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Jeroen van den Brink

Publications and source records attributed to Jeroen van den Brink.

At least 73 records · Page 4Linked to original sources

Non-Hermitian topology in the quantum Hall effect of graphene

Quantum Hall phases have recently emerged as a platform to investigate non-Hermitian topology in condensed-matter systems. This platform is particularly interesting due to its tunability, which allows to modify the properties and topology of the investigated non-Hermitian phases by tuning external parameters of the system such as the magnetic field. Here, we show the tunability of non-Hermitian topology chirality in a graphene heterostructure using a gate voltage. By changing the charge carrier density, we unveil some novel properties specific to different quantum Hall regimes. First, we find that the best quantization of the non-Hermitian topological invariant is interestingly obtained at very high filling factor rather than on well-quantized quantum Hall plateaus. This is of particular importance for the efficient operation of devices based on non-Hermitian topology. Moreover, we observe an additional non-Hermitian topological phase in the insulating nu=0 quantum Hall plateau, which survives at lower fields than the opening of the nu=0 gap, confirming a recent prediction of a disorder-induced trivial phase. Our results evidence graphene as a promising platform for the study of non-Hermitian physics and of emergent phases in such topological devices.

cond-mat.mes-hall↗

Dissipationless transport signature of topological nodal lines

Topological materials, such as topological insulators or semimetals, usually not only reveal the nontrivial properties of their electronic wavefunctions through the appearance of stable boundary modes, but also through very specific electromagnetic responses. The anisotropic longitudinal magnetoresistance of Weyl semimetals, for instance, carries the signature of the chiral anomaly of Weyl fermions. However for topological nodal line semimetals -- materials where the valence and conduction bands cross each other on one-dimensional curves in the three-dimensional Brillouin zone -- such a characteristic has been lacking. Here we report the discovery of a peculiar charge transport effect generated by topological nodal lines: a dissipationless transverse signal in the presence of coplanar electric and magnetic fields, which originates from a Zeeman-induced conversion of topological nodal lines into Weyl nodes under infinitesimally small magnetic fields. We evidence this dissipationless topological response in trigonal \ce{PtBi2} persisting up to room temperature, and unveil the extensive topological nodal lines in the band structure of this non-magnetic material. These findings provide a new pathway to engineer Weyl nodes by arbitrary small magnetic fields and reveal that bulk topological nodal lines can exhibit non-dissipative transport properties.

cond-mat.mes-hall↗

Superselection Rules, Bosonization Duality in 1+1 Dimensions and Momentum-Space Entanglement

We investigate the effects of the presence of conserved charges on the momentum-space entanglement of Quantum Field Theories (QFTs). We show that if a given model has superselection sectors, then it allows for different notions of momentum modes, each associated with a complete set of commuting observables. Applying this idea to investigate the entanglement of momentum degrees of freedom on both sides of the abelian Bosonization duality, we find that different tensor product partitions are mapped into each other and give explicit examples to sustain our findings. The conditions on which our conclusions may be generalized to other duality transformations, which require the introduction of a notion stricter than the most general possible, are laid and directions for further work are given.

hep-th↗

Fluctuation induced piezomagnetism in local moment altermagnets

It was recently discovered that, depending on their symmetries, collinear antiferromagnets may break spin degeneracy in momentum space, even in absence of spin-orbit coupling. Such systems, dubbed altermagnets, have electronic bands with a spin-momentum texture set mainly by the combined crystal-magnetic symmetry. This discovery motivates the question which novel physical properties derive from altermagnetic order. Here we show that one consequence of altermagnetic order is a fluctuation-driven piezomagnetic response. Using two Heisenberg models of d-wave altermagnets, a checkerboard one and one for rutiles, we determine the fluctuation induced piezomagnetic coefficients considering temperature induced transversal spin fluctuations. We establish in addition that magnetic fluctuations induce an anisotropic thermal spin conductivity.

cond-mat.str-el↗

Altermagnetic anomalous Hall effect emerging from electronic correlations

While altermagnetic materials are characterized by a vanishing net magnetic moment, their symmetry in principle allows for the existence of an anomalous Hall effect (AHE). Here we introduce a model with altermagnetism in which the emergence of an AHE is driven by interactions. This model is grounded in a modified Kane-Mele framework with antiferromagnetic (AFM) spin-spin correlations. Quantum Monte Carlo simulations show that the system undergoes a finite temperature phase transition governed by a primary AFM order parameter accompanied by a secondary one of Haldane type. The emergence of both orders turns the metallic state of the system, away from half-filling, to an altermagnet with a finite anomalous Hall conductivity. A mean field ansatz corroborates these results, which pave the way into the study of correlation induced altermagnets with finite Berry curvature.

