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Jeff D. Thompson

Publications and source records attributed to Jeff D. Thompson.

At least 19 recordsLinked to original sources

High-fidelity neutral atom gates leveraging low-rank Hessian optimization

Quantum optimal control can produce fast and robust multi-qubit gates, but experimentally calibrating the resulting high-dimensional waveforms remains challenging because direct searches over large parameter spaces converge slowly. Building on the low-rank structure of quantum-control landscapes, we develop and benchmark a Hessian-based calibration method for optimal-control gates. The method identifies the few waveform directions that affect fidelity to leading order, with the number of directions set by the accessible leakage and coherent error channels, and optimizes only within this principal space using closed-loop experimental feedback. We apply this approach to an amplitude-robust controlled-Z gate on metastable-state 171Yb nuclear-spin qubits. Experimentally, we verify the predicted Hessian-sensitive directions and demonstrate rapid convergence of the optimization protocol. The optimized gate reaches a raw fidelity of 0.9959(2), increasing to 0.99902(7) after postselection on no detected loss, and the performance is essentially unchanged under laser-power variations of up to 20%. We further show that the same fidelity Hessian directions can correct certain Hamiltonian parameter errors. These results establish low-rank Hessian optimization as an efficient and physically motivated calibration strategy for high-dimensional optimal-control gates, which is broadly applicable to many qubit types.

quant-ph

Fast single-atom preparation in optical tweezers via Rydberg blockade

Continuously replenished optical tweezer arrays will unlock unlimited-depth quantum circuits with neutral atom qubits. A key bottleneck limiting the cycle time of these systems is removing atoms from tweezers initially loaded with more than one atom. In the conventional technique of light-assisted collisions, slow collisional dynamics limit the timescale for removing excess atoms to several milliseconds. Here, we propose and demonstrate a scheme for selectively removing one atom at a time from multiply occupied tweezers on a microsecond timescale, using intra-tweezer Rydberg blockade and autoionization. We demonstrate the protocol in $^{171}$Yb in two complementary regimes. With two-photon Rydberg excitation from the ground state, we reduce multi-atom probability to 1% in 64.8 $\mu$s, while retaining single atoms in 58.2(2)% of the tweezers, which is comparable to the filling fraction achieved with light-assisted collisions under the same experimental conditions, but over two orders of magnitude faster. With single-photon excitation from the metastable state $^3P_0$, reduced single-atom loss enables a higher filling fraction of 74.8(3)%, at the cost of additional temporal overhead to prepare the atoms in $^3P_0$. The final filling fraction is limited by an unexplained two-body loss mechanism, which, if solved, could enable fast, quasi-deterministic loading.

physics.atom-ph

Native defects and erbium impurities in CaWO4

We perform hybrid density functional calculation to study the energetics, electronic properties, optical transitions, and migration barriers of native defects in CaWO$_4$. Oxygen and calcium vacancies are most likely to form in the absence of doping, but interstitials could also incorporate. Tungsten-related defects are unlikely to be present. The positively charged $V_{\rm O}$ and the negatively charged $V_{\rm Ca}$ are likely to form complexes. Calculated optical transition levels indicate that experimentally observed absorption and emission peaks can be attributed mainly to oxygen-related defects. Calculations of migration barriers allow us to conclude that Ca$_i^{2+}$, $V_{\rm O}^{2+}$ and O$_i^{2-}$ are highly mobile, even below room temperature. We have also examined Er dopants, finding that erbium easily substitutes on the Ca site in a positive charge state. Erbium can form complexes with $V_{\rm Ca}$ and O$_i$, which would deactivate the Er. If Er is introduced by implantation, Er interstitials are likely present, which will produce emission that is prone to spectral diffusion and blinking. Our calculated properties of Er$_i$ explain why annealing at modest temperatures allows the interstitials to move into substitutional sites and point defects to move away, resulting in stable emission.

cond-mat.mtrl-sci

Isotopically enriched epitaxial CaWO$_{4}$ thin films for Er$^{3+}$ spin-photon quantum interfaces

