arXiv subjects
Publications and source records attributed to Jens Eggers.
The nonlinear breakup dynamics of a strip of active chiral fluid is considered, and it is shown that the strip thickness goes to zero as a power law in finite time. Applying slender body theory to the hydrodynamic equations of active chiral fluids, we predict the exponents analytically, and our predictions are shown to be in excellent agreement with numerical simulations. Qualitative agreement between experiment and simulation is also found.
Steady tip streaming in the vanishing flow rate limit has been evidenced both experimentally and numerically in the literature. However, local conical Stokes flow solutions supporting these results at vanishing small scales around the emitting tip have remained elusive. This work presents approximate local conical solutions in liquid-liquid flow focusing and tip streaming, in general, as the limit of a macroscopic vanishing issued flow rate. This provides mathematical foundations for the existence of an asymptotically vanishing scale at the tip of an intermediate conical flow geometry with angle $α$. For a sufficiently small inner-to-outer liquid viscosity ratio $λ$, these solutions exhibit a universal power-law relationship between this ratio and the cone angle as $α=k λ^{1/2}$, where the prefactor $k$, of the order of unity, depends on the geometric details of the macroscopic flow. This confirms the existing proposals that anticipate the use of flow focusing and tip streaming technologies for tight control of microscopic scales, down to those where diffuse liquid-liquid interfaces become manifested.
Despite the large body of research on coalescence, firm agreement between experiment, theory, and computation has not been established for the very first moments following the initial contact of two liquid volumes. Combining a range of experimental and computational modeling approaches in two different geometries, namely drop-drop and drop-bath configurations, we have been able to elucidate the influence of the intervening gas and van der Waals forces on coalescence. For simple liquids considered here, the gas influences both pre- and post-contact regimes, with jump-to-contact being the primary mode of merging. Subsequently, wave-like air pockets are observed and ultimately influence the initial opening dynamics of the neck.
The viscoelastic relaxation time of a polymer solution is often measured using Capillary Breakup Extensional Rheometry (CaBER) where a droplet is placed between two plates which are pulled apart to form a thinning filament. For a slow plate retraction protocol, required to avoid inertio-capillary oscillations for low-viscosity liquids, we show experimentally that the CaBER relaxation time $τ_e$ inferred from the exponential thinning regime is in fact an apparent relaxation time that may increase significantly when increasing the plate diameter and the droplet volume. Similarly, we observe that $τ_e$ increases with the plate diameter for the classical step-strain plate separation protocol of a commercial (Haake) CaBER device and increases with the nozzle diameter for a Dripping-onto-Substrate (DoS) method. This dependence on the flow history before the formation of the viscoelastic filament is in contradiction with polymer models such as Oldroyd-B that predict a filament thinning rate $1/3τ$ ($τ$ being the model's relaxation time) which is a material property independent of geometrical factors. We show that this is not due to artefacts such as solvent evaporation or polymer degradation and that it can only be rationalised by finite extensibility effects (FENE-P model) for a dilute polymer solution in a viscous solvent, but not for semi-dilute solutions in a low-viscosity solvent.
We calculate the effective forces on hard disks near walls embedded inside active nematic liquid crystals. When the disks are sufficiently close to the wall and the flows are sufficiently slow, we can obtain exact expressions for the effective forces. We find these forces and the dynamics of disks near the wall depend both on the properties of the active nematic and on the anchoring conditions on the disks and the wall. Our results show that the presence of active stresses attract planar anchored disks to walls if the activity is extensile, and repel them if contractile. For normal anchored disks the reverse is true; they are attracted in contractile systems, and repelled in extensile ones.
The classical Cox-Voinov theory of contact line motion provides a relation between the macroscopically observable contact angle, and the microscopic wetting angle as a function of contact line velocity. Here we investigate how viscoelasticity, specifically the normal stress effect, modifies wetting dynamics. Using the thin film equation for the second-order fluid, it is found that the normal stress effect is dominant at small scales. We show that the effect can be incorporated in the Cox-Voinov theory through an apparent microscopic angle, which differs from the true microscopic angle. The theory is applied to the classical problems of drop spreading and dip-coating, which shows how normal stress facilitates (inhibits) the motion of advancing (receding) contact lines. For rapid advancing motion, the apparent microscopic angle can tend to zero in which case the dynamics is described by a new regime that was already anticipated in Boudaoud (2007).
