arXiv subjects

Ji Ma

Publications and source records attributed to Ji Ma.

At least 55 records · Page 3Linked to original sources

arXiv2024

Probabilistic Visibility-Aware Trajectory Planning for Target Tracking in Cluttered Environments

Target tracking has numerous significant civilian and military applications, and maintaining the visibility of the target plays a vital role in ensuring the success of the tracking task. Existing visibility-aware planners primarily focus on keeping the target within the limited field of view of an onboard sensor and avoiding obstacle occlusion. However, the negative impact of system uncertainty is often neglected, rendering the planners delicate to uncertainties in practice. To bridge the gap, this work proposes a real-time, non-myopic trajectory planner for visibility-aware and safe target tracking in the presence of system uncertainty. For more accurate target motion prediction, we introduce the concept of belief-space probability of detection (BPOD) to measure the predictive visibility of the target under stochastic robot and target states. An Extended Kalman Filter variant incorporating BPOD is developed to predict target belief state under uncertain visibility within the planning horizon. To reach real-time trajectory planning, we propose a computationally efficient algorithm to uniformly calculate both BPOD and the chance-constrained collision risk by utilizing linearized signed distance function (SDF), and then design a two-stage strategy for lightweight calculation of SDF in sequential convex programming. Extensive simulation results with benchmark comparisons show the capacity of the proposed approach to robustly maintain the visibility of the target under high system uncertainty. The practicality of the proposed trajectory planner is validated by real-world experiments.

cs.RO↗

arXiv2024

Gapless spin excitations in nanographene-based antiferromagnetic spin-1/2 Heisenberg chains

Haldane's seminal work established two fundamentally different types of excitation spectra for antiferromagnetic Heisenberg quantum spin chains: gapped excitations in integer-spin chains and gapless excitations in half-integer-spin chains. In finite-length half-integer spin chains, quantization, however, induces a gap in the excitation spectrum, with the upper bound given by the Lieb-Schulz-Mattis (LSM) theorem. Here, we investigate the length-dependent excitations in spin-1/2 Heisenberg chains obtained by covalently linking olympicenes--Olympic rings shaped nanographenes carrying spin-1/2--into one-dimensional chains. The large exchange interaction (J~38 mV) between olympicenes and the negligible magnetic anisotropy in these nanographenes make them an ideal platform for studying quantum spin excitations, which we directly measure using inelastic electron tunneling spectroscopy. We observe a power-law decay of the lowest excitation energy with increasing chain length L, remaining below the LSM boundary. In a long chain with L = 50, a nearly V-shaped excitation continuum is observed, reinforcing the system's gapless nature in the thermodynamic limit. Finally, we visualize the standing wave of a single spinon confined in odd-numbered chains using low-bias current maps. Our results provide compelling evidence for the realization of a one-dimensional analog of a gapless spin liquid.

cond-mat.mtrl-sci↗

arXiv2024

Topological Woodward-Hoffmann classification for cycloadditions in polycyclic aromatic azomethine ylides

The study of cycloaddition mechanisms is central to the fabrication of extended sp2 carbon nanostructures. Reaction modeling in this context has focused mostly on putative, energetically preferred, exothermic products with limited consideration for symmetry allowed or forbidden mechanistic effects. Here, we introduce a scheme for classifying symmetry-forbidden reaction coordinates in Woodward-Hoffmann correlation diagrams. Topological classifiers grant access to the study of reaction pathways and correlation diagrams in the same footing, for the purpose of elucidating mechanisms and products of polycyclic aromatic azomethine ylide (PAMY) cycloadditions with pentacene-yielding polycyclic aromatic hydrocarbons with an isoindole core in the solid-state and on surfaces as characterized by mass spectrometry and scanning tunneling microscopy, respectively. By means of a tight-binding reaction model and density functional theory (DFT) we find topologically-allowed pathways if a product is endothermic, and topologically-forbidden if a product is exothermic. Our work unveils topological classification as a crucial element for reaction modeling for nanographene engineering, and highlights its fundamental role in the design of cycloadditions in on-surface and solid-state chemical reactions, while underscoring that exothermic pathways can be topologically-forbidden.

physics.chem-ph↗

arXiv2024

Thermal spin-crossover and temperature-dependent zero-field splitting in magnetic nanographene chains

