Searcharxiv⌕ Search

arXiv subjects

Jia-Xin Yin

Publications and source records attributed to Jia-Xin Yin.

At least 19 recordsLinked to original sources

Topological pair density waves in kagome superconductors

The pair density wave (PDW) is an unconventional superconducting state exhibiting periodic pairing modulations due to pairing with finite momentum Q. In two dimensions, multiple Q components of the PDW can have a non-trivial relative phase, breaking time-reversal symmetry and resulting in a topological electronic structure. Here we review progress on exploring such topological PDWs (TPDWs) and discuss their potential realization in kagome superconductors. We first introduce the concept of a TPDW starting from the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state and examine the challenges toward its realization. We then discuss the possibility of a TPDW in the kagome lattice, which intertwines with chiral superconductivity and loop currents, thus connecting to models describing the quantum anomalous Hall effect. Furthermore, we review the experimental signatures of a TPDW in AV3Sb5 (A = Cs, Rb, K) superconductors and highlight related quantum effects, including switchable chiral pairing modulations, Bogoliubov Fermi states, the superconducting diode effect, and the anomalous thermal Hall effect. Finally, we project the future research opportunities of this correlated topological quantum phase and discuss its broad implications for finite-momentum pairing, topological matter, and chiral superconductivity.

cond-mat.supr-con↗

One-Step Epitaxial Access to Rhombohedral Graphene Flat-Band States on Step-Bunched SiC

Rhombohedral graphene multilayers provide a moiré-free platform for correlated and topological flat-band physics, but direct, transfer-free epitaxial access to thickness-tunable multilayers remains limited. Here we report a one-step graphitization route on 4$^\circ$ off-axis 4H-SiC, in which high-temperature flash annealing simultaneously drives self-organized step bunching and multilayer graphene formation. Atomic-resolution cross-sectional scanning transmission electron microscopy identify local ABC registry and distinguish rhombohedral from Bernal stacking. The thickness is tuned from bilayer to more than twenty layers by varying single parameter, the annealing temperature. Angle-resolved photoemission spectroscopy directly tracks the thickness-dependent evolution from interface-dominated low-energy states toward pronounced near-Fermi-level flat-band spectral weight in thick multilayers. Low-temperature scanning tunneling microscopy and spectroscopy on a 17-layer film further reveal a 13.4 meV low-energy spectral reconstruction and a $\sqrt{3} \times \sqrt{3}$ Kekulé-like modulation, providing microscopic signatures consistent with an intervalley-mixed electronic texture. This one-step, transfer-free approach establishes step-bunched SiC as an epitaxial platform that links stacking engineering with moiré-free correlated flat-band electronic states.

cond-mat.mtrl-sci↗

Discovery of a symmetry-driven electronic cascade in a $d$-wave altermagnet

Altermagnets host magnetic compensation together with non-relativistic spin-split bands, a coexistence enabled by crystal symmetry. Yet whether and how crystal symmetry organizes collective electronic order remains largely unexplored. Here we uncover a symmetry-driven cascade of finite-$q$ charge order in a $d$-wave altermagnet Rb$_{1-δ}$V$_2$Te$_2$O, using phase-resolved scanning tunneling microscopy. A primary density-wave instability drives an initial electronic reconstruction, followed by the emergence of a nematic component and an off-axis modulation with wave vectors geometrically tied to the preceding orders. Phase-resolved spectroscopy distinguishes these components through separate contrast-inversion energies and maps out branch-selective spectral-weight redistribution within the off-axis mode. Together with doping and temperature evolution, these observations establish a highly coordinated hierarchy of coupled density-wave instabilities, consistent with successive symmetry lowering. This multi-component hierarchy can be well described in the Landau framework through sequential softening of the charge orders, where bilinear coupling to their compatible octupolar partners at the lower-symmetry stages enables mutual stabilization within an intertwined charge-multipole state. Such a transparent realization of a charge-order cascade shows how altermagnetic symmetry can extend beyond band formation to organize collective electronic order, offering a new perspective on emergent many-body states in correlated quantum materials.

