arXiv subjects

Jeroen van den Brink

Publications and source records attributed to Jeroen van den Brink.

At least 127 records · Page 7Linked to original sources

arXiv2021

Extended high-harmonic spectra through cascade resonance in confined quantum systems

The study of high-harmonic generation in confined quantum systems is vital to establishing a complete physical picture of harmonic generation from atoms and molecules to bulk solids. Based on a multilevel approach, we demonstrate how intraband resonances significantly influence the harmonic spectra via charge pumping to the higher subbands and, thus, redefine the cutoff laws. As a proof of principle, we consider the interaction of graphene nanoribbons, with zigzag as well as armchair terminations, and resonant fields polarized along the cross-ribbon direction. Here, this effect is particularly prominent due to many nearly equi-separated energy levels. In such a scenario, a cascade resonance effect can take place in high-harmonic generation when the field strength is above a critical threshold, which is completely different from the harmonic generation mechanism of atoms, molecules and bulk solids. We further discuss the implications not only for other systems in a nanoribbon geometry, but also systems where only a few subbands (energy levels) meet this frequency-matching condition by considering a generalized multilevel Hamiltonian. Our study highlights that cascade resonance bears fundamentally distinct influence on the laws of harmonic generation, specifically the cutoff laws based on laser duration, field strength, and wavelength, thus unraveling new insights in solid-state high-harmonic generation.

cond-mat.mes-hall↗

arXiv2021

Non-Hermitian skin effect of dislocations and its topological origin

We demonstrate that dislocations in two-dimensional non-Hermitian systems can give rise to density accumulation or depletion through the localization of an extensive number of states. These effects are shown by numerical simulations in a prototype lattice model and expose a different face of non-Hermitian skin effect, by disentangling it from the need for boundaries. We identify a topological invariant responsible for the dislocation skin effect, which takes the form of a ${\mathbb Z}_2$ Hopf index that depends on the Burgers vector characterizing the dislocations. Remarkably, we find that this effect and its corresponding signature for defects in Hermitian systems falls outside of the known topological classification based on bulk-defect correspondence.

cond-mat.mes-hall↗

arXiv2021

Chirality flip of Weyl nodes and its manifestation in strained MoTe$_2$

Due to their topological charge, or chirality, the Weyl cones present in topological semimetals are considered robust against arbitrary perturbations. One well-understood exception to this robustness is the pairwise creation or annihilation of Weyl cones, which involves the overlap of two oppositely charged nodes in energy and momentum. Here we show that their topological charge can in fact change sign, in a process that involves the merging of not two, but three Weyl nodes. This is facilitated by the presence of rotation and time-reversal symmetries, which constrain the relative positions of Weyl cones in momentum space. We analyze the chirality flip process, showing that transport properties distinguish it from the conventional, double Weyl merging. Moreover, we predict that the chirality flip occurs in MoTe$_2$, where experimentally accessible strain leads to the merging of three Weyl cones close to the Fermi level. Our work sets the stage to further investigate and observe such chirality flipping processes in different topological materials.

cond-mat.mes-hall↗

arXiv2021

Axion Mie Theory of Electron Energy Loss Spectroscopy in Topological Insulators

Electronic topological states of matter exhibit novel types of responses to electromagnetic fields. The response of strong topological insulators, for instance, is characterized by a so-called axion term in the electromagnetic Lagrangian which is ultimately due to the presence of topological surface states. Here we develop the axion Mie theory for the electromagnetic response of spherical particles including arbitrary sources of fields, i.e., charge and current distributions. We derive an axion induced mixing of transverse magnetic and transverse electric modes which are experimentally detectable through small induced rotations of the field vectors. Our results extend upon previous analyses of the problem. Our main focus is on the experimentally relevant problem of electron energy loss spectroscopy in topological insulators, a technique that has so far not yet been used to detect the axion electromagnetic response in these materials.

