arXiv subjects

Jigang Wang

Publications and source records attributed to Jigang Wang.

At least 37 records · Page 2Linked to original sources

arXiv2024

Two-dimensional coherent spectrum of high-spin models via a quantum computing approach

We present and benchmark a quantum computing approach to calculate the two-dimensional coherent spectrum (2DCS) of high-spin models. Our approach is based on simulating their real-time dynamics in the presence of several magnetic field pulses, which are spaced in time. We utilize the adaptive variational quantum dynamics simulation (AVQDS) algorithm for the study due to its compact circuits, which enables simulations over sufficiently long times to achieve the required resolution in frequency space. Specifically, we consider an antiferromagnetic quantum spin model that incorporates Dzyaloshinskii-Moriya interactions and single-ion anisotropy. The obtained 2DCS spectra exhibit distinct peaks at multiples of the magnon frequency, arising from transitions between different eigenstates of the unperturbed Hamiltonian. By comparing the one-dimensional coherent spectrum with 2DCS, we demonstrate that 2DCS provides a higher resolution of the energy spectrum. We further investigate how the quantum resources scale with the magnitude of the spin using two different binary encodings of the high-spin operators: the standard binary encoding and the Gray code. At low magnetic fields both encodings require comparable quantum resources, but at larger field strengths the Gray code is advantageous. Numerical simulations for spin models with increasing number of sites indicate a polynomial system-size scaling for quantum resources. Lastly, we compare the numerical 2DCS with experimental results on a rare-earth orthoferrite system. The observed strength of the magnonic high-harmonic generation signals in the 2DCS of the quantum high-spin model aligns well with the experimental data, showing significant improvement over the corresponding mean-field results.

quant-ph↗

arXiv2024

Multi-Dimensional Coherent Spectroscopy of Light-Driven States and their Collective Modes in Multi-Band Superconductors

We present a comprehensive theory of light-controlled multi-band superconductivity and apply it to predict distinctive signatures of light-driven superconducting (SC) states in terahertz multi-dimensional coherent spectroscopy (THz-MDCS) experiments. We first derive gauge-invariant Maxwell-Bloch equations for multi-band BCS superconductors. For this, we go beyond previously considered Anderson pseudo-spin precession models to include quantum transport effects. By calculating the THz-MDCS spectra measured experimentally, we then identify unique signatures of finite-momentum Cooper-pairing states that live longer than the laser pulse. These non-equilibrium SC states are characterized by long-lived canting of Anderson pseudo-spins. The pseudo-spin oscillators that describe the properties of these SC states are parametrically driven by both finite-momentum Cooper pairing and by time oscillations of the order parameter relative phase. We show that such strong parametric driving leads to drastic changes in the THz-MDCS spectral shape from the predictions of third-order nonlinear susceptibility calculations. These spectral changes strongly depend on the interband-to-intraband interaction ratio and on the collective modes of the light-driven state.

cond-mat.supr-con↗

arXiv2024

Observation of the Magnonic Dicke Superradiant Phase Transition

Two-level atoms coupled with single-mode cavity photons are predicted to exhibit a quantum phase transition when the coupling strength exceeds a critical value, entering a phase in which atomic polarization and photonic field are finite even at zero temperature and without external driving. However, this phenomenon, the superradiant phase transition (SRPT), is forbidden by a no-go theorem due to the existence of the diamagnetic term in the Hamiltonian. Here, we present spectroscopic evidence for a magnonic SRPT in ErFeO$_3$, where the role of the photonic mode (two-level atoms) in the photonic SRPT is played by an Fe$^{3+}$ magnon mode (Er$^{3+}$ spins). The absence of the diamagnetic term in the Fe$^{3+}$-Er$^{3+}$ exchange coupling ensures that the no-go theorem does not apply. Terahertz and gigahertz magnetospectroscopy experiments revealed the signatures of the SRPT -- a kink and a softening, respectively, of two spin-magnon hybridized modes at the critical point.

quant-ph↗

arXiv2023

One In-Situ Extraction Algorithm for Monitoring Bunch-by-Bunch Profile in the Storage Ring