Nanographene-based magnetism at interfaces offers an avenue to designer quantum materials towards novel phases of matter and atomic-scale applications. Key to spintronics applications at the nanoscale is bistable spin-crossover which however remains to be demonstrated in nanographenes. Here we show that antiaromatic 1,4-disubstituted pyrazine-embedded nanographene derivatives, which promote magnetism through oxidation to a non-aromatic radical are prototypical models for the study of carbon-based thermal spin-crossover. Scanning tunneling spectroscopy studies reveal symmetric spin excitation signals which evolve at Tc to a zero-energy peak, and are assigned to the transition of a S = 3/2 high-spin to a S = 1/2 low-spin state by density functional theory. At temperatures below and close to the spin-crossover Tc, the high-spin S= 3/2 excitations evidence pronouncedly different temperature-dependent excitation energies corresponding to a zero-field splitting in the Hubbard-Kanamori Hamiltonian. The discovery of thermal spin crossover and temperature-dependent zero-field splitting in carbon nanomaterials promises to accelerate quantum information, spintronics and thermometry at the atomic scale.

physics.chem-ph↗

arXiv2024

Building spin-1/2 antiferromagnetic Heisenberg chains with diaza-nanographenes

Understanding and engineering the coupling of spins in nanomaterials is of central importance for designing novel devices. Graphene nanostructures with π-magnetism offer a chemically tunable platform to explore quantum magnetic interactions. However, realizing spin chains bearing controlled odd-even effects with suitable nanographene systems is challenging. Here, we demonstrate the successful on-surface synthesis of spin-1/2 antiferromagnetic Heisenberg chains with parity-dependent magnetization based on antiaromatic diaza-hexa-peri-hexabenzocoronene (diaza-HBC) units. Using distinct synthetic strategies, two types of spin chains with different terminals were synthesized, both exhibiting a robust odd-even effect on the spin coupling along the chain. Combined investigations using scanning tunneling microscopy, non-contact atomic force microscopy, density functional theory calculations, and quantum spin models confirmed the structures of the diaza-HBC chains and revealed their magnetic properties, which has an S = 1/2 spin per unit through electron donation from the diaza-HBC core to the Au(111) substrate. Gapped excitations were observed in even-numbered chains, while enhanced Kondo resonance emerged in odd-numbered units of odd-numbered chains due to the redistribution of the unpaired spin along the chain. Our findings provide an effective strategy to construct nanographene spin chains and unveil the odd-even effect in their magnetic properties, offering potential applications in nanoscale spintronics.

cond-mat.mtrl-sci↗

arXiv2024

AHMF: Adaptive Hybrid-Memory-Fusion Model for Driver Attention Prediction

Accurate driver attention prediction can serve as a critical reference for intelligent vehicles in understanding traffic scenes and making informed driving decisions. Though existing studies on driver attention prediction improved performance by incorporating advanced saliency detection techniques, they overlooked the opportunity to achieve human-inspired prediction by analyzing driving tasks from a cognitive science perspective. During driving, drivers' working memory and long-term memory play crucial roles in scene comprehension and experience retrieval, respectively. Together, they form situational awareness, facilitating drivers to quickly understand the current traffic situation and make optimal decisions based on past driving experiences. To explicitly integrate these two types of memory, this paper proposes an Adaptive Hybrid-Memory-Fusion (AHMF) driver attention prediction model to achieve more human-like predictions. Specifically, the model first encodes information about specific hazardous stimuli in the current scene to form working memories. Then, it adaptively retrieves similar situational experiences from the long-term memory for final prediction. Utilizing domain adaptation techniques, the model performs parallel training across multiple datasets, thereby enriching the accumulated driving experience within the long-term memory module. Compared to existing models, our model demonstrates significant improvements across various metrics on multiple public datasets, proving the effectiveness of integrating hybrid memories in driver attention prediction.

cs.CV↗

arXiv2024

DOZE: A Dataset for Open-Vocabulary Zero-Shot Object Navigation in Dynamic Environments

