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Ji Zou

Publications and source records attributed to Ji Zou.

At least 19 recordsLinked to original sources

Universal Right-Hand Chirality of Evanescent Vector Fields

A locking between propagation direction $\hat{\bf q}$, spin $\hat{\bf S}$, and surface or interface normal $\hat{\bf n}$ -- a phenomenon broadly termed \textit{chirality} -- pervades evanescent or surface waves in optics, magnetism, plasmonics, and acoustics. Yet, it is not known whether the phenomenon is universal or bound to conditions. Here, we unveil that any \textit{source-free} vector field that propagates along $\hat{\bf q}$ and is evanescent along $\hat{\bf n}$, the existence of a spin automatically enforces a rigid, right-handed locking among $\hat{\bf q}$, $\hat{\bf S}$, and $\hat{\bf n}$, that is characterized by a chirality index $C_{\bf q}\equiv \hat{\bf n}\cdot(\hat{\bf S}\times \hat{\bf q})>0$. For an arbitrary propagation direction defined by $\hat{\bf q}\cdot \hat{\bf S}\equiv \eta\in [-1,1]$, i.e., not necessarily transverse spin, we derive a fundamental upper bound $C_{\bf q}\le \sqrt{1-\eta^2}$. The universal absence of left-handed evanescent (source-less) vector fields underscores the fundamental physical non-equivalence of mirror-image configurations -- a principle echoed by parity violation, the natural excess of enantiomers in chiral molecules, and the fixed chirality of DNA.

cond-mat.mes-hall

Perspective: Quantum Computing on Magnetic Racetrack

Magnetic domain walls have long been pursued as carriers of classical information for storage and processing. With the ability to create, control, and probe domain walls at the nanoscale, they are recently recognized as an ideal platform for studying macroscopic quantum effects and provide a natural blueprint for building scalable quantum computing architectures. In particular, the experimentally demonstrated high mobility of domain walls makes them not only suitable as stationary qubits but also as flying qubits, which may offer advantages over currently explored quantum computing platforms. In this Perspective, we outline our current understanding of the essential ingredients and key requirements for realizing universal quantum computation based on magnetic domain walls. We highlight promising concrete material platforms and identify the experiments that are still needed to advance this concept. We also discuss the potential challenges and point to new opportunities in this emerging research direction at the interface between magnetism and quantum information science.

cond-mat.mes-hall

Emergent ac Effect in Nonreciprocal Coupled Condensates

We report an emergent ac Josephson-like effect arising without external bias, driven by the interplay between nonreciprocity and nonlinearity in coupled condensates. Using a minimal model of three mutually nonreciprocally coupled condensates, we uncover a rich landscape of dynamical phases governed by generalized Josephson equations. This goes beyond the Kuramoto framework owing to inherent nonreciprocity and dynamically evolving effective couplings, leading to static and dynamical ferromagnetic and (anti)vortex states with nontrivial phase winding. Most strikingly, we identify an ac phase characterized by the emergence of two distinct frequencies, which spontaneously break the time-translation symmetry: one associated with the precession of the global U(1) Goldstone mode and the other with a stabilized limit cycle in a five-dimensional phase space. This phase features bias-free autonomous oscillatory currents beyond conventional Josephson dynamics. We further examine how instabilities develop in the ferromagnetic and vortex states, and how they drive transitions into the ac regime. Interestingly, the transition is hysteretic: phases with different winding numbers destabilize under distinct conditions, reflecting their inherently different nonlinear structures. Our work lays the foundation for exploring nonreciprocity-driven novel dynamical phases in a broad class of condensate platforms.

cond-mat.mes-hall

Three-dimensional imaging of individual carbon atoms

Carbon is fundamental to science and technology due to its diverse bonding configurations, structural versatility, and essential role in defining the mechanical, chemical, electronic, and quantum properties of materials. However, direct three-dimensional (3D) imaging of individual carbon atoms remains a long-standing challenge. Here, we use twisted bilayer graphene (TBG) as a model system and demonstrate ptychographic atomic electron tomography (pAET) for determining the 3D atomic coordinates of individual carbon atoms with a precision of 0.11 angstrom. The resulting 3D atomic model uncovers chiral lattice distortions driven by van der Waals interactions that exhibit meron-like and skyrmion-like structural textures. These findings provide direct insight into the interplay between 3D chiral lattice deformation and electronic properties in moire-engineered carbon systems. Beyond TBG, pAET offers a versatile approach for 3D atomic-scale imaging of carbon-based and other light-element materials that are central to advances in physics, chemistry, materials science, and nanotechnology.

cond-mat.mtrl-sci

Heisenberg-limited metrology from the quantum-quench dynamics of an anisotropic ferromagnet

