arXiv subjects

Jeehoon Kim

Publications and source records attributed to Jeehoon Kim.

At least 19 recordsLinked to original sources

arXiv2026

Topological Hall Effect in Antiferromagnetic Co doped Fe$_3$GaTe$_2$

Fe$_3$GaTe$_2$ is van der Waals (vdW) ferromagnet with a Curie temperature $T_C$ ranging from 350 K to 380 K, followed upon cooling by a ferrimagnetic transition near room temperature. Substituting Fe with Co was previously reported to induce antiferromagnetism (AFM) at a Co fraction dependent Neel temperature $T_N$. In this work, we confirm the overall phase diagram of the Fe$_{3-x}$Co$_x$GaTe$_2$ series as a function of $x$ and temperature via magnetization and electrical transport measurements. For $x \simeq 0.6$ the Hall effect is observed to mimic the magnetization as the AF ground state is suppressed by the external magnetic field via a metamagnetic transition, thus displaying an anomalous Hall response. At low temperatures, we also observe a pronounced topological Hall signal peaking at $\mu_0H$ = 4 T, or within the metamagnetic transition region of fields. This observation points to the presence of magnetic field-induced chiral spin textures, such as skyrmions upon approaching magnetization saturation. Magnetic force microscopy (MFM) reveals the emergence of nearly circular magnetic domains, with diameters on the order of 100 to 200 nm, within the antiferromagnetic phase. A detailed analysis of the MFM images indicates that the topological Hall effect is closely linked to the field-induced stabilization of magnetic domain structures, likely exhibiting chiral textures. This observation suggests the possible formation of skyrmions already in the AFM phase, i.e., AFM skyrmions, that evolve into ferromagnetic (FM) ones upon increasing the magnetic field. Consequently, Co-doped Fe$_3$GaTe$_2$ might provide a platform to investigate the transformation of skyrmions, initially coupled antiferromagnetically into ferromagnetic skyrmions, and to explore its impact on the topological and skyrmion Hall effects.

cond-mat.mes-hall↗

arXiv2025

Effect of C additives with 0.5% in weight on structural, optical and superconducting properties of Ta-Nb-Hf-Zr-Ti high entropy alloy films

We investigated the superconducting (SC) properties of Ta-Nb-Hf-Zr-Ti high-entropy alloy (HEA) thin films with 0.5% weight C additives. The C additives stabilize the structural properties and enhance the SC critical properties, including $\mu_0$Hc$_2$ (13.45 T) and Tc (7.5 K). The reflectance of the C-added HEA film is enhanced in the low-energy region, resulting in a higher optical conductivity, which is consistent with the lower electrical resistivity. In addition, we observed SC vortices in the C-added HEA film using magnetic force microscopy. The magnetic penetration depths ($\lambda$) of the pure HEA and C-added HEA films were estimated from their Meissner force curves by comparing them with those of a reference Nb film. At 4.2 K, the {\lambda} of the C-added film is 360 nm, shorter than that of the pure HEA film (560 nm), indicating stronger superconductivity against an applied magnetic field.

cond-mat.supr-con↗

arXiv2025

Local Inversion Symmetry Breaking and Thermodynamic Evidence for Ferrimagnetism in Fe3GaTe2

The layered compound Fe3GaTe2 is attracting attention due to its high Curie temperature, low dimensionality, and the presence of topological spin textures above room temperature, making Fe$_3$GaTe$_2$ a good candidate for applications in spintronics. Here, we show, through transmission electron microscopy (TEM) techniques, that Fe$_3$GaTe$_2$ single crystals break local inversion symmetry while maintaining global inversion symmetry according to X-ray diffraction. Coupled to the observation of N\'{e}el skyrmions via Lorentz-TEM, our structural analysis provides a convincing explanation for their presence in centrosymmetric materials. Magnetization measurements as a function of the temperature displays a sharp first-order thermodynamic phase-transition leading to a reduction in the magnetic moment. This implies that the ground state of Fe$_3$GaTe$_2$ is globally ferrimagnetic and not a glassy magnetic state composed of ferrimagnetic, and ferromagnetic domains as previously claimed. Neutron diffraction studies indicate that the ferromagnetic to ferrimagnetic transition upon reducing the external magnetic field is associated with a change in the magnetic configuration/coupling between Fe1 and Fe2 moments. We observe a clear correlation between the hysteresis observed in both the skyrmion density and the magnetization of Fe$_3$GaTe$_2$. This indicates that its topological spin textures are affected by the development of ferrimagnetism upon cooling. Observation, via magnetic force microscopy, of magnetic bubbles at the magnetic phase boundary suggests skyrmions stabilized by the competition among magnetic phases and distinct exchange interactions. Our study provides an explanation for the observation of N\'eel skyrmions in centrosymmetric systems, while exposing a correlation between the distinct magnetic phases of Fe$_3$GaTe$_2$ and topological spin textures.

