arXiv subjects

Jens Limpert

Publications and source records attributed to Jens Limpert.

At least 19 recordsLinked to original sources

arXiv2025

Unleashing HHG Efficiency: The Role of Driving Pulse Duration

High harmonic generation (HHG) is a crucial technology for compact, high-brightness extreme ultraviolet (XUV) and soft X-ray sources, which are key to advancing both fundamental and applied sciences. The availability of advanced driving lasers, with tunable wavelength, power, and pulse duration, opens new opportunities for optimizing HHG-based sources. While scaling laws for wavelength are well understood, this work focuses on how pulse duration impacts HHG efficiency and introduces a unified framework that links microscopic dynamics to macroscopic performance. We establish a practical scaling law for the single-atom dipole moment under phase-matching conditions, demonstrating a 1/t dependence at 515 nm wavelength. By connecting this microscopic scaling to macroscopic conversion efficiency, we provide clear guidelines for optimizing HHG output across different gases and driving wavelengths. Furthermore, we identify fundamental constraints, including the carrier-envelope-phase (CEP) walk-off, which limits efficiency at longer driver wavelengths and becomes especially significant for very short pulses. All predictions are based on simple, accessible formulas, eliminating the need for complex numerical simulations. Experiments confirm these predictions and highlight when short pulses are advantageous, particularly in scenarios where CEP walk-off and absorption effects are minimized. These findings offer practical principles for designing next-generation HHG sources, capable of Watt-level average power and extended spectral reach, enabling more versatile and powerful HHG-based XUV and soft X-ray sources.

physics.optics↗

arXiv2025

Laser-driven high-flux source of coherent quasi-monochromatic extreme ultraviolet radiation for coincidence spectroscopy

We present a source of coherent extreme ultraviolet (XUV) radiation with a flux of 10$^{13}$ photons per second at 26.5 eV. The source is based on high-harmonic generation (HHG) in argon and pumped by a frequency-doubled 100 kHz repetition rate fiber laser providing 30 fs pulses centered at 515 nm. We report on the characterization of the source and the generated XUV radiation using optical imaging and photoelectron spectroscopy. The generated radiation is quasi-monochromatized using a suitably coated XUV mirror and used for coincidence spectroscopy of ions and electrons generated from a cold gas target. The high intensity of the focused XUV pulses is confirmed by the observation of two-photon double ionization in argon. Moreover, we demonstrate the capability to perform pump-probe experiments using XUV and visible laser pulses.

physics.atom-ph↗

arXiv2025

Coincidence measurement of two-photon double ionization of argon through an autoionizing resonance

We present coincidence measurements of two-photon double-ionization (TPDI) of argon driven by femtosecond pulses tunable around 26.5 eV photon energy, which are obtained from a high-harmonic generation source. The measured photoelectron spectra are interpreted with regard to three TPDI mechanisms. Theoretical predictions are obtained by an approximate model for direct TPDI and atomic structure calculations, which are implemented into a Monte Carlo simulation. The prevailing mechanism involves the excitation and prompt photoionization of an autoionizing resonance in neutral argon. We provide evidence for pronounced electron-electron interaction in this ultrafast ionization process. Furthermore, we show that the dominant TPDI mechanism can be altered by slight tuning of the photon energy. The present work paves the way for scrutinizing and controlling non-linear photoionization in the extreme ultraviolet using table-top sources.

physics.atom-ph↗

arXiv2025

Quantitative EUV ptychography reveals nanoscale morphological responses of bacteria under physiological and antibiotic stress

Table-top extreme ultraviolet (EUV) ptychography enables nanoscale, label-free, and quantitative imaging with intrinsic elemental sensitivity, offering a unique modality for subcellular profiling of bacterial morphology and composition. In this work, we apply a state-of-the-art EUV ptychographic microscope to systematically investigate the structural and compositional features of two model prokaryotic bacteria, Escherichia coli and Bacillus subtilis. With quantitative amplitude and phase reconstructions at 44 nm resolution on a tabletop, we visualize subtle phenomena during bacterial sporulation based on distinct morphological signatures. Notably, we examine the single-cell response of B. subtilis to the antibiotic monazomycin, uncovering ultrastructural disruption and compositional alterations. To further characterize the phenotypic variations, we perform multivariate statistical analysis on extracted morphological features, revealing diversity and clustering patterns associated with defined biological states. This work establishes EUV ptychography as a powerful, element-sensitive imaging platform for label-free bacterial imaging, showcasing its promise for biomedical and antimicrobial research.