Zero-Shot Object Navigation (ZSON) requires agents to autonomously locate and approach unseen objects in unfamiliar environments and has emerged as a particularly challenging task within the domain of Embodied AI. Existing datasets for developing ZSON algorithms lack consideration of dynamic obstacles, object attribute diversity, and scene texts, thus exhibiting noticeable discrepancies from real-world situations. To address these issues, we propose a Dataset for Open-Vocabulary Zero-Shot Object Navigation in Dynamic Environments (DOZE) that comprises ten high-fidelity 3D scenes with over 18k tasks, aiming to mimic complex, dynamic real-world scenarios. Specifically, DOZE scenes feature multiple moving humanoid obstacles, a wide array of open-vocabulary objects, diverse distinct-attribute objects, and valuable textual hints. Besides, different from existing datasets that only provide collision checking between the agent and static obstacles, we enhance DOZE by integrating capabilities for detecting collisions between the agent and moving obstacles. This novel functionality enables the evaluation of the agents' collision avoidance abilities in dynamic environments. We test four representative ZSON methods on DOZE, revealing substantial room for improvement in existing approaches concerning navigation efficiency, safety, and object recognition accuracy. Our dataset can be found at https://DOZE-Dataset.github.io/.

cs.CV↗

arXiv2024

C3L: Content Correlated Vision-Language Instruction Tuning Data Generation via Contrastive Learning

Vision-Language Instruction Tuning (VLIT) is a critical training phase for Large Vision-Language Models (LVLMs). With the improving capabilities of open-source LVLMs, researchers have increasingly turned to generate VLIT data by using open-source LVLMs and achieved significant progress. However, such data generation approaches are bottlenecked by the following challenges: 1) Since multi-modal models tend to be influenced by prior language knowledge, directly using LVLMs to generate VLIT data would inevitably lead to low content relevance between generated data and images. 2) To improve the ability of the models to generate VLIT data, previous methods have incorporated an additional training phase to boost the generative capacity. This process hurts the generalization of the models to unseen inputs (i.e., "exposure bias" problem). In this paper, we propose a new Content Correlated VLIT data generation via Contrastive Learning (C3L). Specifically, we design a new content relevance module which enhances the content relevance between VLIT data and images by computing Image Instruction Correspondence Scores S(I2C). Moreover, a contrastive learning module is introduced to further boost the VLIT data generation capability of the LVLMs. A large number of automatic measures on four benchmarks show the effectiveness of our method.

cs.CV↗

arXiv2024

CAMON: Cooperative Agents for Multi-Object Navigation with LLM-based Conversations

Visual navigation tasks are critical for household service robots. As these tasks become increasingly complex, effective communication and collaboration among multiple robots become imperative to ensure successful completion. In recent years, large language models (LLMs) have exhibited remarkable comprehension and planning abilities in the context of embodied agents. However, their application in household scenarios, specifically in the use of multiple agents collaborating to complete complex navigation tasks through communication, remains unexplored. Therefore, this paper proposes a framework for decentralized multi-agent navigation, leveraging LLM-enabled communication and collaboration. By designing the communication-triggered dynamic leadership organization structure, we achieve faster team consensus with fewer communication instances, leading to better navigation effectiveness and collaborative exploration efficiency. With the proposed novel communication scheme, our framework promises to be conflict-free and robust in multi-object navigation tasks, even when there is a surge in team size.

cs.RO↗

arXiv2024

Magnetic Excitations in Ferromagnetically Coupled Spin-1 Nanographenes

In the quest for high-spin building blocks to form covalently bonded 1D or 2D materials with controlled magnetic interactions, $π$-electron magnetism provides an ideal framework to engineer large ferromagnetic interactions between nanographenes. As a first step in this direction, we investigate the spin properties of ferromagnetically coupled triangulenes, triangular nanographenes with spin $S = 1$. Combining in-solution synthesis of rationally designed molecular precursors and on-surface synthesis, we achieve covalently bonded $S = 2$ triangulene dimers and $S = 3$ trimers on Au(111). Starting from the triangulene dimer, we thoroughly characterize its low-energy magnetic excitations using inelastic electron tunneling spectroscopy (IETS). IETS reveals conductance steps identified as a quintet to triplet excitation, and a zero-bias peak stemming from higher-order spin-spin scattering of the 5-fold degenerate ferromagnetic ground state. The Heisenberg picture captures the relevant parameters of inter-triangulene ferromagnetic exchange, and its successful extension to the larger $S = 3$ system confirms the model's accuracy. We expect that the addition of ferromagnetically coupled building blocks to the toolbox of magnetic nanographenes opens new opportunities to design carbon materials with complex magnetic ground states.

cond-mat.mes-hall↗

arXiv2024

How Far Are We to GPT-4V? Closing the Gap to Commercial Multimodal Models with Open-Source Suites