The emerging field of quantum magnonics seeks to understand and harness the quantum properties of magnons -- quantized collective spin excitations in magnets. Squeezed magnon states arise naturally as the equilibrium ground states of anisotropic ferromagnets and antiferromagnets, representing an important class of nonclassical magnon states. In this work, we show how a qubit-conditioned quantum quench of an anisotropic ferromagnet can be used for Heisenberg-limited parameter estimation based on measurements of the qubit only. In the presence of ground-state squeezing, the protocol yields information about the eigenmode frequency of the coupled magnon-qubit system, whereas no information is gained in the absence of such squeezing. The protocol therefore leverages genuine quantum correlations in the form of magnonic squeezing while simultaneously relying on the equilibrium character of this squeezing -- a feature distinctive to magnetic systems.

quant-ph

Topological Spin Textures Enabling Quantum Transmission

Quantum spintronics is an emerging field focused on developing novel applications by utilizing the quantum coherence of magnetic systems. A key challenge in this context is achieving scalable long-range quantum information transmission in magnetic systems. Here, we propose a novel transmission scheme based on topological spin textures in a hybrid architecture combining a magnetic racetrack and localized spin qubits. We demonstrate this principle by employing the domain wall (DW), the most fundamental texture, to transport quantum signal between distant qubits. We introduce a measurement-free protocol that utilizes DW mobility to enable high-fidelity and tunable entanglement generation. Furthermore, we demonstrate that spin qubits can function as quantum stations on the racetrack, enabling flexible state transfer among fast-moving DWs on a single track. Finally, we discuss concrete material platforms to implement the proposed scheme. Our work introduces a new hybrid quantum platform that merges topological spin textures with solid-state qubits, offering a scalable architecture for quantum information processing and opening promising directions for quantum spintronics.

cond-mat.mes-hall

Density Matrix Renormalization Group Study of Domain Wall Qubits

Nanoscale topological spin textures in magnetic systems are emerging as promising candidates for scalable quantum architectures. Despite their potential as qubits, previous studies have been limited to semiclassical approaches, leaving a critical gap: the lack of a fully quantum demonstration. Here, we address this challenge by employing the density-matrix renormalization group (DMRG) method to establish domain wall (DW) qubits in coupled quantum spin-1/2 chains. We calculate the ground-state energies and excitation gaps of the system and find that DWs with opposite chiralities form a well-defined low-energy sector, distinctly isolated from higher excited states in the presence of anisotropies. This renders the chirality states suitable for encoding quantum information, serving as robust qubits. Interestingly, when a magnetic field is applied, we observe tunneling between quantum DW states with opposite chiralities. Through quantum simulations, we construct an effective qubit Hamiltonian that exhibits strongly anisotropic $g$-factors, offering a way to implement single-qubit gates. Furthermore, we obtain an effective interacting Hamiltonian for two mobile DWs in coupled quantum spin chains from DMRG simulations, enabling the implementation of two-qubit gates.Single-qubit and two-qubit gates are also demonstrated in real-time simulations using the time-dependent variational principle. Our work represents a critical step from semiclassical constructions to a fully quantum demonstration of the potential of DW textures for scalable quantum computing, establishing a solid foundation for future quantum architectures based on topological magnetic textures.

cond-mat.mes-hall

Directional entanglement of spin-orbit locked nitrogen-vacancy centers by magnons

We address that the stray magnetic field emitted by the excited quantum states of the nitrogen-vacancy (NV) centers is spin-momentum locked, such that the spin transfer to nearby ferromagnetic nanostructures is unidirectional. This may allow the controlled excitation of propagating magnons by NV centers in diamond. A pair of NV spin qubits exchange virtual magnons in a magnetic nanowire in a chiral manner that leads to directional quantum entanglement. A magnon-based ``quantum-entanglement isolator" should be a useful device in future quantum information technology.

cond-mat.mes-hall

Robust Tripartite Entanglement Generation via Correlated Noise in Spin Qubits

We investigate the generation of genuine tripartite entanglement in a triangular spin-qubit system due to spatially correlated noise. In particular, we demonstrate how the formation of a highly entangled dark state -- a W state -- enables robust, long-lived tripartite entanglement. Surprisingly, we find that environmentally induced coherent coupling does not play a crucial role in sustaining this entanglement. This contrasts sharply with the two-qubit case, where the induced coupling significantly influences the entanglement dynamics. Furthermore, we explore two promising approaches to enhance the tripartite entanglement by steering the system towards the dark state: post-selection and coherent driving. Our findings offer a robust method for generating high-fidelity tripartite entangled states with potential applications in quantum computation.

