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Jhinhwan Lee

Publications and source records attributed to Jhinhwan Lee.

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Evolution of inhomogeneities in two-dimensional disordered superconductors in a magnetic field

Emerging granularity in superconducting films by tuning disorder is a well-studied topic, both theoretically and experimentally. However, the orbital magnetic field generates a vortex lattice and contributes to the formation of periodic inhomogeneities. Here, we study superconducting films in the simultaneous presence of disorder and a magnetic field, examining how inhomogeneities in various superconducting correlations evolve under these two perturbations. By performing scanning tunneling spectroscopy (STS) on thin films of \ce{Sr2VO_{3-\text{x}}FeAs} layer structures under both zero and finite orbital magnetic fields, we report impressive similarities between our theoretical results and the experimental findings. Our results have strong implications for identifying the nature of vortices in disordered superconductors, demonstrating a crossover from Abrikosov to Josephson character with increasing disorder, and provide predictive guidance for interpreting STS and current mapping data in complex superconductors.

cond-mat.supr-con

Anderson transition of in-gap quasiparticles in a quasi-two-dimensional disordered superconductor

The Anderson transition of Bogoliubov-de Gennes (BdG) quasiparticles in superconducting state has been studied theoretically for last three decades. However, its experimental proof is lacking. In particular, the relationship of the superconducting order-parameter fluctuations and the Anderson transition of BdG quasiparticles have not been well understood. Our study, based on scanning tunneling microscopy measurements, investigates how BdG quasiparticles become Anderson-localized and delocalized as a function of energy and applied magnetic field in a quasi-two-dimensional Fe-based superconductor with sufficient zero-bias BdG quasiparticles. The anomalous multifractal spectra based on the spatial distributions of the pairing gaps and the coherent peak heights suggest that superconducting fluctuations play a key role in the delocalization of in-gap BdG quasiparticles. Our real-space Hartree-Fock-BCS-Anderson simulations and renormalization group analysis with pairing fluctuations support quasiparticle localization and suggest that enhanced pairing fluctuations lead to delocalization of BdG quasiparticles and "weak localization" of phase-fluctuating Cooper pairs in quasi-two-dimensional disordered superconductors. The present study proposes that the 10-fold way classification scheme has to be generalized to take order-parameter fluctuations in actual quantum matter. Also, it shed light on how ac energy loss due to quasiparticles at Fermi level can be controlled in a quasi-2d superconductor with sufficient pairing fluctuation.

cond-mat.str-el

First prototype of a biaxially textured YBa$_{2}$Cu$_{3}$O$_{7-x}$ microwave cavity in a high magnetic field for dark matter axion search

A high-quality factor microwave resonator in the presence of a strong magnetic field could have a wide range of applications, such as axion dark matter searches where the two aspects must coexist to enhance the experimental sensitivity. We introduce a polygon-shaped cavity design with bi-axially textured YBa$_{2}$Cu$_{3}$O$_{7-x}$ superconducting tapes covering the entire inner wall. Using a 12-sided polygon cavity, we obtain substantially improved quality factors of the TM$_{010}$ mode at 6.9 GHz at 4 K with respect to a copper cavity and observe no considerable degradation in the presence of magnetic fields up to 8 T. This corresponds to the first demonstration of practical applications of superconducting radio frequency technology for axion and other research areas requiring low loss in a strong magnetic field. We address the importance of the successful demonstration and discuss further improvements.

physics.ins-det

Superconducting cavity in a high magnetic field

A high Q-factor microwave resonator in a high magnetic field could be used in a wide range of applications, especially for enhancing the scanning speed in axion dark matter research. In this letter, we introduce a polygon-shaped resonant cavity with commercial YBCO tapes covering the entire inner wall. We demonstrated that the maximum Q-factor (TM$_{010}$, 6.93 GHz) of the superconducting YBCO cavity was about 6 times higher than that of a copper cavity and showed no significant degradation up to 8 T at 4 K. This is the first indication of the possible applications of HTS technology to the research areas requiring low loss in a strong magnetic field at high radio frequencies.

