arXiv subjects

Jeffrey Holzgrafe

Publications and source records attributed to Jeffrey Holzgrafe.

11 recordsLinked to original sources

arXiv2025

Coherent control of a superconducting qubit using light

Quantum communications technologies require a network of quantum processors connected with low loss and low noise communication channels capable of distributing entangled states. Superconducting microwave qubits operating in cryogenic environments have emerged as promising candidates for quantum processor nodes. However, scaling these systems is challenging because they require bulky microwave components with high thermal loads that can quickly overwhelm the cooling power of a dilution refrigerator. Telecommunication frequency optical signals, meanwhile, can be fabricated in significantly smaller form factors while avoiding challenges due to high signal loss, noise sensitivity, and thermal loads due to their high carrier frequency and propagation in silica optical fibers. Transduction of information via coherent links between optical and microwave frequencies is therefore critical to leverage the advantages of optics for superconducting microwave qubits, while also enabling superconducting processors to be linked with low-loss optical interconnects. Here, we demonstrate coherent optical control of a superconducting qubit. We achieve this by developing a microwave-optical quantum transducer that operates with up to 1.18% conversion efficiency with low added microwave noise, and demonstrate optically-driven Rabi oscillations in a superconducting qubit.

quant-ph↗

arXiv2022

Reduced Material Loss in Thin-film Lithium Niobate Waveguides

Thin-film lithium niobate has shown promise for scalable applications ranging from single-photon sources to high-bandwidth data communication systems. Realization of the next generation high-performance classical and quantum devices, however, requires much lower optical losses than the current state of the art ($\sim$10 million). Unfortunately, material limitations of ion-sliced thin-film lithium niobate have not been explored, and therefore it is unclear how high-quality factor can be achieved in this platform. Here we evaluate the material limited quality factor of thin-film lithium niobate photonic platform can be as high as $Q\approx 1.8\times10^{8}$ at telecommunication wavelengths, corresponding to a propagation loss of 0.2 dB/m.

physics.optics↗

arXiv2021

Optically-Heralded Entanglement of Superconducting Systems in Quantum Networks

Networking superconducting quantum computers is a longstanding challenge in quantum science. The typical approach has been to cascade transducers: converting to optical frequencies at the transmitter and to microwave frequencies at the receiver. However, the small microwave-optical coupling and added noise have proven formidable obstacles. Instead, we propose optical networking via heralding end-to-end entanglement with one detected photon and teleportation. In contrast to cascaded direct transduction, our scheme absorbs the low optical-microwave coupling efficiency into the heralding step, thus breaking the rate-fidelity trade-off. Moreover, this technique unifies and simplifies entanglement generation between superconducting devices and other physical modalities in quantum networks.

quant-ph↗

arXiv2021

Integrated photonics on thin-film lithium niobate

Lithium niobate (LN), an outstanding and versatile material, has influenced our daily life for decades: from enabling high-speed optical communications that form the backbone of the Internet to realizing radio-frequency filtering used in our cell phones. This half-century-old material is currently embracing a revolution in thin-film LN integrated photonics. The success of manufacturing wafer-scale, high-quality, thin films of LN on insulator (LNOI), accompanied with breakthroughs in nanofabrication techniques, have made high-performance integrated nanophotonic components possible. With rapid development in the past few years, some of these thin-film LN devices, such as optical modulators and nonlinear wavelength converters, have already outperformed their legacy counterparts realized in bulk LN crystals. Furthermore, the nanophotonic integration enabled ultra-low-loss resonators in LN, which unlocked many novel applications such as optical frequency combs and quantum transducers. In this Review, we cover -- from basic principles to the state of the art -- the diverse aspects of integrated thin-film LN photonics, including the materials, basic passive components, and various active devices based on electro-optics, all-optical nonlinearities, and acousto-optics. We also identify challenges that this platform is currently facing and point out future opportunities. The field of integrated LNOI photonics is advancing rapidly and poised to make critical impacts on a broad range of applications in communication, signal processing, and quantum information.