physics.optics↗

arXiv2021

Infinite Berry Curvature of Weyl Fermi Arcs

We show that Weyl Fermi arcs are generically accompanied by a divergence of the surface Berry curvature scaling as $1/k^2$, where $k$ is the distance to a hot-line in the surface Brillouin zone that connects the projection of Weyl nodes with opposite chirality but which is distinct from the Fermi arc itself. Such surface Berry curvature appears whenever the bulk Weyl dispersion has a velocity tilt toward the surface of interest. This divergence is reflected in a variety of Berry curvature mediated effects that are readily accessible experimentally, and in particular leads to a surface Berry curvature dipole that grows linearly with the thickness of a slab of a Weyl semimetal material in the limit of long lifetime of surface states. This implies the emergence of a gigantic contribution to the non-linear Hall effect in such devices.

cond-mat.mes-hall↗

arXiv2021

Deconfined criticality and bosonization duality in easy-plane Chern-Simons two-dimensional antiferromagnets

Two-dimensional quantum systems with competing orders can feature a deconfined quantum critical point, yielding a continuous phase transition that is incompatible with the Landau-Ginzburg-Wilson scenario, predicting instead a first-order phase transition. This is caused by the LGW order parameter breaking up into new elementary excitations at the critical point. Canonical candidates for deconfined quantum criticality are quantum antiferromagnets with competing magnetic orders, captured by the easy-plane CP$^1$ model. A delicate issue however is that numerics indicates the easy-plane CP$^1$ antiferromagnet to exhibit a first-order transition. Here we show that an additional topological Chern-Simons term in the action changes this picture completely in several ways. We find that the topological easy-plane antiferromagnet undergoes a second-order transition with quantized critical exponents. Further, a particle-vortex duality naturally maps the partition function of the Chern-Simons easy-plane antiferromagnet into one of massless Dirac fermions.

cond-mat.str-el↗

arXiv2021

Finite temperature fluctuation-induced order and responses in magnetic topological insulators

We derive an effective field theory model for magnetic topological insulators and predict that a magnetic electronic gap persists on the surface for temperatures above the ordering temperature of the bulk. Our analysis also applies to interfaces of heterostructures consisting of a ferromagnetic and a topological insulator. In order to make quantitative predictions for MnBi$_2$Te$_4$, and for EuS-Bi$_2$Se$_3$ heterostructures, we combine the effective field theory method with density functional theory and Monte Carlo simulations. For MnBi$_2$Te$_4$ we predict an upwards Néel temperature shift at the surface up to $15 \%$, while the EuS-Bi$_2$Se$_3$ interface exhibits a smaller relative shift. The effective theory also predicts induced Dzyaloshinskii-Moriya interactions and a topological magnetoelectric effect, both of which feature a finite temperature and chemical potential dependence.

cond-mat.str-el↗

arXiv2021

Spin Hall effect emerging from a chiral magnetic lattice without spin-orbit coupling

The spin Hall effect (SHE), which converts a charge current into a transverse spin current, has long been believed to be a phenomenon induced by the spin--orbit coupling. Here, we propose an alternative mechanism to realize the intrinsic SHE through a chiral magnetic structure that breaks the spin rotation symmetry. No spin--orbit coupling is needed even when the scalar spin chirality vanishes, different from the case of the topological Hall effect. In known chiral antiferromagnetic compounds Mn$_3X$ ($X=$ Ga, Ge, and Sn), for example, we indeed obtain large spin Hall conductivities based on \textit{ab initio} calculations. Apart further developing the conceptual understanding of the SHE, our work suggests an alternative strategy to design spin Hall materials without involving heavy elements, which may be advantageous for technological applications.

cond-mat.mtrl-sci↗

arXiv2021

Observation of orbital order in the Van der Waals material 1T-TiSe2

Besides magnetic and charge order, regular arrangements of orbital occupation constitute a fundamental order parameter of condensed matter physics. Even though orbital order is difficult to identify directly in experiments, its presence was firmly established in a number of strongly correlated, three-dimensional Mott insulators. Here, reporting resonant X-ray scattering experiments on the layered Van der Waals compound $1T$-TiSe$_2$, we establish the emergence of orbital order in a weakly correlated, quasi-two-dimensional material. Our experimental scattering results are consistent with first-principles calculations that bring to the fore a generic mechanism of close interplay between charge redistribution, lattice displacements, and orbital order. It demonstrates the essential role that orbital degrees of freedom play in TiSe$_2$, and their importance throughout the family of correlated Van der Waals materials.