physics.app-ph

Maintaining high Q-factor of superconducting YBa$_2$Cu$_3$O$_{7-x}$ microwave cavity in a high magnetic field

A high Q-factor microwave resonator in a high magnetic field could be of great use in a wide range of fields, from accelerator design to axion dark matter search. The natural choice of material for the superconducting cavity to be placed in a high field is a high temperature superconductor (HTS) with a high critical field. The deposition, however, of a high-quality, grain-aligned HTS film on a three-dimensional surface is technically challenging. We have fabricated a polygon-shaped resonant cavity with commercial YBa$_2$Cu$_3$O$_{7-x}$ (YBCO) tapes covering the entire inner wall and measured the Q-factor at 4 K at 6.93 GHz as a function of an external DC magnetic field. We demonstrated that the high Q-factor of the superconducting YBCO cavity showed no significant degradation from 1 T up to 8 T. This is the first indication of the possible applications of HTS technology to the research areas requiring a strong magnetic field at high radio frequencies.

physics.ins-det

Barrier-bound States in Flat-band Systems

As the fundamental quantum mechanical theory predicts, it is believed that electronic states can be bound only to potential wells and not to potential barriers in any dimension and their energies should be below the background potential. However, with the help of atomic lattice potentials with a flat electron band in momentum space in the background, an atomically thin 1D potential barrier can possess barrier-centered bound states above the background potential. Here we provide a theoretical proof using Green function pole analysis with Dyson equation that shows the existence of barrier-bound-states whose energy is elevated from the flat band energy nearly by the barrier height. The phenomenon is believed to be independently confirmed in a system of Pd monolayer on a flat oxide substrate with Stoner ferromagnetism using spin-polarized STM technique and through comparison with real-space QPI simulations using realistic 2D Pd band structure.

cond-mat.mes-hall

Real-time digital signal recovery for a low-pass transfer function system with multiple complex poles

In order to solve the problems of waveform distortion and signal delay by many physical and electrical systems with linear low-pass transfer characteristics with multiple complex poles, a general digital-signal-processing (DSP)-based method of real-time recovery of the original source waveform from the distorted output waveform is proposed. From the convolution kernel representation of a multiple-pole low-pass transfer function with an arbitrary denominator polynomial with real valued coefficients, it is shown that the source waveform can be accurately recovered in real time using a particular moving average algorithm with real-valued DSP computations only, even though some or all of the poles are complex. The proposed digital signal recovery method is DC-accurate and unaffected by initial conditions, transient signals, and resonant amplitude enhancement. The noise characteristics of the data recovery shows inverse of the low-pass filter characteristics. This method can be applied to most sensors and amplifiers operating close to their frequency response limits or around their resonance frequencies to accurately deconvolute the multiple-pole characteristics and to improve the overall performances of data acquisition systems and digital feedback control systems.

physics.ins-det

Versatile Variable Temperature and Magnetic Field Scanning Probe Microscope for Advanced Material Research

We have built a variable temperature scanning probe microscope (SPM) that covers 4.6 K - 180 K and up to 7 Tesla whose SPM head fits in a 52 mm bore magnet. It features a temperature-controlled sample stage thermally well isolated from the SPM body in good thermal contact with the liquid helium bath. It has a 7 sample holder storage carousel at liquid helium temperature for systematic studies using multiple samples and field emission targets intended for spin-polarized spectroscopic-imaging scanning tunneling microscopy (STM) study on samples with various compositions and doping conditions. The system is equipped with a UHV sample preparation chamber and mounted on a two-stage vibration isolation system made of a heavy concrete block and a granite table on pneumatic vibration isolators. A quartz resonator (qPlus) based non-contact atomic force microscope (AFM) sensor is used for simultaneous STM/AFM operation for research on samples with highly insulating properties such as strongly underdoped cuprates and strongly correlated electron systems.