cond-mat.mtrl-sci↗

arXiv2024

Vortex confinement through an unquantized magnetic flux

Geometrically confined superconductors often experience a breakdown in the quantization of magnetic flux owing to the incomplete screening of the supercurrent against the field penetration. In this study, we report that the confinement of a magnetic field occurs regardless of the dimensionality of the system, extending even to 1D linear potential systems. By utilizing a vector-field magnetic force microscope, we successfully create a vortex-antivortex pair connected by a 1D unquantized magnetic flux in ultra-thin superconducting films. Through an investigation of the manipulation and thermal behavior of the vortex pair, we uncover a long-range interaction mediated by the unquantized magnetic flux. These findings suggest a universal phenomenon of unquantized magnetic flux formation, independent of the geometry of the system. Our results present an experimental route for probing the impact of confinement on superconducting properties and order parameters in unconventional superconductors characterized by extremely low dimensionality.

cond-mat.supr-con↗

arXiv2023

Tuning vortex critical velocity in Mo$_2$N thin films via striped magnetic domain configuration

We report on the impact of the magnetic domain stripe configuration on the critical velocity of vortices in superconducting/ferromagnetic bilayers. Using a 23 nm thick Mo$_2$N film, covered by a 48 nm FePt layer with tunable nanosized striped domains, we demonstrate that flux instability at low magnetic fields depends on the orientation of the stripes. When the stripes are perpendicular to the applied current and act as vortex guides, the velocity values reach 5 km/s, duplicating those found when configured parallel to the current, creating winding vortex paths. Our results indicate that vortex critical velocities can be tuned by configuring different domain structures, providing a platform to understand vortex dynamics in superconducting microstrips.

cond-mat.supr-con↗

arXiv2023

Microscopic Insights into London Penetration Depth: Application to CeCoIn$^{}_{5}$

We propose a comprehensive theoretical formulation of magnetic penetration depth, $\lambda(T)$, based on the microscopic calculations for a general superconducting gap symmetry. Our findings admit the significant role of band structure and Fermi surface topology together with the symmetry of superconducting order parameter. We employ our findings pertaining to the heavy-fermion superconductor CeCoIn$_5$ to explore both local and non-local behaviors in response to an external magnetic field across varying temperatures. Our calculations in the low-temperature regime offer compelling macroscopic evidence of the nodal character within the superconducting state with $d_{x^2-y^2}$ symmetry. Furthermore, our findings align with the characteristics of London-type superconductivity, holding significant implications for upcoming experiments.

cond-mat.supr-con↗

arXiv2022

Reversibly controlled ternary polar states and ferroelectric bias promoted by boosting square-tensile-strain

Interaction between dipoles often emerges intriguing physical phenomena, such as exchange bias in the magnetic heterostructures and magnetoelectric effect in multiferroics, which lead to advances in multifunctional heterostructures. However, the defect-dipole tends to be considered the undesired to deteriorate the electronic functionality. Here, we report deterministic switching between the ferroelectric and the pinched states by exploiting a new substrate of cubic perovskite, BaZrO$_{3}$, which boosts square-tensile-strain to BaTiO$_{3}$ and promotes four-variants in-plane spontaneous polarization with oxygen vacancy creation. First-principles calculations propose a complex of an oxygen vacancy and two Ti$^{3+}$ ions coins a charge-neutral defect-dipole. Cooperative control of the defect-dipole and the spontaneous polarization reveals ternary in-plane polar states characterized by biased/pinched hysteresis loops. Furthermore, we experimentally demonstrate that three electrically controlled polar-ordering states lead to switchable and non-volatile dielectric states for application of non-destructive electro-dielectric memory. This discovery opens a new route to develop functional materials via manipulating defect-dipoles and offers a novel platform to advance heteroepitaxy beyond the prevalent perovskite substrates.