cond-mat.str-el↗

Fermi arcs dominating the electronic surface properties of trigonal PtBi$_2$

Materials combining topologically non-trivial behavior and superconductivity offer a potential route for quantum computation. However, the set of available materials intrinsically realizing these properties are scarce. Recently, surface superconductivity has been reported in PtBi$_2$ in its trigonal phase and an inherent Weyl semimetal phase has been predicted. Here, based on scanning tunneling microscopy experiments, we reveal the signature of topological Fermi arcs in the normal state patterns of the quasiparticle interference. We show that the scattering between Fermi arcs dominates the interference spectra, providing conclusive evidence for the relevance of Weyl fermiology for the surface electronic properties of trigonal PtBi$_2$.

cond-mat.supr-con↗

Topological Weyl Altermagnetism in CrSb

Altermagnets constitute a novel, third fundamental class of collinear magnetic ordered materials, alongside with ferro- and antiferromagnets. They share with conventional antiferromagnets the feature of a vanishing net magnetization. At the same time they show a spin-splitting of electronic bands, just as in ferromagnets, caused by the atomic exchange interaction. On the other hand, topology has recently revolutionized our understanding of condensed matter physics, introducing new phases of matter classified by intrinsic topological order. Here we connect the worlds of altermagnetism and topology, showing that the electronic structure of the altermagnet CrSb is topological and hosts a novel Weyl semimetallic state. Using high-resolution and spin angleresolved photoemission spectroscopy, we observe a large momentum-dependent spin-splitting in CrSb, reaching up to 1 eV, that induces altermagnetic Weyl nodes with an associated magnetic quantum number. At the surface we observe their spin-polarized topological Fermi-arcs. This establishes that in altermagnets the large energy scale intrinsic to the spin-splitting - orders of magnitude larger than the relativistic spin-orbit coupling - creates its own realm of robust electronic topology.

cond-mat.mtrl-sci↗

Impact of crystal symmetries and Weyl nodes on high-harmonic generation in Weyl semimetal TaAs

High-harmonic generation (HHG) offers an all-optical approach to discern structural symmetries through its selection rules and probe topological phases with its spectral signatures. Here we develop a universal theoretical framework -- the Jones matrix formalism -- establishing the fundamental relationship between pulse-crystal shared symmetries and HHG selection rules. Applying this to the Weyl semimetal (WSM) material TaAs, shows that the anomalous harmonics excited by linearly and circularly polarized pulses are governed respectively by the shared twofold and fourfold rotational symmetries of laser pulses and lattice, rather than the topology of Weyl nodes. The common observables of HHG, including intensity, circular dichroism, ellipticity dependence, and carrier-envelope phase dependence, are not found to carry a signature of the Weyl cones. This insight into TaAs can be extended to other WSMs, indicating that HHG is not a particularly effective tool for investigating the topological features of WSMs. However, the Jones matrix formalism lays the groundwork for both HHG probing crystal symmetry and controlling harmonic polarization states.

cond-mat.mtrl-sci↗

Electronic structure of the surface superconducting Weyl semimetal PtBi$_2$

Trigonal PtBi$_2$ is a layered semimetal without inversion symmetry, featuring 12 Weyl points in the vicinity of the Fermi energy. Its topological Fermi arcs were recently shown to superconduct at low temperatures where bulk superconductivity is absent. Here, we perform first-principles calculations to investigate in detail the bulk and surface electronic structure of PtBi$_2$, and obtain the spin texture as well as the momentum-dependent localization of the arcs. Motivated by the experimentally observed recovery of inversion symmetry under pressure or upon doping, we interpolate between the two structures and determine the energy and momentum dependence of the Weyl nodes. For deeper insights into the surface superconductivity of PtBi$_2$, we construct a symmetry-adapted effective four-band model that accurately reproduces the Weyl points of PtBi$_2$. We supplement this model with an analysis of the symmetry-allowed pairings between the Fermi arcs, which naturally mix spin-singlet and spin-triplet channels. Moreover, the presence of surface-only superconductivity facilitates an intrinsic superconductor-semimetal-superconductor Josephson junction, with the semimetallic phase sandwiched between the two superconducting surfaces. For a phase difference of $π$, zero-energy Andreev bound states develop between the two terminations.

cond-mat.supr-con↗

Layer dependent topological phases and transitions in TaRhTe$_4$: From monolayer and bilayer to bulk

