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Jean-Pierre Tchapet Njafa

Publications and source records attributed to Jean-Pierre Tchapet Njafa.

11 recordsLinked to original sources

Temperature-Driven Sequential Modeling for the Prediction of Annual Power Conversion Efficiency Profiles of Organic Photovoltaic Materials: Douala Case Study

Organic photovoltaic (OPV) materials are promising candidates for distributed solar energy in tropical regions, yet existing virtual screening tools report static power conversion efficiency (PCE) values at standard testing conditions (STC) that fail to capture the temperature-driven performance degradation experienced under real deployment conditions. Here we introduce a Climate-Native computational framework that forecasts the annual PCE profile of OPV donor molecules under geographically realistic operating conditions. The framework combines GFN2-xTB molecular dynamics with an equivariant graph neural network surrogate ($268$ Neyman-stratified CEP molecules; $120,600$ training geometries; $\sim 1050\times$ speedup over explicit quantum chemistry) and sequential deep learning models trained on annual time series anchored in NASA POWER climate data for Douala, Cameroon, and validated by zero-shot transfer to Yaoundé and Maroua. Applied to $\sim 30,000$ molecules from the Harvard Clean Energy Project (CEP) and validated against $350$ HOPV15 experimental device measurements, the framework demonstrates that sequential models trained on full molecular dynamics trajectories outperform time-averaged baselines ($35\%$-$48\%$ relative MAE improvement over static baselines), confirming that thermal conformational dynamics carry information beyond mean geometry. We further introduce a seasonal stability score that reranks OPV candidates by performance consistency under tropical conditions, identifying molecules whose deployment suitability differs substantially from their static PCE ranking.

cond-mat.mtrl-sci↗

Selective Vibronic Excitation for Coherent Energy Transport in Photosynthetic and Agrivoltaic Systems

Partitioning the photonic environment into resonant and off-resonant modes provides a mechanism for dephasing suppression in photosynthetic energy transfer. Aligning the excitation spectrum with underdamped vibronic resonances in the Fenna-Matthews-Olson (FMO) complex prepares vibronically dressed states with reduced coupling to dissipative fluctuations, inducing a biexponential coherence decay: a rapid initial dephasing (τfast {\approx} 37fs) followed by persistent inter-band coherences extending beyond 1ps-a > 3x extension of the effective coherence window relative to broadband excitation (τc = 280fs). This improves forward transfer yields by 39% at 295K. PT-HOPS/SBD simulations establish that dual-band filtering at 750nm and 820nm targets vibronic resonances while bypassing dephasing-dominated noise. This enhancement is robust against static disorder (σ = 50 cm-1), with an ensemble-averaged increase of η = 0.39 {\pm} 0.04. These results identify selective vibronic excitation as a foundational design principle for coherence-assisted transport. This framework extends to symbiotic agrivoltaic systems, where organic photovoltaics function as active spectral filters to co-optimize excitonic transport alongside the photosynthetic requirements of underlying crops.

quant-ph↗

Data-Driven Design Rules for TADF Emitters from a High-Throughput Screening of 747 Molecules

TADF emitter performance depends on both thermodynamic and kinetic factors. We analyze 747 experimentally known TADF molecules computationally to extract quantitative design guidelines. Using a validated xTB-based workflow, we examine how architecture, geometry, and electronic structure affect photophysical properties. Among architectures, D-A-D frameworks achieve the smallest \deltaest. A favorable torsional angle of $50°-90°$ balances small $ΔE_{\text{ST}}$ with the spin--orbit coupling needed for reverse intersystem crossing. Clustering separates high-performance candidates and highlights multi-resonance emitters for blue emission. From these results, we identify 127 candidates with predicted $ΔE_{\text{ST}} < 0.1 eV$ and oscillator strength $f > 0.1$. These HTVS-derived design guidelines and candidates can guide future TADF emitter development.

physics.app-ph↗

Computational discovery of bifunctional organic semiconductors for energy and biosensing

The discovery of synthetically accessible organic semiconductors with exceptional performance remains a critical bottleneck in materials science. While these materials offer compelling advantages - structural modularity, mechanical flexibility, and cost-effective solution processing - for applications in photovoltaics and biosensors, identifying candidates that balance high efficiency with practical synthesis presents significant challenges. To address this challenge, we developed a high-throughput screening approach using 17 458 molecules from the PubChemQC B3LYP/6-31G*//PM6 dataset. Our strategy employs a composite metric, PCESAScore = PCE - SAScore, which systematically balances power conversion efficiency (PCE) predictions from the Scharber model against synthetic accessibility scores. This approach successfully identified seven multi-functional candidates that demonstrate both exceptional photovoltaic performance (PCE up to 36.1 %) and strong protein-binding affinity for biosensing applications. Notably, molecule 4550 emerged as the optimal candidate, exhibiting a ligand efficiency of 0.340 kcal/mol/heavy atom with 100 % target promiscuity. Our computational framework integrates machine learning, density functional theory, and molecular docking to bridge the gap between theoretical performance and experimental feasibility. These findings establish a systematic pathway for discovering synthetically compatible organic semiconductors that can simultaneously address energy conversion and molecular recognition challenges.

