically active region

GeSn alloys are nowadays considered as the most promising materials to build Group IV laser sources on silicon (Si) in a full complementary metal oxide semiconductor-compatible approach. Recent GeSn laser developments rely on increasing the band structure directness, by increasing the Sn content in thick GeSn layers grown on germanium (Ge) virtual substrates (VS) on Si. These lasers nonetheless suffer from a lack of defect management and from high threshold densities. In this work we examine the lasing characteristics of GeSn alloys with Sn contents ranging from 7 \% to 10.5 \%. The GeSn layers were patterned into suspended microdisk cavities with different diameters in the 4-\SI{8 }{\micro\meter} range. We evidence direct band gap in GeSn with 7 \% of Sn and lasing at 2-\SI{2.3 }{\micro\meter} wavelength under optical injection with reproducible lasing thresholds around \SI{10 }{\kilo\watt\per\square\centi\meter}, lower by one order of magnitude as compared to the literature. These results were obtained after the removal of the dense array of misfit dislocations in the active region of the GeSn microdisk cavities. The results offer new perspectives for future designs of GeSn-based laser sources.

physics.optics↗