arXiv subjects

Jeremy Upham

Publications and source records attributed to Jeremy Upham.

At least 19 recordsLinked to original sources

arXiv2026

Generating quantum entanglement from sunlight

Energy consumption is becoming a serious bottleneck for integrating quantum technologies within the existing global information infrastructure. In photonic architectures, considerable energy overheads stem from using lasers, whose high coherence was long considered indispensable for quantum state preparation. Here, we demonstrate that natural, incoherent sunlight can successfully produce quantum-entangled states via spontaneous parametric down-conversion. We detect polarization-entangled photon pairs with a concurrence of $0.905\pm0.053$ and a Bell state fidelity of $0.939\pm0.027$. Importantly, the system violates Bell's inequality with $S=2.5408\pm0.2171$, exceeding the classical threshold of 2, while maintaining generation rates comparable to laser-based setups. These findings pave the way for sustainable quantum applications in resource-limited environments like interplanetary missions.

quant-ph↗

arXiv2025

An epsilon-near-zero-based nonlinear platform for ultrafast re-writable holography

We re-examine real-time holography for all-optical structuring of light and optical computation using a contemporary material: a subwavelength-thick, spatially unstructured film of indium tin oxide (ITO). When excited by spatially structured light at epsilon-near-zero frequencies, the film acts as an efficient and reconfigurable diffractive optical platform for all-optical modulation of light such as spatial structuring and optical computations. We demonstrate a few percent of absolute diffraction efficiency over greater than 300 nm bandwidth around telecom wavelengths using a film four orders of magnitude thinner than and up to six orders of magnitude faster than standard holographic materials. Our findings highlight the potential of using epsilon-near-zero-based nanostructures for efficient modulation of spatially structured light and rapid prototyping without complex nanofabrication processes.

physics.optics↗

arXiv2025

All-optical turbulence mitigation for free-space quantum key distribution using stimulated parametric down-conversion

In this work, we propose and demonstrate a turbulence-resilient scheme for free-space quantum communication. By leveraging the phase conjugation property of stimulated parametric down-conversion, our scheme enables all-optical dynamic correction of spatial-mode distortion induced by atmospheric turbulence, thereby enhancing the secure key rate in high-dimensional quantum key distribution. We develop a theoretical model that provides detailed guidelines for selecting the optimal basis and spatial properties needed to maximize the efficiency of the proposed scheme. Both numerical simulations and experimental results show that, even under strong turbulence, our scheme can reduce the quantum error rates well below the security threshold. These results highlight the potential of nonlinear optical approaches as powerful tools for robust quantum communication in realistic free-space environments. Our work could have important implications for the practical implementation of secure quantum channels over long free-space distances.

quant-ph↗

arXiv2025

Can We Conjugate the Orbital Angular Momentum of a Single Photon with Nonlinear Optics? A Theoretical Analysis

Stimulated parametric down-conversion (StimPDC) produces an idler beam that exhibits a phase conjugate of the spatial structure of the classical seed beam. Extending this effect to the single-photon regime can, in principle, enable the control of the orbital angular momentum of single photons. However, its experimental implementation remains challenging due to the lower photon flux of realistic single-photon sources compared to a classical pump beam, which causes the StimPDC process to occur less frequently compared to its spontaneous counterpart. To overcome this, we propose a cascaded parametric down-conversion scheme, in which the signal photon from a spontaneously down-converted pair seeds the StimPDC process, while the idler photon heralds the seed's presence. This configuration uses coincidence detection to effectively post-select for stimulated events among the background of spontaneous contributions. We show that phase conjugation at the single-photon level manifests as a bias towards equal orbital angular momentum between the heralding idler and the stimulated idler. Our results offer a practical route to manipulate single-photon correlations in the orbital angular momentum degree of freedom and could have implications for applications such as free-space quantum communication and quantum-enhanced sensing.

physics.optics↗

arXiv2025

Violation of local realism with spatially multimode parametric down-conversion pumped by spatially incoherent light

We experimentally demonstrate a violation of local realism with highly spatially multimode polarization-entangled two-photon states produced by spontaneous parametric down-conversion (SPDC) pumped by a spatially incoherent light source-a light-emitting diode (LED). While existing studies have observed such a violation only by post-selecting the LED-pumped SPDC photons into a single spatial detection mode, we achieve a Clauser-Horne-Shimony-Holt inequality violation of $S = 2.532 \pm 0.069 > 2$ using a spatially multimode detection setup that collects nearly 4,080 SPDC spatial modes. These results indicate that coherent pump sources, such as lasers, are not required for SPDC-based entanglement generation. Our work could enable novel and practical sources of entangled photons for quantum technologies such as device-independent quantum key distribution and quantum-enhanced sensing.

