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Jeroen van den Brink

Publications and source records attributed to Jeroen van den Brink.

At least 37 records · Page 2Linked to original sources

Magnetic-field tuning of the spin dynamics in the quasi-2D van der Waals antiferromagnet CuCrP$_{2}$S$_{6}$

The use of antiferromagnets in magnetoelectronic devices as counterparts of ferromagnets is a new, rapidly developing trend in spintronics that leverages antiferromagnetic (AFM) magnons for transmitting of spin currents. Van der Waals (vdW) antiferromagnets are particularly attractive in this respect as they possess tunable magnetic properties and can be easily integrated into spintronic devices. In this work we use electron spin resonance (ESR) spectroscopy to assess the potential of the vdW AFM compound CuCrP$_{2}$S$_{6}$ for magnonic applications by exploring the magnetic field ($H$) dependence of the spectrum of magnon excitations below its AFM ordering temperature $T_{\rm N} \approx 30$ K and the correlated spin dynamics above $T_{\rm N}$. ESR reveals prominent ferromagnetic (FM) spin correlations that persist far above $T_{\rm N}$ suggesting an intrinsically two-dimensional character of the spin dynamics in CuCrP$_{2}$S$_{6}$. Most interestingly, at $T < T_{\rm N}$, CuCrP$_{2}$S$_{6}$ features two non-degenerate, i.e., distinct in energy AFM magnon modes at $H = 0$ which can be tuned to the FM type of collective spin excitations with increasing $H$. These remarkable properties are favorable for the induction and control of unidirectional spin current in CuCrP$_{2}$S$_{6}$ and suggest it as a new functional material for magnetoelectronics.

cond-mat.str-el↗

Feynman paradox in a spherical axion insulator

We show that a small charged probe near a spherical topological insulator causes the latter to rotate around a symmetry axis defined by the center of the sphere and the position of the charge outside the latter. The rotation occurs when the distance from the charge to the center of the sphere is changed. This phenomenon occurs due to induced static fields and is a consequence of the axion electrodynamics underlying the electromagnetic response of a topological insulator. Assuming a regime where the charged probe can be regarded as a point charge $q=Ne$, where $N$ is a positive integer and $e$ is the elementary electric charge, we obtain that the rotation frequency is given by $ω=(Nα)^2Υ(ε,d/a)/I$, where $I$ is the moment of inertia, $α$ is the fine-structure constant, and the function $Υ$ depends on the dielectric constant $ε$ and the relative distance $d/a$ of the charge from the center of the sphere of radius $a$. Since the point charge also induces Hall currents on the surface, we compute also their associated angular momentum. This allows us to derive an exact expression for the electronic velocity on the surface as a function of $a/d$.

cond-mat.mes-hall↗

Fermi surface and topology of multiband superconductor BeAu

The chiral material BeAu was recently identified as a multiband type-I superconductor with a critical temperature of 3.2 K. As a member of the B20 crystal family (space group $P2_13$), its band structure hosts multifold fermions at high-symmetry points, unpaired Weyl points and even nodal surfaces. This renders BeAu an appealing system to investigate the interplay between superconductivity and topology. Here we present a comprehensive first-principles analysis of BeAu's electronic structure focusing on its Fermi surface's topology and the implications for superconductivity. Together with the presence of four- and six-fold fermions at high-symmetry points, we identify several additional isolated Weyl points near the Fermi level. We also determine the associated topological edge states -- the surface Fermi arcs. Computing the Chern number associated to different Fermi surface sheets, we show that BeAu harbors a $ν= 4$ topological superconducting phase in the presence of $s$-wave pairing of alternating sign ($s_\pm$ pairing). Notably, we also identify a Fermi surface with a Chern number of +6; the highest value reported to date. Finally, our analysis reveals strong inhomogeneity in the orbital character of electronic states at the Fermi level, suggesting a link to the observed multigap superconductivity.

