arXiv subjects

Jiangfeng Du

Publications and source records attributed to Jiangfeng Du.

At least 127 records · Page 7Linked to original sources

arXiv2020

Nanoscale zero-field electron spin resonance spectroscopy

Electron spin resonance (ESR) spectroscopy has broad applications in physics, chemistry and biology. As a complementary tool, zero-field ESR (ZF-ESR) spectroscopy has been proposed for decades and shown its own benefits for investigating the electron fine and hyperfine interaction. However, the ZF-ESR method has been rarely used due to the low sensitivity and the requirement of much larger samples than conventional ESR. In this work, we present a method for deploying ZF-ESR spectroscopy at the nanoscale by using a highly sensitive quantum sensor, the nitrogen-vacancy center in diamond. We also measure the nanoscale ZF-ESR spectrum of a few P1 centers in diamond, and show that the hyperfine coupling constant can be directly extracted from the spectrum. This method opens the door to practical applications of ZF-ESR spectroscopy, such as investigation of the structure and polarity information in spin-modified organic and biological systems.

quant-ph↗

arXiv2020

Single DNA Electron Spin Resonance Spectroscopy in Aqueous Solutions

Magnetic resonance spectroscopy of single biomolecules under near-physiological conditions may substantially advance understanding of biological function, yet remains very challenging. Here we use nitrogen-vacancy centers in diamonds to detect electron spin resonance spectra of individual, tethered DNA duplexes labeled with a nitroxide spin label in aqueous buffer solutions at ambient temperatures. This paves the way for magnetic resonance studies on single biomolecules and their inter-molecular interactions in a native-like environment.

physics.bio-ph↗

arXiv2020

Dynamically encircling an exceptional point in a real quantum system

The exceptional point, known as the non-Hermitian degeneracy, has special topological structure, leading to various counterintuitive phenomena and novel applications, which are refreshing our cognition of quantum physics. One particularly intriguing behavior is the mode switch phenomenon induced by dynamically encircling an exceptional point in the parameter space. While these mode switches have been explored in classical systems, the experimental investigation in the quantum regime remains elusive due to the difficulty of constructing time-dependent non-Hermitian Hamiltonians in a real quantum system. Here we experimentally demonstrate dynamically encircling the exceptional point with a single nitrogen-vacancy center in diamond. The time-dependent non-Hermitian Hamiltonians are realized utilizing a dilation method. Both the asymmetric and symmetric mode switches have been observed. Our work reveals the topological structure of the exceptional point and paves the way to comprehensively explore the exotic properties of non-Hermitian Hamiltonians in the quantum regime.

quant-ph↗

arXiv2020

Experimental sensing quantum atmosphere of a single spin

Understanding symmetry-breaking states of materials is a major challenge in the modern physical sciences. Quantum atmosphere proposed recently sheds light on the hidden world of these symmetry broken patterns. But the requirements for exquisite sensitivity to the small shift and tremendous spatial resolution to local information pose huge obstacles to its experimental manifestation. In our experiment, we prepare time-reversal-symmetry conserved and broken quantum atmosphere of a single nuclear spin and successfully observe their symmetry properties. Our work proves in principle that finding symmetry patterns from quantum atmosphere is conceptually viable. It also opens up entirely new possibilities in the potential application of quantum sensing in material diagnosis.

quant-ph↗

arXiv2019

Pulse-width-induced polarization enhancement of optically-pumped N-V electron spin in diamond

The nitrogen-vacancy (N-V) center in diamond is a widely-used platform for quantum information processing and metrology. The electron-spin state of N-V center could be initialized and readout optically, and manipulated by resonate microwave fields. In this work, we analyze the dependence of electron-spin initialization on widths of laser pulses. We build a numerical model to simulate this process and verify the simulation results in experiment. Both simulations and experiments reveal a fact that shorter laser pulses are helpful to the electron-spin polarization. We therefore propose to use extremely-short laser pulses for electron-spin initialization. In this new scheme, the spin-state contrast could be improved about 10% in experiment by using laser pulses as short as 4 ns in width. Furthermore, we provide a mechanism to explain this effect which is due to the occupation time in the meta-stable spin-singlet states of N-V center. Our new scheme is applicable in a broad range of NV-based applications in the future.