physics.optics↗

arXiv2020

Reconfigurable electro-optic frequency shifter

Here we demonstrate an on-chip electro-optic frequency shifter that is precisely controlled using only a single-tone microwave signal. This is accomplished by engineering the density of states of, and coupling between, optical modes in ultra-low loss electro-optic waveguides and resonators realized in lithium niobate nanophotonics. Our device provides frequency shifts as high as 28 GHz with measured shift efficiencies of ~99% and insertion loss of <0.5 dB. Importantly, the device can be reconfigured as a tunable frequency-domain beam splitter, in which the splitting ratio and splitting frequency are controlled by microwave power and frequency, respectively. Using the device, we also demonstrate (non-blocking) frequency routing through an efficient exchange of information between two distinct frequency channels, i.e. swap operation. Finally, we show that our scheme can be scaled to achieve cascaded frequency shifts beyond 100 GHz. Our device could become an essential building-block for future high-speed and large-scale classical information processors as well as emerging frequency-domain photonic quantum computers.

physics.optics↗

arXiv2020

Cavity electro-optics in thin-film lithium niobate for efficient microwave-to-optical transduction

Linking superconducting quantum devices to optical fibers via microwave-optical quantum transducers may enable large scale quantum networks. For this application, transducers based on the Pockels electro-optic (EO) effect are promising for their direct conversion mechanism, high bandwidth, and potential for low-noise operation. However, previously demonstrated EO transducers require large optical pump power to overcome weak EO coupling and reach high efficiency. Here, we create an EO transducer in thin-film lithium niobate, leveraging the low optical loss and strong EO coupling in this platform. We demonstrate a transduction efficiency of up to $2.7\times10^{-5}$, and a pump-power normalized efficiency of $1.9\times10^{-6}/\mathrm{μW}$. The transduction efficiency can be improved by further reducing the microwave resonator's piezoelectric coupling to acoustic modes, increasing the optical resonator quality factor to previously demonstrated levels, and changing the electrode geometry for enhanced EO coupling. We expect that with further development, EO transducers in thin-film lithium niobate can achieve near-unity efficiency with low optical pump power.

quant-ph↗

arXiv2019

Quantum interference of electromechanically stabilized emitters in nanophotonic devices

Photon-mediated coupling between distant matter qubits may enable secure communication over long distances, the implementation of distributed quantum computing schemes, and the exploration of new regimes of many-body quantum dynamics. Nanophotonic devices coupled to solid-state quantum emitters represent a promising approach towards realization of these goals, as they combine strong light-matter interaction and high photon collection efficiencies. However, the scalability of these approaches is limited by the frequency mismatch between solid-state emitters and the instability of their optical transitions. Here we present a nano-electromechanical platform for stabilization and tuning of optical transitions of silicon-vacancy (SiV) color centers in diamond nanophotonic devices by dynamically controlling their strain environments. This strain-based tuning scheme has sufficient range and bandwidth to alleviate the spectral mismatch between individual SiV centers. Using strain, we ensure overlap between color center optical transitions and observe an entangled superradiant state by measuring correlations of photons collected from the diamond waveguide. This platform for tuning spectrally stable color centers in nanophotonic waveguides and resonators constitutes an important step towards a scalable quantum network.

physics.app-ph↗

arXiv2019

Nanoscale NMR Spectroscopy using Self-Calibrating Nanodiamond Quantum Sensors

Conventional nuclear magnetic resonance (NMR) spectroscopy relies on acquiring signal from a macroscopic ensemble of molecules to gain information about molecular structure and dynamics. Transferring this technique to nanoscale sample sizes would enable molecular analysis without the effects of averaging over spatial and temporal inhomogeneities and without the need for macroscopic volumes of analyte, both inherent to large ensemble measurements. Nanoscale NMR based on nitrogen vacancy (NV) centers inside bulk diamond chips achieves single nuclear spin sensitivity and the resolution required to determine chemical structure, but their detection volume is limited to a few nanometers above the diamond surface for the most sensitive devices. This precludes them from use for nuclear spin sensing with nanoscale resolution inside thicker structures, such as cells. Here, we demonstrate the detection of NMR signals from multiple nuclear species in a (19 nm)3 volume using versatile NV-NMR devices inside nanodiamonds that have a typical 30 nm diameter. The devices detect a signal generated by a small number of analyte molecules on the order of 1000. To use these devices in situ, the detected signal must be corrected for the unknown geometry of each nanodiamond device. We show that such a calibration could be performed by exploiting the signal from a thin layer of nuclei on the diamond surface. These results, combined with the low toxicity of nanodiamonds and their amenability to surface functionalization, indicate that nanodiamond NV-NMR devices could become a useful tool for nanoscale NMR-based sensing inside living cells.