cond-mat.mes-hall↗

Probing Quantum Geometric Phases via Scanning Tunneling Microscopy

The quantum geometric phase intrinsically dictates the geometry, topology, and many-body correlations of electronic wave functions. While quantum geometric phases are conventionally inferred through momentum-space probes or macroscopic transport measurements, their direct visualization and quantification in real space have historically been restricted by the spatial averaging of bulk techniques. Scanning tunneling microscopy and spectroscopy (STM/STS) circumvent this limitation, leveraging atomic-scale spatial resolution and high energy sensitivity to resolve local electronic phase profiles directly. This review highlights recent progress across four representative methodologies: probing the Aharonov-Bohm (AB) geometric phase via nanoscale real space interferometry; extracting the Berry phase from defect-induced quasiparticle interference and wavefront dislocations; reconstructing the complex phase structure in symmetric systems, such as magic-angle graphene, using order parameter decomposition; and mapping the phase textures and topological defects of pair density wave (PDW) and charge density wave (CDW) in unconventional superconductors utilizing the numerical 2D lock-in technique. Together, these developments show how quantum phases can be translated onto real space and locally resolvable observables. Phase-resolved STM imaging provides stringent constraints on topological states of matter, symmetry-breaking patterns, and strong electronic correlations, outlining a robust framework for in situ phase engineering in quantum materials.

cond-mat.mes-hall↗

Phase-sensitive evidence for pair density waves in a kagome superconductor

Pair density wave (PDW) exhibits periodic amplitude and sign modulations of the superconducting order parameter. Such a pairing state has long been proposed to be highly sensitive to nonmagnetic scattering, but its experimental realization remains elusive. Here we discover a nonmagnetic PDW-breaking effect in a kagome superconductor, using designer atomic nonmagnetic impurities and high-precision scanning tunneling microscopy (STM) at a base temperature of 30mK. We detect 2x2 pair density modulations by Josephson STM with a superconducting tip and 2x2 pairing gap modulations by normal STM. We find that the pairing modulations in both cases are substantially suppressed upon doping the kagome lattice with dilute isovalent nonmagnetic impurities, whereas the charge order and uniform superconductivity remain robust. We further identify the correlation between atomic dopants and the local suppression of PDW. We attribute these findings to a nonmagnetic pair-breaking effect, arising from the phase modulation of PDW in the kagome d-orbital. Taken together with its signatures in other state-of-the-art spectroscopy and transport measurements linked by theory, our findings support the ground state of the kagome superconductor as a correlated topological phase with superconducting loop currents.

cond-mat.supr-con↗

Charge density wave in a band insulator

Charge density wave (CDW) implies a periodic modulation of the charge density. Typically observed in metallic systems, CDWs arise from Fermi surface instabilities, resulting in the total or partial gapping of the Fermi surface. Here, we present experimental evidence for a CDW state emerging in a band insulator which has no Fermi surface. The bulk and surface of our material platform, Bi4Br4, is gapped over the entire Brillouin zone. Through topographic and spectroscopic imaging at low temperatures, we unveil an unexpected unidirectional charge modulation in Bi4Br4, breaking the lattice translation symmetry. The CDW develops at temperatures below 40 K and adds an energy gap atop the existing insulating gap of Bi4Br4. Furthermore, our transport measurements reveal nonlinear electrical conduction, a phenomenon conventionally associated with the sliding or phason mode of incommensurate CDWs. These highly unusual observations represent a new type of CDW and demand a new theoretical framework for CDWs.

cond-mat.str-el↗

Josephson spectroscopy study of kagome superconductors toward the deep point-contact regime

Josephson scanning tunneling microscopy (JSTM) has emerged as an important technique for probing the superconducting order parameter at the atomic scale. However, the Josephson current in JSTM may behave quite differently when the coupling strength varies. Here, we push the junction to the deep point-contact regime, reaching a normal-state junction resistance of only 0.15 $h/2e^2 \simeq 2~{\rm k}Ω$. We demonstrate, using kagome superconductors, that the zero-bias conductance, a key characteristic of the Josephson current, deviates strongly from the quadratic dependence on the normal-state conductance upon entering the deep point-contact regime. Furthermore, we observe a striking saturation of the zero-bias conductance, which we show arises from the series resistance in the circuit. This also serves as a cautious reminder when interpreting zero-bias conductance saturation or quantization in studies of exotic physics such as that of Majorana zero modes if the tip-sample junction resistance is extremely small. Finally, we identify an optimum regime where JSTM can be used as an atomic-scale probe for studying pair-density wave states in materials with low superconducting transition temperature, such as AV3Sb5 kagome superconductors.

cond-mat.supr-con↗

Type-I and Type-II Saddle Points and a Topological Flat Band in a Bi-Pyrochlore Superconductor CsBi2