In this report, we introduce InternVL 1.5, an open-source multimodal large language model (MLLM) to bridge the capability gap between open-source and proprietary commercial models in multimodal understanding. We introduce three simple improvements: (1) Strong Vision Encoder: we explored a continuous learning strategy for the large-scale vision foundation model -- InternViT-6B, boosting its visual understanding capabilities, and making it can be transferred and reused in different LLMs. (2) Dynamic High-Resolution: we divide images into tiles ranging from 1 to 40 of 448$\times$448 pixels according to the aspect ratio and resolution of the input images, which supports up to 4K resolution input. (3) High-Quality Bilingual Dataset: we carefully collected a high-quality bilingual dataset that covers common scenes, document images, and annotated them with English and Chinese question-answer pairs, significantly enhancing performance in OCR- and Chinese-related tasks. We evaluate InternVL 1.5 through a series of benchmarks and comparative studies. Compared to both open-source and proprietary models, InternVL 1.5 shows competitive performance, achieving state-of-the-art results in 8 of 18 benchmarks. Code has been released at https://github.com/OpenGVLab/InternVL.

cs.CV↗

arXiv2024

ASPIRe: An Informative Trajectory Planner with Mutual Information Approximation for Target Search and Tracking

This paper proposes an informative trajectory planning approach, namely, \textit{adaptive particle filter tree with sigma point-based mutual information reward approximation} (ASPIRe), for mobile target search and tracking (SAT) in cluttered environments with limited sensing field of view. We develop a novel sigma point-based approximation to accurately estimate mutual information (MI) for general, non-Gaussian distributions utilizing particle representation of the belief state, while simultaneously maintaining high computational efficiency. Building upon the MI approximation, we develop the Adaptive Particle Filter Tree (APFT) approach with MI as the reward, which features belief state tree nodes for informative trajectory planning in continuous state and measurement spaces. An adaptive criterion is proposed in APFT to adjust the planning horizon based on the expected information gain. Simulations and physical experiments demonstrate that ASPIRe achieves real-time computation and outperforms benchmark methods in terms of both search efficiency and estimation accuracy.

cs.RO↗

arXiv2024

Tunable topological phases in nanographene-based spin-1/2 alternating-exchange Heisenberg chains

Unlocking the potential of topological order within many-body spin systems has long been a central pursuit in the realm of quantum materials. Despite extensive efforts, the quest for a versatile platform enabling site-selective spin manipulation, essential for tuning and probing diverse topological phases, has persisted. Here, we utilize on-surface synthesis to construct spin-1/2 alternating-exchange Heisenberg (AH) chains[1] with antiferromagnetic couplings $J_1$ and $J_2$ by covalently linking Clar's goblets -- nanographenes each hosting two antiferromagnetically-coupled unpaired electrons[2]. Utilizing scanning tunneling microscopy, we exert atomic-scale control over the spin chain lengths, parities and exchange-coupling terminations, and probe their magnetic response by means of inelastic tunneling spectroscopy. Our investigation confirms the gapped nature of bulk excitations in the chains, known as triplons[3]. Besides, the triplon dispersion relation is successfully extracted from the spatial variation of tunneling spectral amplitudes. Furthermore, depending on the parity and termination of chains, we observe varying numbers of in-gap $S=1/2$ edge spins, enabling the determination of the degeneracy of distinct topological ground states in the thermodynamic limit-either 1, 2, or 4. By monitoring interactions between these edge spins, we identify the exponential decay of spin correlations. Our experimental findings, corroborated by theoretical calculations, present a phase-controlled many-body platform, opening promising avenues toward the development of spin-based quantum devices.

cond-mat.mtrl-sci↗

arXiv2024

VoroNav: Voronoi-based Zero-shot Object Navigation with Large Language Model

In the realm of household robotics, the Zero-Shot Object Navigation (ZSON) task empowers agents to adeptly traverse unfamiliar environments and locate objects from novel categories without prior explicit training. This paper introduces VoroNav, a novel semantic exploration framework that proposes the Reduced Voronoi Graph to extract exploratory paths and planning nodes from a semantic map constructed in real time. By harnessing topological and semantic information, VoroNav designs text-based descriptions of paths and images that are readily interpretable by a large language model (LLM). In particular, our approach presents a synergy of path and farsight descriptions to represent the environmental context, enabling LLM to apply commonsense reasoning to ascertain waypoints for navigation. Extensive evaluation on HM3D and HSSD validates VoroNav surpasses existing benchmarks in both success rate and exploration efficiency (absolute improvement: +2.8% Success and +3.7% SPL on HM3D, +2.6% Success and +3.8% SPL on HSSD). Additionally introduced metrics that evaluate obstacle avoidance proficiency and perceptual efficiency further corroborate the enhancements achieved by our method in ZSON planning. Project page: https://voro-nav.github.io

cs.RO↗

arXiv2024

Distributed Optimal Output Consensus Control of Heterogeneous Multi-Agent Systems with Safety Constraints