cond-mat.str-el↗

arXiv2021

Engineering spectral properties of non-interacting lattice Hamiltonians

We investigate the spectral properties of one-dimensional lattices with position-dependent hopping amplitudes and on-site potentials that are smooth bounded functions of position. We find an exact integral form for the density of states (DOS) in the limit of an infinite number of sites, which we derive using a mixed Bloch-Wannier basis consisting of piecewise Wannier functions. Next, we provide an exact solution for the inverse problem of constructing the position-dependence of hopping in a lattice model yielding a given DOS. We confirm analytic results by comparing them to numerics obtained by exact diagonalization for various incarnations of position-dependent hoppings and on-site potentials. Finally, we generalize the DOS integral form to multi-orbital tight-binding models with longer-range hoppings and in higher dimensions.

cond-mat.mes-hall↗

arXiv2021

Ab initio ligand field approach to determine electronic multiplet properties

A method is developed to calculate the ligand field (LF) parameters and the multiplet spectra of local magnetic centers with open $d$- and $f$-shells in solids in a parameter-free way. This method proceeds from density functional theory and employs Wannier projections of nonmagnetic band structures onto local $d$- or $f$-orbitals. Energies of multiplets and optical, as well as X-ray spectra are determined by exact numerical diagonalization of a local Hamiltonian describing Coulomb, LF, and spin-orbit interactions. The method is tested for several 3$d$- and 5$f$-compounds for which the LF parameters and multiplet spectra are experimentally well known. In this way, we obtain good agreement with experiment for La$_2$NiO$_4$, CaCuO$_2$, Li$_2$CuO$_2$, ZnO:Co, and UO$_2$.

cond-mat.str-el↗

arXiv2021

Synthetic gravitational horizons in low-dimensional quantum matter

We propose a class of lattice models realizable in a wide range of setups whose low-energy dynamics exactly reduces to Dirac fields subjected to (1+1)-dimensional gravitational backgrounds, including (anti-)de Sitter spacetime. Wave-packets propagating on the lattice exhibit an eternal slowdown for power-law position-dependent hopping integrals $t(x)\propto x^γ$ when $γ\geq 1$, signalling the formation of black hole event horizons. For $γ< 1$ instead the wave-packets behave radically different and bounce off the horizon. We show that the eternal slowdown relates to a zero-energy spectral singularity of the lattice model and that the semiclassical wave packets trajectories coincide with the geodesics on (1+1)D dilaton gravity, paving the way for new and experimentally feasible routes to mimic black hole horizons and realize (1+1)D spacetimes as they appear in certain gravity theories.

cond-mat.mes-hall↗

arXiv2021

Unraveling the orbital physics in a canonical orbital system KCuF$_3$

We explore the existence of the collective orbital excitations, orbitons, in the canonical orbital system KCuF$_3$. Using the Cu $L_3$-edge resonant inelastic X-ray scattering we show that the non-dispersive high-energy peaks result from the Cu$^{2+}$ $dd$ orbital excitations. These high-energy modes show good agreement with the {\it ab-initio} quantum chemistry calculation based on a single cluster, indicating that the $dd$ excitations are highly localized. At the same time, the low-energy excitations present clear dispersion. They match extremely well with the two-spinon continuum following the comparison with Mueller Ansatz calculations. The localized $dd$ excitations and the observation of the strongly dispersive magnetic excitations suggest that orbiton dispersion is below the resolution detection limit. Our results can reconcile with the strong {\it local} Jahn-Teller effect in KCuF$_3$, which predominantly drives orbital ordering.

cond-mat.str-el↗

arXiv2021

Ferromagnetic helical nodal line and Kane-Mele spin-orbit coupling in kagome metal Fe3Sn2

The two-dimensional kagome lattice hosts Dirac fermions at its Brillouin zone corners K and K', analogous to the honeycomb lattice. In the density functional theory electronic structure of ferromagnetic kagome metal Fe$_3$Sn$_2$, without spin-orbit coupling we identify two energetically split helical nodal lines winding along $z$ in the vicinity of K and K' resulting from the trigonal stacking of the kagome layers. We find that hopping across A-A stacking introduces a layer splitting in energy while that across A-B stacking controls the momentum space amplitude of the helical nodal lines. The effect of spin-orbit coupling is found to resemble that of a Kane-Mele term, where the nodal lines can either be fully gapped to quasi-two-dimensional massive Dirac fermions, or remain gapless at discrete Weyl points depending on the ferromagnetic moment orientation. Aside from numerically establishing Fe$_3$Sn$_2$ as a model Dirac kagome metal, our results provide insights into materials design of topological phases from the lattice point of view, where paradigmatic low dimensional lattice models often find realizations in crystalline materials with three-dimensional stacking.