The divergence of the electron density of states (DOS) plays an important role in enhancing many-body interactions and inducing various quantum phases in low-dimensional systems. However, such unique electronic structures remain experimentally elusive in three-dimensional (3D) systems, particularly those with strong spin-orbit coupling (SOC). Using angle-resolved photoemission spectroscopy and first-principles calculations for a Laves-phase superconductor CsBi$_2$, which features a Bi-pyrochlore 3D network with strong SOC, we identify two characteristic electronic structures with a large DOS. One is a dispersionless topological flat band with p-orbital character, locally formed around the U-K line, which enhances DOS near the Fermi level. The other involves type-I and type-II saddle points connected by a flat band, which cooperatively produce an enhancement in the DOS. Our findings suggest a novel mechanism for achieving a DOS enhancement and lay a foundation for exploring exotic phenomena driven by the interplay of multiple singularities with a large DOS, nontrivial topology, and strong SOC in 3D pyrochlores.

cond-mat.mes-hall↗

Switchable chiral 2x2 pair density wave in pure CsV3Sb5

We investigate electron pairing in a super clean kagome superconductor CsV3Sb5 with a residual resistivity ratio (RRR) of 290. By using the dilution-refrigerator-based scanning tunneling microscopy (STM) at the Synergetic Extreme Condition User Facility (SECUF), we find that the pairing gap exhibits chiral 2x2 modulations, and their chirality can be controlled by magnetic field training. We introduce nonmagnetic impurities to observe the complete suppression of 2x2 pairing modulations in presence of persistent 2x2 charge order. This nonmagnetic pair-breaking effect provides phase-sensitive evidence for pair-density-wave (PDW) induced pairing modulations. Our results support switchable chiral 2x2 PDW in this super clean kagome superconductor.

cond-mat.supr-con↗

Interlayer Charge-density-wave Vector Phase Induced Structural Chirality

Chiral charge density waves (CDWs) have attracted intense interest due to their exotic quantum properties, yet the microscopic origin of structural chirality emerging from correlated charge order remains elusive. Here, we reveal that the interlayer phases of CDW wave vectors, an overlooked degree of freedom, play a crucial role in driving chiral structural displacements in layered CDW materials. By explicitly incorporating the interlayer phases in first-principles calculations, we successfully obtained the chiral structure of the CDW phases of AV$_3$Sb$_5$ (A= K, Rb, and Cs) and 1T-TiSe$_2$. The electronic and optical properties of the predicted chiral structures are consistent with experimental measurements of these materials in their CDW phases. We further predict that 1T-NbSe$_2$ is a promising material candidate for realizing chiral CDW order. Beyond materials prediction, our theory reveals that the chiral CDW can be manipulated by electron filling. Our study opens new avenues for discovering, designing, and engineering chiral CDW materials.

cond-mat.mtrl-sci↗

Unusual Dual Flat Bands and two-dimensional Dirac-node Arc State in Kagome Metal Ni3In2S2

Kagome materials are at the frontier of condensed matter physics. An ideal kagome lattice features only one geometrically frustrated flat band spanning the entire momentum space and a single Dirac cone at the Brillouin-zone corners. However, for the first time, here we observe unusual flat-band and Dirac physics in the newly discovered "322" kagome material Ni3In2S2 by combining high-resolution synchrotron- and laser-based angle-resolved photoemission spectroscopy with a micro-focused beam, scanning tunneling microscopy, and first-principles calculations. We resolve two distinct electronic flat-band states located in close proximity to the Fermi level: a robust Topological Surface Flat Band at ~40 meV below the Fermi level on the Sulfur-terminated surface, originating from weak topological insulator states, and a kagome lattice-derived flat band at ~100 meV binding energy with an ultranarrow bandwidth (~5 meV). Instead of the single Dirac cone, the Indium-terminated surface hosts a rare two-dimensional Dirac-node arc state, where the gapless Dirac nodes extend along an open one-dimensional line crossing the Brillouin-zone boundary, exhibiting sharp linear dispersion, exceptionally high Fermi velocity, and pronounced circular dichroism. These findings establish Ni3In2S2 as a unique topological kagome metal in which multiple flat-band states of different physical origin coexist with an unusual Dirac-node arc, opening an avenue for discovering flat-band--driven and topology-enabled quantum phenomena.

