arXiv subjects

Jianming Zhao

Publications and source records attributed to Jianming Zhao.

At least 37 records · Page 2Linked to original sources

arXiv2023

Microwave spectroscopy and Zeeman effect of cesium $(n+2)D_{5/2}\rightarrow nF_{J}$ Rydberg transitions

We report on high-resolution microwave spectroscopy of cesium Rydberg $(n+2)D_{5/2}\rightarrow nF_{J}$ transitions in a cold atomic gas. Atoms laser-cooled and trapped in a magnetic-optical trap are prepared in the $D$ Rydberg state using a two-photon laser excitation scheme. A microwave field transmitted into the chamber with a microwave horn drives the Rydberg transitions, which are probed via state selective field ionization. Varying duration and power of the microwave pulse, we observe Fourier side-band spectra as well as damped, on-resonant Rabi oscillations with pulse areas up to $\gtrsim 3 π$. Furthermore, we investigate the Zeeman effect of the clearly resolved $nF_J$ fine-structure levels in fields up to 120~mG, where the transition into $nF_{7/2}$ displays a thee-peak Zeeman pattern, while $nF_{5/2}$ shows a two-peak pattern. Our theoretical models explain all observed spectral characteristics, showing good agreement with the experiment. Our measurements provide a pathway for the study of high-angular-momentum Rydberg states, initialization and coherent manipulation of such states, Rydberg-atom macrodimers, and other Rydberg-atom interactions. Furthermore, the presented methods are suitable for calibration of microwave radiation as well as for nulling and calibration of DC magnetic fields in experimental chambers for cold atoms.

physics.atom-ph↗

arXiv2023

Quantum defects of $n$F$_J$ levels of Cs Rydberg atoms

We present precise measurements of the quantum defects of cesium $n$F$_J$ Rydberg levels. We employ high-precision microwave spectroscopy of $(n+2)\mathrm{D}_{5/2}\rightarrow n\mathrm{F}_{5/2,7/2}$ transitions for $n=45$ to 50 in a cold-atom setup. Cold cesium $(n+2)$D$_{5/2}$ atoms, prepared via two-photon laser excitation, are probed by scanning weak microwave fields interacting with the atoms across the $n\mathrm{F}_{5/2,7/2}$ resonances. Transition spectra are acquired using state-selective electric-field ionization and time-gated ion detection. Transition-frequency intervals are obtained by Lorentzian fits to the measured spectral lines, which have linewidths ranging between 70~kHz and 190~kHz, corresponding to about one to three times the Fourier limit. A comprehensive analysis of relevant line-shift uncertainties and line-broadening effects is conducted. We find quantum defect parameters $δ_{0}(\mathrm{F}_{5/2})=0.03341537(70)$ and $δ_{2}(\mathrm{F}_{5/2})=-0.2014(16)$, as well as $δ_{0}(\mathrm{F}_{7/2})=0.0335646(13)$ and $δ_{2}(\mathrm{F}_{7/2})=-0.2052(29)$, for $J=5/2$ and $J=7/2$, respectively. Fine structure parameters $A_{FS}$ and $B_{FS}$ for Cs $n{\rm{F}}_J$ are also obtained. Results are discussed in context with previous works, and the significance of the results is discussed.

physics.atom-ph↗

arXiv2023

Dephasing of ultracold cesium $80D_{5/2}$-Rydberg Electromagnetically Induced Transparency

We study Rydberg electromagnetically induced transparency (EIT) of a cascade three-level atom involving 80$D_{5/2}$ state in a strong interaction regime employing a cesium ultracold cloud. In our experiment, a strong coupling laser couples 6$P_{3/2}$ to 80$D_{5/2}$ transition, while a weak probe, driving 6$S_{1/2}$ to 6$P_{3/2}$ transition, probes the coupling induced EIT signal. At the two-photon resonance, we observe that the EIT transmission decreases slowly with time, which is a signature of interaction induced metastability. The dephasing rate $γ_{\rm OD}$ is extracted with optical depth OD = $γ_{\rm OD}t$. We find that the optical depth linearly increases with time at onset for a fixed probe incident photon number $R_{\rm in}$ before saturation. The dephasing rate shows a nonlinear dependence on $R_{\rm in}$. The dephasing mechanism is mainly attributed to the strong dipole-dipole interactions, which leads to state transfer from $nD_{5/2}$ to other Rydberg states. We demonstrate that the typical transfer time $τ_{0(80D)}$ obtained by the state selective field ionization technique is comparable with the decay time of EIT transmission $τ_{0({\rm EIT})}$. The presented experiment provides a useful tool for investigating the strong nonlinear optical effects and metastable state in Rydberg many-body systems.