We consider a suspension of non-interacting flat elastic particles in a Newtonian fluid. We model a flat shape as three beads, carried along by the flow according to Stokes' law, and connected by nonlinear springs, chosen such that the energy is quadratic in the area. In analogy with common dumbbell models involving two beads connected by linear springs, we solve the stochastic equations of motion exactly to compute the constitutive law for the stress tensor of a flat elastic particle suspension. A lower convected time derivative naturally arises as part of the constitutive law, but surprisingly the rheological response in strong extensional and strong contracting flows is similar to that of the classical Oldroyd-B model associated with dumbbell suspensions.
We consider a confined sheared active polar liquid crystal with a uniform orientation and study the effect of variations in the magnitude of polarization. Restricting our analysis to one-dimensional geometries, we demonstrate that with asymmetric boundary conditions, this system is characterized, macroscopically, by a linear shear stress vs. shear strain relationship that does not pass through the origin: At a zero strain rate, the fluid sustains a non-zero stress. Analytic solutions for the polarization, density, and velocity fields are derived for asymptotically large or small systems and are shown by comparison with precise numerical solutions to be good approximations for finite-size systems.
The E(xplicit)I(implicit)N(null) method was developed recently to remove numerical instability from PDEs, adding and subtracting an operator $\mathcal{D}$ of arbitrary structure, treating the operator implicitly in one case, and explicitly in the other. Here we extend this idea by devising an adaptive procedure to find an optimal approximation for $\mathcal{D}$. We propose a measure of the numerical error which detects numerical instabilities across all wavelengths, and adjust each Fourier component of $\mathcal{D}$ to the smallest value such that numerical instability is suppressed. We show that for a number of nonlinear and non-local PDEs, in one and two dimensions, the spectrum of $\mathcal{D}$ adapts automatically and dynamically to the theoretical result for marginal stability. Our method thus has the same stability properties as a fully implicit method, while only requiring the computational cost comparable to an explicit solver. The adaptive implicit part is diagonal in Fourier space, and thus leads to minimal overhead compared to the explicit method.
In this paper we compute the linear stability of similarity solutions of the breakup of viscous liquid threads, in which the viscosity and inertia of the liquid are in balance with the surface tension. The stability of the similarity solution is determined using numerical continuation to find the dominant eigenvalues. Stability of the first two solutions (those with largest minimum radius) is considered. We find that the first similarity solution, which is the one seen in experiments and simulations, is linearly stable with a complex nontrivial eigenvalue, which could explain the phenomenon of break-up producing sequences of small satellite droplets of decreasing radius near a main pinch-off point. The second solution is seen to be linearly unstable. These linear stability results compare favorably to numerical simulations for the stable similarity solution, while a profile starting near the unstable similarity solution is shown to very rapidly leave the linear regime.
A slender thread of elastic hydrogel is susceptible to a surface instability that is reminiscent of the classical Rayleigh-Plateau instability of liquid jets. The final, highly nonlinear states that are observed in experiments arise from a competition between capillarity and large elastic deformations. Combining a slender analysis and fully three-dimensional numerical simulations, we present the phase map of all possible morphologies for an unstable neo-Hookean cylinder subjected to capillary forces. Interestingly, for softer cylinders we find the coexistence of two distinct configurations, namely, cylinders-on-a-string and beads-on-a-string. It is shown that for a given set of parameters, the final pattern is selected via a dynamical evolution. To capture this, we compute the dispersion relation and determine the characteristic wavelength of the dynamically selected profiles. The validity of the "slender" results is confirmed via simulations and these results are consistent with experiments on elastic and viscoelastic threads.
Numerous physical models have been proposed to explain how cell motility emerges from internal activity, mostly focused on how crawling motion arises from internal processes. Here we offer a classification of self-propulsion mechanisms based on general physical principles, showing that crawling is not the only way for cells to move on a substrate. We consider a thin drop of active matter on a planar substrate and fully characterize its autonomous motion for all three possible sources of driving: (i) the stresses induced in the bulk by active components, which allow in particular tractionless motion, (ii) the self-propulsion of active components at the substrate, which gives rise to crawling motion, and (iii) a net capillary force, possibly self-generated, and coupled to internal activity. We determine travelling-wave solutions to the lubrication equations as a function of a dimensionless activity parameter for each mode of motion. Numerical simulations are used to characterize the drop motion over a wide range of activity magnitudes, and explicit analytical solutions in excellent agreement with the simulations are derived in the weak-activity regime.
