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Jiacheng Gao

Publications and source records attributed to Jiacheng Gao.

At least 19 recordsLinked to original sources

SLIDE: Shuffle Shamir Secret Shares Uniformly with Linear Online Communication and Guaranteed Output Delivery

We revisit shuffle protocols for Shamir secret sharing. Existing constructions either produce non-uniform shuffles or incur high communication and round complexity, sometimes exponential in the number of parties. We propose two new shuffle protocols that achieve uniform shuffling with communication complexity $O((k+l)n^2m\log m/\log k)$ for an $m$-by-$l$ matrix shared among $n$ parties, where $k\leq m$ is a tunable parameter. The first protocol is concretely efficient, while the second achieves the best-known $O(nml)$ online communication and $O(n)$ rounds. Experiments show significant improvements in online efficiency and total cost over prior work. Our key technical ingredient is a novel permutation sharing technique that represents permutations using smaller permutation matrices, making their application significantly more efficient. The first protocol applies independent secret permutations sequentially, while the second builds on shuffle correlation to achieve optimal online complexity. We further extend shuffle correlation to support guaranteed output delivery with linear online communication, yielding SLIDE, the first protocol to achieve both $O(nml)$ online communication and guaranteed output delivery. Our constructions rely only on basic Shamir secret sharing over any field of size greater than $n$. As shuffling is a fundamental primitive for MPC tasks such as sorting and oblivious data structures, our results enable more efficient and scalable secure computation in practice.

cs.CR

Inference for Multiple Change-points in Piecewise Locally Stationary Time Series

Change-point detection and locally stationary time series modeling are two major approaches for the analysis of non-stationary data. The former aims to identify stationary phases by detecting abrupt changes in the dynamics of a time series model, while the latter employs (locally) time-varying models to describe smooth changes in dependence structure of a time series. However, in some applications, abrupt and smooth changes can co-exist, and neither of the two approaches alone can model the data adequately. In this paper, we propose a novel likelihood-based procedure for the inference of multiple change-points in locally stationary time series. In contrast to traditional change-point analysis where an abrupt change occurs in a real-valued parameter, a change in locally stationary time series occurs in a parameter curve, and can be classified as a jump or a kink depending on whether the curve is discontinuous or not. We show that the proposed method can consistently estimate the number, locations, and the types of change-points. Two different asymptotic distributions corresponding respectively to jump and kink estimators are also established. Extensive simulation studies and a real data application to financial time series are provided.

stat.ME

A robust and tunable Luttinger liquid in correlated edge of transition-metal second-order topological insulator Ta$_2$Pd$_3$Te$_5$

The interplay between topology and interaction always plays an important role in condensed matter physics and induces many exotic quantum phases, while rare transition metal layered material (TMLM) has been proved to possess both. Here we report a TMLM Ta$_2$Pd$_3$Te$_5$ has the two-dimensional second-order topology (also a quadrupole topological insulator) with correlated edge states - Luttinger liquid. It is ascribed to the unconventional nature of the mismatch between charge- and atomic- centers induced by a remarkable double-band inversion. This one-dimensional protected edge state preserves the Luttinger liquid behavior with robustness and universality in scale from micro- to macro- size, leading to a significant anisotropic electrical transport through two-dimensional sides of bulk materials. Moreover, the bulk gap can be modulated by the thickness, resulting in an extensive-range phase diagram for Luttinger liquid. These provide an attractive model to study the interaction and quantum phases in correlated topological systems.

cond-mat.mes-hall

Evidence for an Excitonic Insulator State in Ta$_2$Pd$_3$Te$_5$

The excitonic insulator (EI) is an exotic ground state of narrow-gap semiconductors and semimetals arising from spontaneous condensation of electron-hole pairs bound by attractive Coulomb interaction. Despite research on EIs dating back to half a century ago, their existence in real materials remains a subject of ongoing debate. In this study, through systematic experimental and theoretical investigations, we provide evidence for the existence of an EI ground state in a van der Waals compound Ta$_2$Pd$_3$Te$_5$. Density-functional-theory calculations suggest that it is a semimetal with a small band overlap, whereas various experiments exhibit an insulating ground state with a clear band gap. Upon incorporating electron-hole Coulomb interaction into our calculations, we obtain an EI phase where the electronic symmetry breaking opens a many-body gap. Angle-resolved photoemission spectroscopy measurements exhibit that the band gap is closed with a significant change in the dispersions as the number of thermally excited charge carriers becomes sufficiently large in both equilibrium and nonequilibrium states. Structural measurements reveal a slight breaking of crystal symmetry with exceptionally small lattice distortion in the insulating state, which cannot account for the significant gap opening. Therefore, we attribute the insulating ground state with a gap opening in Ta$_2$Pd$_3$Te$_5$ to exciton condensation, where the coupling to the symmetry-breaking electronic state induces a subtle change in the crystal structure.