In this paper, we develop a novel dynamic distributed optimal safe consensus protocol to simultaneously achieve safety requirements and output optimal consensus. Specifically, we construct a distributed projection optimization algorithm with an expanding constraint set in the decision-making layer, while we propose a reference tracking safety controller to ensure that each agent's output remains within a shrinking safety set in the control layer.We also establish the convergence and safety analysis of the closed-loop system using the small-gain theorem and time-varying control barrier function (CBF) theory, respectively. Besides, unlike previous works on distributed optimal consensus, our approach does not require prior knowledge of the local objective or gradient function and adopts a mild assumption on the dynamics of multiagent systems (MASs) by using the transmission zeros condition.

math.OC↗

arXiv2023

Learning List-Level Domain-Invariant Representations for Ranking

Domain adaptation aims to transfer the knowledge learned on (data-rich) source domains to (low-resource) target domains, and a popular method is invariant representation learning, which matches and aligns the data distributions on the feature space. Although this method is studied extensively and applied on classification and regression problems, its adoption on ranking problems is sporadic, and the few existing implementations lack theoretical justifications. This paper revisits invariant representation learning for ranking. Upon reviewing prior work, we found that they implement what we call item-level alignment, which aligns the distributions of the items being ranked from all lists in aggregate but ignores their list structure. However, the list structure should be leveraged, because it is intrinsic to ranking problems where the data and the metrics are defined and computed on lists, not the items by themselves. To close this discrepancy, we propose list-level alignment -- learning domain-invariant representations at the higher level of lists. The benefits are twofold: it leads to the first domain adaptation generalization bound for ranking, in turn providing theoretical support for the proposed method, and it achieves better empirical transfer performance for unsupervised domain adaptation on ranking tasks, including passage reranking.

cs.IR↗

arXiv2023

OpenMSD: Towards Multilingual Scientific Documents Similarity Measurement

We develop and evaluate multilingual scientific documents similarity measurement models in this work. Such models can be used to find related works in different languages, which can help multilingual researchers find and explore papers more efficiently. We propose the first multilingual scientific documents dataset, Open-access Multilingual Scientific Documents (OpenMSD), which has 74M papers in 103 languages and 778M citation pairs. With OpenMSD, we pretrain science-specialized language models, and explore different strategies to derive "related" paper pairs to fine-tune the models, including using a mixture of citation, co-citation, and bibliographic-coupling pairs. To further improve the models' performance for non-English papers, we explore the use of generative language models to enrich the non-English papers with English summaries. This allows us to leverage the models' English capabilities to create better representations for non-English papers. Our best model significantly outperforms strong baselines by 7-16% (in mean average precision).

cs.CL↗

arXiv2023

Tailoring magnetism of nanographenes via tip-controlled dehydrogenation

Atomically precise graphene nanoflakes, called nanographenes, have emerged as a promising platform to realize carbon magnetism. Their ground state spin configuration can be anticipated by Ovchinnikov-Lieb rules based on the mismatch of π-electrons from two sublattices. While rational geometrical design achieves specific spin configurations, further direct control over the π-electrons offers a desirable extension for efficient spin manipulations and potential quantum device operations. To this end, we apply a site-specific dehydrogenation using a scanning tunneling microscope tip to nanographenes deposited on a Au(111) substrate, which shows the capability of precisely tailoring the underlying π-electron system and therefore efficiently manipulating their magnetism. Through first-principles calculations and tight-binding mean-field-Hubbard modelling, we demonstrate that the dehydrogenation-induced Au-C bond formation along with the resulting hybridization between frontier π-orbitals and Au substrate states effectively eliminate the unpaired π-electron. Our results establish an efficient technique for controlling the magnetism of nanographenes.

cond-mat.mtrl-sci↗