cond-mat.supr-con↗

Non-collinear Altermagnetic Phases in the Mott Insulator NiS$_2$

Altermagnets (A$\ell$Ms) constitute a novel family of magnetic materials characterized by the absence of net magnetization and the presence of spin-polarized band structures. Whereas A$\ell$M phases were initially proposed in collinear structures, the recently discovered noncollinear chiral A$\ell$Ms stand out for their distinct hedgehog spin texture and multifunctionality in spintronics. In this work, we deepen the characterization of these systems by constructing a Landau theory for noncollinear achiral A$\ell$Ms. Furthermore, we demonstrate that the achiral symmetry of the crystal is reflected in the spin texture in reciprocal space, which presents only spatial-even multipoles. These multipoles, distinguished from those in collinear A$\ell$Ms via the high-order secondary order parameters, can couple to many phenomena such as the spin Hall effect and piezomagnetic effect. To exemplify our theory, we study the noncollinear achiral magnet NiS$_2$ within the framework of altermagnetism, showcasing both spin Hall and piezomagnetic effects in a prototypical correlated Mott insulator that provides an ideal platform to explore the interplay between strong electronic correlations, crystal symmetry, and altermagnetic spin textures. Interestingly, altermagnetism emerges in two magnetic ordered phases of NiS$_2$ upon lowering the temperature. The non-collinearity strengthens the robustness of A$\ell$M order, as the anti-ferromagnetism induced by the strong correlations will not impose effective time-reversal symmetry as in the collinear case. Our results suggest non-collinear achiral A$\ell$Ms as a promising platform for spintronics applications due to the potential to achieve various spin textures with different magnetic orders.

cond-mat.mtrl-sci↗

A Kapitza Pendulum Route to Supercurrent Tunnel Diodes

Superconducting diodes that support nonreciprocal supercurrent flow in principle constitute attractive, non-dissipative, circuit elements for superconducting electronics. But their realization faces fundamental challenges, as conventional Josephson tunnel junctions are inherently reciprocal. Existing approaches to break reciprocity typically involve magnetism or spin-orbit coupling, which often increase device complexity and limit reproducibility. Here, we demonstrate an alternative dynamical route to supercurrent nonreciprocity based on parametric driving. By applying a frequency-modulated supercurrent amplitude we show that effective higher-order, nonharmonic terms are generated in the current-phase relation. Leveraging mathematical equivalences with the Kapitza pendulum, we show that these terms dynamically break reciprocity. This establishes the concept of a Kapitza supercurrent diode and demonstrates that nonreciprocal superconducting transport can be engineered by nonequilibrium driving conventional Josephson tunnel junctions. We propose two implementations of the Kapitza supercurrent diode - via gate-controlled superconducting interferometers or flux-driven double-loop SQUIDs - to achieve nonreciprocal supercurrent transport within experimentally accessible frequencies $ω/2π\sim 1$-$10\,\mathrm{GHz}$.

cond-mat.supr-con↗

Generating ferro-spinetic polarizations in altermagnetic insulators

Altermagnets are a novel class of fully spin-compensated magnetic materials that nevertheless have spin-split electronic bands, offering novel perspectives for spintronics applications. Based on a rigorous analysis of altermagnetic many-body models and their symmetry we establish the important role of two fundamental types of polarizations in altermagnetic insulators: the charge and the spinetic one, where the latter corresponds to a macroscopic spin-displacement field. First principles calculations confirm and quantify their presence in real materials. The two polarizations are directly coupled and emerge in orthogonal directions when inversion symmetry is broken, either by the system developing a spontaneously ferroelectric polarization (in ferroelectric altermagnets), or by a charge displacement induced by an external electric field (for inversion invariant altermagnetic insulators). This presence of large and switchable spin accumulations constitute an attractive fundamental feature of altermagnetic insulators.

cond-mat.str-el↗

Real critical exponents from the $\varepsilon$-expansion in an interacting $U(1)$ model with non-Hermitian $Z_4$ anisotropy