cond-mat.mtrl-sci

Magnetic-field modulation of topological electronic states and emergent magneto-transport in a magnetic Weyl semimetal

The modulation of topological electronic states by an external magnetic field is highly desired for condensed matter physics. Schemes to achieve this have been proposed theoretically, but few can be realized experimentally. Here, combining transverse transport, theoretical calculations, and scanning tunneling microscopy/spectroscopy (STM/S) investigations, we provide an observation that the topological electronic states, accompanied by an emergent magneto-transport phenomenon, were modulated by applying magnetic fields through induced non-collinear magnetism in the magnetic Weyl semimetal EuB6. A giant unconventional anomalous Hall effect (UAHE) is found during the magnetisation re-orientation from easy axis to hard ones in magnetic fields, with a UAHE peak around the low field of 5 kOe. Under the reasonable spin-canting effect, the folding of the topological anti-crossing bands occurs, generating a strong Berry curvature that accounts for the observed UAHE. Field-dependent STM/S reveals a highly synchronous evolution of electronic density of states, with a dI/dV peak around the same field of 5 kOe, which provides evidence to the folded bands and excited UAHE by external magnetic fields. This finding elucidates the connection between the real-space non-collinear magnetism and the k-space topological electronic states and establishes a novel manner to engineer the magneto-transport behaviours of correlated electrons for future topological spintronics.

cond-mat.mtrl-sci

Magnetic band representations, Fu-Kane-like symmetry indicators and magnetic topological materials

To realize novel topological phases and to pursue potential applications in low-energy consumption spintronics, the study of magnetic topological materials is of great interest. Starting from the theory of nonmagnetic topological quantum chemistry [Bradlyn et al., Nature 547, 298 (2017)], we have obtained irreducible (co)representations and compatibility relations (CRs) in momentum space, and we constructed a complete list of magnetic band (co)representations (MBRs) in real space for other MSGs with anti-unitary symmetries (i.e. type-III and type-IV MSGs). The results are consistent with the magnetic topological quantum chemistry [Elcoro et al., Nat. Comm. 12, 5965 (2021)]. Using the CRs and MBRs, we reproduce the symmetry-based classifications for MSGs, and we obtain a set of Fu-Kane-like formulas of symmetry indicators (SIs) in both spinless (bosonic) and spinful (fermionic) systems, which are implemented in an automatic code - TopMat - to diagnose topological magnetic materials. The magnetic topological materials, whose occupied states can not be decomposed into a sum of MBRs, are consistent with nonzero SIs. Lastly, using our online code, we have performed spin-polarized calculations for magnetic compounds in the materials database and find many magnetic topological candidates.

cond-mat.mtrl-sci

Interaction Driven Topological Phase Transition in Monolayer CrCl$_2$(pyrazine)$_2$

The quadratic band crossing points (QBCPs) at Fermi level in two-dimension have been proposed to be unstable under electron-electron interaction. The possible interaction driven states include quantum anomalous Hall (QAH) state and various nematic ordered states. In this work, motivated by the discovery of ferromagnetic van der Waals layered metal-organic framework CrCl$_2$(pyrazine)$_2$, we theoretically propose that the single layer of CrCl$_2$(pyrazine)$_2$ might realize one or some of these interaction driven states based on the QBCP protected by $C_4$ symmetry. By introducing the short-range density-density type repulsion interactions into this system, we have found the phase diagram depending on different interaction range and strength. The exotic phases include the staggered chiral flux state manifesting QAH effect, the site-nematic insulator and the site-nematic Dirac semimetal state. The QAH state is robust against perturbations breaking the QBCP but it is weakened by increasing temperature. The metal-organic framework is tunable by changing the transition-metal elements, which might improve the gap size and stability of this interaction induced QAH state.

cond-mat.mtrl-sci

Twisted nodal wires and three-dimensional quantum spin Hall effect in distorted square-net compounds