Rare earth ion (REI)-doped oxide thin films are attractive for the application of quantum interconnects due to their stable optical levels and scalability$^{1-3}$. Among them, Er$^{3+}$ doped CaWO$_{4}$ is promising because it possesses narrow optical linewidth transitions and a long spin coherence time$^{4-6}$. The electron spin coherence is limited at high temperatures by paramagnetic impurities and by the presence of the 14.3% $^{183}$W nuclear spin. To further increase the spin coherence time at millikelvin temperatures, where the paramagnetic impurities are frozen out, our approach is to synthesize chemically and isotopically purified thin films as a host material. We first grow non-isotopically enriched Er$^{3+}$ doped CaWO$_{4}$ thin films, which exhibit a 214(13) MHz photoluminescence (PL) inhomogeneous linewidth, indicating the thin film has high crystalline quality. We then grow isotopically enriched CaWO$_{4}$ thin films using an isotopically purified $^{186}$WO$_{3}$ source. Time of flight secondary ion mass spectrometry (ToF-SIMS) was used to measure the relative concentration of W isotopes. $^{183}$W, the only W isotope that has a net nuclear spin and is the major cause of spin decoherence, was at a relative abundance of 1.2%, a factor of 10 lower than natural abundance. We also observed PL emission from single ions after integrating nano-photonic devices with the thin film. These results establish isotopically engineered CaWO$_{4}$ thin films as a promising platform for future studies of nuclear-spin-limited coherence and for scalable rare-earth-ion-based quantum nanophotonic devices.

quant-ph

Scalable Postselection of Quantum Resources

The large overhead imposed by quantum error correction is a critical challenge to the realization of quantum computers, and motivates searching for alternative error correcting codes and fault-tolerant circuit constructions. Postselection is a powerful tool that builds large programs out of probabilistically generated sub-circuits, and has been shown to increase the threshold of quantum error correction based on fusing fixed-size resource states or concatenated codes. In this work, we present an approach to lower the overhead of quantum computing using scalable postselection, based on directly postselecting sub-circuits with a size extensive in the code distance using decoder soft information. We introduce a metric, the partial gap, that estimates what the logical gap of a resource state will be after it is consumed, and show that postselection based on the partial gap leads to scalable improvements in the logical error rate. In the specific context of implementing logical gates via teleportation through a cluster state, we demonstrate that scalable postselection provides a $4\times$ reduction in the overhead per logical gate, at the same logical error probability.

quant-ph

Extended Rydberg Lifetimes in a Cryogenic Atom Array

We report on the realization of a $^{133}$Cs optical tweezer array in a cryogenic blackbody radiation (BBR) environment. By enclosing the array within a 4K radiation shield, we measure long Rydberg lifetimes, up to $406 (36)\,\mu$s for the $55 P_{3/2}$ Rydberg state, a factor of 3.3(3) longer than the room-temperature value. We employ single-photon coupling for coherent manipulation of the ground-Rydberg qubit. We measure a small differential dynamic polarizability of the transition, beneficial for reducing dephasing due to light intensity fluctuations. Our results pave the path for advancing neutral-atom two-qubit gate fidelities as their error budgets become increasingly dominated by $T_1$ relaxation of the ground-Rydberg qubit.

physics.atom-ph

Scalable accuracy gains from postselection in quantum error correcting codes

Decoding stabilizer codes such as the surface and toric codes involves evaluating free-energy differences in a disordered statistical mechanics model, in which the randomness comes from the observed pattern of error syndromes. We study the statistical distribution of logical failure rates across observed syndromes in the toric code, and show that, within the coding phase, logical failures are predominantly caused by exponentially unlikely syndromes. Therefore, postselecting on not seeing these exponentially unlikely syndrome patterns offers a scalable accuracy gain. In general, the logical error rate can be suppressed from $p_f$ to $p_f^b$, where $b \geq 2$ in general; in the specific case of the toric code with perfect syndrome measurements, we find numerically that $b = 3.1(1)$. Our arguments apply to general topological stabilizer codes, and can be extended to more general settings as long as the decoding failure probability obeys a large deviation principle.