In quantum optics and condensed matter physics non-Hermitian phenomena are often studied under the assumption of an open physical system. However, there are examples of intrinsically non-Hermitian, though often $\mathcal{PT}$ (parity-time) symmetric, not necessarily open systems, in which case the concept of gain and loss relative to an underlying environment is not primordial. A particularly intriguing example with experimental consequences in the literature is QCD at finite density. Motivated by the existence of such inherently non-Hermitian systems, here we study the critical behavior of a $U(1)$-invariant Lagrangian perturbed by a complex, $\mathcal{PT}$ symmetric $Z_{4}$ anisotropy. We find real critical exponents both in the region of unbroken and broken $\mathcal{PT}$ symmetry. In the former the coupling constants for fixed points or lines are real, whereas in the latter they become complex. Importantly, the most stable fixed point corresponds to the flow at large distances towards an effectively Hermitian $U(1)$ symmetric system. This constitutes an example where both the $U(1)$ and the Hermitian character are emergent features of the theory. This tells us about the importance and physical meaning of some non-Hermitian systems beyond interpretations involving gain and loss.

quant-ph↗

Non-Hermitian topology of quantum spin-Hall systems to detect edge-state polarization

We study the non-Hermitian topology of multi-terminal transport in a quantum spin-Hall device described by the Bernevig-Hughes-Zhang model. We show that breaking time-reversal symmetry alone does not imply non-reciprocal transport or a non-Hermitian conductance matrix. Instead, non-Hermitian topology arises only when transport becomes directionally imbalanced. We identify two distinct mechanisms that generate such a response: spin-selective coupling at the contacts and an out-of-plane Zeeman field that unbalances the counter-propagating helical edge modes. We show, for unpolarized leads, that the spin polarization-dependent response to Zeeman fields, provides a transport-based probe of the intrinsic spin polarization of the helical edge states. Moreover, we demonstrate that non-Hermitian skin effect is more sensitive than conductance elements to detect the spin polarization of the edge states. Our results clarify the conditions required for non-Hermitian topology in quantum spin-Hall transport and establish non-Hermitian skin effect as a diagnostic tool for spin-selective coupling and edge-state polarization.

cond-mat.mes-hall↗

Non-linear anomalous Edelstein response at altermagnetic interfaces

In altermagnets, time-reversal symmetry breaking spin-polarizes electronic states, while total magnetization remains zero. In addition, at altermagnetic surfaces Rashba-spin orbit coupling is activated due to broken inversion symmetry, introducing a competing spin-momentum locking interaction. Here we show that their interplay leads to the formation of complex, chiral spin textures that offer novel, non-linear spin-to-charge conversion properties. Whereas altermagnetic order suppresses the canonical linear in-plane Rashba-Edelstein response, we establish the presence of an \textit{anomalous} transversal Edelstein effect for planar applied electric and magnetic field, or alternatively, an in-plane magnetization. Additionally, we predict a purely electric-field-driven non-linear out-of-plane magnetization. We compute the anomalous response within a general altermagnet $d$-wave model, with parameters extracted from the ab-initio electronic structure of an altermagnetic bilayer. Our results suggest altermagnetic surfaces as a promising platform for unconventional spintronic functionalities.

cond-mat.mtrl-sci↗

Revealing altermagnetic Fermi surfaces with two Kondo impurities

Motivated by recent advances in the study of altermagnetism, or unconventional magnetism, and in the realization and manipulation of two-impurity Kondo physics in real materials, we propose a phase-sensitive method to explore unconventional magnetic symmetries. Our method can be implemented with spin-resolved scanning tunneling microscopy to study two-impurity Kondo phenomena on altermagnetic metals by varying the distance and orientation between magnetic impurities. Using quantum Monte Carlo simulations, we analyze the spin splitting of the Kondo resonance, whose spatial distribution sensitively captures the symmetry of the underlying altermagnetic order. Furthermore, the impurity spin correlations reflects the anisotropy of the RKKY interaction due to the altermagnetic Fermi surface splitting. This work provides a framework for studying the competition between the Kondo effect, the RKKY interaction and altermagnetism, in the simplest possible system.

cond-mat.str-el↗

Non-Hermitian topological devices with Chern insulators

Multi-terminal topological devices are a new generation of electronic devices with quantized properties robust against imperfections. In magnetic topological insulators, dissipationless edge states give functional devices in zero magnetic field, of interest for quantum metrology (resistance standard) or topological electronics (Chern networks). Here we show that a new generation of simple quantum circuits (disk, ring) with non-Hermitian topology, based on the interconnection of 1D Chern states in the quantum anomalous Hall regime, can have a much stronger quantization of their invariant than that of the Chern invariant itself, when measured in a non-metrology grade setup - that is, in industry-relevant conditions. Remarkably, the chirality-related topological skin effect is realized without the need of a magnetic field or an electrical gate, with a record degree of localization for a quantum Hall device. This new type of topological quantum devices based on magnets, with an exponential response that can be switched at small magnetic fields (about 200mT), can operate at liquid-Helium temperature with a good quantization and have some potential as cryogenic sensors for applications in high-precision impedance or magnetic field measurements.

