Jean-Paul Boucher | Searcharxiv

arXiv2017

Phase Diagram and Soliton Picture of an Ideal Spin-Peierls Compound D-F$_{5}$PNN

We investigate magnetic properties of an $S$=1/2 quasi-one dimensional organic antiferromagnet, D-F$_{5}$PNN using magnetization measurements taken at temperatures as low as 0.5 K. Three distinct phases were observed consisting of uniform, dimerized (D), and incommensurate (I) spin structures in the magnetic field versus temperature plane, where a significant hysteresis appears between D-I transitions in the field scan measurements. A combination of magnon ($S$=1) and soliton ($S$=1/2) excitations have successfully reproduced the observed magnetic susceptibility. In addition, such excitations provide a reasonable interpretation of the temperature dependent electron spin resonance (ESR) spectra. By comparison with the theoretical study, we conclude that D-F$_{5}$PNN is an ideal compound for investigating the spin-Peierls transition.

cond-mat.str-el↗

arXiv1999

Soliton Lattices in the Incommensurate Spin-Peierls Phase: Local Distortions and Magnetizations

It is shown that nonadiabatic fluctuations of the soliton lattice in the spin-Peierls system CuGeO_3 lead to an important reduction of the NMR line widths. These fluctuations are the zero-point motion of the massless phasonic excitations. Furthermore, we show that the discrepancy of X-ray and NMR soliton widths can be understood as the difference between a distortive and a magnetic width. Their ratio is controlled by the frustration of the spin system. By this work, theoretical and experimental results can be reconciled in two important points.

cond-mat.str-el↗