quant-ph↗

arXiv2025

Full-field mapping of spatially varying polarization entanglement generated from spontaneous parametric down-conversion

Two-photon states generated from spontaneous parametric down-conversion (SPDC) can display entanglement in all degrees of freedom (DoFs) of light, including spatial, temporal, and polarization. The coupling between different DoFs of a two-photon state has been shown to display rich structures that enable novel and robust information processing schemes. While existing literature has studied these couplings by post-selecting the SPDC field, a comprehensive understanding of the inherent spatial-polarization coupling produced in the SPDC process is still lacking. This work produces a full spatial map of the polarization entanglement generated across the entire SPDC field, which contains an entire class of near-maximally polarization-entangled states with an average concurrence of 0.8303 +/- 0.0004. The spatial-polarization coupling manifests as radially or linearly varying polarization-entangled states, whose wavefunctions are dependent on the transverse momenta of the down-converted photons and the pump beam, respectively. Our study lays important groundwork for further exploiting the coupling between entanglement in different DoFs for future quantum technologies

quant-ph↗

arXiv2024

Efficient characterization of spatial Schmidt modes of multiphoton entangled states produced from high-gain parametric down-conversion

The ability to efficiently characterize the spatial correlations of entangled states of light is critical for applications of many quantum technologies such as quantum imaging. Here, we demonstrate highly efficient theoretical and experimental characterization of the spatial Schmidt modes and the Schmidt spectrum of bright multiphoton entangled states of light produced from high-gain parametric down-conversion. In contrast to previous studies, we exploit the approximate quasihomogeneity and isotropy of the signal field and dramatically reduce the numerical computations involved in the experimental and theoretical characterization procedures. In our particular case where our experimental data sets consist of 5000 single-shot images of 256*256 pixels each, our method reduced the overall computation time by 2 orders of magnitude. This speed-up would be even more dramatic for larger input sizes. Consequently, we are able to rapidly characterize the Schmidt modes and Schmidt spectrum for a range of pump amplitudes and study their variation with increasing gain. Our results clearly reveal the broadening of the Schmidt modes and narrowing of the Schmidt spectrum for increasing gain with good agreement between theory and experiment.

quant-ph↗

arXiv2024

Fast control of the transverse structure of a light beam using acousto-optic modulators

Fast, reprogrammable control over the transverse structure of light beams plays an essential role in applications such as structured illumination microscopy, optical trapping, and quantum information processing. Existing technologies, such as liquid crystal on silicon spatial light modulators (LCoS-SLMs) and digital micromirror devices (DMDs), suffer from limited refresh rates, low damage thresholds, and high insertion loss. Acousto-optic modulators (AOMs) can resolve the above issues, as they typically handle higher laser power and offer lower insertion loss. By effectively mapping the temporal radio-frequency (RF) waveforms onto the spatial diffraction patterns of the optical field, individual AOMs have been shown to generate one-dimensional (1D) spatial modes at a pixel refresh rate of nearly 20 MHz. We extend this concept to enable fast modulation in a two-dimensional (2D) space using a double-AOM scheme. We demonstrate the generation of 2D Hermite-Gaussian (HG_nm) modes with an average fidelity of 81%, while the highest-order mode generated, HG_53, retains a fidelity of 56%.

physics.optics↗

arXiv2024

Modeling beam propagation in a moving nonlinear medium

Fully describing light propagation in a rotating, anisotropic medium with thermal nonlinearity requires modeling the interplay between nonlinear refraction, birefringence, and the nonlinear group index. Incorporating these factors into a generalized nonlinear Schr\"odinger equation and fitting them to recent experimental results reveals two key relationships: the photon drag effect can have a nonlinear component that is dependent on the motion of the medium, and the temporal dynamics of the moving birefringent nonlinear medium create distorted figure-eight-like transverse trajectories at the output. The beam trajectory can be accurately modelled with a full understanding of the propagation effects. Efficiently modeling these effects and accurately predicting the beam's output position has implications for optimizing applications in velocimetry and beam-steering. Understanding the roles of competitive nonlinearities gives insight into the creation or suppression of nonlinear phenomena like self-action effects.

physics.optics↗

arXiv2023

Photon Number Resolving Detection with a Single-Photon Detector and Adaptive Storage Loop