quant-ph↗

arXiv2019

Room temperature test of the Continuous Spontaneous Localization model using a levitated micro-oscillator

The Continuous Spontaneous Localization (CSL) model predicts a tiny break of energy conservation via a weak stochastic force acting on physical systems, which triggers the collapse of the wave function. Mechanical oscillators are a natural way to test such a force; in particular levitated micro-mechanical oscillator has been recently proposed to be an ideal system. We report a proof-of-principle experiment with a micro-oscillator generated by a micro-sphere diamagnetically levitated in a magneto-gravitational trap under high vacuum. Due to the ultra-low mechanical dissipation, the oscillator provides a new upper bound on the CSL collapse rate, which gives an improvement of two orders of magnitude over the previous bounds in the same frequency range, and partially reaches the enhanced collapse rate suggested by Adler. Although being performed at room temperature, our experiment has already exhibits advantages over those operating at low temperatures previously reported. Our results experimentally show the potential of magneto-gravitational levitated mechanical oscillator as a promising method for testing collapse model. Further improvements in cryogenic experiments are discussed.

quant-ph↗

arXiv2019

Manipulation of a Micro-object Using Topological Hydrodynamic Tweezers

Manipulating micro-scale object plays paramount roles in a wide range of fundamental researches and applications. At micro-scale, various methods have been developed in the past decades, including optical, electric, magnetic, aerodynamic and acoustic methods. However, these non-contact forces are susceptible to external disturbance, and so finding a way to make micro-scale object manipulation immune to external perturbations is challenging and remains elusive. Here we demonstrate a method based on new trapping mechanism to manipulate micro-scale object in a gas flow at ambient conditions. We first show that the micro-droplet is entrapped into a trapping ring constructed by a particular toroidal vortex. The vortex works as tweezers to control the position of the micro-droplet. We then show that the micro-droplet can be transported along the trapping ring. By virtue of the topological character of the gas flow, the transport path is able to bypass external strong perturbations automatically. We further demonstrate a topological transfer process of the micro-droplet between two hydrodynamic tweezers. Our method provides an integrated toolbox to manipulate a micro-scale object, with an intrinsic mechanism that protects the target object from external disturbances.

physics.flu-dyn↗

arXiv2019

Observation of anti-PT symmetry phase transition in the magnon-cavity-magnon coupled system

As the counterpart of PT symmetry, abundant phenomena and potential applications of anti-PT symmetry have been predicted or demonstrated theoretically. However, experimental realization of the coupling required in the anti-PT symmetry is difficult. Here, by coupling two YIG spheres to a microwave cavity, the large cavity dissipation rate makes the magnons coupled dissipatively with each other, thereby obeying a two-dimensional anti-PT Hamiltonian. In terms of the magnon-readout method, a new method adopted here, we demonstrate the validity of our method in constructing an anti-PT system and present the counterintuitive level attraction process. Our work provides a new platform to explore the anti-PT symmetry properties and paves the way to study multi-magnoncavity-polariton systems.

quant-ph↗

arXiv2019

Observation of dynamical phase transitions in a topological nanomechanical system

Dynamical phase transitions (DPTs), characterized by non-analytic behaviors in time domain, extend the equilibrium phase transitions to far-from-equilibrium situations. It has been predicted that DPTs can be precisely identified by the discontinuities of the Pancharatnam geometric phase (PGP) during the time evolution. However, PGP always mixes with dynamical phase and the experimental observation of DPTs by PGP is still absent. Here, we theoretically present a novel scheme for eliminating the dynamical phase by taking advantage of chiral symmetry in the Su-Schrieffer-Heeger (SSH) model, and experimentally observe DPTs by directly measuring PGP in a quenched topological nanomechanical lattice. Time-dependent topological structures of the SSH model are configured by eight strong-coupled high-quality-factor nanomechanical oscillators. By measuring the vibration phase and the normalized amplitude of the edge oscillator, we show a direct classical analog of DPTs. Furthermore, we experimentally demonstrate the robustness of DPTs against weak structure disorders, and numerically explore the relation between DPTs and the equilibrium phase boundary. This work not only establishes the quantitative method to identify DPTs, but also opens the door for studying non-equilibrium topological dynamics with a well-controlled nanomechanical system.

