arXiv subjects

Jianwang Cai

Publications and source records attributed to Jianwang Cai.

8 recordsLinked to original sources

arXiv2023

Giant orbit-to-charge conversion induced via the inverse orbital Hall effect

We investigate the orbit-to-charge conversion in YIG/Pt/nonmagnetic material (NM) trilayer heterostructures. With the additional Ru layer on the top of YIG/Pt stacks, the charge current signal increases nearly an order of magnitude in both longitudinal spin Seebeck effect (SSE) and spin pumping (SP) measurements. Through thickness dependence studies of the Ru metal layer and theoretical model, we quantitatively clarify different contributions of the increased SSE signal that mainly comes from the inverse orbital Hall effect (IOHE) of Ru, and partially comes from the orbital sink effect in the Ru layer. A similar enhancement of SSE(SP) signals is also observed when Ru is replaced by other materials (Ta, W, and Cu), implying the universality of the IOHE in transition metals. Our findings not only suggest a more efficient generation of the charge current via the orbital angular moment channel but also provides crucial insights into the interplay among charge, spin, and orbit.

cond-mat.mtrl-sci↗

arXiv2020

Timescales and contribution of heating and helicity effect in helicity-dependent all-optical switching

The manipulation of the magnetic direction by using the ultrafast laser pulse is attractive for its great advantages in terms of speed and energy efficiency for information storage applications. However, the heating and helicity effects induced by circularly polarized laser excitation are entangled in the helicity-dependent all-optical switching (HD-AOS), which hinders the understanding of magnetization dynamics involved. Here, by applying a dual-pump laser excitation, first with a linearly polarized (LP) laser pulse followed by a circularly polarized (CP) laser pulse, we identify the timescales and contribution from heating and helicity effects in HD-AOS with a Pt/Co/Pt triple layer. When the sample is preheated by the LP laser pulses to a nearly fully demagnetized state, CP laser pulses with a much-reduced power switches the sample's magnetization. By varying the time delay between the two pump pulses, we show that the helicity effect, which gives rise to the deterministic helicity induced switching, onsets instantly upon laser excitation, and only exists for less than 0.2 ps close to the laser pulse duration of 0.15 ps. The results reveal that that the transient magnetization state upon which CP laser pulses impinge is the key factor for achieving HD-AOS, and importantly, the tunability between heating and helicity effects with the unique dual-pump laser excitation approach will enable HD-AOS in a wide range of magnetic material systems for the potential ultrafast spintronics applications.

cond-mat.mtrl-sci↗

arXiv2020

Defect-Correlated Skyrmions and Controllable Generation in Perpendicularly Magnetized CoFeB Ultrathin Films

Skyrmions have attracted significant interest due to their topological spin structures and fascinating physical features. The skyrmion phase arises in materials with Dzyaloshinskii-Moriya (DM) interaction at interfaces or in volume of non-centrosymmetric materials. However, although skyrmions were generated experimentally, one critical intrinsic relationship between fabrication, microstructures, magnetization and the existence of skyrmions remains to be established. Here, two series of CoFeB ultrathin films with controlled atomic scale structures are employed to reveal this relationship. By inverting the growth order, the amount of defects can be artificially tuned, and skyrmions are shown to be preferentially formed at defect sites. The stable region and the density of the skyrmions can be efficiently controlled in the return magnetization loops by utilizing first-order reversal curves to reach various metastable states. These findings establish the general and intrinsic relationship from sample preparation to skyrmion generation, offering an universal method to control skyrmion density.

cond-mat.mes-hall↗

arXiv2020

Ghost spintronic THz-emitter-array microscope

Terahertz (THz) wave shows great potential in non-destructive testing, bio detection and cancer imaging. Recent progresses on THz wave near-field probes/apertures enable mechanically raster scanning of an object's surface in the near-field region, while an efficient, non-scanning, non-invasive, deeply sub-diffraction-limited imaging still remains challenging. Here, we demonstrate a THz near-field microscopy using a reconfigurable spintronic THz emitter array (STEA) with computational ghost imaging. By illuminating an object with the reconfigurable STEA in near field and computing the correlation measurements, we reconstruct its image with deeply sub-diffraction resolution. By circulating an external magnetic field, the in-line polarization rotation of THz waves is realized, making the fused image contrast polarization-free. The time-of-flight (TOF) measurements of coherent THz pulses further enables to resolve objects at different distances or depths. The demonstrated ghost spintronic THz-emitter-array microscope (GHOSTEAM) is a new imaging tool for THz near-field real-time imaging (with potential of video framerate), especially opening up paradigm-shift opportunities in non-intrusive label-free bioimaging in a broadband frequency range from 0.1 THz to 30 THz (namely 3.3-1000 cm-1).