cond-mat.mes-hall↗

Altermagnetic polarons: the fate of alter magnetic band splittings at strong coupling

While a spin-dependent band splitting is one of the characteristic features of altermagnets, the conventional band picture itself breaks down in the many altermagnets that are correlated Mott materials. We employ two numerical many-body methods, the self-consistent Born approximation and variational cluster approach, to explore this strongly correlated regime and investigate hole motion in Mott altermagnets. Our results reveal that spin-dependent spectral-weight transfer is the dominant signature of Mott altermagnetism. This pronounced spin-momentum locking of the quasiparticle spectral weight arises from the formation of altermagnetic polarons, whose dynamics are governed by the interplay between free hole motion and the coupling of the hole to magnon excitations in the altermagnet. We demonstrate this effect by calculating ARPES spectra for three canonical altermagnetic systems: the checkerboard $J$-$J'$ model, a variant describing the transition-metal--ion sites of the inverse Lieb lattice, and the Kugel-Khomskii spin-orbital altermagnet based on cubic vanadates RVO$_3$ (R=La, Pr, Nd, Y).

cond-mat.str-el↗

Magnon topology driven by altermagnetism

Altermagnets present a class of fully compensated collinear magnetic order, where the two sublattices are not related merely by time-reversal combined with lattice translation or inversion, but require an additional lattice rotation. This distinctive symmetry leads to a characteristic splitting of the magnon bands; however the splitting is only partial -- residual degeneracies persist along certain lines in the Brillouin zone as a consequence of the underlying altermagnetic rotation. We consider a two-dimensional $d$-wave altermagnetic spin model on the checkerboard lattice and introduce additional interactions such as an external magnetic field and Dzyaloshinskii-Moriya interactions, that lift these degeneracies. The resulting magnon bands become fully gapped and acquire non-trivial topology, characterized by nonzero Chern numbers. We demonstrate the crucial role of altermagnetism for the generation of the Berry curvature. As a direct consequence of the topological magnons, we find finite thermal Hall conductivity $κ_{xy}$, which exhibits a characteristic low-temperature scaling, $κ_{xy}\propto T^4$. Moreover, $κ_{xy}$ changes sign under reversal of the magnetic field, exhibiting a sharp jump across zero field at low temperatures. We also demonstrate topologically protected chiral edge modes in a finite strip geometry.

cond-mat.str-el↗

Ginzburg-Landau theory for unconventional surface superconductivity in PtBi$_2$

Recent experimental evidence suggests the presence of an unconventional, nodal surface-su\-per\-con\-duc\-ting state in trigonal PtBi\textsubscript{2}. We construct a Ginzburg--Landau theory for the three superconducting order parameters, which correspond to the three irreducible representations of the point group $C_{3v}$. The irreducible representations $A_1$ and $A_2$ are the most likely. We develop a systematic method to determine the symmetry-allowed terms and apply it to derive all terms up to fourth order in the three order parameters. The Ginzburg--Landau functional also includes coupling to the magnetic field. The functional is employed to determine the effect of an applied uniform magnetic field on the nodal structure for $A_1$ and $A_2$ pairing. The results facilitate clear-cut experimental differentiation between these symmetries. We also predict field-induced helical superconductivity.