quant-ph↗

arXiv2019

Experimental dissipative quantum sensing

Quantum sensing utilizes quantum systems as sensors to capture weak signal, and provides new opportunities in nowadays science and technology. The strongest adversary in quantum sensing is decoherence due to the coupling between the sensor and the environment. The dissipation will destroy the quantum coherence and reduce the performance of quantum sensing. Here we show that quantum sensing can be realized by engineering the steady-state of the quantum sensor under dissipation. We demonstrate this protocol with a magnetometer based on ensemble Nitrogen-Vacancy centers in diamond, while neither high-quality initialization/readout of the sensor nor sophisticated dynamical decoupling sequences is required. Thus our method provides a concise and decoherence-resistant fashion of quantum sensing. The frequency resolution and precision of our magnetometer are far beyond the coherence time of the sensor. Furthermore, we show that the dissipation can be engineered to improve the performance of our quantum sensing. By increasing the laser pumping, magnetic signal in a broad audio-frequency band from DC up to 140 kHz can be tackled by our method. Besides the potential application in magnetic sensing and imaging within microscopic scale, our results may provide new insight for improvement of a variety of high-precision spectroscopies based on other quantum sensors.

quant-ph↗

arXiv2019

Dynamically Polarizing Spin Register of NV Centers in Diamond using Chopped Laser Pulses

Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose and demonstrate a magnetic-field-independent, deterministic and highly efficient polarization scheme by introducing chopped laser pulses into the double-resonance initialization method. With this method, we demonstrate initialization of single-nuclear-spin approaching $98.1\%$ and a $^{14}N$-$^{13}C$ double-nuclear-spin system approaching $96.8\%$ at room temperature. The initialization is limited by a nuclear-spin depolarization effect due to chopped laser excitation. Our approach could be extended to NV systems with more nuclear spins and would be a useful tool in future applications such as nano-MRI and single-cell NMR.

quant-ph↗

arXiv2019

Breaking the quantum adiabatic speed limit by jumping along geodesics

Quantum adiabatic evolutions find a broad range of applications in quantum physics and quantum technologies. The traditional form of the quantum adiabatic theorem limits the speed of adiabatic evolution by the minimum energy gaps of the system Hamiltonian. Here, we experimentally show using a nitrogen-vacancy center in diamond that, even in the presence of vanishing energy gaps, quantum adiabatic evolution is possible. This verifies a recently derived necessary and sufficient quantum adiabatic theorem and offers paths to overcome the conventionally assumed constraints on adiabatic methods. By fast modulation of dynamic phases, we demonstrate near-unit-fidelity quantum adiabatic processes in finite times. These results challenge traditional views and provide deeper understanding on quantum adiabatic processes, as well as promising strategies for the control of quantum systems.

quant-ph↗

arXiv2019

Structural analysis of nuclear spin clusters via two-dimensional nanoscale nuclear magnetic resonance spectroscopy

Two-dimensional Nuclear Magnetic Resonance (NMR) is essential in molecular structure determination. The Nitrogen-Vacancy (NV) center in diamond has been proposed and developed as an outstanding quantum sensor to realize NMR in nanoscale. In this work, we develop a scheme for two-dimensional nanoscale NMR spectroscopy based on quantum controls on an NV center. We carry out a proof of principle experiment on a target of two coupled $^{13}$C nuclear spins in diamond. A COSY-like sequences is used to acquire the data on time domain, which is then converted to frequency domain with the fast Fourier transform (FFT). With the two-dimensional NMR spectrum, the structure and location of the set of nuclear spin are resolved. This work marks a fundamental step towards resolving the structure of a single molecule.

quant-ph↗

arXiv2019

Searching for an Exotic Spin-Dependent Interaction between Electrons at the Nanometer Scale with Molecular Rulers

