arXiv subjects

Jierong Wang

Publications and source records attributed to Jierong Wang.

4 recordsLinked to original sources

arXiv2026

A cryogenic apparatus for coupling two-dimensional materials to a confocal multimode optical cavity

Two-dimensional van der Waals materials exhibit a variety of correlated electron phases, and optical driving offers a promising route toward manipulating them. For example, cavity-enhanced, continuous-wave (CW) Raman excitation has been suggested as a way to coherently and superradiantly populate phonons or charge density waves via material excitons. A steady-state phonon population may be sustained with sufficiently strong electron-phonon coupling to drive novel collective response. We describe an apparatus built to meet the requirements of such an experimental program: Namely, an ultrahigh-vacuum system housing a length-tunable confocal Fabry-Pérot cavity with an intracavity sample, both cryogenically cooled and stabilized against vibrations. A four-axis nanopositioner aligns the sample and supports electrical leads for sample carrier density modulation and transport measurements. Transmission through the multimode cavity enables in situ sample imaging for alignment; the sample is a transition metal dichalcogenide in this work. Operating near the confocal geometry concentrates the optical field into a localized supermode that substantially enhances light-matter coupling. This enhancement is preserved despite the millimeter-scale cavity length, which provides room for sample alignment and exchange.

quant-ph↗

arXiv2026

Long-Range Fermi-Polaron Blockade in Monolayer MoSe$_2$

Strong optical nonlinearities at the few-photon level are a central goal for quantum photonics, yet they remain difficult to realize in solid-state systems. In doped two-dimensional semiconductors, coupling between excitons and a degenerate Fermi sea gives rise to exciton-Fermi polarons, many-body quasiparticles whose optical response is governed by fermionic correlations. Here, using femtosecond pump-probe transient absorption microscopy, we directly image the spatially resolved nonlinear optical response of exciton-Fermi polarons in monolayer MoSe$_2$. We observe a pronounced spatial suppression of resonant absorption associated with the attractive Fermi polaron, from which we extract an optical blockade radius that is more than ten times larger than that of the neutral exciton. Microscopic analysis indicates that this extended nonlinearity arises primarily from fermion-mediated interactions between exciton-Fermi polarons. Our results establish exciton-Fermi polarons in two-dimensional semiconductors as electrically tunable, strongly interacting optical quasiparticles, and identify them as a promising platform for ultralow-power nonlinear optical devices.

cond-mat.mes-hall↗

arXiv2024

Direct Exfoliation of Nanoribbons from Bulk van der Waals Crystals

Confinement of monolayers into quasi-one-dimensional atomically-thin nanoribbons could lead to novel quantum phenomena beyond those achieved in their bulk and monolayer counterparts. However, current experimental availability of nanoribbon species beyond graphene has been limited to bottom-up synthesis or top-down patterning. In this study, we introduce a versatile and direct lithography-free approach to exfoliate a variety of bulk van der Waals (vdW) crystals into nanoribbons. Akin to the Scotch tape exfoliation in producing monolayers, this technique provides convenient access to a wide range of nanoribbons derived from their corresponding bulk crystals, including MoS2, WS2, MoSe2, WSe2, MoTe2, WTe2, ReS2, and hBN. The nanoribbons are single-crystalline, parallel-aligned, flat, and have high aspect ratio. We demonstrated the electrical, magnetic, and optical properties from the confinement, strain, and edge configurations of these nanoribbons. This versatile preparation technique will pave the way for future experimental investigation and broad applications in optoelectronic, sensing, electronic and quantum devices.

cond-mat.mtrl-sci↗

arXiv2022

Controlling frustrated magnetism on the kagome lattice by uniaxial-strain tuning

It is predicted that strongly interacting spins on a frustrated lattice may lead to a quantum disordered ground state or even form a quantum spin liquid with exotic low-energy excitations. However, a thorough tuning of the frustration strength, separating its effects from those of disorder and other factors, is pending. Here we break the symmetry of a kagome-lattice compound in a controlled manner by applying $in$ $situ$ uniaxial stress. The transition temperature of $\rm Y_3Cu_9(OH)_{18}OCl_8$ is linearly enhanced with strain, $ΔT_{\rm N}/T_{\rm N} \approx 10\%$ upon in-plane compression of order $1\%$, providing clear evidence for a release of frustration and its pivotal role for magnetic order. Our comprehensive $^1$H NMR results suggest a $\overrightarrow{Q}=(1/3\times 1/3)$ state under unstrained conditions and further reveal an incomplete antiferromagnetic transition with fluctuating moments in this strongly frustrated system.

cond-mat.str-el↗