cond-mat.mtrl-sci↗

arXiv2020

Electronic correlations and magnetic interactions in infinite-layer NdNiO$_2$

The large antiferromagnetic exchange coupling in the parent high-$T_{\rm c}$ cuprate superconductors is believed to play a crucial role in pairing the superconducting carriers. The recent observation of superconductivity in hole-doped infinite-layer (IL-) NdNiO$_2$ brings to the fore the relevance of magnetic coupling in high-$T_{\rm c}$ superconductors, particularly because no magnetic ordering is observed in the undoped IL-NdNiO$_2$ unlike in parent copper oxides. Here, we investigate the electronic structure and the nature of magnetic exchange in IL-NdNiO$_2$ using state-of-the-art many-body quantum chemistry methods. From a systematic comparison of the electronic and magnetic properties with isostructural cuprate IL-CaCuO$_2$, we find that the on-site dynamical correlations are significantly stronger in IL-NdNiO$_2$ compared to the cuprate analog. These dynamical correlations play a critical role in the magnetic exchange resulting in an unexpectedly large antiferromagnetic nearest neighbor isotropic $J$ of 77 meV between the Ni$^{1+}$ ions within the $ab$-plane. While we find many similarities in the electronic structure between the nickelate and the cuprate, the role of electronic correlations is profoundly different in the two. We further discuss the implications of our findings in understanding the origin of superconductivity in nickelates.

cond-mat.str-el↗

arXiv2020

Plasmons in anisotropic Dirac systems

We consider the plasmon excitations in anisotropic two-dimensional Dirac systems, be it either anisotropic graphene or surfaces of topological insulators. Generalizing the exact density-density response function one finds a plasmon dispersion that is anisotropic already at the lowest frequencies. Asymptotic expressions are obtained for the dispersion in this regime. We show that the plasmon properties of the complete material class of anisotropic Dirac systems are characterized by just two dimensionless material parameters. The strong anisotropy can be used to guide the plasmon modes, introducing new functionalities to the field of Dirac plasmonics.

cond-mat.mtrl-sci↗

arXiv2020

Bosonization in 2+1 dimensions via Chern-Simons bosonic particle-vortex duality

Dualities provide deep insight into physics by relating two seemingly distinct theories. Here we consider a duality between lattice fermions and bosons in (2+1) spacetime dimensions, relating free massive Dirac fermions to Abelian Chern-Simons Higgs (ACSH) bosons. To establish the duality we represent the exact partition function of the lattice fermions in terms of the writhe of fermionic worldlines. On the bosonic side the partition function is expressed in the writhe of the vortex loops of the particle-vortex dual of the ACSH Lagrangian. In the continuum and scaling limit we show these to be identical. This result can be understood from the closed fermionic worldlines being direct mappings of the ACSH vortex loops, with the writhe keeping track of particle statistics.

hep-th↗

arXiv2020

A $j_\mathrm{eff} = 1/2$ pseudospinon continuum in CaIrO$_3$

In so-called $j_\mathrm{eff} = 1/2$ systems, including some iridates and ruthenates, the coherent superposition of $t_\mathrm{2g}$ orbitals in the ground state gives rise to hopping processes that strongly depend on the bond geometry. Resonant inelastic x-ray scattering (RIXS) measurements on CaIrO$_3$ reveal a prototypical $j_\mathrm{eff} = 1/2$ pseudospinon continuum, a hallmark of one-dimensional (1D) magnetic systems despite its three-dimensional crystal structure. The experimental spectra compare very well to the calculated magnetic dynamical structure factor of weakly coupled spin-1/2 chains. We attribute the onset of such quasi-1D magnetism to the fundamental difference in the magnetic interactions between the $j_\mathrm{eff} = 1/2$ pseudospins along the corner- and edge-sharing bonds in CaIrO$_3$.

cond-mat.str-el↗