We propose that a type of molecular rulers, which contains two electron spins with precisely adjustable distance by varying the length of the shape-persistent polymer chains, can be utilized to constrain the axial-vector mediated interaction between electron spins at the nanometer scale. With measurements of the coupling strengths between two electron spins within different molecular rulers, an improved laboratory bound of exotic dipole-dipole interaction between electrons is established within the force range from 3 to 220 nm. The upper bound of the coupling $g_A^e g_A^e/4π\hbar c $ at 200 nm is $|g_A^e g_A^e/4π\hbar c| \leq 4.9\times10^{-13}$, which is about 20 times more stringent than previous limits.

physics.atom-ph↗

arXiv2019

Experimental observation of dynamical bulk-surface correspondence for topological phases

We experimentally demonstrate a dynamical classification approach for investigation of topological quantum phases using a solid-state spin system through nitrogen-vacancy (NV) center in diamond. Similar to the bulkboundary correspondence in real space at equilibrium, we observe a dynamical bulk-surface correspondence in the momentum space from a dynamical quench process. An emergent dynamical topological invariant is precisely measured in experiment by imaging the dynamical spin-textures on the recently defined band-inversion surfaces, with high topological numbers being implemented. Importantly, the dynamical classification approach is shown to be independent of quench ways and robust to the decoherence effects, offering a novel and practical strategy for dynamical topology characterization, especially for high dimensional gapped topological phases.

cond-mat.mes-hall↗

arXiv2019

Quantum Simulation of Resonant Transitions for Solving the Eigen-problem of an Effective Water Hamiltonian

It is difficult to calculate the energy levels and eigenstates of a large physical system on a classical computer because of the exponentially growing size of the Hilbert space. In this work, we experimentally demonstrate a quantum algorithm which could solve this problem via simulated resonant transitions. Using a four-qubit quantum simulator in which two qubits are used as ancillas for control and measurement, we obtain the energy spectrum of a 2-qubit low-energy effective Hamiltonian of the water molecule. The simulated transitions allow the state of the quantum simulator to transform and access large regions of the Hilbert space, including states that have no overlap with the initial state. Furthermore, we make use of this algorithm to efficiently prepare specific eigenstates on the simulator according to the measured eigenenergies.

quant-ph↗

arXiv2019

Floquet dynamical quantum phase transitions

Dynamical quantum phase transitions (DQPTs) are manifested by time-domain nonanalytic behaviors of many-body systems.Introducing a quench is so far understood as a typical scenario to induce DQPTs.In this work, we discover a novel type of DQPTs, termed "Floquet DQPTs", as intrinsic features of systems with periodic time modulation.Floquet DQPTs occur within each period of continuous driving, without the need for any quenches.In particular, in a harmonically driven spin chain model, we find analytically the existence of Floquet DQPTs in and only in a parameter regime hosting a certain nontrivial Floquet topological phase. The Floquet DQPTs are further characterized by a dynamical topological invariant defined as the winding number of the Pancharatnam geometric phase versus quasimomentum.These findings are experimentally demonstrated with a single spin in diamond.This work thus opens a door for future studies of DQPTs in connection with topological matter.

quant-ph↗

arXiv2018

Observation of parity-time symmetry breaking in a single spin system

A fundamental axiom of quantum mechanics requires the Hamiltonians to be Hermitian which guarantees real eigen-energies and probability conservation. However, a class of non-Hermitian Hamiltonians with Parity-Time ($\mathcal{PT}$) symmetry can still display entirely real spectra. The Hermiticity requirement may be replaced by $\mathcal{PT}$ symmetry to develop an alternative formulation of quantum mechanics. A series of experiments have been carried out with classical systems including optics, electronics, microwaves, mechanics and acoustics. However, there are few experiments to investigate $\mathcal{PT}$ symmetric physics in quantum systems.Here we report the first observation of the $\mathcal{PT}$ symmetry breaking in a single spin system. We have developed a novel method to dilate a general $\mathcal{PT}$ symmetric Hamiltonian into a Hermitian one, which can be realized in a practical quantum system.Then the state evolutions under $\mathcal{PT}$ symmetric Hamiltonians, which range from $\mathcal{PT}$ symmetric unbroken to broken regions, have been experimentally observed with a single nitrogen-vacancy (NV) center in diamond. Due to the universality of the dilation method, our result opens a door for further exploiting and understanding the physical properties of $\mathcal{PT}$ symmetric Hamiltonian in quantum systems.

quant-ph↗