cond-mat.supr-con↗

Room temperature Planar Hall effect in nanostructures of trigonal-PtBi2

Trigonal-PtBi2 has recently garnered significant interest as it exhibits unique superconducting topological surface states due to electron pairing on Fermi arcs connecting bulk Weyl nodes. Furthermore, topological nodal lines have been predicted in trigonal-PtBi2, and their signature was measured in magnetotransport as a dissipationless, i.e. odd under a magnetic field reversal, anomalous planar Hall effect. Understanding the topological superconducting surface state in trigonal-PtBi2 requires unravelling the intrinsic geometric properties of the normal state electronic wavefunctions and further studies of their hallmarks in charge transport characteristics are needed. In this work, we reveal the presence of a strong dissipative, i.e. even under a magnetic field reversal, planar Hall effect in PtBi2 at low magnetic fields and up to room temperature. This robust response can be attributed to the presence of Weyl nodes close to the Fermi energy. While this effect generally follows the theoretical prediction for a planar Hall effect in a Weyl semimetal, we show that it deviates from theoretical expectations at both low fields and high temperatures. We also discuss the origin of the PHE in our material, and the contributions of both the topological features in PtBi2 and its possible trivial origin. Our results strengthen the topological nature of PtBi2 and the strong influence of quantum geometric effects on the electronic transport properties of the low energy normal state.

cond-mat.mes-hall↗

Photostriction-Driven Phase Transition in Layered Chiral NbOX$_2$ Crystals: Electrical-Field-Controlled Enantiomer Selectivity

Chiral crystals offer an unique platform for controlling structural handedness through external stimuli. However, the ability to select between structural enantiomers remains challenging, both theoretically and experimentally. In this work, we demonstrate a two-step pathway for enantiomer selectivity in layered chiral NbOX$_2$ (X = Cl, Br, I) crystals based on photostriction-driven phase transitions. Ab-initio simulations reveal that optical excitation is capable of inducing a structural phase transition in NbOX$_2$ from the monoclinic ($C2$) ground state to the higher-symmetry ($C2/m$) structure. In the resulting transient high-symmetry state, an applied electric field breaks the residual inversion-symmetry degeneracy, selectively stabilizing one enantiomeric final state configuration over the other. Our results establish a combined optical-electrical control scheme for chiral materials, enabling reversible and non-contact enantiomer selection with potential applications in ultrafast switching, optoelectronics, and chiral information storage.

cond-mat.mtrl-sci↗

Axion electrodynamics of Weyl superconductors with broken time-reversal symmetry

The low-energy effective description of Weyl semimetals is defined by the axion electrodynamics, which captures the effects arising due to the presence of nodes of opposite chirality in the electronic structure. Here we explore the magnetoelectric response of time-reversal breaking (TRB) Weyl superconductors in the London regime. The influence of the axion contribution leads to an increase in the London penetration depth$-$a behavior that can be anticipated by first considering the photon spectrum of a TRB Weyl semimetal. Moreover, we find that both the Meissner state and the vortex phase feature an interplay between the electric and magnetic fields. This leads to a nonvanishing electromagnetic angular momentum, which we calculate for a number of geometrical configurations.

cond-mat.supr-con↗

Strongly Entangled Kondo and Kagome Lattices and the Emergent Magnetic Ground State in Heavy-Fermion Kagome Metal YbV$_6$Sn$_6$

Applying angle-resolved photoemission spectroscopy and density functional theory calculations, we present compelling spectroscopic evidence demonstrating the intertwining and mutual interaction between the Kondo and kagome sublattices in heavy-fermion intermetallic compound YbV$_6$Sn$_6$. We reveal the Yb 4$f$-derived states near the Fermi level, along with the presence of bulk kagome bands and topological surface states. We unveil strong interactions between the 4$f$ and itinerant electrons, where the kagome bands hosting the Dirac fermions and van Hove singularities predominate. Such findings are well described using a $c$-$f$ hybridization model. On the other hand, our systematic characterization of magnetic properties demonstrates an unusually enhanced antiferromagnetic ordering, where the kagome-derived van Hove singularities near $E_F$ play a vital role in determining the unconventional nature of the Ruderman-Kittel-Kasuya-Yosida interaction and Kondo coupling. These unique kagome-state-mediated exchange interactions have never been reported before and could lead to a novel phase diagram and various quantum critical behaviors in YbV$_6$Sn$_6$ and its siblings. Our results not only expand the family of exotic quantum phases entangled with kagome structure to the strongly correlated regime, but also establish YbV$_6$Sn$_6$ as an unprecedented platform to explore unconventional many-body physics beyond the standard Kondo picture.

cond-mat.str-el↗