The recently synthesized ternary quasi-2D material TaRhTe$_4$ is a bulk Weyl semimetal with an intrinsically layered structure, which poses the question how the topology of its electronic structure depends on layers separations. Experimentally these separations may be changed for instance by intercalation of the bulk, or by exfoliation to reach monolayer or few-layer structures. Here we show that in the monolayer limit a quantum spin Hall insulator (QSHI) state emerges, employing density functional calculations as well as a minimal four-orbital tight-binding model that we develop. Even for weak spin-orbit couplings the QSHI is present, which has an interesting edge state that features Rashba-split bands with quadratic band minima. Further we find that a weak topological insulator (WTI) manifests in the bilayer system due to sizable intralayer hopping, contrary to the common lore that only weak interlayer interactions between stacked QSHIs lead to WTIs. Stacked bilayers give rise to a phase diagram as function of the interlayer separation that comprises a Weyl semimetal, WTI and normal insulator phases. These insights on the evolution of topology with dimension can be transferred to the family of layered ternary transition metal tellurides.

cond-mat.mtrl-sci↗

Chiral Meissner effect in time-reversal invariant Weyl superconductors

Weyl semimetals have nodes in their electronic structure at which electrons attain a definite chirality. Due to the chiral anomaly, the non-conservation of charges with given chirality, the axion term appears in their effective electromagnetic action. We determine how this affects the properties of time-reversal invariant Weyl {\it superconductors} (SCs) in the London regime. For type II SCs the axion coupling generates magnetic $B$-fields transverse to vortices, which become unstable at a critical coupling so that a transition into type I SC ensues. In this regime an applied $B$-field not only decays inside the SC within the London penetration depth, but the axion coupling generates an additional perpendicular field. Consequently, when penetrating into the bulk the $B$-field starts to steadily rotate away from the applied field. At a critical coupling the screening of the magnetic field breaks down. The novel chiral superconducting state that emerges has a periodically divergent susceptibility that separates onsets of chiral Meissner regimes. The chiral anomaly thus leaves very crisp experimental signatures in structurally chiral Weyl SCs with an axion response.

cond-mat.supr-con↗

Two-dimensional Discommensurations: an extension to McMillan's Ginzburg-Landau Theory

Charge density waves (CDW) profoundly affect the electronic properties of materials and have an intricate interplay with other collective states, like superconductivity and magnetism. The well-known macroscopic Ginzburg-Landau theory stands out as a theoretical method for describing CDW phenomenology without requiring a microscopic description. In particular, it has been instrumental in understanding the emergence of domain structures in several CDW compounds, as well as the influence of critical fluctuations and the evolution towards or across lock-in transitions. In this context, McMillan's foundational work introduced discommensurations as the objects mediating the transition from commensurate to incommensurate CDW, through an intermediate nearly commensurate phase characterised by an ordered array of phase slips. Here, we extend the simplified, effectively one-dimensional, setting of the original model to a fully two-dimensional analysis. We find exact and numerical solutions for several types of discommensuration patterns and provide a framework for consistently describing multi-component CDW embedded in quasi-two-dimensional atomic lattices.

cond-mat.str-el↗

Correlation between electronic polarization and shift current in cubic and hexagonal semiconductors LiZn$X$ ($X$ = P, As, Sb)

The rectified bulk photovoltaic effect (BPVE) in noncentrosymmetric semiconductors, also called shift current, is considered promising for optoelectronic devices, terahertz emission and possibly solar energy harvesting. A clear understanding of the shift current mechanism and search for materials with large shift current is, therefore, of immense interest. $ABC$ semiconductors LiZn$X$ ($X$ = N, P, As, and Sb) can be stabilized in cubic as well as hexagonal morphologies lacking inversion symmetry$-$an ideal platform to investigate the significant contributing factors to shift current, such as the role of structure and chemical species. Using density-functional calculations properly accounting for the electronic bandgaps, the shift current conductivities in LiZn$X$ ($X$ = P, As, Sb) are found to be approximately an order of magnitude larger than the well-known counterparts and peak close to the maximum solar radiation intensity. Notably, hexagonal LiZnSb shows a peak shift current conductivity of $\sim -75 ~\rm{\rmμ}$A/V$^2$ and Glass coefficient of $ -20$ $\times$ 10$^{-8}$ cm/V, comparable to the highest predicted values in literature. Our comparative analysis reveals a quantitative relationship between the shift current response and the electronic polarization. These findings not only posit Li-Zn-based $ABC$ semiconductors as viable material candidates for potential applications but also elucidates key aspects of the structure-BPVE relationship.

