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Jiang-Xiazi Lin

Publications and source records attributed to Jiang-Xiazi Lin.

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Transport-Noise Witnesses of Electronic Multipartite Entanglement

Entanglement among particles is a defining feature of strongly correlated quantum materials, distinguishing them from conventional metals and semiconductors. The ability to certify intrinsic entanglement among interacting electrons in solid-state materials is important not only for classifying quantum states of matter, but also for developing material-based quantum technologies. Here, we introduce a transport-based protocol for witnessing multipartite entangled electronic states, based on the equilibrium noise spectrum as an experimentally accessible observable. The appropriately integrated, symmetrized, and projected current noise obeys an upper bound that can be derived from microscopic model parameters and is invariant with respect to the choice of electronic basis. We benchmark this framework in several paradigmatic systems, including twisted bilayer graphene, twisted bilayer MoTe$_2$, and Hubbard models, certifying entanglement in the fractional Chern insulating state. The method extends recently developed scattering-based entanglement witnesses to ultralow-temperature materials, where conventional spectroscopic probes are inaccessible but candidate entangled states are expected to arise.

cond-mat.str-el

Observation of giant nonlinear Hall conductivity in Bernal bilayer graphene

In a system of two-dimensional electrons, a combination of broken symmetry, interactions, and nontrivial topology can conspire to give rise to a nonlinear transport regime, where electric current density scales as the square of electric field. This regime has become a venue for exciting discoveries such as the nonlinear Hall effect and diode-like nonreciprocal transport. However, interpretation of experimental data is challenging in the nonlinear regime as DC transport is described by a rank-3 conductivity tensor with 6 free parameters. Here, we resolve this challenge by analytically solving for the nonlinear potential distribution across the disk sample for an arbitrary linear and nonlinear conductivity tensors. This allows us to unambiguously extract all components of the nonlinear tensor from experimental measurement. Using this novel tool, we identify giant nonlinear Hall effect in Bernal bilayer graphene. Our methodology provides the first systematic framework for interpreting nonlinear transport and uncovers a new route towards understanding quasi-2D materials.

cond-mat.mes-hall

Angle-resolved transport nonreciprocity and spontaneous symmetry breaking in twisted trilayer graphene

The ability to identify and characterize spontaneous symmetry breaking is central to our understanding of 2D materials with strong correlation, such as the moiré flat bands in magic-angle twisted graphene bilayer and trilayer. In this work, we utilize angle-resolved measurements of transport nonreciprocity to investigate spontaneous symmetry breaking in twisted trilayer graphene. By analyzing the angular dependence of nonreciprocity in both longitudinal and transverse channels, we are able to identify the symmetry axis associated with the underlying electronic order. We report that a hysteretic rotation in the mirror axis can be induced by thermal cycles and a large current bias, which offers unambiguous evidence for the spontaneous breaking of rotational symmetry. Moreover, the onset of nonreciprocity with decreasing temperature coincides with the emergence of orbital ferromagnetism. Combined with the angular dependence of the superconducting diode effect, our findings uncover a direct link between rotational and time-reversal symmetry breaking. These symmetry requirements point towards the exchange-driven instabilities in the momentum space as a possible origin for transport nonreciprocity in tTLG.

cond-mat.mes-hall

Spontaneous momentum polarization and diodicity in Bernal bilayer graphene

The low-temperature phase diagram of multilayer graphene heterostructures is largely defined by the exchange-driven instability that lifts the four-fold isospin degeneracy. Such instability gives rise to the quarter- and half-metal phases, which are key to our understanding of other emergent phenomena. Recent theoretical works shed light on a new type of Coulomb-driven instability. It is proposed that the exchange interaction between trigonal-warping-induced Fermi pockets could induce charge carriers to condense into one of the Fermi pockets, giving rise to a net polarization in the momentum space. Here, we report the observation of spontaneous momentum polarization in Bernal bilayer graphene using angle-resolved nonlinear transport measurement at the second-harmonic frequency. With excellent angular precision, we show that the polar axis of the momentum polarization is tunable with varying carrier density, electric field, and magnetic field. The dominating influence of the momentum-space instability reveals a natural connection between broken symmetries, and the isospin degeneracy lifting in the half- and quarter-metal phases.

cond-mat.mes-hall

Electron spin resonance and collective excitations in magic-angle twisted bilayer graphene

