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Jianxiong Zhao

Publications and source records attributed to Jianxiong Zhao.

2 recordsLinked to original sources

Anisotropic Spin Polarization and magnetic spin hall effect in Ferromagnets

Spin-dependent transport in ferromagnets underpins the development of high-density spintronic memories. Spin-dependent transport in strong spin-orbit-coupled ferromagnets exhibits a significant anisotropy. Both the overall spin polarization during charge transport and the magnetic spin Hall conductivity are found to exhibit pronounced anisotropy when the magnetization is tilted away from the crystallographic easy axis or when the electric field is rotated relative to the crystal axes. These anisotropic responses originate primarily from spin-orbit coupling, which is identified as the key driver of the large anisotropy observed in ferromagnet. Furthermore, strain tunability of the magnetic spin Hall anisotropy is demonstrated, with tensile strain progressively enhancing the oscillatory amplitude of the spin Hall conductivity. These findings establish strong spin-orbit-coupled ferromagnets as a platform for anisotropic spin-current generation and field-free spintronic devices that exploit intrinsic material anisotropy for improved performance and energy efficiency.

cond-mat.mes-hall↗

Looping metal-support interaction in heterogeneous catalysts during redox reactions

Metal-support interfaces fundamentally govern the catalytic performance of heterogeneous systems through complex interactions. Here, utilizing operando transmission electron microscopy, we uncovered a type of looping metal-support interaction in NiFe-Fe3O4 catalysts during hydrogen oxidation reaction. At the NiFe-Fe3O4 interfaces, lattice oxygens react with NiFe-activated H atoms, gradually sacrificing themselves and resulting in dynamically migrating interfaces. Meanwhile, reduced iron atoms migrate to the {111} surface of Fe3O4 support and react with oxygen molecules. Consequently, the hydrogen oxidation reaction separates spatially on a single nanoparticle and is intrinsically coupled with the redox reaction of the Fe3O4 support through the dynamic migration of metal-support interfaces. Our work provides previously unidentified mechanistic insight into metal-support interactions and underscores the transformative potential of operando methodologies for studying atomic-scale dynamics.

cond-mat.mtrl-sci↗