physics.bio-ph↗

arXiv2023

Broadband ptychography using curved wavefront illumination

We examine the interplay between spectral bandwidth and illumination curvature in ptychography. By tailoring the divergence of the illumination, broader spectral bandwidths can be tolerated without requiring algorithmic modifications to the forward model. In particular, a strong wavefront curvature transitions a far-field diffreaction geometry to an effectively near-field one, which is lees affected by temporal coherence effects. The relaxed temporal coherence requirements allow for leveraging wider spectral bandwidths and larger illumination spots. Our findings open up new avenues towards utilizing pink and broadband beams for increased flux and throughput at both synchrotron facilities and lab-scale beamlines.

physics.optics↗

arXiv2023

High-speed and wide-field nanoscale table-top ptychographic EUV imaging and beam characterization with a sCMOS detector

We present high-speed and wide-field EUV ptychography at 13.5 nm wavelength using a table-top high-order harmonic source. By employing a scientific complementary metal oxide semiconductor (sCMOS) detector the scan time for sub-20 nm high-resolution measurements were significantly reduced by up to a factor of five. The fast frame rate of sCMOS enables wide-field imaging with a field of view of 100 μm x 100 μm with an imaging speed of 4.6 Mpix/h. Furthermore, fast EUV wavefront characterization is employed using a combination of the sCMOS detector with orthogonal probe relaxation.

physics.ins-det↗

arXiv2022

Visualizing the ultra-structure of microorganisms using table-top extreme ultraviolet imaging

Table-top extreme ultraviolet (EUV) microscopy offers unique opportunities for label-free investigation of biological samples. Here, we demonstrate ptychographic EUV imaging of two dried, unstained model specimens: germlings of a fungus (Aspergillus nidulans), and bacteria (Escherichia coli) cells at 13.5 nm wavelength. We find that the EUV spectral region, which to date has not received much attention for biological imaging, offers sufficient penetration depths for the identification of intracellular features. By implementing a position-correlated ptychography approach, we demonstrate a millimeter-squared field of view enabled by infrared illumination combined with sub-60 nm spatial resolution achieved with EUV illumination on selected regions of interest. The strong element contrast at 13.5 nm wavelength enables the identification of the nanoscale material composition inside the specimens. Our work will advance and facilitate EUV imaging applications and enable further possibilities in life science.

physics.bio-ph↗

arXiv2022

Carrier-envelope offset stable, coherently combined ytterbium-doped fiber CPA delivering 1 kW of average power

We present a carrier-envelope offset (CEO) stable ytterbium-doped fiber chirped-pulse amplification system employing the technology of coherent beam combining and delivering more than 1 kW of average power at a pulse repetition rate of 80 MHz. The CEO stability of the system is 220 mrad rms, characterized out-of-loop with an f-to-2f interferometer in a frequency offset range of 10 Hz to 20 MHz. The high-power amplification system boosts the average power of the CEO stable oscillator by five orders of magnitude while increasing the phase noise by only 100 mrad. No evidence of CEO noise deterioration due to coherent beam combining is found. Low-frequency CEO fluctuations at the chirped-pulse amplifier are suppressed by a slow loop feedback. To the best of our knowledge, this is the first demonstration of a coherently combined laser system delivering an outstanding average power and high CEO stability at the same time.

