arXiv subjects

Jiří Kabát

Publications and source records attributed to Jiří Kabát.

6 recordsLinked to original sources

arXiv2026

Optically Induced Thermal Runaway in Phase-Change VO2 Nanostructures

While thermal runaway occurs across diverse physical disciplines, its presence in subwavelength phase-change photonics remains unexplored because existing thermo-optical models break down near sharp optical transitions. Here, we introduce an iterative multiphysics framework coupling full-wave electrodynamics with heat transfer, and we discover optically induced thermal runaway in vanadium dioxide (VO2) nanostructures. The runaway switching threshold depends on the illumination wavelength, ambient temperature, and underlying substrate, with external thermal biasing significantly reducing the optical intensity required for runaway ignition. Our results push forward the modeling of sharp photothermal transitions and provide essential design principles for active metasurfaces, neuromorphic photonic devices, and nanoscale thermal management.

physics.optics↗

arXiv2026

Reconfigurable plasmonic hot spots enabled by composite VO2-gold plasmonic antennas

We theoretically investigate the formation of electric and magnetic hot spots with reconfigurable plasmonic antennas. We consider three material systems offering different levels of reconfigurability: gold with the static response, vanadium dioxide which allows for ON/OFF switching, and composite gold-vanadium dioxide material platform which offers a possibility to switch between the electric and magnetic hot spot within a single antenna. Using bowtie and diabolo antennas as a case study, we evaluate optical response functions (scattering and absorption cross-sections, electric and magnetic field enhancement). We demonstrate that the composite material system brings, in addition to enhanced reconfigurability, also novel features of plasmonic antennas, such as strong optical absorption and a joint electric-magnetic hotspot.

physics.optics↗

arXiv2026

Tuning of Localized Surface Plasmons in Vanadium Dioxide Nanoparticles via Size and Insulator-Metal Transition

Vanadium dioxide has been identified as a promising phase-changing material for use in tunable plasmonic devices. In this study, we present a comprehensive modal analysis of single-phase and multi-phase vanadium dioxide nanoparticles. In-situ high-resolution electron energy loss spectroscopy was utilized to experimentally resolve the dipole plasmon peak, higher-order and breathing plasmonic modes, and bulk losses as a function of nanoparticle size. Furthermore, the focus is directed toward capturing the dynamic nanoscale optical response throughout the metal-insulator transition in a vanadium dioxide nanoparticle. This system possesses the ability to be gradually switched on and off in terms of the emergence of near-infrared plasmonic absorption. The switching is accompanied by a gradual spectral shift of the absorption peak, amounting to 0.18 eV for a 120 nm nanoparticle. It is envisioned that this phenomenon can be generalized to larger nanostructures with a higher aspect ratio, thereby introducing a wider tunability of the system, which is essential for functional nanodevices based on vanadium dioxide.

physics.optics↗

arXiv2024

Coexisting phases of individual VO$_2$ nanoparticles for multilevel nanoscale memory

Vanadium dioxide (VO$_2$) has received significant interest in the context of nanophotonic metamaterials and memories owing to its reversible insulator-metal transition associated with significant changes in its optical and electronic properties. While the VO$_2$ transition has been extensively studied for several decades, the hysteresis dynamics of individual single-crystal VO$_2$ nanoparticles (NPs) remains largely unexplored. Here, employing transmission electron microscopy techniques, we investigate phase transitions of single VO$_2$ NPs in real time. Our analysis reveals the statistical distribution of the transition temperature and steepness and how they differ during forward (heating) and backward (cooling) transitions. We assess the stability of coexisting phases in individual NPs and prove the persistent multilevel memory at near-room temperatures using only a few VO$_2$ NPs. Our findings shed new light on the underlying physical mechanisms governing the hysteresis of VO$_2$ and establish VO$_2$ NPs as a promising component of optoelectronic and memory devices with enhanced functionalities.

cond-mat.mes-hall↗

arXiv2024

Efficient nanoscale imaging of solid-state phase transitions by transmission electron microscopy demonstrated on vanadium dioxide nanoparticles

We present annular dark field scanning transmission electron microscopy (ADF-STEM) as an efficient, fast, and non-destructive nanoscale tool for monitoring solid-state phase transition. Using metal-insulator transition in vanadium dioxide nanoparticles as an example, we characterize lattice and electronic signatures of the phase transition using analytical transmission electron microscopy including diffraction and electron energy-loss spectroscopy. We demonstrate that ADF-STEM shows a clear contrast across the transition, interpreted with the help of convergent electron beam diffraction as stemming from the crystal-lattice modification accompanying the transition. In addition, ADF-STEM utilizes 3--6 orders of magnitude lower electron dose when compared to electron microscopy techniques able to reveal the phase transition with the same spatial resolution and universality. The benefits of ADF-STEM are emphasized by recording a full hysteresis loop for the metal-insulator transition of a single vanadium dioxide nanoparticle. Our study opens the prospect for fast, non-destructive, large-area and nanoscale characterization of solid-state phase transitions.

cond-mat.mtrl-sci↗

arXiv2024

Analytical electron microscopy analysis of insulating and metallic phases in nanostructured vanadium dioxide

Vanadium dioxide (VO$_2$) is a strongly-correlated material that exhibits insulator-to-metal transition (IMT) near room temperature, which makes it a promising candidate for applications in nanophotonics or optoelectronics. However, creating VO$_2$ nanostructures with the desired functionality can be challenging due to microscopic inhomogeneities that can significantly impact the local optical and electronic properties. Thin lamellas, produced by focused ion beam milling from a homogeneous layer, provide a useful prototype for studying VO$_2$ at the truly microscopic level using a scanning transmission electron microscope (STEM). High-resolution imaging is used to identify structural inhomogeneities while electron energy-loss spectroscopy (EELS) supported by statistical analysis helps to detect V$_x$O$_y$ stoichiometries with a reduced oxidation number of vanadium at the areas of thickness below 70 nm. On the other hand, the thicker areas are dominated by vanadium dioxide, where the signatures of IMT are detected in both core-loss and low-loss EELS experiments with in-situ heating. The experimental results are interpreted with ab-initio and semi-classical calculations. This work shows that structural inhomogeneities such as pores and cracks present no harm to the desired optical properties of VO$_2$ samples.

cond-mat.mtrl-sci↗