cond-mat.stat-mech

Coherent control of interacting solid-state spins below the diffraction limit

Optically addressed atomic defects in the solid-state are widely used as single-photon sources and memories for quantum network applications. The solid-state environment allows for a high density of electron and nuclear spins with the potential to form registers for coherent information processing. However, it is challenging to reliably address individual spins at nanometer separations where interactions are large. Rare-earth ions offer a unique solution, as their narrow homogeneous optical linewidth allows frequency-domain resolution of a large number of emitters without regard to their spatial separation. In this work, we realize coherent optical and spin control of a pair of interacting Er$^{3+}$ ions, together with a nearby nuclear spin ancilla. We demonstrate two-qubit electron-electron gates and use them to perform repeated quantum non-demolition measurements on one of the Er$^{3+}$ ions. We also demonstrate electron-nuclear gates to allow coherent storage and retrieval of qubit information in a nuclear spin, and show that the nuclear spin coherence survives readout of the electron spin. These techniques can be readily scaled to larger numbers of electron and nuclear spins, paving the way for massively multiplexed quantum network nodes.

quant-ph

Microwave spectroscopy and multi-channel quantum defect analysis of ytterbium Rydberg states

The complex Rydberg structure of ytterbium atoms is shaped by multiple low-lying ion-core-excited states and strong channel interactions, which presents both opportunities and challenges for quantum information processing and precision metrology. In this work, we extend high-resolution microwave spectroscopy and multichannel quantum defect theory (MQDT) modeling of singly excited $6sn\ell$ Rydberg states in $^{174}$Yb and $^{171}$Yb to include the $\ell = 3$ ($f$) and $\ell = 4$ ($g$) series. Our measurements reveal $p$-$f$ mixing in odd-parity Rydberg states of $^{171}$Yb, which we incorporate by combined MQDT models for $6snp$ and $6snf$ series. Additionally, we observe that for $\ell = 4$ the spin-orbit interaction dominates over the exchange interaction, such that the $6sng$ states are more accurately described in a $jj$-coupled basis. We validate our models by comparing the predicted Landé $g$-factors and static dipole polarizabilities with experimental measurements, finding excellent agreement. These results provide important input for designing high-fidelity entangling gates with ytterbium atoms.

physics.atom-ph

Fast, continuous and coherent atom replacement in a neutral atom qubit array

Neutral atom quantum processors are a promising platform for scalable quantum computing. An obstacle to implementing deep quantum circuits is managing atom loss, which constitutes a significant fraction of all errors. Current approaches are either not capable of replacing lost atoms in the middle of a circuit -- and therefore restricted to fixed, short circuit depths -- or require more than an order of magnitude longer time than gate and measurement operations to do so. In this work, we demonstrate fast, continuous atom replacement leveraging the metastable $^{171}$Yb qubit. A continuously loaded reservoir near the computation zone enables on-demand atom extraction with tweezers up to 500 times per second. New qubit arrays can be prepared 30 times per second when including single-atom preparation, non-destructive imaging and initialization. Importantly, existing qubits are completely undisturbed by the reloading process, owing to the extreme isolation of the metastable qubit from cooling and imaging light. This work establishes a complete foundation for implementing fast quantum circuits with unlimited depth, removing a final roadblock for fault-tolerant quantum computing with neutral atoms.