In a strongly correlated system, collective excitations contain key information regarding the electronic order of the underlying ground state. An abundance of collective modes in the spin and valley isospin channels of magic-angle graphene moiré bands has been alluded to by a series of recent experiments. However, direct observation of collective excitations has remained elusive due to the lack of a spin probe. In this work, we use a resistively-detected electron spin resonance technique to look for low-energy collective excitations in magic-angle twisted bilayer graphene. We report direct observation of collective modes in the form of microwave-induced resonance near half filling of the moiré flatbands. The frequency-magnetic field dependence of these resonance modes sheds light onto the nature of intervalley spin coupling, allowing us to extract parameters such as intervalley exchange interaction and spin stiffness. Two independent observations testify that the generation and detection of the microwave resonance relies on the strong correlation within the flat moiré energy band. First, the onset of robust resonance response coincides with the spontaneous flavor polarization at half moiré filling, and remains absent in the density range where the underlying Fermi surface is isospin unpolarized. Second, we performed the same resonance measurement on graphene monolayer and bilayer samples, including twisted bilayer with a large twist angle, where flatband physics is absent. We observe no indication of resonance response in these samples across a large range of carrier density, microwave frequency and power. A natural explanation is that the resonance response near the magic angle originates from "Dirac revivals" and the resulting isospin order.

cond-mat.mes-hall

A new flavor of correlation and superconductivity in small twist-angle trilayer graphene

When layers of graphene are rotationally misaligned by the magic angle, the moiré superlattice features extremely flat bands. Due to the enhanced density of states, the Coulomb interaction induces a variety of instabilities. The most prominent occur at integer filling and are therefore commonly attributed to spontaneous polarization of the moiré unit cell's `flavor' degrees of freedom -- spin, valley, and the flat-band degeneracy. As the dominant member of the hierarchy, these correlated states are thought to crucially determine further instabilities at lower energy scales, such as superconductivity and weaker incompressible states at fractional filling. In this work, we examine the behavior of twisted trilayer graphene in a window of twist angle around $1.3^{\circ}$, well below the expected magic angle of $1.55^{\circ}$. In this small twist angle regime, we find surprisingly narrow bands, which are populated with both an abundance of correlation-driven states at fractional filling as well as robust superconductivity. The absence of linear-in-$T$ resistivity without significant reduction of the superconducting transition temperature, provides insights into the origin of both phenomena. Most remarkably, the hierarchy between integer and fractional filling is absent, indicating that flavor polarization does not play a governing role. The prominence of fractional filling in the small twist angle regime also points towards a longer-range effective Coulomb interaction. Combined, our results shed new light on outstanding questions in the field, while establishing the small twist angle regime as a new paradigm for exploring novel flavors of moiré physics.

cond-mat.mes-hall

Zero-field superconducting diode effect in small-twist-angle trilayer graphene

The critical current of a superconductor can be different for opposite directions of current flow when both time-reversal and inversion symmetry are broken. %When time-reversal and inversion symmetry are simultaneously broken, the critical current of a 2D superconductor is expected to depend on the directions of current flow. Such nonreciprocal behavior in superconducting transport, which creates a superconducting diode, has recently been demonstrated experimentally by breaking these symmetries with an applied magnetic field \cite{Ando2020diodes} or by construction of a magnetic tunnel junction \cite{Diez2021magnetic}. Here we report an intrinsic superconducting diode effect which is present at zero external magnetic field in mirror symmetric twisted trilayer graphene (tTLG). Such nonreciprocal behavior, with sign that can be reversed through training with an out-of-plane magnetic field, provides direct evidence of the microscopic coexistence between superconductivity and time-reversal symmetry breaking. In addition to the magnetic-field trainability, we show that the zero-field diode effect can be controlled by varying carrier density or twist angle. In accordance with these experimental controls, a natural interpretation for the origin of the intrinsic diode effect is an imbalance in valley occupation of the underlying Fermi surface, which likely leads to finite-momentum Cooper pairing and nematicity in the superconducting phase.

cond-mat.mes-hall

Spin-orbit driven ferromagnetism at half moiré filling in magic-angle twisted bilayer graphene

Strong electron correlation and spin-orbit coupling (SOC) provide two non-trivial threads to condensed matter physics. When these two strands of physics come together, a plethora of quantum phenomena with novel topological order have been predicted to emerge in the correlated SOC regime. In this work, we examine the combined influence of electron correlation and SOC on a 2-dimensional (2D) electronic system at the atomic interface between magic-angle twisted bilayer graphene (tBLG) and a tungsten diselenide (\WSe) crystal. In such a structure, strong electron correlation within the moiré flatband stabilizes correlated insulating states at both quarter and half-filling, whereas SOC transforms these Mott-like insulators into ferromagnets, evidenced by robust anomalous Hall effect with hysteretic switching behavior. The coupling between spin and valley degrees of freedom is unambiguously demonstrated as the magnetic order is shown to be tunable with an in-plane magnetic field, or a perpendicular electric field. In addition, we examine the influence of SOC on the isospin order and stability of superconductivity. Our findings establish an efficient experimental knob to engineer topological properties of moiré bands in twisted bilayer graphene and related systems.

cond-mat.mes-hall