As the brightness of synchrotron radiation (SR) light sources improves, the operation stability of light sources is weakened. To explore various beam instability related issues in light sources, one transverse beam diagnostics system for bunch-by-bunch (BbB) profile measurement has been established at Hefei Light Source-II (HLS-II). In this paper, one in-situ extraction algorithm in the data processing backend of the system is developed for BbB profiles, so as to provide important beam information of the machine operation in time.

physics.acc-ph↗

arXiv2023

Evidence for highly damped Higgs mode in infinite-layer nickelates

The dynamics of Higgs mode in superconductors, manifested as coherent oscillations of the superconducting order parameter amplitude, provides vital insights into the nature of the superconducting gap structure and symmetry. Here we utilize two-dimensional terahertz coherent spectroscopy to investigate Higgs dynamics of a newly discovered infinite-layer nickelate superconductor. While we observe distinct nonlinear terahertz responses from the superconducting state, well-defined long-lived Higgs modes, as commonly observed in $s$-wave superconductors, are entirely absent in the nickelate film. Instead, we find the coherent nonlinear terahertz response is dominated by the quasiparticle excitations. These observations strongly indicate that the Higgs mode in infinite-layer nickelates is heavily damped by the quasiparticle excitations at arbitrarily low energies, which is a characteristic of $d$-wave pairing symmetry. Additionally, by examining the temperature dependence of the nonlinear terahertz response, we discover short-range superconducting fluctuations in the vicinity of $T_\mathrm{c}$. Our findings provide proof of a new $d$-wave system and establish a foundation for investigating the unconventional superconductivity in nickelates.

cond-mat.supr-con↗

arXiv2023

Low-energy electrodynamics of infinite-layer nickelates: evidence for d-wave superconductivity in the dirty limit

The discovery of superconductivity in infinite-layer nickelates establishes a new category of unconventional superconductors that share structural and electronic similarities with cuprates. Despite exciting advances, such as the establishment of a cuprate-like phase diagram and the observation of charge order and short-range antiferromagnetic fluctuation, the key issues of superconducting pairing symmetry, gap amplitude, and superconducting fluctuation remain elusive. In this work, we utilize static and ultrafast terahertz spectroscopy to address these outstanding problems. We demonstrate that the equilibrium terahertz conductivity and nonequilibrium terahertz responses of an optimally Sr-doped nickelate film ($T_c$ = 17 K) are in line with the electrodynamics of $d$-wave superconductivity in the dirty limit. The gap-to-$T_c$ ratio 2$Δ/k_\mathrm{B}T_\mathrm{c}$ is extracted to be 3.4, indicating the superconductivity falls in the weak-coupling regime. In addition, we observed significant superconducting fluctuation near $T_\mathrm{c}$, while it does not extend into the deep normal state as optimally hole-doped cuprates. Our result highlights a new $d$-wave system which closely resembles the electron-doped cuprates, expanding the family of unconventional superconductivity in oxides.

cond-mat.supr-con↗

arXiv2023

Ab-initio Simulations of Coherent Phonon-Induced Pumping of Carriers in Zirconium Pentatelluride

Laser-driven coherent phonons can act as modulated strain fields and modify the adiabatic ground state topology of quantum materials. Here we use time-dependent first-principles and effective model calculations to simulate the effect of the coherent phonon induced by strong terahertz electric field on electronic carriers in the topological insulator ZrTe$_5$. We show that a coherent $A_\text{1g}$ Raman mode modulation can effectively pump carriers across the band gap, even though the phonon energy is about an order of magnitude smaller than the equilibrium band gap. We reveal the microscopic mechanism of this effect which occurs via Landau-Zener-Stückelberg tunneling of Bloch electrons in a narrow region in the Brillouin zone center where the transient energy gap closes when the system switches from strong to weak topological insulator. The quantum dynamics simulation results are in excellent agreement with recent pump-probe experiments in ZrTe$_5$ at low temperature.

cond-mat.mtrl-sci↗

arXiv2023

Chirality manipulation of ultrafast phase switchings in a correlated CDW-Weyl semimetal