cond-mat.mtrl-sci↗

arXiv2022

Nanoscale Thermal Imaging of VO$_2$ via Poole-Frenkel Conduction

We present a method for nanoscale thermal imaging of insulating thin films using atomic force microscopy (AFM), and we demonstrate its utility on VO$_2$. We sweep the applied voltage $V$ to a conducting AFM tip in contact mode and measure the local current $I$ through the film. By fitting the $IV$ curves to a Poole-Frenkel conduction model at low $V$, we calculate the local temperature with spatial resolution better than 50 nm using only fundamental constants and known film properties. Our thermometry technique enables local temperature measurement of \textit{any} insulating film dominated by the Poole-Frenkel conduction mechanism, and can be extended to insulators that display other conduction mechanisms.

cond-mat.str-el↗

arXiv2021

Interlayer Exchange Interaction Driven Topological Phase Transition in Antiferromagnetic Electride Gd$_2$O

Based on first-principles calculations, we discover a two-dimensional layered antiferromagnetic (AFM) electride Gd$_2$O, where anionic excess electrons exist in the interstitial spaces between positively charged cationic layers. It is revealed that each cationic layer composed of three-atom-thick Gd$-$O$-$Gd stacks has in-plane ferromagnetic and out-of-plane AFM superexchange interactions between the localized Gd 4$f$ spins through O 2$p$ orbitals. Furthermore, the interlayer superexchange mediated by the hybridized Gd-5$d$ and interstitial-$s$-like states involves intimate couplings between the spin, lattice, and charge degrees of freedom, thereby inducing simultaneous magnetic, structural, and electronic phase transitions. The resulting ground state with the simple hexagonal lattice hosts massless Dirac fermions protected by nonsymmorphic magnetic symmetry, as well as massive Dirac fermions. We thus demonstrate that the anionic excess electrons in Gd$_2$O play a crucial role in the emergence of magnetic Dirac semimetal states, therefore offering an intriguing interplay between 2D magnetic electrides and topological physics.

cond-mat.mtrl-sci↗

arXiv2020

Local characterization of a heavy-fermion superconductor via sub-Kelvin magnetic force microscopy

Using magnetic force microscopy operating at sub-Kelvin temperatures we characterize the heavy-fermion superconductor CeCoIn$_5$. We pinpoint the absolute London penetration depth $λ(0) = 435 \pm 20$ nm and report its temperature dependence, which is closely linked to the symmetry of the superconducting gap. In addition, we directly measure the pinning force of individual Abrikosov vortices and estimate the critical current density $j_c = 9 \times 10^4$ A/cm$^2$. In contrast to the related, well-established tunnel diode oscillator technique, our method is capable of resolving inhomogeneities $locally$ on the micrometer-scale at ultra-low temperature.

cond-mat.supr-con↗

arXiv2020

Strong antiferromagnetic proximity coupling in a heterostructured superconductor Sr$_2$VO$_3$FeAs

We report observation of strong magnetic proximity coupling in a heterostructured superconductor Sr$_2$VO$_3$FeAs, determined by the upper critical fields $H_{c2}(T)$ measurements up to 65 T. Using the resistivity and the radio-frequency measurements for both $H \parallel ab$ and $H \parallel c$, we found a strong upward curvature of $H_{c2}^c(T)$, together with a steep increase of $H_{c2}^{ab}(T)$ near $T_c$, yielding the anisotropic factor $γ_H=H_{c2}^{ab}/H_{c2}^c$ up to $\sim$ 20, the largest value among iron-based superconductors. These are attributed to the Jaccarino-Peter effect, rather than to the multiband effect, due to strong exchange interaction between itinerant Fe spins of the FeAs layers and localized V spins of Mott-insulating SrVO$_3$ layers. These findings provide evidence for strong antiferromagnetic proximity coupling, comparable with the intralayer superexchange interaction of SrVO$_3$ layer and sufficient to induce magnetic frustration in Sr$_2$VO$_3$FeAs.