Recently, square-net materials have attracted lots of attention for the Dirac semimetal phase with negligible spin-orbit coupling (SOC) gap, e.g. ZrSiS/LaSbTe and CaMnSb$_2$. In this paper, we demonstrate that the Jahn-Teller effect enlarges the nontrivial SOC gap in the distorted structure, e.g. LaAsS and SrZnSb$_2$. Its distorted $X$ square-net layer ($X=$ P, As, Sb, Bi) resembles a quantum spin Hall (QSH) insulator. Since these QSH layers are simply stacked in the $\hat{x}$ direction and weakly coupled, three-dimensional QSH effect can be expected in these distorted materials, such as insulating compounds CeAs$_{1+x}$Se$_{1-y}$ and EuCdSb$_2$. Our detailed calculations show that it hosts two twisted nodal wires without SOC [each consists of two noncontractible time-reversal symmetry- and inversion symmetry-protected nodal lines touching at a fourfold degenerate point], while with SOC it becomes a topological crystalline insulator with symmetry indicators $(000; 2)$ and mirror Chern numbers $(0, 0)$. The nontrivial band topology is characterized by a generalized spin Chern number $C_{s+}=2$ when there is a gap between two sets of $\hat{s}_{x}$ eigenvalues. The nontrivial topology of these materials can be well reproduced by our tight-binding model and the calculated spin Hall conductivity is quantized to $σ^{x}_{yz} = (\frac{\hbar}{e})\frac{G_xe^2}{πh}$ with $G_x$ a reciprocal lattice vector.

cond-mat.mtrl-sci

Unprotected quadratic band crossing points and quantum anomalous Hall effect in FeB2 monolayer

Quadratic band crossing points (QBCPs) and quantum anomalous Hall effect (QAHE) have attracted the attention of both theoretical and experimental researchers in recent years. Based on first-principle calculations, we find that the FeB$_2$ monolayer is a nonmagnetic semimetal with QBCPs at $K$. Through symmetry analysis and $\mathbf{k}\cdot\mathbf{p}$ invariant theory, we find that the QBCP is not protected by rotation symmetry and consists of two Dirac points with same chirality (Berry phase of $2π$). Once introducing Coulomb interactions, we find that there is a spontaneous-time-reversal-breaking instability of the spinful QBCPs, which gives rise to a $C=2$ QAH insulator with orbital moment ordering.

cond-mat.mes-hall

Unconventional Materials: the mismatch between electronic charge centers and atomic positions

The complete band representations (BRs) have been constructed in the work of topological quantum chemistry. Each BR is expressed by either a localized orbital at a Wyckoff site in real space, or by a set of irreducible representations in momentum space. In this work, we define unconventional materials with a common feature of the mismatch between average electronic centers and atomic positions. They can be effectively diagnosed as whose occupied bands can be expressed as a sum of elementary BRs (eBRs), but not a sum of atomic-orbital-induced BRs (aBRs). The existence of an essential BR at an empty site is described by nonzero real-space invariants (RSIs). The "valence" states can be derived by the aBR decomposition, and unconventional materials are supposed to have an uncompensated total "valence" state. The high-throughput screening for unconventional materials has been performed through the first-principles calculations. We have discovered 423 unconventional compounds, including thermoelectronic materials, higher-order topological insulators, electrides, hydrogen storage materials, hydrogen evolution reaction electrocatalysts, electrodes, and superconductors. The diversity of these interesting properties and applications would be widely studied in the future.

cond-mat.mtrl-sci

The Role of Shift Vector in High-Harmonic Generation from Non-Centrosymmetric Topological Insulators under Strong Laser Fields

As a promising avenue to obtain new extreme ultraviolet light source and detect electronic properties, high-harmonic generation (HHG) has been actively developed in both theory and experiment. In solids lacking inversion symmetry, when electrons undergo a nonadiabatic transition, a directional charge shift occurs and is characterized by shift vector, which measures the real-space shift of the photoexcited electron and hole. For the first time, we have revealed that shift vector plays prominent roles in the real-space tunneling mechanism of three-step model for electrons under strong laser fields. Since shift vector is determined by the topological properties of related wave functions, we expect HHG with its contribution can provide direct knowledge on the band topology in noncentrosymmetric topological insulators (TIs). In both Kane-Mele model and realistic material BiTeI, we have found that the shift vector reverses when band inversion happens during the topological phase transition between normal and topological insulators. Under oscillating strong laser fields, the reversal of shift vector leads to completely opposite radiation time of high-order harmonics. This makes HHG a feasible all-optical strong-field method to directly identify the band inversion in non-centrosymmetric TIs.