physics.ins-det

Switching Magnetism and Superconductivity with Spin-Polarized Current in Iron-Based Superconductor

We have explored a new mechanism for switching magnetism and superconductivity in a magnetically frustrated iron-based superconductor using spin-polarized scanning tunneling microscopy (SPSTM). Our SPSTM study on single crystal Sr$_2$VO$_3$FeAs shows that a spin-polarized tunneling current can switch the Fe-layer magnetism into a non-trivial $C_4$ (2$\times$2) order, not achievable by thermal excitation with unpolarized current. Our tunneling spectroscopy study shows that the induced $C_4$ (2$\times$2) order has characteristics of plaquette antiferromagnetic order in Fe layer and strongly suppressed superconductivity. Also, thermal agitation beyond the bulk Fe spin ordering temperature erases the $C_4$ state. These results suggest a new possibility of switching local superconductivity by changing the symmetry of magnetic order with spin-polarized and unpolarized tunneling currents in iron-based superconductors.

cond-mat.supr-con

Correlation of Fe-based Superconductivity and Electron-Phonon Coupling in an FeAs/Oxide Heterostructure

Interfacial phonons between iron-based superconductors (FeSCs) and perovskite substrates have received considerable attention due to the possibility of enhancing preexisting superconductivity. Using scanning tunneling spectroscopy, we studied the correlation between superconductivity and e-ph interaction with interfacial-phonons in an iron-based superconductor Sr$_2$VO$_3$FeAs ($T_c \approx$ 33 K) made of alternating FeSC and oxide layers. The quasiparticle interference measurement over regions with systematically different average superconducting gaps due to the e-ph coupling locally modulated by O vacancies in VO$_2$ layer, and supporting self-consistent momentum-dependent Eliashberg calculations provide a unique real-space evidence of the forward-scattering interfacial phonon contribution to the total superconducting pairing.

cond-mat.supr-con

Atomic-scale observation and manipulation of plaquette antiferromagnetic order in iron-based superconductor

The symmetry requirement and the origin of magnetic orders coexisting with superconductivity have been strongly debated issues of iron-based superconductors (FeSCs). Observation of C$_4$-symmetric antiferromagnetism in violation of the inter-band nesting condition of spin-density waves in superconducting ground state will require significant change in our understanding of the mechanism of FeSC. The superconducting material Sr$_2$VO$_3$FeAs, a bulk version of monolayer FeSC in contact with a perovskite layer with its magnetism (T$_N$ ~ 50 K) and superconductivity (T$_c$ ~ 37 K) coexisting at parent state, has no reported structural orthorhombic distortion and thus makes a perfect system to look for theoretically expected C$_4$ magnetisms. Based on variable temperature spin-polarized scanning tunneling microscopy (SPSTM) with newly discovered imaging mechanism that removes the static surface reconstruction (SR) pattern by fluctuating it rapidly with spin-polarized tunneling current, we could visualize underlying C$_4$ symmetric (2$\times$2) magnetic domains and its phase domain walls. We find that this magnetic order is perfectly consistent with the plaquette antiferromagnetic order in tetragonal Fe spin lattice expected from theories based on the Heisenberg exchange interaction of local Fe moments and the quantum order by disorder. The inconsistency of its modulation Q vectors from the nesting condition also implies that the nesting-based C$_2$ symmetric magnetism is not a unique prerequisite of high-T$_c$ FeSC. Furthermore, the plaquette antiferromagnetic domain wall dynamics under the influence of small spin torque effect of spin-polarized tunneling current are shown to be consistent with theoretical simulation based on the extended Landau-Lifshitz-Gilbert equation.

cond-mat.supr-con

Real-time digital signal recovery for a multi-pole low-pass transfer function system