physics.atom-ph↗

arXiv2023

Superradiance-induced multistability in driven Rydberg lattice gases

We study steady state phases of a one-dimensional array of Rydberg atoms coupled by a microwave (MW) field where the higher energy Rydberg state decays to the lower energy one via single-body and collective (superradiant) decay. Using mean-field approaches, we examine the interplay among the MW coupling, intra-state van der Waals (vdW) interaction, and single-body and collective dissipation between Rydberg states. A linear stability analysis reveals that a series of phases, including uniform, antiferromagnetic, oscillatory, and bistable and multistable phases can be obtained. Without the vdW interaction, only uniform phases are found. In the presence of the vdW interaction, multistable solutions are enhanced when increasing the strength of the superradiant decay rate. Our numerical simulations show that the bistable and multistable phases are stabilized by superradiance in a long chain. The critical point between the uniform and multistable phases and its scaling with the atom number is obtained. Through numerically solving the master equation of a finite chain, we show that the mean-field multistable phase could be characterized by expectation values of Rydberg populations and two-body correlations between Rydberg atoms in different sites.

quant-ph↗

arXiv2022

Continuous-frequency weak electric field measurement with Rydberg atoms

We demonstrate a continuous frequency electric field measurement based on the far off-resonant AC stark effect in a Rydberg atomic vapor cell. In this configuration, a strong far off-resonant field, denoted as a local oscillator (LO) field, acts as a gain shifting the Rydberg level to a high sensitivity region. An incident weak signal field with a few hundreds of kHz difference from the LO field is mixed with the LO field in Rydberg system to generate an intermediate frequency (IF) signal, which is read out by the Rydberg electromagnetically induced transparency (Rydberg-EIT) spectroscopy. Not like resonant EIT-AT spectra, we realize the electric field measurement of the signal frequency from 2 GHz to 5 GHz using a single Rydberg state. A minimum detectable filed strength is down to 2.31~$μ$V/cm and a linear dynamic range is over 65~dB. The minimum detectable filed is comparable with a resonant microwave-dressed Rydberg heterodyne receiver using the same system, which is 1.45~$μ$V/cm. We also show the system has an inherent polarization selectivity feature. Our method can provide a high sensitivity of electric field measurement and be extended to arbitrary frequency measurements.

physics.atom-ph↗

arXiv2021

Experimental Observation of Partial Parity-Time Symmetry and Its Phase Transition with a Laser-Driven Cesium Atomic Gas

Realization and manipulation of parity-time (PT) symmetry in multidimensional systems are highly desirable for exploring nontrivial physics and uncovering exotic phenomena in non-Hermitian systems. Here, we report the first experimental observation of partial PT (pPT) symmetry in a cesium atomic gas coupled with laser fields, where a two-dimensional pPT-symmetric optical potential for probe laser beam is created. A transition of the pPT symmetry from an unbroken phase to a broken one is observed through changing the beam-waist ratio of the control and probe laser beams, and the domains of unbroken, broken, and non-pPT phases are also discriminated unambiguously. Moreover, we develop a technique to precisely determine the location of the exceptional point of the pPT symmetry breaking by measuring the asymmetry degree of the probe-beam intensity distribution. The findings reported here pave the way for controlling multidimensional laser beams in non-Hermitian systems via laser-induced atomic coherence, and have potential applications for designing new types of light amplifiers and attenuators

physics.optics↗

arXiv2021

Observation of Blackbody Radiation Enhanced Superradiance in ultracold Rydberg Gases