We report on a new mode of self-propulsion exhibited by compact drops of active liquids on a substrate which, remarkably, is tractionless, i.e., which imparts no mechanical stress locally on the surface. We show, both analytically and by numerical simulation, that the equations of motion for an active nematic drop possess a simple self-propelling solution, with no traction on the solid surface and in which the direction of motion is controlled by the winding of the nematic director field across the drop height. The physics underlying this mode of motion has the same origins as that giving rise to the zero viscosity observed in bacterial suspensions. This topologically protected tractionless self-propusion provides a robust physical mechanism for efficient cell migration in crowded environments like tissues.
We point out unconventional mechanical properties of confined active fluids, such as bacterial suspensions, under shear. Using a minimal model of an active liquid crystal with no free parameters, we predict the existence of a window of bacteria concentration for which a suspension of \textit{E.~Coli} effectively behaves, at steady-state, as a negative viscosity fluid and reach quantitative agreement with experimental measurements. Our theoretical analysis further shows that a negative apparent viscosity is due to a non-monotonic local velocity profile, and is associated with a non-monotonic stress vs. strain rate flow curve. This implies that fixed stress and fixed strain rate ensembles are not equivalent for active fluids.
Bringing a rigid object into contact with a soft elastic tube causes the tube to conform to the surface of the object, resulting in contact lines. The curvature of the tube walls near these contact lines is often large and is typically regularized by the finite bending rigidity of the tube. Here, we show using experiments and a Föppl--von Kármán-like theory that a second mechanism of curvature regularization occurs when the tube is axially stretched. The radius of curvature obtained is unrelated to the bending rigidity of the tube walls, increases with the applied stretching force and decreases with sheet thickness, in contrast with the effects of finite bending rigidity. %Moreover, the axial force decreases the contact area between the tube and the intruding object, potentially reducing the drag necessary to propel the object through the tube. We show that these features are due to an interplay between geometry and mechanics specific to elastic tubes, but one that is absent from both planar sheets and spherical shells.
We propose a novel microfluidic "opposed-flow" geometry in which the continuous fluid phase is fed into a junction in a direction opposite the dispersed phase. This pulls out the dispersed phase into a micron-sized jet, which decays into micron-sized droplets. As the driving pressure is tuned to a critical value, the jet radius vanishes as a power law down to sizes below 1 $μ$m. By contrast, the conventional "coflowing" junction leads to a first order jetting transition, in which the jet disappears at a finite radius of several $μ$m, to give way to a "dripping" state, resulting in much larger droplets. We demonstrate the effectiveness of our method by producing the first microfluidic silicone oil emulsions with a sub micron particle radius, and utilize these droplets to produce colloidal clusters.
We present a novel framework for the study of disclinations in two-dimensional active nematic liquid crystals, and topological defects in general. The order tensor formalism is used to calculate exact multi-particle solutions of the linearized static equations inside a uniformly aligned state. Topological charge conservation requires a fixed difference between the number of half charges. Starting from a set of hydrodynamic equations, we derive a low-dimensional dynamical system for the parameters of the static solutions, which describes the motion of a half-disclination pair, or of several pairs. Within this formalism, we model defect production and annihilation, as observed in experiments. Our dynamics also provide an estimate for the critical density at which production and annihilation rates are balanced.
We consider a free liquid sheet, taking into account the dependence of surface tension on temperature, or concentration of some pollutant. The sheet dynamics are described within a long-wavelength description. In the presence of viscosity, local thinning of the sheet is driven by a strong temperature gradient across the pinch region, resembling a shock. As a result, for long times the sheet thins exponentially, leading to breakup. We describe the quasi one-dimensional thickness, velocity, and temperature profiles in the pinch region in terms of similarity solutions, which posses a universal structure. Our analytical description agrees quantitatively with numerical simulations.