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Jianbin Xu

Publications and source records attributed to Jianbin Xu.

27 records · Page 2Linked to original sources

Ultrawideband solid-state terahertz phase shifter electrically modulated by tunable conductive interface in total internal reflection geometry

Phase modulation plays a crucial role in various terahertz applications, including biomedical imaging, high-rate communication, and radar detection. Existing terahertz phase shifters typically rely on tuning the resonant effect of metamaterial structures to achieve a narrow bandwidth phase shift. However, the terahertz band offers a wide bandwidth resource, which has great advantages in high longitudinal resolution detection, high-capacity communication, spectral imaging and so on. Here, we propose and demonstrate an ultrawideband terahertz phase shifting mechanism that utilizes an optical conductivity tuneable interface combined with a non-resonant metasurface operating in the total internal reflection geometry. This approach effectively modulates the phase of the reflected terahertz signal in an ultrawideband. To implement this mechanism, we designed a structure consisting of graphene-loaded non-resonant periodic metal microslits arranged in the total internal reflection geometry. By controlling the gate voltage of the graphene within a range of 5 V, an averaged ~120° continuous phase shift in the frequency range of 0.4 to 1.2 THz was achieved. Notably, in the frequency range of 1 to 1.2 THz, the phase modulation exhibited a linear relationship with the driving voltage. Our device demonstrated minimal fluctuations in the reflected amplitude, with a deviation of less than 1 dB and an insertion loss of less than 10 dB. Additionally, the modulation speed of this solid-state device reached the kHz level. Remarkably, the phase modulation bandwidth (Δf/f) achieved approximately 100% of the arithmetic centre frequency at 0.8 THz, surpassing the definition of ultrawideband, which typically encompasses 20% of the centre frequency. To the best of our knowledge, this is the first and most wideband phase shifter developed for the terahertz regime to date.

physics.optics↗

Accurate prediction of heat conductivity of water by a neuroevolution potential

We propose an approach that can accurately predict the heat conductivity of liquid water. On the one hand, we develop an accurate machine-learned potential based on the neuroevolution-potential approach that can achieve quantum-mechanical accuracy at the cost of empirical force fields. On the other hand, we combine the Green-Kubo method and the spectral decomposition method within the homogeneous nonequilibrium molecular dynamics framework to account for the quantum-statistical effects of high-frequency vibrations. Excellent agreement with experiments under both isobaric and isochoric conditions within a wide range of temperatures is achieved using our approach.

physics.comp-ph↗

Twist-Dependent Anisotropic Thermal Conductivity in Homogeneous MoS$_2$ Stacks

Thermal transport property of homogeneous twisted molybdenum disulfide (MoS$_2$) is investigated using non-equilibrium molecular dynamics simulations with the state-of-art force fields. The simulation results demonstrate that the cross-plane thermal conductivity strongly depends on the interfacial twist angle, while it has only a minor effect on the in-plane thermal conductivity, exhibiting a highly anisotropic nature. A frequency-decomposed phonon analysis showed that both the cross-plane and in-plane thermal conductivity of MoS$_2$ are dominated by the low-frequency phonons below 15 THz. As the interfacial twist angle increases, these low-frequency phonons significantly attenuate the phonon transport across the interface, leading to impeded cross-plane thermal transport. However, the in-plane phonon transport is almost unaffected, which allows for maintaining high in-plane thermal conductivity. Additionally, our study revealed the strong size dependence for both cross-plane and in-plane thermal conductivities due to the low-frequency phonons of MoS$_2$. The maximum in-plane to cross-plane thermal anisotropy ratio is estimated as 400 for twisted MoS$_2$ from our simulation, which is in the same order of magnitude as recent experimental results (~900). Our study highlights the potential of twist engineering as a tool for tailoring the thermal transport properties of layered materials.

physics.comp-ph↗

Transmission-matrix Quantitative Phase Profilometry for Accurate and Fast Thickness Mapping of 2D Materials

The physical properties of two-dimensional (2D) materials may drastically vary with their thickness profiles. Current thickness profiling methods for 2D material (e.g., atomic force microscopy and ellipsometry) are limited in measurement throughput and accuracy. Here we present a novel high-speed and high-precision thickness profiling method, termed Transmission-Matrix Quantitative Phase Profilometry (TM-QPP). In TM-QPP, picometer-level optical pathlength sensitivity is enabled by extending the photon shot-noise limit of a high sensitivity common-path interferometric microscopy technique, while accurate thickness determination is realized by developing a transmission-matrix model that accounts for multiple refractions and reflections of light at sample interfaces. Using TM-QPP, the exact thickness profiles of monolayer and few-layered 2D materials (e.g., MoS2, MoSe2 and WSe2) are mapped over a wide field of view within seconds in a contact-free manner. Notably, TM-QPP is also capable of spatially resolving the number of layers of few-layered 2D materials.

physics.optics↗

Variable thermal transport in black, blue, and violet phosphorene from extensive atomistic simulations with a neuroevolution potential

