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Jianfeng Guo

Publications and source records attributed to Jianfeng Guo.

24 records · Page 2Linked to original sources

Controllable CVD-Growth of 2D Cr5Te8 Nanosheets with Thickness-Dependent Magnetic Domains

As a typical 2D magnetic material with self-intercalated structure, Cr5Te8 exhibits many fascinating magnetic properties. Although the ferromagnetism of 2D Cr5Te8 has been reported, the study of its magnetic domain is still blank. Herein, we successfully fabricated 2D Cr5Te8 nanosheets with controlled thickness and lateral size by chemical vapor deposition (CVD). Then magnetic property measurement system suggested Cr5Te8 nanosheets possessing intense out-of-plane ferromagnetism with the Curie temperature of 179 K. Most importantly, we found magnetic bubbles and thickness-dependent maze-like magnetic domains by cryogenic magnetic force microscopy (MFM) for the first time. The domain width of the maze-like magnetic domains increases rapidly with decreasing sample thickness, while domain contrast decreases. This indicates dipolar interaction is the dominant role over exchange interaction and magnetic anisotropy. Our work not only paves a way for the controllable growth of 2D magnetic materials, but also suggests new directions for controlling magnetic phases and systematically adjusting domain properties.

cond-mat.mes-hall↗

Emergent Electronic Kagome Lattice in Correlated Charge-Density-Wave State of 1T-TaS$_2$

Quantum materials with tunable correlated and/or topological electronic states, such as the electronic Kagome lattice, provide an ideal platform to study the exotic quantum properties. However, the real-space investigations on the correlated electronic Kagome lattice have been rarely reported. Herein, we report on the electronic Kagome lattice emerging in the correlated charge-density-wave (CDW) state of 1T-TaS$_2$ at ~200 K via variable-temperature scanning tunneling microscopy (VT-STM). This emergent Kagome lattice can be considered a fractional electron-filling superstructure with reduced translational and rotational symmetries, confirmed by STM measurements and density functional theory simulations. The characteristic band structure and density of states of this electronic Kagome lattice are further explored based on theoretical calculations. Our results demonstrate a self-organized electronic Kagome lattice from the correlated CDW state via the effective tuning parameter of temperature and provide a platform to directly explore the interplay of correlated electrons and topological physics.

cond-mat.mtrl-sci↗

A Fast Convergent Ordered-Subsets Algorithm with Subiteration-Dependent Preconditioners for PET Image Reconstruction

We investigated the imaging performance of a fast convergent ordered-subsets algorithm with subiteration-dependent preconditioners (SDPs) for positron emission tomography (PET) image reconstruction. In particular, we considered the use of SDP with the block sequential regularized expectation maximization (BSREM) approach with the relative difference prior (RDP) regularizer due to its prior clinical adaptation by vendors. Because the RDP regularization promotes smoothness in the reconstructed image, the directions of the gradients in smooth areas more accurately point toward the objective function's minimizer than those in variable areas. Motivated by this observation, two SDPs have been designed to increase iteration step-sizes in the smooth areas and reduce iteration step-sizes in the variable areas relative to a conventional expectation maximization preconditioner. The momentum technique used for convergence acceleration can be viewed as a special case of SDP. We have proved the global convergence of SDP-BSREM algorithms by assuming certain characteristics of the preconditioner. By means of numerical experiments using both simulated and clinical PET data, we have shown that the SDP-BSREM algorithms substantially improve the convergence rate, as compared to conventional BSREM and a vendor's implementation as Q.Clear. Specifically, SDP-BSREM algorithms converge 35\%-50\% faster in reaching the same objective function value than conventional BSREM and commercial Q.Clear algorithms. Moreover, we showed in phantoms with hot, cold and background regions that the SDP-BSREM algorithms approached the values of a highly converged reference image faster than conventional BSREM and commercial Q.Clear algorithms.

math.NA↗

Coexisting Ferromagnetic-antiferromagnetic Phase and Manipulation in Magnetic Topological Insulator MnBi4Te7

Magnetic topological insulators (MTIs) have received a lot of attention due to the existence of various quantum phenomena such as quantum anomalous Hall effect (QAHE) and topological magnetoelectric effect, etc. The intrinsic superlattice-like layered MTIs, MnBi2Te4/(Bi2Te3)n, have been extensively investigated mainly through the transport measurements, while the direct investigation of their superlattice-sensitive magnetic behaviors is relatively rare. Here, we report a microscopic real-space investigation of magnetic phase behaviors in MnBi4Te7 using cryogenic magnetic force microscopy (MFM). The intrinsic robust A-type antiferromagnetic (AFM), and emerged surface spin-flop (SSF), canted AFM (CAFM), ferromagnetic (FM)+CAFM, forced FM phases are sequentially visualized via the increased external magnetic field, in agreement with the metamagnetic behavior in the M-H curve. The temperature-dependent magnetic phase evolution behaviors are further investigated to obtain the complete H-T phase diagram of MnBi4Te7. The tentative local phase manipulation via the stray field of the magnetic tip is demonstrated by transforming the AFM to FM phase in its surface layers of MnBi4Te7. Our study the not only provide key real-space ingredients for understanding their complicated magnetic, electronic, and topological properties of these intrinsic MTIs, but also suggest new directions for manipulating spin textures and locally controlling their exotic properties.

cond-mat.mtrl-sci↗

Epitaxial fabrication of AgTe monolayer on Ag(111) and the sequential growth of Te film

Transition-metal chalcogenides (TMCs) materials have attracted increasing interest both for fundamental research and industrial applications. Among all these materials, two-dimensional (2D) compounds with honeycomb-like structure possess exotic electronic structures. Here, we report a systematic study of TMC monolayer AgTe fabricated by direct depositing Te on the surface of Ag(111) and annealing. Few intrinsic defects are observed and studied by scanning tunneling microscopy, indicating that there are two kinds of AgTe domains and they can form gliding twin-boundary. Then, the monolayer AgTe can serve as the template for the following growth of Te film. Meanwhile, some Te atoms are observed in the form of chains on the top of the bottom Te film. Our findings in this work might provide insightful guide for the epitaxial growth of 2D materials for study of novel physical properties and for future quantum devices.

cond-mat.mtrl-sci↗

Toplayer-Dependent Crystallographic Orientation Imaging in the Bilayer Two-Dimensional Materials with Transverse Shear Microscopy

Nanocontact properties of two-dimensional (2D) materials are closely dependent on their unique nanomechanical systems, such as the number of atomic layers and the supporting substrate. Here, we report a direct observation of toplayer-dependent crystallographic orientation imaging of 2D materials with the transverse shear microscopy (TSM). Three typical nanomechanical systems, MoS2 on the amorphous SiO2/Si, graphene on the amorphous SiO2/Si, and MoS2 on the crystallized Al2O3, have been investigated in detail. This experimental observation reveals that puckering behaviour mainly occurs on the top layer of 2D materials, which is attributed to its direct contact adhesion with the AFM tip. Furthermore, the result of crystallographic orientation imaging of MoS2/SiO2/Si and MoS2/Al2O3 indicated that the underlying crystalline substrates almost do not contribute to the puckering effect of 2D materials. Our work directly revealed the top layer dependent puckering properties of 2D material, and demonstrate the general applications of TSM in the bilayer 2D systems.

cond-mat.mtrl-sci↗