physics.optics↗

arXiv2022

The scaling potential of beam-splitter-based coherent beam combination

The impact of nonlinear refraction and residual absorption on the achievable peak and average power in beam-splitter-based coherent beam combination is analyzed theoretically. While the peak power remains limited only by the aperture size, a fundamental average power limit is given by the thermo-optical and thermo-mechanical properties of the beam splitter material and its coatings. Based on our analysis, 100 kW average power can be obtained with state-of-the-art optics at maintained high beam quality (M2 {\leq} 1.1) and at only 2% loss of combining efficiency. This result indicates that the power-scaling potential of today's beam-splitter-based coherent beam combination is far from being depleted. A potential scaling route to megawatt-level average power is discussed for optimized beam splitter geometry.

physics.optics↗

arXiv2022

Multipass cell for high-power few-cycle compression

A multipass cell for nonlinear compression to few-cycle pulse duration is introduced comprising dielectrically enhanced silver mirrors on silicon substrates. Spectral broadening with 388 W output average power and 776 μJ pulse energy is obtained at 82% cell transmission. A high output beam quality (M2<1.2) and a high spatio-spectral homogeneity (97.5%) as well as the compressibility of the output pulses to 6.9 fs duration are demonstrated. Finite element analysis reveals scalability of this cell to 2 kW average output power.

physics.optics↗

arXiv2022

Gas-plasma based generation of broadband THz radiation with 640 mW average power

We present a high-power source of broadband terahertz radiation covering the whole THz spectral region (0.1-30 THz). The two-color gas plasma generation process is driven by a state-of-the-art Ytterbium fiber chirped pulse amplification system based on coherent combination of 16 rod-type amplifiers. Prior to the THz generation, the pulses are spectrally broadened in a multi-pass-cell and compressed to 37 fs with a pulse-energy of 1.3 mJ at a repetition rate of 500 kHz. A gas-jet scheme has been employed for the THz generation, increasing the efficiency of the process to 0.1%. The air-biased-coherent-detection scheme is implemented to characterize the full bandwidth of the generated radiation. A THz average power of 640 mW is generated, which is the highest THz average power achieved to date. This makes this source suitable for a variety of applications, e.g. spectroscopy of strongly absorbing samples or driving nonlinear effects for the studies of material properties.

physics.optics↗

arXiv2022

Transverse mode instability and thermal effects in thulium-doped fiber amplifiers under high thermal loads

We experimentally analyze the average-power-scaling capabilities of ultrafast, thulium-doped fiber amplifiers. It has been theoretically predicted that thulium-doped fiber laser systems, with an emission wavelength around 2 um, should be able to withstand much higher heat-loads than their Yb-doped counterparts before the onset of transverse mode instability (TMI) is observed. In this work we experimentally verify this theoretical prediction by operating thulium doped fibers at very high heat-load. In separate experiments we analyze the performance of two different large-core, thulium-doped fiber amplifiers. The first experiment aims at operating a short, very-large core, thulium-doped fiber amplifier at extreme heat-load levels of more than 300 W/m. Even at this extreme heat-load level, the onset of TMI is not observed. The second experiment maximizes the extractable average-output power from a large-core, thulium-doped, fiber amplifier. We have achieved a pump-limited average output power of 1.15 kW without the onset of TMI. However, during a longer period of operation at this power level the amplifier performance steadily degraded and TMI could be observed for average powers in excess of 847 W thereafter. This is the first time, to the best of our knowledge, that TMI has been reported in a thulium-doped fiber amplifier.

physics.optics↗

arXiv2021

Material-specific high-resolution table-top extreme ultraviolet microscopy

Microscopy with extreme ultraviolet (EUV) radiation holds promise for high-resolution imaging with excellent material contrast, due to the short wavelength and numerous element-specific absorption edges available in this spectral range. At the same time, EUV radiation has significantly larger penetration depths than electrons. It thus enables a nano-scale view into complex three-dimensional structures that are important for material science, semiconductor metrology, and next-generation nano-devices. Here, we present high-resolution and material-specific microscopy at 13.5 nm wavelength. We combine a highly stable, high photon-flux, table-top EUV source with an interferometrically stabilized ptychography setup. By utilizing structured EUV illumination, we overcome the limitations of conventional EUV focusing optics and demonstrate high-resolution microscopy at a half-pitch lateral resolution of 16 nm. Moreover, we propose mixed-state orthogonal probe relaxation ptychography, enabling robust phase-contrast imaging over wide fields of view and long acquisition times. In this way, the complex transmission of an integrated circuit is precisely reconstructed, allowing for the classification of the material composition of mesoscopic semiconductor systems.