physics.optics

The evolution of Weyl nodes in Ni doped thallium niobate pyrochlore Tl$_{2-x}$Ni$_x$Nb$_2$O$_7$

Magnetic Weyl semimetal (WSM) is of great importance both for fundamental physics and potential applications due to its spontaneous magnetism, robust band topology, and enhanced Berry curvature. It possesses many unique quantum effects, including large intrinsic anomalous Hall effect, Fermi arcs, and chiral anomaly. In this work, using ab initio calculations, we propose that Ni doped pyrochlore Tl$_2$Nb$_2$O$_7$ is a magnetic WSM caused by exchange field splitting on bands around its quadratic band crossing point. The exchange field tuned by Ni 3d on-site Coulomb interaction parameter $U$ drives the evolution of Weyl nodes and the resulting topological phase transition. Since Weyl nodes can exist at generic point in Brillouin zone and are hard to be exactly identified, the creation and annihilation of them, i.e., the change in their number, chirality and distribution, have been consistently confirmed with a combined theoretical approach, which employs parity criterion, symmetry indicator analysis and the Wilson loop of Wannier center. We find that Weyl nodes remain in a quite large range of $U$ and are close to Fermi level, which makes the experimental observation very possible. We think this method and our proposal of magnetic WSM will be useful in finding more WSMs and adding our understanding on the topological phase transition.

cond-mat.mtrl-sci

Robust Weyl Semimetal and Pressure-induced Superconductivity in Quasi-One-Dimensional (NbSe4)2I

A search for the single material system that simultaneously exhibits topological phase and intrinsic superconductivity has been largely limited, although such a system is far more favorable especially for the quantum device applications. Except artificially engineered topological superconductivity in heterostructure systems, another alternative is to have superconductivity arising from the topological materials by pressure or other clean technology. Here, based on first-principles calculations, we first show that quasi-one-dimensional compound (NbSe4)2I represents a rare example of a chiral Weyl semimetal in which the set of symmetry-related Weyl points (WPs) exhibit the same chiral charge at a certain energy. The net chiral charge (NCC) of the below Fermi level EF (or a certain energy) can be tuned by pressure. In addition, a partial disorder induced by pressure accompanied with superconductivity emerges. Although amorphization of the iodine sub-lattice under high pressure, the one-dimensional NbSe4 chains in (NbSe4)2I remain intact and provide a superconducting channel in one dimension. Our combined theoretical and experimental research provide critical insight into a new phase of the one-dimensional system, in which distinctive phase transitions and correlated topological states emerge upon compression.

cond-mat.supr-con

Application of topological quantum chemistry in electrides

The recently developed theory of topological quantum chemistry (TQC) has built a close connection between band representations in momentum space and orbital characters in real space. It provides an effective way to diagnose topological materials, leading to the discovery of lots of topological materials after the screening of all known nonmagnetic compounds. On the other hand, it can also efficiently reveal spacial orbital characters, including average charge centers and site-symmetry characters. By using TQC theory with the computed irreducible representations in the first-principles calculations, we demonstrate that the electrides with excess electrons serving as anions at vacancies can be well identified by analyzing band representations (BRs), which cannot be expressed as a sum of atomic-orbital-induced band representations (aBRs). In fact, the floating bands (formed by the excess electrons) belong to the BRs induced from the "pseudo-orbitals" centered at vacancies. In other words, the electrides are proved to be unconventional ionic crystals, where a set of occupied bands is not a sum of aBRs but necessarily contains a BR from vacancies. The TQC theory provides a promising avenue to pursue more electride candidates in ionic crystals.

cond-mat.mtrl-sci

Strong electron-phonon coupling in 3D tungsten nitride and coexistence of intrinsic superconductivity and topological nodal line in its 2D limit