quant-ph

Topological transport of vorticity on curved magnetic membranes

In this work, we study the transport of vorticity on curved dynamical two-dimensional magnetic membranes. We find that topological transport can be controlled by geometrically reducing symmetries, enabling processes absent from flat magnetic systems. To this end, the vorticity 3-current is constructed, which obeys a continuity equation immune to local disturbances of the magnetic texture and spatiotemporal fluctuations of the membrane. We show how electric current can manipulate vortex transport in geometrically nontrivial magnetic systems. As an illustrative example, we propose a minimal setup that realizes an experimentally feasible energy storage device and discuss its thermodynamic efficiency in terms of a vortexoelectric counterpart of the thermoelectric figure of merit $ZT$.

cond-mat.mes-hall

Spin-orbit locking of magnons with localized microwave fields

We address the photonic spin-orbit coupling known from nano-optics and plasmonics in the microwave regime. The spin $\mathbf{S}$ and momentum $\mathbf{q}$ of microwaves emitted by an excited magnetic particle are locked by $\mathbf{q}\cdot\mathbf{S}=0$ with a fixed chirality $\hat{\mathbf{n}}\cdot(\hat{\bf S}\times\hat{\bf q})=1$ when evanescent along $\hat{\mathbf{n}}\perp {\bf q}$. This field excites magnons in a nearby magnetic film in the form of directional beams that rotate with the magnetization direction. The exchange of these magnons between two distant nanomagnets leads to a highly tunable strong coupling and entangles their excited states.

cond-mat.mes-hall

Magnonic $φ$ Josephson junctions and synchronized precession

There has been a growing interest in non-Hermitian physics. One of its main goals is to engineer dissipation and to explore ensuing functionality. In magnonics, the effect of dissipation due to local damping on magnon transport has been explored. However, the effects of non-local damping on the magnonic analog of the Josephson effect remain missing, despite that non-local damping is inevitable and has been playing a central role in magnonics. Here, we uncover theoretically that a surprisingly rich dynamics can emerge in magnetic junctions due to intrinsic non-local damping, using analytical and numerical methods. In particular, under microwave pumping, we show that coherent spin precession in the right and left insulating ferromagnet (FM) of the junction becomes synchronized by non-local damping and thereby a magnonic analog of the $φ$ Josephson junction emerges, where $φ$ stands here for the relative precession phase of right and left FM in the stationary limit. Remarkably, $φ$ decreases monotonically from $ π$ to $π/2$ as the magnon-magnon interaction, arising from spin anisotropies, increases. Moreover, we also find a magnonic diode effect giving rise to rectification of magnon currents. Our predictions are readily testable with current device and measurement technologies at room temperatures.

cond-mat.mes-hall

Tunable Ultrafast Dynamics of Antiferromagnetic Vortices in Nanoscale Dots

Topological vortex textures in magnetic disks have garnered great attention due to their interesting physics and diverse applications. However, up to now, the vortex state has mainly been studied in microsize ferromagnetic disks, which have oscillation frequencies confined to the GHz range. Here, we propose an experimentally feasible ultrasmall and ultrafast vortex state in an antiferromagnetic nanodot surrounded by a heavy metal, which is further harnessed to construct a highly tunable vortex network. We theoretically demonstrate that, interestingly, the interfacial Dzyaloshinskii-Moriya interaction (iDMI) induced by the heavy metal at the boundary of the dot acts as an effective chemical potential for the vortices in the interior. Mimicking the creation of a superfluid vortex by rotation, we show that a magnetic vortex state can be stabilized by this iDMI. Subjecting the system to an electric current can trigger vortex oscillations via spin-transfer torque, which reside in the THz regime and can be further modulated by external magnetic fields. Furthermore, we show that coherent coupling between vortices in different nanodisks can be achieved via an antiferromagnetic link. Remarkably, this interaction depends on the vortex polarity and topological charge and is also exceptionally tunable through the vortex resonance frequency. This opens up the possibility for controllable interconnected networks of antiferromagnetic vortices. Our proposal therefore introduces a new avenue for developing high-density memory, ultrafast logic devices, and THz signal generators, which are ideal for compact integration into microchips.

cond-mat.mes-hall

Tracing Dirac points of topological surface states by ferromagnetic resonance

Ferromagnetic resonance is used to reveal features of the buried electronic band structure at interfaces between ferromagnetic metals and topological insulators. By monitoring the evolution of magnetic damping, the application of this method to a hybrid structure consisting of a ferromagnetic layer and a 3D topological insulator reveals a clear fingerprint of the Dirac point and exhibits additional features of the interfacial band structure not otherwise observable. The underlying spin-pumping mechanism is discussed in the framework of dissipation of angular momentum by topological surface states (TSSs). Tuning of the Fermi level within the TSS was verified both by varying the stoichiometry of the topological insulator layer and by electrostatic backgating and the damping values obtained in both cases show a remarkable agreement. The high energy resolution of this method additionally allows us to resolve the energetic shift of the local Dirac points generated by local variations of the electrostatic potential. Calculations based on the chiral tunneling process naturally occurring in TSS agree well with the experimental results.