cond-mat.mtrl-sci↗

Wavefunction-Free Approach for Predicting Nonlinear Responses in Weyl Semimetals

By sidestepping the intractable calculations of many-body wavefunctions, density functional theory (DFT) has revolutionized the prediction of ground states of materials. However, predicting nonlinear responses--critical for next-generation quantum devices--still relies heavily on explicit wavefunctions, limiting computational efficiency. In this letter, using the circular photogalvanic effect (CPGE) in Weyl semimetals as a representative example, we realize a 1000-fold computational speedup by eliminating the explicit dependence on wavefunctions. Our approach leverages the one-to-one correspondence between free parameters of Weyl fermions and the associated responses to obtain precise wavefunction-free formulations. Applying our methodology, we systematically investigated known Weyl semimetals and revealed that Ta$_3$S$_2$ exhibits photocurrents an order of magnitude greater than those observed in TaAs, with potential for an additional order-of-magnitude enhancement under strain. To further demonstrate the generality of our approach, we obtained a wavefunction-free formula for the Berry-curvature dipole in Weyl semimetals. Our work paves the way for substantially more efficient screening and optimization of nonlinear electromagnetic properties in topological quantum materials.

cond-mat.mtrl-sci↗

Many-body electronic structure in pyrochlore superconductor CsBi2 and spin liquid Pr2Ir2O7

The pyrochlore lattice materials can exhibit geometrical frustration, while the related many-body electronic states remain elusive. In this work, we performed scanning tunneling microscopy measurements on the pyrochlore superconductor CsBi2 and spin liquid Pr2Ir2O7 at 0.3 K. For the first time, we obtained atomically resolved images of their (111) surfaces, revealing a hexagonal lattice or a kagome lattice. Tunneling spectroscopy in CsBi2 reveals a nearly fully opened superconductivity gap. The ratio of 2Δ/kBTC = 4.7 suggests relatively strong coupling superconductivity, as compared with that in kagome superconductors AV3Sb5 (A = K, Rb, Cs). In contrast to the previous study categorizing CsBi2 as a type-I superconductor, the applied magnetic field induces a hexagonal vortex lattice in which each vortex core exhibits an intriguing three-fold symmetry state. In Pr2Ir2O7, we observed a spatially homogeneous Kondo-lattice resonance, which is compared with that in the kagome Kondo-lattice material CsCr6Sb6. We further discover that the Kondo resonance exhibits a spatial modulation with three-fold symmetry, and the applied magnetic field induces a Zeeman splitting of the Kondo resonance with intriguing atomic site dependence. We discuss the relations of these many-body electronic phenomena with the pyrochlore lattice geometry and its charge or spin frustration. Our systematic observations offer atomic-scale insights into the many-body electronic structures of the geometrically frustrated pyrochlore superconductors and spin liquids.

cond-mat.str-el↗

Observation of Fermi-surface-dependent anisotropic Cooper pairing in kagome superconductor CsV3Sb5

In the recently discovered kagome superconductor AV3Sb5 (A = K, Rb, and Cs), superconductivity is intertwined with an unconventional charge density wave order. The pairing symmetry remains elusive owing to the lack of direct measurement of the superconducting gap in the momentum space. Here, utilizing laser-based ultra-high-resolution and low-temperature angle-resolved photoemission spectroscopy, we observe Fermi-surface-dependent anisotropic Cooper pairing in kagome superconductor CsV3Sb5. We detect a highly anisotropic superconducting gap structure with anisotropy exceeding 80% and a gap maximum along the V-V bond direction on a Fermi surface originating from the 3d-orbital electrons of the V kagome lattice. This is in stark contrast to the isotropic superconducting gap structure on the Fermi surface occupied by Sb 5p-orbital electrons. Our direct observation of the Fermi-surface-dependent anisotropic pairing in CsV3Sb5 is fundamental for understanding the intertwined orders in the ground state of kagome superconductors.

cond-mat.supr-con↗

Effects of background rotation and anisotropy in the holographic description of type-II superconductors