Three-component fermion beyond the conventional Dirac Weyl Majorana classification attracts extensive attentions recently and many efforts have been paid to explore their superconductivity. Based on first-principles calculations, we systematically investigate the electron-phonon coupling (EPC) in the three-component fermion materials WN, WC and TaN. The EPC in pristine and pressured WC and TaN are to small to induce superconductivity. Electron doping can efficiently enhance the EPC strength and the predicted Tcs reach the value of experiments. Upon 0.6 electron/unitcell doping, the EPC strength of TaN is boosted by two orders of magnitude and Tc can even be as high as 27 K, revealing the crucial role of charge doping in the formation of superconductivity observed in WC and TaN. In stark contrast, pristine WN exhibits overwhelmingly strong EPC and can be a good superconductor with a high transition temperature Tc of 31 K. The strong EPC in WN are dictated by a synergistic effect of strong Fermi nesting and large deformation potential. Going down from three-dimension (3D) to three-dimension (2D), WN thin film (i.e. monolayer W3N4) is also an intrinsic superconductor with Tc of 11 K. Most importantly, monolayer W3N4 host Dirac nodal lines protected by mirror symmetry in the absence of spin-orbit coupling (SOC), Including SOC, the Dirac nodal lines split into three pairs of spinful Weyl rings. These nodal lines lies closely near the Fermi level, they are pure and clean without other nontrivial bands, which is scarce in real materials and making the exotic topological properties easily accessible in experiment. The coexistence of superconductivity with high transition temperature and topological states in WN and its 2D film provide a promising platform for exploring topological superconductivity.

cond-mat.supr-con

High-throughput screening for Weyl Semimetals with S$_{4}$ Symmetry

Based on irreducible representations (or symmetry eigenvalues) and compatibility relations, a material can be predicted to be a topological/trivial insulator [satisfying compatibility relations] or a topological semimetal [violating compatibility relations]. However, Weyl semimetals usually go beyond this symmetry-based strategy. In other words, Weyl nodes could emerge in a material, no matter if its occupied bands satisfy compatibility relations, or if the symmetry indicators are zero. In this work, we propose a new topological invariant $χ$ for the systems with S$_4$ symmetry [i.e., the improper rotation S$_4$ ($\equiv$ IC$_{4z}$) is a proper four-fold rotation (C$_{4z}$) followed by inversion (I)], which can be used to diagnose the Weyl semimetal phase. Moreover, $χ$ can be easily computed through the one-dimensional Wilson-loop technique. By applying this method to the high-throughput screening in first-principles calculations, we predict a lot of Weyl semimetals in both nonmagnetic and magnetic compounds. Various interesting properties (e.g. magnetic frustration effects, superconductivity and spin-glass order, etc.) are found in predicted Weyl semimetals, which provide realistic platforms for future experimental study of the interplay between Weyl fermions and other exotic states.

cond-mat.mtrl-sci

Irvsp: to obtain irreducible representations of electronic states in the VASP

We present an open-source program irvsp, to compute irreducible representations of electronic states for all 230 space groups with an interface to the Vienna ab-initio Simulation Package. This code is fed with plane-wave-based wavefunctions (e.g. WAVECAR) and space group operators (listed in OUTCAR), which are generated by the VASP package. This program computes the traces of matrix presentations and determines the corresponding irreducible representations for all energy bands and all the k-points in the three-dimensional Brillouin zone. It also works with spin-orbit coupling (SOC), i.e., for double groups. It is in particular useful to analyze energy bands, their connectivities, and band topology, after the establishment of the theory of topological quantum chemistry. Accordingly, the associated library - irrep_bcs.a - is developed, which can be easily linked to by other ab-initio packages. In addition, the program has been extended to orthogonal tight-binding (TB) Hamiltonians, e.g. electronic or phononic TB Hamiltonians. A sister program ir2tb is presented as well.

cond-mat.mtrl-sci

Spin Excitations and Spin Wave Gap in the Ferromagnetic Weyl Semimetal Co$_3$Sn$_2$S$_2$

We report a comprehensive neutron scattering study on the spin excitations in the magnetic Weyl semimetal Co$_3$Sn$_2$S$_2$ with quasi-two-dimensional structure. Both in-plane and out-of-plane dispersions of the spin waves are revealed in the ferromagnetic state, similarly dispersive but damped spin excitations persist into the paramagnetic state. The effective exchange interactions have been estimated by a semi-classical Heisenberg model to consistently reproduce the experimental $T_C$ and spin stiffness. However, a full spin wave gap below $E_g=2.3$ meV is observed at $T=4$ K, much larger than the estimated magnetic anisotropy energy ($\sim0.6$ meV), while its temperature dependence indicates a significant contribution from the Weyl fermions. These results suggest that Co$_3$Sn$_2$S$_2$ is a three-dimensional correlated system with large spin stiffness, and the low-energy spin dynamics could interplay with the topological electron states.

cond-mat.str-el