An ensemble of excited atoms can synchronize emission of light collectively in a process known as superradiance when its characteristic size is smaller than the wavelength of emitted photons. The underlying superradiance depends strongly on electromagnetic (photon) fields surrounding the atomic ensemble. High mode densities of microwave photons from $300\,$K blackbody radiation (BBR) significantly enhance decay rates of Rydberg states to neighbouring states, enabling superradiance that is not possible with bare vacuum induced spontaneous decay. Here we report observations of the superradiance of ultracold Rydberg atoms embedded in a bath of room-temperature photons. The temporal evolution of the Rydberg $|nD\rangle$ to $|(n+1)P\rangle$ superradiant decay of Cs atoms ($n$ the principal quantum number) is measured directly in free space. Theoretical simulations confirm the BBR enhanced superradiance in large Rydberg ensembles. We demonstrate that the van der Waals interactions between Rydberg atoms change the superradiant dynamics and modify the scaling of the superradiance. In the presence of static electric fields, we find that the superradiance becomes slow, potentially due to many-body interaction induced dephasing. Our study provides insights into many-body dynamics of interacting atoms coupled to thermal BBR, and might open a route to the design of blackbody thermometry at microwave frequencies via collective, dissipative photon-atom interactions.

physics.atom-ph↗

arXiv2020

Cesium $nD_{J}$+$6S_{1/2}$ Rydberg molecules and their permanent electric dipole moments

Cs$_2$ Rydberg-ground molecules consisting of a Rydberg, $nD_{J}$ (33 $\leq$ $n$ $\leq$ 39), and a ground state atom, 6$S_{1/2} (F=$3 or 4$)$, are investigated by photo-association spectroscopy in a cold atomic gas. We observe vibrational spectra that correspond to triplet $^TΣ$ and mixed $^{S,T}Σ$ molecular states. We establish scaling laws for the energies of the lowest vibrational states vs principal quantum number and obtain zero-energy singlet and triplet $s$-wave scattering lengths from experimental data and a Fermi model. Line broadening in electric fields reveals the permanent molecular electric-dipole moments; measured values agree well with calculations. We discuss the negative polarity of the dipole moments, which differs from previously reported cases.

physics.atm-clus↗

arXiv2019

Observation of many-body dynamics of Rydberg atoms based on antiblockade using two-color excitation

We investigate a long-range interaction between $64D_{5/2}$ Rydberg-atom pairs and antiblockade effect employing a two-color excitation scheme. The first color (pulse A) is set to resonantly excite the Rydberg transition and prepare a few seed atoms, which establish a blockade region due to strong long-range interaction between Rydberg-atom pairs. The second color (pulse B) is blue detuned relative to Rydberg transition and enables further Rydberg excitation of atoms by counteracting the blockade effect. It is found that a few seed atoms lead to a huge difference of the Rydberg excitation with pulse B. The dynamic evolution of antiblockade excitation by varying the pulse-B duration at 30-MHz blue detuning is also investigated. The evolution result reveals that a small amount of seed atoms can trigger an avalanche Rydberg excitation. A modified superatom model is used to simulate the antiblockade effect and relevant dynamic evolution. The simulations are consistent with the experimental measurements.

physics.atom-ph↗

arXiv2018

Adiabatic potentials of cesium $(nD_J)_2$ Rydberg-Rydberg macrodimers

Electrostatic multipole interactions generate long-range Rydberg-Rydberg macrodimer. We calculate the adiabatic potentials of cesium $(nD_{J})_2$ Rydberg macrodimers for principal quantum numbers $n$ ranging from 56 to 62, for $J=3/2$ and $5/2$, and for the allowed values of the conserved sum of the atomic angular-momentum components along the internuclear axis, $M$. For most combinations $(n, M, J)$ exactly one binding potential exists, which should give rise to Rydberg macrodimer states. We study the dependence of the adiabatic potentials on the size of the two-body basis sets used in the calculation, and on the maximal order, $q_{max}$, of the multipole terms included in the calculation. We determine the binding energies and lengths of the binding adiabatic potentials, and investigate their scaling behaviors as a function of the effective principal quantum number; these parameters are relevant to experimental preparation of Rydberg-atom macrodimers. Avoided crossings between adiabatic potentials affect the well shapes and the scaling behaviors differently in two distinct domains in $n$. We discuss an experimental scheme for preparing $(nD_J)_2$ Rydberg-atom macrodimers using two-color double-resonant photoassociation.

physics.atom-ph↗

arXiv2018

Atom-based quantum receiver for amplitude- and frequency-modulated baseband signals in high-frequency radio communication