Photon number resolving (PNR) measurements are beneficial or even necessary for many applications in quantum optics. Unfortunately, PNR detectors are usually large, slow, expensive, and difficult to operate. However, if the input signal is multiplexed, photon "click" detectors, that lack an intrinsic photon number resolving capability, can still be used to realize photon number resolution. Here, we investigate the operation of a single click detector, together with a storage line with tunable outcoupling. Using adaptive feedback to adjust the storage outcoupling rate, the dynamic range of the detector can in certain situations be extended by up to an order of magnitude relative to a purely passive setup. An adaptive approach can thus allow for photon number variance below the quantum shot noise limit under a wider range of conditions than using a passive multiplexing approach. This can enable applications in quantum enhanced metrology and quantum computing.

quant-ph↗

arXiv2023

Strong Reverse Saturation and Fast-Light in Ruby

We observe a strong reverse saturation of absorption in ruby at a wavelength of 473 nm. With an intensity-modulated laser, we observe that the peaks of the pulses appear more than a hundred microseconds earlier than the reference signal. A theoretical model based on coherent population oscillation would suggest a fast-light effect with an extremely large and negative group index of $-(1.7\pm0.1)\times 10^6$. We propose that this pulse advancement can also be described by time-dependent absorption of ruby. Our study helps to understand the nature of the fast- and slow-light effects in transition-metal-doped crystals such as ruby and alexandrite.

physics.optics↗

arXiv2021

Fourier-Engineered Plasmonic Lattice Resonances

Resonances in optical systems are useful for many applications, such as frequency comb generation, optical filtering, and biosensing. However, many of these applications are difficult to implement in optical metasurfaces because traditional approaches for designing multi-resonant nanostructures require significant computational and fabrication efforts. To address this challenge, we introduce the concept of Fourier lattice resonances (FLRs) in which multiple desired resonances can be chosen a priori and used to dictate the metasurface design. Because each resonance is supported by a distinct surface lattice mode, each can have a high quality factor. Here, we experimentally demonstrate several metasurfaces with arbitrarily placed resonances (e.g., at 1310 and 1550 nm) and Q-factors as high as 800 in a plasmonic platform. This flexible procedure requires only the computation of a single Fourier transform for its design, and is based on standard lithographic fabrication methods, allowing one to design and fabricate a metasurface to fit any specific, optical-cavity-based application. This work represents an important milestone towards the complete control over the transmission spectrum of a metasurface.

physics.optics↗

arXiv2021

Flat Magic Window

Magic windows (or mirrors) consist of optical devices with a surface deformation or thickness distribution devised in such a way to form a desired image. The associated image intensity distribution has been shown to be related to the Laplacian of the height of the surface relief. We experimentally realize such devices with flat optics employing optical spin-to-orbital angular momentum coupling, which represent a new paradigm for light manipulation. The desired pattern and experimental specifications for designing the flat optics was implemented with a re-configurable spatial light modulator which acted as the magic mirror. The flat plate, optical spin-to-orbital angular momentum coupler, is then fabricated by spatially structuring nematic liquid crystals. The plate is used to demonstrate the concept of a polarization-switchable magic window, where, depending on the input circular polarization handedness, one can display either the desired image or the image resulting from the negative of the window's phase.

physics.optics↗

arXiv2021

Cross-polarized surface lattice resonances in a rectangular lattice plasmonic metasurface

Multiresonant metasurfaces could enable many applications in filtering, sensing and nonlinear optics. However, developing a metasurface with more than one high-quality-factor or high-Q resonance at designated resonant wavelengths is challenging. Here, we experimentally demonstrate a plasmonic metasurface exhibiting different, narrow surface lattice resonances by exploiting the polarization degree of freedom where different lattice modes propagate along different dimensions of the lattice. The surface consists of aluminum nanostructures in a rectangular periodic lattice. The resulting surface lattice resonances were measured around 630 nm and 1160 nm with Q-factors of ~50 and ~800, respectively. The latter is a record-high plasmonic Q-factor within the near-infrared type-II window. Such metasurfaces could benefit applications such as frequency conversion and all-optical switching.

physics.optics↗

arXiv2021

Relaxed phase-matching constraints in zero-index waveguides

The nonlinear optical response of materials is the foundation upon which applications such as frequency conversion, all-optical signal processing, molecular spectroscopy, and nonlinear microscopy are built. However, the utility of all such parametric nonlinear optical processes is hampered by phase-matching requirements. Quasi-phase-matching, birefringent phase matching, and higher-order-mode phase matching have all been developed to address this constraint, but the methods demonstrated to date suffer from the inconvenience of only being phase-matched for a single, specific arrangement of beams, typically co-propagating, resulting in cumbersome experimental configurations and large footprints for integrated devices. Here, we experimentally demonstrate that these phase-matching requirements may be satisfied in a parametric nonlinear optical process for multiple, if not all, configurations of input and output beams when using low-index media. Our measurement constitutes the first experimental observation of direction-independent phase matching for a medium sufficiently long for phase matching concerns to be relevant. We demonstrate four-wave mixing from spectrally distinct co- and counter-propagating pump and probe beams, the backward-generation of a nonlinear signal, and excitation by an out-of-plane probe beam. These results explicitly show that the unique properties of low-index media relax traditional phase-matching constraints, which can be exploited to facilitate nonlinear interactions and miniaturize nonlinear devices, thus adding to the established exceptional properties of low-index materials.