quant-ph

Logical qubits with erasure conversion using metastable neutral atoms

Implementing large-scale quantum algorithms with practical advantage will require fault-tolerance achieved through quantum error correction, but the associated overhead is prohibitive. This overhead can be reduced by engineering physical qubits with fewer errors, and by shaping the residual errors to be more easily correctable. In this work, we demonstrate quantum error correcting codes and logical qubit circuits in a metastable ytterbium-171 nuclear spin qubit with a noise bias towards erasure errors. These errors can be located separately from any syndrome information diagnosing the error, and we demonstrate adaptive circuit execution based on erasure information. We show that dephasing errors on the qubit during coherent transport can be strongly suppressed, and implement entangling gates that maintain a high fidelity in the presence of gate beam inhomogeneity or pointing errors. Furthermore, we demonstrate logical qubit encoding in the [[4, 2, 2]] code, with error correction during decoding based on mid-circuit erasure measurements despite the fact that the code is too small to correct any Pauli errors. Finally, we demonstrate logical qubit teleportation between multiple code blocks with conditionally selected ancillas based on mid-circuit erasure checks, a key part of leakage-robust error correction schemes using neutral atoms.

quant-ph

Enhancement of Microwave to Optical Spin-Based Quantum Transduction via a Magnon Mode

We propose a new method for converting single microwave photons to single optical sideband photons based on spinful impurities in magnetic materials. This hybrid system is advantageous over previous proposals because (i) the implementation allows much higher transduction rates ($10^{3}$ times faster at the same optical pump Rabi frequency) than state-of the art devices, (ii) high-efficiency transduction is found to happen in a significantly larger space of device parameters (in particular, over $1$ GHz microwave detuning), and (iii) it does not require mode volume matching between optical and microwave resonators. We identify the needed magnetic interactions as well as potential materials systems to enable this speed-up using erbium dopants for telecom compatibility. This is an important step towards realizing high-fidelity entangling operations between remote qubits and will provide additional control of the transduction through perturbation of the magnet.

quant-ph

Spectroscopy and modeling of $^{171}$Yb Rydberg states for high-fidelity two-qubit gates

Highly excited Rydberg states and their interactions play an important role in quantum computing and simulation. These properties can be predicted accurately for alkali atoms with simple Rydberg level structures. However, an extension of these methods to more complex atoms such as alkaline-earth atoms has not been demonstrated or experimentally validated. Here, we present multichannel quantum defect (MQDT) models for highly excited $^{174}$Yb and $^{171}$Yb Rydberg states with $L \leq 2$. The models are developed using a combination of existing literature data and new, high-precision laser and microwave spectroscopy in an atomic beam, and validated by detailed comparison with experimentally measured Stark shifts and magnetic moments. We then use these models to compute interaction potentials between two Yb atoms, and find excellent agreement with direct measurements in an optical tweezer array. From the computed interaction potential, we identify an anomalous Förster resonance that likely degraded the fidelity of previous entangling gates in $^{171}$Yb using $F=3/2$ Rydberg states. We then identify a more suitable $F=1/2$ state, and achieve a state-of-the-art controlled-Z gate fidelity of $F=0.994(1)$, with the remaining error fully explained by known sources. This work establishes a solid foundation for the continued development of quantum computing, simulation and entanglement-enhanced metrology with Yb neutral atom arrays.

physics.atom-ph

Massively multiplexed nanoscale magnetometry with diamond quantum sensors

Single nitrogen vacancy (NV) centers in diamond have been used extensively for high-sensitivity nanoscale sensing, but conventional approaches use confocal microscopy to measure individual centers sequentially, limiting throughput and access to non-local physical properties. Here we design and implement a multiplexed NV sensing platform that allows us to read out many single NV centers simultaneously using a low-noise camera. Using this platform, we coherently manipulate and read out the spin states of hundreds of individual NV centers in parallel, achieving comparable magnetic field sensitivity to confocal measurements. We also implement a parallelized version of spin-to-charge-conversion readout for low NV center spin state readout noise and use it to demonstrate multiplexed covariance magnetometry, in which we measure six two-point magnetic field correlators from four NV centers simultaneously. The number of correlators we can measure is limited only by the available laser power, opening the door to massively multiplexed covariance magnetometry. Our platform significantly increases the throughput and broadens the applications of nanoscale sensing using diamond quantum sensors.

quant-ph

An instructional lab apparatus for quantum experiments with single nitrogen-vacancy centers in diamond