An optical probe of cesium Rydberg atoms generated in a thermal vapor cell is used to retrieve a baseband signal modulated onto a 16.98-GHz carrier wave in real-time, demonstrating an atom-based quantum receiver suitable for microwave communication. The 60$S_{1/2}$ Rydberg level of cesium atoms in the cell is tracked via electromagnetically induced transparency (EIT), an established laser-spectroscopic method. The microwave carrier is resonant with the 60$S_{1/2}$ $\rightarrow$ 60$P_{1/2}$ Rydberg transition, resulting in an Autler-Townes (AT) splitting of the EIT signal. Amplitude modulation of the carrier wave results in a corresponding modulation in the optically retrieved AT splitting. Frequency modulation causes a change in relative height of the two AT peaks, which can be optically detected and processed to retrieve the modulation signal. The optical retrieval of the baseband signal does not require electronic demodulation. The method is suitable for carrier frequencies within a range from $\sim 1$~GHz to hundreds of GHz. The baseband bandwidth, which is $\sim$~20~Hz in the present demonstration, can be increased by faster spectroscopic sampling.

quant-ph↗

arXiv2017

Cs nDJ Rydberg-atom macrodimers formed by long-range multipole interaction

Long-range macrodimers formed by D-state cesium Rydberg atoms are studied in experiments and in calculations. Cesium 62DJ-62DJ Rydberg-atom macrodimers, bonded via long-range multipole interaction, are prepared by two-color photo-association in a cesium atom trap. The first color (pulse A) resonantly excites seed Rydberg atoms, while the second (pulse B, detuned by the molecular binding energy) resonantly excites the Rydberg-atom macrodimer states below the 62DJ pair asymptotes. The Rydberg-atom molecules are measured by extraction of auto-ionization products and Rydberg-atom electric-field ionization, and ion detection. Molecular spectra are compared with calculations of adiabatic molecular potentials. The lifetime of the molecules is obtained from exponential fits to the dependence of the molecular signal on the detection delay time; lifetimes of about 6 us are found.

physics.atom-ph↗

arXiv2017

Transition from electromagnetically induced transparency to Autler-Townes splitting in cold cesium atoms

Electromagnetically induced transparency (EIT) and Aulter-Townes splitting (ATS) are two similar yet distinct phenomena that modify the transmission of a weak probe field through an absorption medium in the presence of a coupling field, featured in a variety of three-level atomic systems. In many applications it is important to distinguish EIT from ATS splitting. We present EIT and ATS spectra in a cold-atom three-level cascade system, involving the 35$S_{1/2}$ Rydberg state of cesium. The EIT linewidth, $γ_{EIT}$, defined as the full width at half maximum (FWHM), and the ATS splitting, $γ_{ATS}$, defined as the peak-to-peak distance between AT peak pairs, are used to delineate the EIT and ATS regimes and to characterize the transition between the regimes. In the cold-atom medium, in the weak-coupler (EIT) regime $γ_{EIT}$ $\approx$ A + B($Ω_{c}^2$ + $Ω_{p}^2)/Γ_{eg}$, where $Ω_{c}$ and $Ω_{p}$ are the coupler and probe Rabi frequencies, $Γ_{eg}$ is the spontaneous decay rate of the intermediate 6P$_{3/2}$ level, and parameters $A$ and $B$ that depend on the laser linewidth. We explore the transition into the strong-coupler (ATS) regime, which is characterized by the linear relation $γ_{ATS}$ $\approx$ $Ω_{c}$. The experiments are in agreement with numerical solutions of the Master equation.

physics.atom-ph↗

arXiv2017

Nonlinear Zeeman effect, line shapes and optical pumping in electromagnetically induced transparency

We perform Zeeman spectroscopy on a Rydberg electromagnetically induced transparency (EIT) system in a room-temperature Cs vapor cell, in magnetic fields up to 50~Gauss and for several polarization configurations. The magnetic interactions of the $\vert 6S_{1/2}, F_g=4 \rangle$ ground, $\vert 6P_{3/2}, F_e=5 \rangle$ intermediate, and $\vert 33S_{1/2} \rangle$ Rydberg states that form the ladder-type EIT system are in the linear Zeeman, quadratic Zeeman, and the deep hyperfine Paschen-Back regimes, respectively. Starting in magnetic fields of about 5~Gauss, the spectra develop an asymmetry that becomes paramount in fields $\gtrsim40$~Gauss. We use a quantum Monte Carlo wave-function approach to quantitatively model the spectra. Simulated spectra are in good agreement with experimental data. The asymmetry in the spectra is, in part, due to level shifts caused by the quadratic Zeeman effect, but it also reflects the complicated interplay between optical pumping and EIT in the magnetic field. Relevance to measurement applications is discussed. %The simulations are also used to study optical pumping in the magnetic field and to investigate the interplay between optical pumping and EIT, which reduces photon scattering and optical pumping.