In order to solve the problems of waveform distortion and signal delay by many physical and electrical systems with multi-pole linear low-pass transfer characteristics, a simple digital-signal-processing (DSP)-based method of real-time recovery of the original source waveform from the distorted output waveform is proposed. A mathematical analysis on the convolution kernel representation of the single-pole low-pass transfer function shows that the original source waveform can be accurately recovered in real time using a particular moving average algorithm applied on the input stream of the distorted waveform, which can also significantly reduce the overall delay time constant. This method is generalized for multi-pole low-pass systems and has noise characteristics of the inverse of the low-pass filter characteristics. This method can be applied to most sensors and amplifiers operating close to their frequency response limits to improve the overall performances of data acquisition systems and digital feedback control systems.

physics.ins-det

Prediction of ultra-high ON/OFF ratio nanoelectromechanical switching from covalently-bound C60 chains

Applying a first-principles computational approach, we have systematically analyzed the effects of [2+2] cycloaddition oligomerization of fullerene C60 chains on their junction electronic and charge transport properties. For hypothetical infinite C60 chains, we first establish that the polymerization can in principle increase conductance by several orders of magnitude due to the strong orbital hybridizations and band formation. On the other hand, our simulations of the constant-height scanning tunneling microscope (STM) configuration shows that, in agreement with the recent experimental conclusion, the junction electronic structure and device characteristics are virtually unaffected by the C60 chain oligomerization. We further predict that the switching characteristics including even the ON/OFF-state assignment will sensitively depend on the substrate metal species due to the Fermi-level pinning at the substrate-side contact and the subsequent energy level bending toward the STM tip-side contact. We finally demonstrate that a force-feedbacked nanoelectromechanical approach in which both of the C60-electrode distances are kept at short distances before and after switching operations can achieve a metal-independent and significantly improved switching performance due to the Fermi-level pinning in both contacts and the large intrinsic conductance switching capacity of the C60 chain oligomerization.

cond-mat.mes-hall

A high-resolution cross-sectional analysis for Fourier-transform scanning tunneling spectroscopy and fully-phased Green-function-based quasiparticle scattering theories

The Fourier-transform scanning tunneling spectroscopy (FTSTS) contains rich signals related to the quasiparticle scattering interference and/or the density-wave-like orders which are crucial in interpretation of the ground states and the phase transitions in quasi-2D strongly correlated electron systems such as cuprate and pnictide high-Tc superconductors. The octet model has been used to describe the FTSTS data according to the simplified banana band model of cuprates in superconducting ground state and worked well deep inside the superconducting dome, but away from the superconducting ground state the description starts to show severe limitations, such as appearance of particle-hole asymmetry of the quasiparticle band as will be discussed later. The first efforts to describe the FTSTS signals based on the fully-phased Green's function-based quasiparticle scattering interference theory, however lacked the full similarity to the FTSTS data, in part due to the lack of accurate information on the tunneling and scattering matrix elements. In this paper we discuss how the noise due to the potential disorder and the various artifacts in the raw FTSTS data can be handled by a simple cross-sectional analysis with an isotropic Gaussian averaging and modeling the set-point effect by an energy-independent and position-dependent factor to the density of states function. The result shows that in the cross-sectional presentation an enhanced correlation exists between the FTSTS data and the theoretical simulation even without the accurate model for the tunneling and the scattering matrix elements and without the assumption for particle-hole symmetry, suggesting that it can be a new starting point of a more robust quantum physical analysis framework appropriate for the phase transition study in the high-Tc superconductors and other strongly correlated electron systems.

cond-mat.supr-con

Intra-unit-cell electronic nematicity of the high-Tc copper-oxide pseudogap states