cond-mat.mtrl-sci↗

Emergent Quadrupolar Order in the Spin-$1/2$ Kitaev-Heisenberg Model

Motivated by the largely unexplored domain of multi-polar ordered spin states in the Kitaev-Heisenberg (KH) systems we investigate the ground state dynamics of the spin-$\frac{1}{2}$ KH model, focusing on quadrupolar (QP) order in 2-leg ladder and two-dimensional honeycomb lattice geometries. Employing exact diagonalization and density-matrix renormalization group methods, we analyze the QP order parameter and correlation functions. Our findings reveal a robust QP order across a wide range of the phase diagram, influenced by the interplay between Heisenberg and Kitaev interactions. Notably, we observe an enhancement of QP order near Kitaev quantum spin liquid (QSL) phases, despite the absence of long-range spin-spin correlations. This highlights a complex relationship between QP order and QSLs, offering new insights into quantum magnetism in low-dimensional systems. Our findings provide a rational explanation for the observed nonlinear magnetic susceptibility in $α$-RuCl$_3$.

cond-mat.str-el↗

Observation of giant circular dichroism induced by electronic chirality

Chiral phases of matter, characterized by a definite handedness, abound in nature, ranging from the crystal structure of quartz to spiraling spin states in helical magnets. In $1T$-TiSe$_2$ a source of chirality has been proposed that stands apart from these classical examples as it arises from combined electronic charge and quantum orbital fluctuations. This may allow its chirality to be accessed and manipulated without imposing either structural or magnetic handedness. However, direct bulk evidence that broken inversion symmetry and chirality are intrinsic to TiSe$_2$ remains elusive. Here, employing resonant elastic scattering of x-rays, we reveal the presence of giant circular dichroism up to $\sim$ 40$\%$ at forbidden Bragg peaks that emerge at the charge and orbital ordering transition. The dichroism varies dramatically with incident energy and azimuthal angle. Comparison to calculated scattering intensities unambiguously traces its origin to bulk chiral electronic order in ${\mathrm{TiSe}}_2$ and establishes resonant elastic x-ray scattering as a sensitive probe to electronic chirality.

cond-mat.str-el↗

Emergence of vortex state in the $S=1$ Kitaev-Heisenberg model with single-ion anisotropy

The search for Kitaev spin liquid states has recently broadened to include a number of honeycomb materials with integer spin moments. The qualitative difference with their spin-1/2 counterparts is the presence of single-ion anisotropy (SIA). This motivates our investigation of the effects of SIA on the ground state of the spin-$1$ Kitaev-Heisenberg (KH) model using the density-matrix renormalization group which allows construction of detailed phase diagrams around the Kitaev points. We demonstrate that positive out-of-plane SIA induces an in-plane vortex state without the need for off-diagonal interactions. Conversely, negative SIA facilitates the emergence of a ferromagnetic state in presence of antiferromagnetic Heisenberg interactions, while a Nèel state can emerge for ferromagnetic Heisenberg coupling. These findings, pertinent even for weak SIA, not only enhance our theoretical understanding of the spin-1 KH model but also propose experimental prospects for observing these novel magnetic states in material realizations.

cond-mat.str-el↗

Data-driven estimation of transfer integrals in undoped cuprates

Undoped cuprates are an abundant class of magnetic insulators, in which the synergy of rich chemistry and sizable quantum fluctuations leads to a variety of magnetic behaviors. Understanding the magnetism of these materials is impossible without the knowledge of the underlying spin model. The typically dominant antiferromagnetic superexchanges can be accurately estimated from the respective electronic transfer integrals. Density functional theory calculations mapped onto an effective one-orbital model in the Wannier basis are an accurate, albeit computationally cumbersome method to estimate such transfer integrals in cuprates. We demonstrate that instead an Artificial Neural Network (ANN), trained on the results of high-throughput calculations, can predict the transfer integrals using the crystal structure as the only input. Descriptors of the ANN model encode the spatial configuration and the chemical composition of the local crystalline environment. A virtual toolbox employing our model can be readily employed to determine leading superexchange paths as well as for rapidly assessing the relevant spin model in yet unknown cuprates.

cond-mat.str-el↗

Two-point spectroscopy of Fibonacci topoelectrical circuits

Topoelectrical circuits are meta-material realizations of topological features of condensed matter systems. In this work, we discuss experimental methods that allow a fast and straightforward detection of the spectral features of these systems from the two-point impedance of the circuit. This allows to deduce the full spectrum of a topoelectrical circuit consisting of N sites from a single two-point measurement of the frequency resolved impedance. In contrast, the standard methods rely on $N^2$ measurements of admittance matrix elements with a subsequent diagonalization on a computer. We experimentally test our approach by constructing a Fibonacci topoelectrical circuit. Although the spectrum of this chain is fractal, i.e., more complex than the spectra of periodic systems, our approach is successful in recovering its eigenvalues. Our work promotes the topoelectrical circuits as an ideal platform to measure spectral properties of various (quasi)crystalline systems.

cond-mat.mes-hall↗