physics.optics↗

arXiv2018

Highly-efficient spintronic terahertz emitter enabled by metal-dielectric photonic crystal

Spintronic terahertz (THz) emitter provides the advantages such as apparently broader spectrum, significantly lower cost, and more flexibility in compared with the commercial THz emitters, and thus attracts great interests recently. In past few years, efforts have been made in optimizing the material composition and structure geometry, and the conversion efficiency has been improved close to that of ZnTe crystal. One of the drawbacks of the current designs is the rather limited laser absorption - more than 50% energy is wasted and the conversion efficiency is thus limited. Here, we theoretically propose and experimentally demonstrate a novel device that fully utilizes the laser intensity and significantly improves the conversion efficiency. The device, which consists of a metal-dielectric photonic crystal structure, utilizes the interference between the multiple scattering waves to simultaneously suppress the reflection and transmission of the laser, and to reshape the laser field distributions. The experimentally detected laser absorption and THz generations show one-to-one correspondence with the theoretical calculations. We achieve the strongest THz pulse emission that presents a 1.7 times improvement compared to the currently designed spintronic emitter. This work opens a new pathway to improve the performance of spintronic THz emitter from the perspective of optics.

cond-mat.mes-hall↗

arXiv2018

Roles of heating and helicity in ultrafast all-optical magnetization switching in TbFeCo

Using time-resolved magneto-optical Kerr effect (TR-MOKE) method, helicity-dependent all-optical magnetization switching (HD-AOS) is observed in ferrimagnetic TbFeCo films. The thermal effect and opto-magneto effects are separately justified after single circularly polarized laser pulse. The integral evolution of this ultrafast switching is characterized on different time scales and the defined magnetization reversal time of 460 fs is the fastest ever observed. Combining the heat effect and inverse Faraday effect (IFE), micromagnetic simulations based on a single macro-spin model are performed that reproduce HD-AOS following a linear reversal mechanism.

cond-mat.mtrl-sci↗

arXiv2017

Tuning the diffusion of magnon in Y3Fe5O12 by light excitation

Deliberate control of magnon transportation will lead to an energy-efficient technology for information transmission and processing. Y3Fe5O12(YIG), exhibiting extremely large magnon diffusion length due to the low magnetic damping constant, has been intensively investigated for decades. While most of the previous works focused on the determination of magnon diffusion length by various techniques, herein we demonstrated how to tune magnon diffusion by light excitation. We found that the diffusion length of thermal magnons is strongly dependent on light wavelength when the magnon is generated by exposing YIG directly to laser beam. The diffusion length, determined by a nonlocal geometry at room temperature, is ~30 um for the magnons produced by visible light (400-650 nm), and ~136-156 um for the laser between 808 nm and 980 nm. The diffusion distance is much longer than the reported value. In addition to thermal gradient, we found that light illumination affected the electron configuration of the Fe3+ ion in YIG. Long wavelength laser triggers a high spin to low spin state transition of the Fe3+ ions in FeO6 octahedron. This in turn causes a substantial softening of the magnon thus a dramatic increase in diffusion distance. The present work paves the way towards an efficient tuning of magnon transport behavior which is crucially important for magnon spintronics.

cond-mat.mtrl-sci↗

arXiv2016

A centrosymmetric hexagonal magnet with superstable biskyrmion magnetic nanodomains in a wide temperature range of 100K to 340K

Here, we report on the experimental discovery of biskyrmion magnetic nanodomains at RT and the observation of a biskyrmion-derived topological Hall effect (THE) in the centrosymmetric hexagonal MnNiGa magnet. Using a phase reconstruction technique based on a transport-of-intensity equation (TIE), we established the texture of the biskyrmion spin. Results from Lorentz transmission electron microscopy (TEM) and the topological Hall effect revealed that the biskyrmion phase is stable over a much wider temperature range (100 K to ~340K) and a larger magnetic field range in our material than in skyrmion-hosting bulk crystals reported previously[1-3,6]. The super-wide operating temperature and the broad range of material options indicate important progress toward the realization of skyrmion-based spintronic devices.

cond-mat.mtrl-sci↗