A recently emerging concept for quantum phase discovery is the controlled gapping of linear band crossings in topological semimetals. For example, achieving topological superconducting and charge-density-wave (CDW) gapping could introduce Majorana zero modes and axion electrodynamics, respectively. Light engineering of correlation gaps in topological materials provides a new avenue of achieving exotic topological phases inaccessible by conventional tuning methods such as doping and straining. Here we demonstrate a light control of correlation gaps and ultrafast phase switchings in a model CDW and polaron insulator (TaSe$_4$)$_2$I recently predicted to be an axion insulator. Our ultrafast terahertz photocurrent spectroscopy reveals a two-step, non-thermal melting of polarons and electronic CDW gap via studying the fluence dependence of a {\em longitudinal} circular photogalvanic current. The helicity-dependent photocurrent observed along the propagation of light reveals continuous ultrafast switchings from the polaronic state, to the CDW (axion) phase, and finally to a hidden Weyl phase as the pump fluence increases. Other distinguishing features corroborating with the light-induced switchings include: mode-selective coupling of coherent phonons to polaron and CDW modulation, and the emergence of a {\em non-thermal} chiral photocurrent above pump threshold of CDW-related phonons. The ultrafast chirality control of correlated topological states revealed here is important to realize axion electrodynamics and quantum computing.

cond-mat.str-el↗

arXiv2023

An Effective Deployment of Contrastive Learning in Multi-label Text Classification

The effectiveness of contrastive learning technology in natural language processing tasks is yet to be explored and analyzed. How to construct positive and negative samples correctly and reasonably is the core challenge of contrastive learning. It is even harder to discover contrastive objects in multi-label text classification tasks. There are very few contrastive losses proposed previously. In this paper, we investigate the problem from a different angle by proposing five novel contrastive losses for multi-label text classification tasks. These are Strict Contrastive Loss (SCL), Intra-label Contrastive Loss (ICL), Jaccard Similarity Contrastive Loss (JSCL), Jaccard Similarity Probability Contrastive Loss (JSPCL), and Stepwise Label Contrastive Loss (SLCL). We explore the effectiveness of contrastive learning for multi-label text classification tasks by the employment of these novel losses and provide a set of baseline models for deploying contrastive learning techniques on specific tasks. We further perform an interpretable analysis of our approach to show how different components of contrastive learning losses play their roles. The experimental results show that our proposed contrastive losses can bring improvement to multi-label text classification tasks. Our work also explores how contrastive learning should be adapted for multi-label text classification tasks.

cs.CL↗

arXiv2022

Cryogenic Magneto-Terahertz Scanning Near-field Optical Microscope (cm-SNOM)

We have developed a versatile near-field microscopy platform that can operate at high magnetic fields and below liquid-helium temperatures. We use this platform to demonstrate an extreme terahertz (THz) nanoscope operation and to obtain the first cryogenic magneto-THz time-domain nano-spectroscopy/imaging at temperatures as low as 1.8 K and magnetic fields of up to 5 T simultaneously. Our cryogenic magneto-THz scanning near-field optical microscopy, or cm-SNOM, instrument comprises three main equipment: i) a 5 T split pair magnetic cryostat with a custom made insert for mounting SNOM inside; ii) an atomic force microscope (AFM) unit that accepts ultrafast THz excitation and iii) a MHz repetition rate, femtosecond laser amplifier for high-field THz pulse generation and sensitive detection. We apply the cm-SNOM to obtain proof of principle measurements of superconducting and topological materials. The new capabilities demonstrated break grounds for studying quantum materials that requires extreme environment of cryogenic operation and applied magnetic fields simultaneously in nanometer space, femtosecond time, and terahertz energy scales.

cond-mat.mes-hall↗

arXiv2021

Local atomic configuration control of superconductivity in the undoped pnictide parent compound BaFe2As2

Emergent superconductivity is strongly correlated with the symmetry of local atomic configuration in the parent compounds of iron-based superconductors. While chemical doping or hydrostatic pressure can change the local geometry, these conventional approaches do not provide a clear pathway in tuning the detailed atomic arrangement predictably, due to the parent compounds complicated structural deformation in the presence of the tetragonal-to-orthorhombic phase transition. Here, we demonstrate a systematic approach to manipulate the local structural configurations in BaFe2As2 epitaxial thin films by controlling two independent structural factors orthorhombicity (in-plane anisotropy) and tetragonality (out-of-plane/in-plane balance) from lattice parameters. We tune superconductivity without chemical doping utilizing both structural factors separately, controlling local tetrahedral coordination in designed thin film heterostructures with substrate clamping and bi-axial strain. We further show that this allows quantitative control of both the structural phase transition, associated magnetism, and superconductivity in the parent material BaFe2As2. This approach will advance the development of tunable thin film superconductors in reduced dimension.