The present work concerns the detailed construction of a holographic model for a type-II s-wave superconductor defined on a 5-dimensional anisotropic rotating black hole. We examine the role of rotation and anisotropy on the properties of the superconductor model focusing on the condensate and the AC conductivity, for which we obtain closed formulas, using both analytical and numerical methods. The results reveal that the rotation is responsible for the appearance of a peak and for introducing an exponentially vanishing behavior in the high-frequency limit of the real component of the AC conductivity. Such a behavior aligns with that observed in high-temperature superconductor models and experiments, where the peak and vanishing behavior result from quasiparticle damping, suggesting a relation between the {\it rotation of a black hole} and {\it quasiparticle damping effects} due to impurities or defects in a superconducting material. This relation supplements the holographic dictionary of the gravity/Condensed Matter Theory correspondence. In addition, we provide a detailed construction of the vortex lattice presented in arXiv:2208.05988 and study its behavior as a function of an external uniform magnetic field. Once again, it is shown that the vortex lattice can be continuously deformed along with a change in the vortex population by virtue of the magnetic field, providing a promising avenue for holographically modeling the vortex lattice deformations observed in experimental studies with superconducting materials. As a concrete example, we describe both the vortex lattice deformation and the increment of the vortex population under the action of an external magnetic field in the LiFeAs type-II superconductor. These effects supplement those previously found for the FeSe type-II superconductor studied in arXiv:2208.05988.

hep-th↗

Atomic perspective on the topological magnetism in kagome metal Co3Sn2S2

Topological quantum materials with kagome lattices have attracted intense interest due to their unconventional electronic structures, which exhibit nontrivial topology, anomalous magnetism, and electronic correlations. Among these, Co3Sn2S2 stands out as a prototypical kagome metal, uniquely combining intrinsic ferromagnetism with topologically nontrivial electronic states. This perspective presents a systematic overview of recent advances in studying kagome metal Co3Sn2S2 achieved through scanning tunneling microscopy. We begin by introducing different methodologies for surface identification and propose using designer layer-selective chemical markers for conclusive surface identification. We then discuss the Berry curvature induced flat band orbital magnetism and the associated unconventional Zeeman effect. Furthermore, we explore boundary states arising from Weyl topology and analyze challenges in detecting Fermi arcs via quasiparticle interference patterns and in uncovering the topological aspect of the edge states. Finally, we review recent observations of spin-orbit-coupled quantum impurity states through spin-polarized tunneling spectroscopy, as well as their connection to Weyl topology and flat band magnetism. We also provide in-depth analysis and constructive comments on the limitations of the current research approach. This review highlights the critical role of scanning tunneling microscopy in unraveling the intricate interplay between topology, magnetism, and correlations at the atomic scale, and the methodology discussed here can be applied to study other topological quantum materials in general.

cond-mat.str-el↗

Charge density wave with suppressed long-range structural modulation in canted antiferromagnetic kagome FeGe

Kagome lattice can host abundant exotic quantum states such as superconductivity and charge density wave (CDW). Recently, successive orders of A-type antiferromagnetism (AFM), CDW and canted AFM have been manifested upon cooling in kagome FeGe. However, the mechanism of CDW and interaction with magnetism remains unclear. Here we investigate the evolution of CDW with temperature across the canted AFM by single-crystal x-ray diffraction, scanning tunneling microscope (STM) and resonant elastic x-ray scattering (REXS). Interestingly, CDW-induced superlattice reflections become weak after the canted AFM, although long-range CDW order is still detectable by STM and REXS. We uncover a novel long-range CDW order with suppressed structural modulation, likely due to the competition for the underlying crystal structure between CDW and canted AFM. Additionally, occupational modulations of Ge1 in the kagome plane and displacive modulations of all atoms were extracted. The results confirm Ge dimerization along the c axis and suggest a dynamic transformation between different CDW domains.

cond-mat.str-el↗

Visualizing higher-fold topology in chiral crystals

Novel topological phases of matter are fruitful platforms for the discovery of unconventional electromagnetic phenomena. Higher-fold topology is one example, where the low-energy description goes beyond Standard Model analogs. Despite intensive experimental studies, conclusive evidence remains elusive for the \textit{multi-gap topological nature of higher-fold chiral fermions}. In this Letter, we leverage a combination of fine-tuned chemical engineering and photoemission spectroscopy with photon energy contrast to discover the higher-fold topology of a chiral crystal. We identify all bulk branches of a higher-fold chiral fermion for the first time, critically important for allowing us to explore unique Fermi arc surface states in multiple inter-band gaps, which exhibit an emergent ladder structure. Through designer chemical gating of the samples in combination with our measurements, we uncover an unprecedented multi-gap bulk boundary correspondence. Our demonstration of multi-gap electronic topology will propel future research on unconventional topological responses.

cond-mat.mtrl-sci↗