cond-mat.mes-hall

Visualizing Magnetic Order in Self-Assembly of Superparamagnetic Nanoparticles

We use soft x-ray vector-ptychographic tomography to determine the three-dimensional magnetization field in superparamagnetic nanoparticles self-assembled at the liquid-liquid interface and reveal the magnetic order induced by layered structure. The spins in individual nanoparticles become more aligned with increasing number of layers, resulting in a larger net magnetization. Our experimental results show a magnetic short-range order in the monolayer due to the proliferation of thermally induced magnetic vortices and a magnetic long-range order in the bilayer and trilayer, stemming from the strengthened dipolar interactions that effectively suppress thermal fluctuations. We also observe a screening effect of magnetic vortices and the attractive interaction between the magnetic vortices with opposite topological charges. Our work demonstrates the crucial role of layered structure in shaping the magnetization of nanoparticle assemblies, providing new opportunities to modulate these properties through strategic layer engineering.

cond-mat.mes-hall

High-fidelity spin qubit shuttling via large spin-orbit interaction

Shuttling spins with high fidelity is a key requirement to scale up semiconducting quantum computers, enabling qubit entanglement over large distances and favoring the integration of control electronics on-chip. To decouple the spin from the unavoidable charge noise, state-of-the-art spin shuttlers try to minimize the inhomogeneity of the Zeeman field. However, this decoupling is challenging in otherwise promising quantum computing platforms such as hole spin qubits in silicon and germanium, characterized by a large spin-orbit interaction and electrically-tunable qubit frequency. In this work, we show that, surprisingly, the large inhomogeneity of the Zeeman field stabilizes the coherence of a moving spin state, thus enabling high-fidelity shuttling also in these systems. We relate this enhancement in fidelity to the deterministic dynamics of the spin which filters out the dominant low-frequency contributions of the charge noise. By simulating several different scenarios and noise sources, we show that this is a robust phenomenon generally occurring at large field inhomogeneity. By appropriately adjusting the motion of the quantum dot, we also design realistic protocols enabling faster and more coherent spin shuttling. Our findings are generally applicable to a wide range of setups and could pave the way toward large-scale quantum processors.

cond-mat.mes-hall

Non-Hermitian Topological Magnonics

Dissipation in mechanics, optics, acoustics, and electronic circuits is nowadays recognized to be not always detrimental but can be exploited to achieve non-Hermitian topological phases or properties with functionalities for potential device applications. As elementary excitations of ordered magnetic moments that exist in various magnetic materials, magnons are the information carriers in magnonic devices with low-energy consumption for reprogrammable logic, non-reciprocal communication, and non-volatile memory functionalities. Non-Hermitian topological magnonics deals with the engineering of dissipation and/or gain for non-Hermitian topological phases or properties in magnets that are not achievable in the conventional Hermitian scenario, with associated functionalities cross-fertilized with their electronic, acoustic, optic, and mechanic counterparts, such as giant enhancement of magnonic frequency combs, magnon amplification, (quantum) sensing of the magnetic field with unprecedented sensitivity, magnon accumulation, and perfect absorption of microwaves. In this review article, we address the unified approach in constructing magnonic non-Hermitian Hamiltonian, introduce the basic non-Hermitian topological physics, and provide a comprehensive overview of the recent theoretical and experimental progress towards achieving distinct non-Hermitian topological phases or properties in magnonic devices, including exceptional points, exceptional nodal phases, non-Hermitian magnonic SSH model, and non-Hermitian skin effect. We emphasize the non-Hermitian Hamiltonian approach based on the Lindbladian or self-energy of the magnonic subsystem but address the physics beyond it as well, such as the crucial quantum jump effect in the quantum regime and non-Markovian dynamics. We provide a perspective for future opportunities and challenges before concluding this article.

cond-mat.mes-hall

Quantum computing on magnetic racetracks with flying domain wall qubits

Domain walls (DWs) on magnetic racetracks are at the core of the field of spintronics, providing a basic element for classical information processing. Here, we show that mobile DWs also provide a blueprint for large-scale quantum computers. Remarkably, these DW qubits showcase exceptional versatility, serving not only as stationary qubits, but also performing the role of solid-state flying qubits that can be shuttled in an ultrafast way. We estimate that the DW qubits are long-lived because they can be operated at sweet spots to reduce potential noise sources. Single-qubit gates are implemented by moving the DW, and two-qubit entangling gates exploit naturally emerging interactions between different DWs. These gates, sufficient for universal quantum computing, are fully compatible with current state-of-the-art experiments on racetrack memories. Further, we discuss possible strategies for qubit readout and initialization, paving the way toward future quantum computers based on mobile topological textures on magnetic racetracks.

cond-mat.mes-hall