cond-mat.str-el↗

arXiv2020

Josephson coupling in high-T$_c$ superconducting junctions using ultra-thin BaTiO$_3$ barriers

We study the electrical transport of vertically-stacked Josephson tunnel junctions using GdBa$_2$Cu$_3$O$_{7-d}$ electrodes and a BaTiO$_3$ barrier with thicknesses between 1 nm and 3 nm. The junctions with an area of 20 mm x 20 mm were fabricated combining optical lithography and ion etching using GdBa$_2$Cu$_3$O$_{7-d}$ (16 nm) / BaTiO$_3$ (1 - 3 nm) / GdBa$_2$Cu$_3$O$_{7-d}$ (16 nm) trilayers growth by sputtering on (100) SrTiO$_3$. Current-voltage measurements at low temperatures show a Josephson coupling for junctions with BaTiO$_3$ barriers of 1 nm and 2 nm. Reducing the barrier thickness bellow a critical thickness seems to suppress the ferroelectric nature of the BaTiO$_3$. The Josephson coupling temperature is strongly reduced for increasing barrier thicknesses, which may be related to the suppression of the superconducting critical temperature in the bottom GdBa$_2$Cu$_3$O$_{7-d}$ due to stress. The Josephson energies at 12 K are of $\approx$ 1.5 mV and $\approx$ 7.5 mV for BaTiO$_3$ barriers of 1 nm and 2 nm. Fraunhofer patterns are consistent with fluctuations in the critical current due to structural inhomogeneities in the barriers. Our results are promising for the development of Josephson junctions using high-T$_c$ electrodes with energy gaps much higher than those usually present in conventional low-temperature superconductors.

cond-mat.supr-con↗

arXiv2018

Imaging the magnetic states in an actinide ferromagnet UMn$_2$Ge$_2$

We present studies of the magnetic domain structure of UMn$_2$Ge$_2$ single crystals using a home-built low temperature magnetic force microscope. The material has two distinct magnetic ordering temperatures, originating from the Mn and U moments. At room temperature, where the Mn moments dominate, there are flower-like domain patterns similar to those observed in uniaxial ferromagnets. After exposing the sample to a one-tesla magnetic field near 40 K, the evolution of the magnetic domains are imaged through zero-field warming up to 200 K. Near the ordering temperature of the uranium moments a clear change in the domain wall motion is observed. The domain size analysis of the flower-like pattern reveals that the domain structure is consistent with a model of branching domains.

cond-mat.mtrl-sci↗

arXiv2018

Transmission/reflection coefficients and Faraday/Kerr rotations as a function of applied magnetic fields in spin-orbit coupled Dirac metals

We reveal the nature of propagation and reflection of light in Weyl metals with broken time reversal symmetry, whose electromagnetic properties are described by axion electrodynamics. These Weyl metals turn out to play the role of a chiral prism: An incident monochromatic wave can split into three waves propagating with different wave numbers, depending on its chirality and polarization (right $\&$ left circular polarizations and linear polarization along the propagating direction). The helicity of the propagating/reflected light is determined by $\textbf{B}_{ext}$ and $\textbf{E}_{light}$, where $\textbf{B}_{ext}$ is the gradient of the $\theta-$field in the axion term given by the applied magnetic field and $\textbf{E}_{light}$ is the electric-field component of the incident light. This implies that the direction of the external magnetic field controls the Faraday/Kerr rotation. In particular, we find that the linear polarization of the oscillating electric field along the propagating direction, which cannot occur in conventional metals, arises when Weyl nodes are aligned along the oscillating magnetic field. We evaluate both transmission/reflection coefficients and Faraday/Kerr rotation angles as a function of both an external magnetic field and frequency for various configurations of light propagation. We propose their strong magnetic-field dependencies as one of the fingerprints of the axion electrodynamics.