physics.optics↗

arXiv2021

Enhanced Nonlinear Optical Responses of Layered Epsilon-Near-Zero Metamaterials at Visible Frequencies

Optical materials with vanishing dielectric permittivity, known as epsilon-near-zero (ENZ) materials, have been shown to possess enhanced nonlinear optical responses in their ENZ region. These strong nonlinear optical properties have been firmly established in homogeneous materials; however, it is as of yet unclear whether metamaterials with effective optical parameters can exhibit a similar enhancement. Here, we probe an optical ENZ metamaterial composed of a subwavelength periodic stack of alternating Ag and SiO$_2$ layers and measure a nonlinear refractive index $n_2 = (1.2 \pm 0.1) \times 10^{-12}$ m$^2$/W and nonlinear absorption coefficient $β= (-1.5 \pm 0.2) \times 10^{-5}$ m/W at its effective zero-permittivity wavelength. The measured $n_2$ is $10^7$ times larger than $n_2$ of fused silica and four times larger than that the $n_2$ of silver. We observe that the nonlinear enhancement in $n_2$ scales as $1/(n_0 \mathrm{Re}[n_0])$, where $n_0$ is the linear effective refractive index. As opposed to homogeneous ENZ materials, whose optical properties are dictated by their intrinsic material properties and hence are not widely tunable, the zero-permittivity wavelength of the demonstrated metamaterials may be chosen to lie anywhere within the visible spectrum by selecting the right thicknesses of the sub-wavelength layers. Consequently, our results offer the promise of a means to design metamaterials with large nonlinearities for applications in nanophotonics at any specified optical wavelength.

physics.optics↗

arXiv2021

Ultra-high-Q resonances in plasmonic metasurfaces

Plasmonic nanostructures hold promise for the realization of ultra-thin sub-wavelength devices, reducing power operating thresholds and enabling nonlinear optical functionality in metasurfaces. However, this promise is substantially undercut by absorption introduced by resistive losses, causing the metasurface community to turn away from plasmonics in favour of alternative material platforms (e.g., dielectrics) that provide weaker field enhancement, but more tolerable losses. Here, we report a plasmonic metasurface with a quality-factor (Q-factor) of 2340 in the telecommunication C band by exploiting surface lattice resonances (SLRs), exceeding the record by an order of magnitude. Additionally, we show that SLRs retain many of the same benefits as localized plasmonic resonances, such as field enhancement and strong confinement of light along the metal surface. Our results demonstrate that SLRs provide an exciting and unexplored method to tailor incident light fields, and could pave the way to flexible wavelength-scale devices for any optical resonating application.

physics.optics↗

arXiv2020

A nonreciprocal optical resonator with broken time-invariance for arbitrarily high time-bandwidth performance

Most present-day resonant systems, throughout physics and engineering, are characterized by a strict time-reversal symmetry between the rates of energy coupled in and out of the system, which leads to a trade-off between how long a wave can be stored in the system and the system bandwidth. Any attempt to reduce the losses of the resonant system, and hence store a (mechanical, acoustic, electronic, optical, atomic, or of any other nature) wave for more time, will inevitably also reduce the bandwidth of the system. Until recently, this time-bandwidth limit has been considered fundamental, arising from basic Fourier reciprocity. A recent theory suggested that it might in fact be overcome by breaking Lorentz reciprocity in the resonant system, reinvigorated a debate about whether (or not) this was indeed the case. Here, we report an experimental realization of a cavity where, inducing nonreciprocity by breaking the time invariance, we do overcome the fundamental time-bandwidth limit of ordinary resonant systems by a factor of 30, in full agreement with accompanying numerical simulations. We show that, although in practice experimental constraints limit our scheme, the time bandwidth product can be arbitrarily large, simply dictated by the finesse of the cavity. Our experimental realization uses a simple macroscopic, time-variant, fiber-optic cavity, where we break Lorentz reciprocity by non-adiabatically opening the cavity, injecting a pulse of large bandwidth, and then closing the cavity, storing the pulse which can be released on-demand at a later time. Our results open the path for designing resonant systems, ubiquitous in physics and engineering, that can simultaneously be broadband (i.e., ultrafast) and possessing long storage times, thereby unleashing fundamentally new functionalities in wave physics and wave-matter interactions.

physics.optics↗