cond-mat.mtrl-sci↗

From orbital analysis to active learning: an integrated strategy for the accelerated design of TADF emitters

Thermally Activated Delayed Fluorescence (TADF) emitters must satisfy two competing requirements: small singlet-triplet energy gaps for thermal upconversion and sufficient spin-orbit coupling for fast reverse intersystem crossing. Predicting these properties accurately demands expensive calculations. We address this using a validated semi-empirical protocol (GFN2-xTB geometries, sTDA/sTD-DFT-xTB excited states) on 747 molecules, combined with charge-transfer descriptors from Natural Transition Orbital analysis. The hole-electron spatial overlap She emerges as a key predictor, accounting for 21% of feature importance for the triplet state alone. Our best model (Support Vector Regression) reaches MAE = 0.024 eV and R2 = 0.96 for $ΔE_{ST}$. Active learning reduces the data needed to reach target accuracy by approximately 25% compared to random sampling. Three application domains are explored: NIR-emitting probes for bioimaging, photocatalytic sensitizers, and fast-response materials for photodetection.

cond-mat.mtrl-sci↗

Validation of Semi-Empirical xTB Methods for High-Throughput Screening of TADF Emitters: A 747-Molecule Benchmark Study

Thermally activated delayed fluorescence (TADF) emitters are essential for next-generation, high-efficiency organic light-emitting diodes (OLEDs), yet their rational design is hampered by the high computational cost of accurate excited-state predictions. Here, we present a comprehensive benchmark study validating semi-empirical extended tight-binding (xTB) methods -- specifically sTDA-xTB and sTD-DFT-xTB -- for the high-throughput screening of TADF materials. Using an unprecedentedly large dataset of \num{747} experimentally characterized emitters, our framework demonstrates a computational cost reduction of over \qty{99}{\percent} compared to conventional TD-DFT, while maintaining strong internal consistency between methods (Pearson $r \approx \num{0.82}$ for \deltaest), validating their utility for relative molecular ranking. Validation against \num{312} experimental \deltaest values reveals a mean absolute error of approximately \qty{0.17}{\electronvolt}, a discrepancy attributed to the vertical approximation inherent to the HTS protocol, underscoring the methods' role in screening rather than quantitative prediction. Through large-scale data analysis, we statistically validate key design principles, confirming the superior performance of Donor-Acceptor-Donor (D-A-D) architectures and identifying an optimal D-A torsional angle range of \qtyrange{50}{90}{\degree} for efficient TADF. Principal Component Analysis reveals that the complex property space is fundamentally low-dimensional, with three components capturing nearly \qty{90}{\percent} of the variance. This work establishes these semi-empirical methods as powerful, cost-effective tools for accelerating TADF discovery and provides a robust set of data-driven design rules and methodological guidelines for the computational materials science community.

cond-mat.mtrl-sci↗

Tunable direct bandgap and optical response in \ch{Mo_{1-x}W_xS2} monolayer alloys: A first-principles investigation

This study presents a comprehensive first-principles investigation of the structural, electronic and optical properties of monolayer \ch{Mo_{1-x}W_xS2} alloys, systematically exploring the full compositional range ($x=0$ to $1$) using density functional theory (DFT). We establish that these alloys are thermodynamically stable and maintain the characteristic 2H crystal structure with minimal structural perturbation upon alloying. A key finding is the preservation of a direct bandgap at the $K$-point across all compositions. This gap exhibits continuous tunability, increasing near-monotonically from \SI{1.696}{\electronvolt} (\ch{MoS2}) to \SI{1.858}{\electronvolt} (\ch{WS2}), a critical feature for tailoring optoelectronic devices. Electronic structure analysis reveals the systematic evolution of the orbital contributions of transition metal $d$ and sulfur $p$ at the edges of the band with composition. Consequently, the optical spectra, evaluated up to \SI{8}{\electronvolt}, show a progressive blueshift in the main features of the interband transition with increasing \ch{W} content, accompanied by predictable changes in key optical constants. Our comprehensive results validate the monolayer \ch{Mo_{1-x} W_xS2} as an electronically versatile platform that offers fine control over electronic and optical properties via alloying, making these tunable direct-gap semiconductors highly promising for next-generation photodetectors, light emitters, and potentially flexible optoelectronic applications exploiting their 2D nature.

cond-mat.mtrl-sci↗

Comparative Analysis of GFN Methods in Geometry Optimization of Small Organic Semiconductor Molecules: A DFT Benchmarking Study