cond-mat.other↗

arXiv2016

Direct observation of the M2 phase with its Mott transition in a VO$_2$ film

In VO$_2$, the explicit origin of the insulator-to-metal transition is still disputable between Peierls and Mott insulators. Along with the controversy, its second monoclinic (M2) phase has received considerable attention due to the presence of electron correlation in undimerized vanadium ions. However, the origin of the M2 phase is still obscure. Here, we study a granular VO$_2$ film using conductive atomic force microscopy and Raman scattering. Upon the structural transition from monoclinic to rutile, we observe directly an intermediate state showing the coexistence of monoclinic M1 and M2 phases. The conductivity near the grain boundary in this regime is six times larger than that of the grain core, producing a donut-like landscape. Our results reveal an intra-grain percolation process, indicating that VO$_2$ with the M2 phase is a Mott insulator.

cond-mat.str-el↗

arXiv2016

Two-parameter scaling theory of the longitudinal magnetoconductivity in a Weyl metal phase: Chiral anomaly, weak disorder, and finite temperature

It is at the heart of modern condensed matter physics to investigate the role of a topological structure in anomalous transport phenomena. In particular, chiral anomaly turns out to be the underlying mechanism for the negative longitudinal magnetoresistivity in a Weyl metal phase. Existence of a dissipationless current channel causes enhancement of electric currents along the direction of a pair of Weyl points or applied magnetic fields ($B$). However, temperature ($T$) dependence of the negative longitudinal magnetoresistivity has not been understood yet in the presence of disorder scattering since it is not clear at all how to introduce effects of disorder scattering into the "topological-in-origin" transport coefficient at finite temperatures. The calculation based on the Kubo formula of the current-current correlation function is simply not known for this anomalous transport coefficient. Combining the renormalization group analysis with the Boltzmann transport theory to encode the chiral anomaly, we reveal how disorder scattering renormalizes the distance between a pair of Weyl points and such a renormalization effect modifies the topological-in-origin transport coefficient at finite temperatures. As a result, we find breakdown of $B/T$ scaling, given by $B/T^{1 + η}$ with $0 < η< 1$. This breakdown may be regarded to be a fingerprint of the interplay between disorder scattering and topological structure in a Weyl metal phase.

cond-mat.dis-nn↗

arXiv2016

Construction of a $^3$He magnetic force microscope with a vector magnet

We constructed a $^3$He magnetic force microscope operating at the base temperature of 300 mK under a vector magnetic field of 2-2-9 T in the $x-y-z$ direction. Fiber optic interferometry as a detection scheme is employed in which two home-built fiber walkers are used for the alignment between the cantilever and the optical fiber. The noise level of the laser interferometer is close to its thermodynamic limit. The capabilities of the sub-Kelvin and vector field are demonstrated by imaging the coexistence of magnetism and superconductivity in a ferromagnetic superconductor (ErNi$_2$B$_2$C) at $T$=500 mK and by probing a dipole shape of a single Abrikosov vortex with an in-plane tip magnetization.

physics.ins-det↗

arXiv2015

Spatially resolved penetration depth measurements and vortex manipulation in the ferromagnetic superconductor ErNi2B2C

We present a local probe study of the magnetic superconductor, ErNi$_2$B$_2$C, using magnetic force microscopy at sub-Kelvin temperatures. ErNi$_2$B$_2$C is an ideal system to explore the effects of concomitant superconductivity and ferromagnetism. At 500 mK, far below the transition to a weakly ferromagnetic state, we directly observe a structured magnetic background on the micrometer scale. We determine spatially resolved absolute values of the magnetic penetration depth $λ$ and study its temperature dependence as the system undergoes magnetic phase transitions from paramagnetic to antiferromagnetic, and to weak ferromagnetic, all within the superconducting regime. In addition, we estimate the absolute pinning force of Abrikosov vortices, which shows a position- and temperature dependence as well, and discuss the possibility of the purported spontaneous vortex formation.

cond-mat.supr-con↗