Hands-on experimental experience with quantum systems in the undergraduate physics curriculum provides students with a deeper understanding of quantum physics and equips them for the fast-growing quantum science industry. Here we present an experimental apparatus for performing quantum experiments with single nitrogen-vacancy (NV) centers in diamond. This apparatus is capable of basic experiments such as single-qubit initialization, rotation, and measurement, as well as more advanced experiments investigating electron-nuclear spin interactions. We describe the basic physics of the NV center and give examples of potential experiments that can be performed with this apparatus. We also discuss the options and inherent trade-offs associated with the choice of diamond samples and hardware. The apparatus described here enables students to write their own experimental control and data analysis software from scratch all within a single semester of a typical lab course, as well as to inspect the optical components and inner workings of the apparatus. We hope that this work can serve as a standalone resource for any institution that would like to integrate a quantum instructional lab into its undergraduate physics and engineering curriculum.

quant-ph

Rephasing spectral diffusion in time-bin spin-spin entanglement protocols

Generating high fidelity spin-spin entanglement is an essential task of quantum repeater networks for the distribution of quantum information across long distances. Solid-state based spin-photon interfaces are promising candidates to realize nodes of a quantum network, but are often limited by spectral diffusion of the optical transition, which results in phase errors on the entangled states. Here, we introduce a method to correct phase errors from quasi-static frequency fluctuations after the entangled state is generated, by shelving the emitters in the excited state to refocus the unknown phase. For quasi-static frequency fluctuations, the fidelity is determined only by the lifetime of the excited state used for shelving, making it particularly suitable for systems with a long-lived shelving state with correlated spectral diffusion. Such a shelving state may be found in Kramers doublet systems such as rare-earth emitters and color centers in Si or SiC interfaced with nanophotonic cavities with a strongly frequency-dependent Purcell enhancement. The protocol can be used to generate high-fidelity entangled spin pairs without reducing the rate of entanglement generation.

quant-ph

Spin-photon entanglement of a single Er$^{3+}$ ion in the telecom band

Long-distance quantum communication using quantum repeaters is an enabling technology for secure communication, distributed quantum computing and quantum-enhanced sensing and metrology. As a building block of quantum repeaters, spin-photon entanglement has been demonstrated with both atomic and solid-state qubits. However, previously demonstrated qubits with long spin coherence do not directly emit photons into the low-loss telecom band that is needed for long-distance communication. Here, we demonstrate spin-photon entanglement using a single Er$^{3+}$ ion in a solid-state crystal, integrated into a silicon nanophotonic circuit. Direct emission into the telecom band enables an entanglement rate of 1.48 Hz over 15.6 km of optical fiber, with a fidelity of 73(3)$\%$. This opens the door to large-scale quantum networks based on scalable nanophotonic devices and many spectrally multiplexed Er$^{3+}$ ions.

quant-ph

High threshold codes for neutral atom qubits with biased erasure errors

The requirements for fault-tolerant quantum error correction can be simplified by leveraging structure in the noise of the underlying hardware. In this work, we identify a new type of structured noise motivated by neutral atom qubits, biased erasure errors, which arises when qubit errors are dominated by detectable leakage from only one of the computational states of the qubit. We study the performance of this model using gate-level simulations of the XZZX surface code. Using the predicted erasure fraction and bias of metastable $^{171}$Yb qubits, we find a threshold of 8.2% for two-qubit gate errors, which is 1.9 times higher than the threshold for unbiased erasures, and 7.5 times higher than the threshold for depolarizing errors. Surprisingly, the improved threshold is achieved without bias-preserving controlled-not gates, and instead results from the lower noise entropy in this model. We also introduce an XZZX cluster state construction for measurement-based error correction, hybrid-fusion, that is optimized for this noise model. By combining fusion operations and deterministic entangling gates, this construction preserves the intrinsic symmetry of the XZZX code, leading to a higher threshold of 10.3% and enabling the use of rectangular codes with fewer qubits. We discuss a potential physical implementation using a single plane of atoms and moveable tweezers.

quant-ph