In the high-transition-temperature (high-Tc) superconductors the pseudogap phase becomes predominant when the density of doped holes is reduced1. Within this phase it has been unclear which electronic symmetries (if any) are broken, what the identity of any associated order parameter might be, and which microscopic electronic degrees of freedom are active. Here we report the determination of a quantitative order parameter representing intra-unit-cell nematicity: the breaking of rotational symmetry by the electronic structure within CuO2 unit cell. We analyze spectroscopic-imaging scanning tunneling microscope images of the intra-unit-cell states in underdoped Bi2Sr2CaCu2O8+δ and, using two independent evaluation techniques, find evidence for electronic nematicity of the states close to the pseudogap energy. Moreover, we demonstrate directly that these phenomena arise from electronic differences at the two oxygen sites within each unit cell. If the characteristics of the pseudogap seen here and by other techniques all have the same microscopic origin, this phase involves weak magnetic states at the O sites that break 90o -rotational symmetry within every CuO2 unit cell.

cond-mat.supr-con

Spectroscopic Fingerprint of Phase-Incoherent Superconductivity in the Cuprate Pseudogap State

A possible explanation for the existence of the cuprate "pseudogap" state is that it is a d-wave superconductor without quantum phase rigidity. Transport and thermodynamic studies provide compelling evidence that supports this proposal, but few spectroscopic explorations of it have been made. One spectroscopic signature of d-wave superconductivity is the particle-hole symmetric "octet" of dispersive Bogoliubov quasiparticle interference modulations. Here we report on this octet's evolution from low temperatures to well into the underdoped pseudogap regime. No pronounced changes occur in the octet phenomenology at the superconductor's critical temperature Tc, and it survives up to at least temperature T ~ 1.5Tc. In the pseudogap regime, we observe the detailed phenomenology that was theoretically predicted for quasiparticle interference in a phase-incoherent d-wave superconductor. Thus, our results not only provide spectroscopic evidence to confirm and extend the transport and thermodynamics studies, but they also open the way for spectroscopic explorations of phase fluctuation rates, their effects on the Fermi arc, and the fundamental source of the phase fluctuations that suppress superconductivity in underdoped cuprates.

cond-mat.supr-con

How Cooper pairs vanish approaching the Mott insulator in Bi2Sr2CaCu2O8+d

The antiferromagnetic ground state of copper oxide Mott insulators is achieved by localizing an electron at each copper atom in real space (r-space). Removing a small fraction of these electrons (hole doping) transforms this system into a superconducting fluid of delocalized Cooper pairs in momentum space (k-space). During this transformation, two distinctive classes of electronic excitations appear. At high energies, the enigmatic 'pseudogap' excitations are found, whereas, at lower energies, Bogoliubov quasi-particles -- the excitations resulting from the breaking of Cooper pairs -- should exist. To explore this transformation, and to identify the two excitation types, we have imaged the electronic structure of Bi2Sr2CaCu2O8+d in r-space and k-space simultaneously. We find that although the low energy excitations are indeed Bogoliubov quasi-particles, they occupy only a restricted region of k-space that shrinks rapidly with diminishing hole density. Concomitantly, spectral weight is transferred to higher energy r-space states that lack the characteristics of excitations from delocalized Cooper pairs. Instead, these states break translational and rotational symmetries locally at the atomic scale in an energy independent fashion. We demonstrate that these unusual r-space excitations are, in fact, the pseudogap states. Thus, as the Mott insulating state is approached by decreasing the hole density, the delocalized Cooper pairs vanish from k-space, to be replaced by locally translational- and rotational-symmetry-breaking pseudogap states in r-space.

cond-mat.supr-con

Real Space Imaging of One-Dimensional Standing Waves: Direct Evidence for a Luttinger Liquid

Electronic standing waves with two different wavelengths were directly mapped near one end of a single-wall carbon nanotube as a function of the tip position and the sample bias voltage with highresolution position-resolved scanning tunneling spectroscopy. The observed two standing waves caused by separate spin and charge bosonic excitations are found to constitute direct evidence for a Luttinger liquid. The increased group velocity of the charge excitation, the power-law decay of their amplitudes away from the scattering boundary, and the suppression of the density of states near the Fermi level were also directly observed or calculated from the two different standing waves.

cond-mat.str-el