physics.optics↗

arXiv2021

Ultraviolet Dual Comb Spectroscopy: A Roadmap

Dual Comb Spectroscopy proved its versatile capabilities in molecular fingerprinting in different spectral regions, but not yet in the ultraviolet (UV). Unlocking this spectral window would expand fingerprinting to the electronic energy structure of matter.This will access the prime triggers of photo-chemical reactions with unprecedented spectral resolution. In this research article, we discuss the milestones marking the way to the first UV dual comb spectrometer. We present experimental and simulated studies towards UV dual comb spectroscopy, directly applied to planned absorption measurements of formaldehyde (centered at 343 nm, 3.6 eV) and argon (80 nm, 16 eV). This will enable an unparalleled relative resolution of up to $10^{-9}$ - with a table-top UV source surpassing any synchrotron linked spectrometer by at least two and any grating-based UV spectrometer by up to six orders of magnitude.

physics.optics↗

arXiv2021

1 kW, 10 mJ, 120 fs coherently combined fiber CPA laser system

An ultrafast fiber chirped-pulse amplification laser system based on coherent combination of 16 ytterbium-doped rod-type amplifiers is presented. It generates 10 mJ pulse energy at 1 kW average power and 120 fs pulse duration. A partially helium-protected, two-staged chirped-pulse amplification grating compressor is implemented to maintain the close to diffraction-limited beam quality by avoiding nonlinear absorption in air.

physics.optics↗

arXiv2021

Impact of thermo-optical effects in coherently-combined multicore fiber amplifiers

In this work we analyze the power scaling potential of amplifying multicore fibers (MCFs) used in coherently-combined systems. In particular, in this study we exemplarily consider rod-type MCFs with 2x2 up to 10x10 Ytterbium doped cores arranged in a squared pattern. We will show that, even though increasing the number of active cores will lead to higher output powers, particular attention has to be paid to arising thermal effects, which potentially degrade the performance of these systems. Additionally, we analyze the influence of the core dimensions on the extractable and combinable output power and pulse energy. This includes a detailed study on the thermal effects that influence the propagating transverse modes and, in turn, the amplification efficiency, the combining efficiency, the onset of nonlinear effect, as well as differences in the optical path lengths between the cores. Considering all these effects under rather extreme conditions, the study predicts that average output powers higher than 10 kW from a single 1 m long Ytterbium-doped MCF are feasible and femtosecond pulses with energies higher than 400 mJ can be extracted and efficiently recombined in a filled-aperture scheme.

physics.optics↗

arXiv2021

Kilowatt-average-power compression of millijoule pulses in a gas-filled multi-pass cell

We demonstrate the reliable generation of 1-mJ, 31-fs pulses with an average power of 1 kW by post-compression of 200-fs pulses from a coherently combined Yb:fiber laser system in an argon-filled Herriott-type multi-pass cell with an overall compression efficiency of 96%. We also analyze the output beam, revealing essentially no spatio-spectral couplings or beam quality loss.

physics.optics↗

arXiv2021

Fiber laser-driven gas plasma-based generation of THz radiation with 50-mW average power

We present on THz generation in the two-color gas plasma scheme driven by a high-power, ultrafast fiber laser system. The applied scheme is a promising approach for scaling the THz average power but it has been limited so far by the driving lasers to repetition rates up to 1 kHz. Here, we demonstrate recent results of THz generation operating at a two orders of magnitude higher repetition rate. This results in a unprecedented THz average power of 50 mW. The development of compact, table-top THz sources with high repetition rate and high field strength is crucial for studying nonlinear responses of materials, particle acceleration or faster data acquisition in imaging and spectroscopy.

physics.optics↗