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Jeffrey J. Schwartz

Publications and source records attributed to Jeffrey J. Schwartz.

2 recordsLinked to original sources

Interlayer Fermi Polarons in Bilayer MoTe$_2$

Atomic bilayers of transition metal dichalcogenides (TMDs) host quantum phases governed by the layer degree of freedom, including bilayer Wigner crystals, fractional Chern insulators, and exciton condensates. These phases are probed primarily through exciton spectroscopy, yet it remains poorly understood how excitons and carriers interact to form Fermi polarons in bilayers, where both the impurity and the Fermi sea carry a layer pseudospin. Progress has been limited because most TMD bilayers have momentum-indirect optical bandgaps, in which non-radiative decay and inhomogeneous broadening obscure the intrinsic spectra. Here, we show that bilayer MoTe$_2$, unlike most TMD bilayers, retains a direct optical bandgap, providing a clean platform for studying bilayer Fermi-polaron physics. In a dual-gated device, an out-of-plane electric field continuously tunes the hybridization between intralayer and interlayer excitons, forming layer-coherent excitons. Upon electrostatic doping, the excitonic spectrum evolves into multiple polaron branches, controlled by both carrier doping and the out-of-plane electric field. Among these, we identify a polaron with no analog in monolayers, in which a layer-coherent exciton is dressed by carriers in the opposite layer, and is quantitatively captured by our field-theoretic model. Our results establish that pseudospin structure in both the impurity and the bath reshapes polaron formation, opening new avenues to many-body states such as Bose-Einstein condensates with interlayer coherence.

cond-mat.mes-hall↗

Assembly of High-Performance van der Waals Devices Using Commercial Polyvinyl Chloride Films

Control over the position, orientation, and stacking order of two-dimensional (2D) materials within van der Waals heterostructures is crucial for applications in electronics, spintronics, optics, and sensing. The most popular strategy for assembling 2D materials uses purpose-built stamps with working surfaces made from one of several different polymers. However, these stamps typically require tedious preparation steps and suffer from poor durability, contamination, and limited applicability to specific 2D materials or surfaces. Here, we demonstrate significant improvements upon current 2D flake transfer and assembly practices by using mechanically durable stamps made from polyvinyl chloride (PVC) thin films. These stamps are simpler to prepare compared with existing methods and can withstand multiple transfer cycles, enabling greater reusability. We use two commercially available PVC films with distinct pick-up and release temperatures. Together, these films also enable polymer-to-polymer flake transfers and stack-and-flip fabrication of inverted heterostructures in one seamless process. Systematic comparisons of cleaning processes confirm the removal of PVC-derived residue from the assembled structures to create atomically clean interfaces. We demonstrate the utility and versatility of these polymer films and transfer process by fabricating graphene/hexagonal boron nitride heterostructure devices with high-performance electrical characteristics. Further, we demonstrate the ability to pick up and to deposit bulk aluminum gallium arsenide nanostructured films, enabling the creation of heterogeneously integrated devices. This technique increases fabrication rates, improves device quality, and enables more complex structures, thereby facilitating nanomaterial assembly in a broad range of applications.

cond-mat.mtrl-sci↗