cond-mat.mes-hall↗

arXiv2018

Error Corrected Spin-State Readout in a Nanodiamond

Quantum state readout is a key component of quantum technologies, including applications in sensing, computation, and secure communication. Readout fidelity can be enhanced by repeating readouts. However, the number of repeated readouts is limited by measurement backaction, which changes the quantum state that is measured. This detrimental effect can be overcome by storing the quantum state in an ancilla qubit, chosen to be robust against measurement backaction and to allow error correction. Here, we protect the electronic-spin state of a diamond nitrogen-vacancy center from measurement backaction using a robust multilevel 14N nuclear spin memory and perform repetitive readout, as demonstrated in previous work on bulk diamond devices. We achieve additional protection using error correction based on the quantum logic of coherent feedback to reverse measurement backaction. The repetitive spin readout scheme provides a 13-fold enhancement of readout fidelity over conventional readout and the error correction a 2-fold improvement in the signal. These experiments demonstrate full quantum control of a nitrogen vacancy center electronic spin coupled to its host 14N nuclear spin inside a ~25 nm nanodiamond, creating a sensitive and biologically compatible platform for nanoscale quantum sensing. Our error-corrected repetitive readout scheme is particularly useful for quadrupolar nuclear magnetic resonance imaging in the low magnetic field regime where conventional repetitive readout suffers from strong measurement backaction. More broadly, methods for correcting longitudinal (bit-flip) errors described here could be used to improve quantum algorithms that require nonvolatile local memory, such as correlation spectroscopy measurements for high resolution sensing.

quant-ph↗

arXiv2018

Controlling the coherence of a diamond spin qubit through strain engineering

The uncontrolled interaction of a quantum system with its environment is detrimental for quantum coherence. In the context of solid-state qubits, techniques to mitigate the impact of fluctuating electric and magnetic fields from the environment are well-developed. In contrast, suppression of decoherence from thermal lattice vibrations is typically achieved only by lowering the temperature of operation. Here, we use a nano-electro-mechanical system (NEMS) to mitigate the effect of thermal phonons on a solid-state quantum emitter without changing the system temperature. We study the silicon-vacancy (SiV) colour centre in diamond which has optical and spin transitions that are highly sensitive to phonons. First, we show that its electronic orbitals are highly susceptible to local strain, leading to its high sensitivity to phonons. By controlling the strain environment, we manipulate the electronic levels of the emitter to probe, control, and eventually, suppress its interaction with the thermal phonon bath. Strain control allows for both an impressive range of optical tunability and significantly improved spin coherence. Finally, our findings indicate that it may be possible to achieve strong coupling between the SiV spin and single phonons, which can lead to the realisation of phonon-mediated quantum gates and nonlinear quantum phononics.

quant-ph↗

arXiv2018

Strain engineering of the silicon-vacancy center in diamond

We control the electronic structure of the silicon-vacancy (SiV) color-center in diamond by changing its static strain environment with a nano-electro-mechanical system. This allows deterministic and local tuning of SiV optical and spin transition frequencies over a wide range, an essential step towards multi-qubit networks. In the process, we infer the strain Hamiltonian of the SiV revealing large strain susceptibilities of order 1 PHz/strain for the electronic orbital states. We identify regimes where the spin-orbit interaction results in a large strain suseptibility of order 100 THz/strain for spin transitions, and propose an experiment where the SiV spin is strongly coupled to a nanomechanical resonator.

quant-ph↗