physics.atom-ph↗

arXiv2017

Atom-based radio-frequency field calibration and polarization measurement using cesium $nD_J$ Floquet states

We investigate atom-based electric-field calibration and polarization measurement of a 100-MHz linearly polarized radio-frequency (RF) field using cesium Rydberg-atom electromagnetically induced transparency (EIT) in a room-temperature vapor cell. The calibration method is based on matching experimental data with the results of a theoretical Floquet model. The utilized 60$D_J$ fine structure Floquet levels exhibit $J$- and $m_j$-dependent AC Stark shifts and splittings, and develop even-order RF-modulation sidebands. The Floquet map of cesium 60$D_J$ fine structure states exhibits a series of exact crossings between states of different $m_j$, which are not RF-coupled. These exact level crossings are employed to perform a rapid and precise ($\pm 0.5\%$) calibration of the RF electric field. We also map out three series of narrow avoided crossings between fine structure Floquet levels of equal $m_j$ and different $J$, which are weakly coupled by the RF field via a Raman process. The coupling leads to narrow avoided crossings that can also be applied as spectroscopic markers for RF field calibration. We further find that the line-strength ratio of intersecting Floquet levels with different $m_j$ provides a fast and robust measurement of the RF field's polarization.

physics.atom-ph↗

arXiv2016

Spectroscopy of cesium Rydberg atoms in strong radio-frequency fields

We study Rydberg atoms modulated by strong radio-frequency (RF) fields with a frequency of 70 MHz. The Rydberg atoms are prepared in a room temperature cesium cell, and their level structure is probed using electromagnetically induced transparency (EIT). As the RF field increases from the weak- into the strong-field regime, the range of observed RF-induced phenomena progresses from AC level shifts through increasingly pronounced and numerous RF-modulation sidebands to complex state-mixing and level-crossings with high-l hydrogen-like states. Weak anharmonic admixtures in the RF field generate clearly visible modifications in the Rydberg-EIT spectra. A Floquet analysis is employed to model the Rydberg spectra, and good agreement with the experimental observations is found. Our results show that all-optical spectroscopy of Rydberg atoms in vapor cells can serve as an antenna-free, atom-based and calibration-free technique to measure and map RF electric fields and to analyze their higher-harmonic contents.

physics.atom-ph↗

arXiv2015

Atom-interferometric measurement of Stark level splittings

Multiple adiabatic/diabatic passages through avoided crossings in the Stark map of cesium Rydberg atoms are employed as beam splitters and recombiners in an atom-interferometric measurement of energy-level splittings. We subject cold cesium atoms to laser-excitation, electric-field and detection sequences that constitute an (internal-state) atom interferometer. For the read-out of the interferometer we utilize state-dependent collisions, which selectively remove atoms of one kind from the detected signal. We investigate the dependence of the interferometric signal on timing and field parameters, and find good agreement with time-dependent quantum simulations of the interferometer. Fourier analysis of the interferometric signals yield coherence frequencies that agree with corresponding energy-level differences in calculated Stark maps. The method enables spectroscopy of states that are inaccessible to direct laser-spectroscopic observation, due to selection rules, and has applications in field metrology.

physics.atom-ph↗

arXiv2015

Dipolar Rydberg-atom gas prepared by adiabatic passage through an avoided crossing

The passage of cold cesium 49S$_{1/2}$ Rydberg atoms through an electric-field-induced multi-level avoided crossing with nearby hydrogen-like Rydberg levels is employed to prepare a cold, dipolar Rydberg atom gas. When the electric field is ramped through the avoided crossing on time scales on the order of 100~ns or slower, the 49S$_{1/2}$ population adiabatically transitions into high-\emph{l} Rydberg Stark states. The adiabatic state transformation results in a cold gas of Rydberg atoms with large electric dipole moments. After a waiting time of about $1~μ$s and at sufficient atom density, the adiabatically transformed highly dipolar atoms become undetectable, enabling us to discern adiabatic from diabatic passage behavior through the avoided crossing. We attribute the state-selectivity to $m$-mixing collisions between the dipolar atoms. The data interpretation is supported by numerical simulations of the passage dynamics and of binary $m$-mixing collisions.

physics.atom-ph↗