This study benchmarks the GFN family of semiempirical methods (GFN1-xTB, GFN2-xTB, GFN0-xTB, and GFN-FF) against density functional theory (DFT) for the evaluation of optimized molecular geometries and electronic properties of small organic semiconductor molecules. This work offers a systematic assessment of these computationally efficient quantum chemical methods and their accuracy-cost profiles when applied to a challenging class of systems, characterized, for instance, by extended $π$-conjugation, conformational flexibility, and sensitivity of properties to subtle structural changes. Two datasets are evaluated: a QM9-derived subset of small organic molecules and the Harvard Clean Energy Project (CEP) database of extended $π$-systems relevant to organic photovoltaics. Structural agreement is quantified using heavy-atom RMSD, equilibrium rotational constants, bond lengths, and angles, while electronic property prediction is assessed via HOMO-LUMO energy gaps. Computational efficiency is assessed via CPU time and scaling behavior. GFN1-xTB and GFN2-xTB demonstrate the highest structural fidelity, while GFN-FF offers an optimal balance between accuracy and speed, particularly for larger systems. The results indicate that GFN-based methods are suitable for high-throughput molecular screening of small organic semiconductors, with the choice of method depending on accuracy-cost trade-offs. The findings support the deployment of GFN approaches in computational pipelines for the discovery of organic electronics and materials, providing information on their strengths and limitations relative to established DFT methods.

cond-mat.mtrl-sci↗

First principal investigation of Structural optical and thermoelectric properties of hybrid organic-inorganic perovskite $[NH_3-(CH_2)_4-NH_3]CdCl_4$ compound

The structural, thermoelectric, and optical properties of $[NH_3-(CH_2)_4-NH_3]CdCl_4$ were studied using Density Functional Theory (DFT) within the ABINIT code. The GGA-PBE functional, plane wave pseudopotentials, a kinetic energy cutoff of $35Ha$, and an 11x8x8 Monkhorst-Pack $k$-point grid were employed. The material comprises inorganic $[CdCl_4]^{2-}$ sheets, organic $[NH_3-(CH_2)_4-NH_3]^{2+}$ layers, and $N-H-Cl$ hydrogen bonds, ensuring sublattice cohesion. Structural optimization used reference crystal data, enabling analysis of alkylene-diammonium chain conformation, intermolecular interactions, and crystal stability. The study highlights the role of $Cd$ in influencing optical and thermoelectric properties. Temperature-induced changes lead to a reduced band gap and enhanced optical absorption, indicating significant electronic structure modifications. These findings propose $[NH_3-(CH_2)_4-NH_3]CdCl_4$ as a promising candidate for optoelectronic applications, particularly after thermal cycling, due to its improved performance under varying conditions.

cond-mat.mtrl-sci↗

Advancing excited-state simulations for TADF emitters: An eXtended Tight-Binding framework for high-throughput screening and design

We present a computationally efficient framework for predicting the excited-state properties of thermally activated delayed fluorescence (TADF) emitters, integrating extended tight-binding (\xtb), simplified Tamm-Dancoff approximation (\stda), and simplified time-dependent density functional theory (\stddft) methods. Benchmarking against Tamm-Dancoff approximation (noted full \tda) demonstrates that this approach accurately captures key photophysical properties, including singlet-triplet energy gaps, excitation energies, and fluorescence spectra, in both vacuum and solvent environments, while achieving over 99\% reduction in computational cost. We analyze a series of representative TADF emitters, revealing a strong correlation between the torsional angle between donor and acceptor units and the solvent-induced redshift in the emission spectrum. This work highlights the potential of semi-empirical methods for high-throughput screening of TADF materials and provides valuable insights for designing next-generation optoelectronic devices. The multi-objective function is one of a kind, and it further enhances our results with an original solution. While acknowledging the limitations of semi-empirical methods for highly complex systems, we outline promising future directions, including hybrid computational approaches and integration with machine learning techniques, to further improve predictive accuracy and accelerate the discovery of advanced functional materials.

physics.optics↗

Quantum associative memory with linear and non-linear algorithms for the diagnosis of some tropical diseases

This paper presents the QAMDiagnos, a model of Quantum Associative Memory (QAM) that can be a helpful tool for medical staff without experience or laboratory facilities, for the diagnosis of four tropical diseases (malaria, typhoid fever, yellow fever and dengue) which have several similar signs and symptoms. The memory can distinguish a single infection from a polyinfection. Our model is a combination of the improved versions of the original linear quantum retrieving algorithm proposed by Ventura and the non-linear quantum search algorithm of Abrams and Lloyd. From the given simulation results, it appears that the efficiency of recognition is good when particular signs and symptoms of a disease are inserted given that the linear algorithm is the main algorithm. The non-linear algorithm helps confirm or correct the diagnosis or give some advice to the medical staff for the treatment. So, our QAMDiagnos that has a friendly graphical user interface for desktop and smart-phone is a sensitive and a low-cost diagnostic tool that enables rapid and accurate diagnosis of four tropical diseases.

physics.med-ph↗