Phosphorus has diverse chemical bonds and even in its two-dimensional form there are three stable allotropes: black phosphorene (Black-P), blue phosphorene (Blue-P), and violet phosphorene (Violet-P). Due to the complexity of these structures, no efficient and accurate classical interatomic potential has been developed for them. In this paper, we develop an efficient machine-learned neuroevolution potential model for these allotropes and apply it to study thermal transport in them via extensive molecular dynamics (MD) simulations. Based on the homogeneous nonequilibrium MD method, the thermal conductivities are predicted to be $12.5 \pm 0.2$ (Black-P in armchair direction), $78.4 \pm 0.4$ (Black-P in zigzag direction), $128 \pm 3$ (Blue-P), and $2.36 \pm 0.05$ (Violet-P) $\mathrm{Wm^{-1}K^{-1}}$. The underlying reasons for the significantly different thermal conductivity values in these allotropes are unraveled through spectral decomposition, phonon eigenmodes, and phonon participation ratio. Under external tensile strain, the thermal conductivity in black-P and violet-P are finite, while that in blue-P appears unbounded due to the linearization of the flexural phonon dispersion that increases the phonon mean free paths in the zero-frequency limit.

physics.comp-ph↗

Near-field radiative heat transfer between hybrid polaritonic structures

Near-field radiative heat transfer between close objects may exceed the far-field blackbody radiation in orders of magnitude when exploiting polaritonic materials. Great efforts have been made to experimentally measure this fundamental stochastic effect but mostly based on simple materials. In this work, we foster an all-optical method to characterize the heat transfer between less explored plasmon-phonon hybrid polaritonic systems made of graphene-SiC heterostructures. A large heat flux about 26 times of the blackbody radiation limit is obtained over a 150-nm vacuum gap, attributed to the couplings of three different surface modes (plasmon, phonon polaritons and frustrated mode). The interaction of polaritonic modes in the hybrid system is also explored to build a switchable thermophotonic device with nearly unity heat flux tunability. This work paves the way for understanding mode-mediated near-field heat transfer and provides a platform for building thermophotonic or thermo-optoelectronic blocks for various applications.

physics.optics↗

Abnormally High Thermal Conductivity in Fivefold Twinned Diamond Nanowires

Fivefold twins (5FTs), discovered nearly 200 years ago, are a common multiply twinned structure that usually dramatically deteriorate the thermal transport properties of nanomaterials. Here, we report the anomalous thermal conductivity ($κ$) in a novel fivefold twinned diamond nanowires (5FT-DNWs). The $κ$ of 5FT-DNWs is effectively enhanced by the defects of 5FT boundaries, and non-monotonically changes with the cross-sectional area ($\textit{S}$). Above the critical $\textit{S}$ = 7.1 nm$^{2}$, 5FT-DNWs show a constant value of $κ$, whereas below it, there appears a sharp increase in $κ$ with decreasing $\textit{S}$. More importantly, 5FT-DNWs with minimal $\textit{S}$ show a superior $κ$ over the bulk diamond. By confirming the Normal-process-dominated scattering event, it is demonstrated that the phonon hydrodynamic behavior plays a determinative role in abnormally high $κ$ of 5FT-DNWs with small $\textit{S}$. The super-transported phonon hydrodynamic phenomenon unveiled in the twinned diamond nanowires may provide a new route for pursuing highly thermally conductive nanomaterials.

physics.comp-ph↗

Controlled synthesis of MoxW1-xTe2 atomic layers with emergent quantum states

Recently, new states of matter like superconducting or topological quantum states were found in transition metal dichalcogenides (TMDs) and manifested themselves in a series of exotic physical behaviors. Such phenomena have been demonstrated to exist in a series of transition metal tellurides including MoTe2, WTe2 and alloyed MoxW1-xTe2. However, the behaviors in the alloy system have been rarely addressed due to their difficulty in obtaining atomic layers with controlled composition, albeit the alloy offers a great platform to tune the quantum states. Here, we report a facile CVD method to synthesize the MoxW1-xTe2 with controllable thickness and chemical composition ratios. The atomic structure of monolayer MoxW1-xTe2 alloy was experimentally confirmed by scanning transmission electron microscopy (STEM). Importantly, two different transport behaviors including superconducting and Weyl semimetal (WSM) states were observed in Mo-rich Mo0.8W0.2Te2 and W-rich Mo0.2W0.8Te2 samples respectively. Our results show that the electrical properties of MoxW1-xTe2 can be tuned by controlling the chemical composition, demonstrating our controllable CVD growth method is an efficient strategy to manipulate the physical properties of TMDCs. Meanwhile, it provides a perspective on further comprehension and shed light on the design of device with topological multicomponent TMDCs materials.

cond-mat.mtrl-sci↗

Room-temperature high detectivity mid-infrared photodetectors based on black arsenic phosphorus

The mid-infrared (MIR) spectral range, pertaining to important applications such as molecular 'fingerprint' imaging, remote sensing, free space telecommunication and optical radar, is of particular scientific interest and technological importance. However, state-of-the-art materials for MIR detection are limited by intrinsic noise and inconvenient fabrication processes, resulting in high cost photodetectors requiring cryogenic operation. We report black arsenic-phosphorus-based long wavelength infrared photodetectors with room temperature operation up to 8.2 um, entering the second MIR atmospheric transmission window. Combined with a van der Waals heterojunction, room temperature specific detectivity higher than 4.9*10^9 Jones was obtained in the 3-5 um range. The photodetector works in a zero-bias photovoltaic mode, enabling fast photoresponse and low dark noise. Our van der Waals heterojunction photodector not only exemplify black arsenic-phosphorus as a promising candidate for MIR opto-electronic applications, but also pave the way for a general strategy to suppress 1/f noise in photonic devices.

cond-mat.mtrl-sci↗