cond-mat.supr-con↗

arXiv2021

Hefei light source storage ring bunch by bunch 3D position measuring system is introduced and a preliminary study is shown

The 4 electrode signals of the beam position detector(BPM) of the STORAGE ring of HEFEI Light Source are directly connected to the domestic oscilloscope with 12bit resolution, 10Gsps sampling rate and 2GHz bandwidth. The acquisition program is run on the cloud host under the Zstack architecture, triggering to read a group of waveforms of 500us each time. The X (horizontal position), Y (vertical position) and Z (longitudinal phase) information of the centroid of 45 bunches 2266 cycles were extracted. The resolution of X and Y of each bunches was about 5um, and the resolution of Z was about 0.5ps. The update period of online operation was about 7 seconds. The three-dimensional tune of each bunch can be obtained by analyzing the three-dimensional position information of each bunch in normal operation. The spectrum peak of the transverse quadrupole oscillation can be observed by analyzing the button and strip electrode signals when beam is incentived.

physics.ins-det↗

arXiv2020

Wavelength conversion through plasmon-coupled surface states

Surface states generally degrade semiconductor device performance by raising the charge injection barrier height, introducing localized trap states, inducing surface leakage current, and altering the electric potential. Therefore, there has been an endless effort to use various surface passivation treatments to suppress the undesirable impacts of the surface states. We show that the giant built-in electric field created by the surface states can be harnessed to enable passive wavelength conversion without utilizing any nonlinear optical phenomena. Photo-excited surface plasmons are coupled to the surface states to generate an electron gas, which is routed to a nanoantenna array through the giant electric field created by the surface states. The induced current on the nanoantennas, which contains mixing product of different optical frequency components, generates radiation at the beat frequencies of the incident photons. We utilize the unprecedented functionalities of plasmon-coupled surface states to demonstrate passive wavelength conversion of nanojoule optical pulses at a 1550 nm center wavelength to terahertz regime with record-high efficiencies that exceed nonlinear optical methods by 4-orders of magnitude. The presented scheme can be used for optical wavelength conversion to different parts of the electromagnetic spectrum ranging from microwave to infrared regimes by using appropriate optical beat frequencies.

physics.optics↗

arXiv2020

Lightwave Terahertz Quantum Manipulation of Non-equilibrium Superconductor Phases and their Collective Modes

We present a gauge-invariant density matrix description of non-equilibrium superconductor (SC) states with spatial and temporal correlations driven by intense terahertz (THz) lightwaves. We derive superconductor Bloch--Maxwell equations of motion that extend Anderson pseudo-spin models to include the Cooper pair center-of-mass motion and electromagnetic propagation effects. We thus describe quantum control of dynamical phases, collective modes, quasi-particle coherence, and high nonlinearities during cycles of carrier wave oscillations, which relate to our recent experiments. Coherent photogeneration of a nonlinear supercurrent with dc component via condensate acceleration by an effective lightwave field dynamically breaks the equilibrium inversion symmetry. Experimental signatures include high harmonic light emission at equilibrium-symmetry-forbidden frequencies, Rabi--Higgs collective modes and quasi-particle coherence, and non-equilibrium moving condensate states tuned by few-cycle THz fields. We use such lightwaves as an oscillating accelerating force that drives strong nonlinearities and anisotropic quasi-particle populations to control and amplify different classes of collective modes, e.g., damped oscillations, persistent oscillations, and overdamped dynamics via Rabi flopping. Recent phase-coherent nonlinear spectroscopy experiments can be modeled by solving the full nonlinear quantum dynamics including self-consistent light--matter coupling.

cond-mat.supr-con↗

arXiv2018

Impact of damping on superconducting gap oscillations induced by intense Terahertz pulses

We investigate the interplay between gap oscillations and damping in the dynamics of superconductors taken out of equilibrium by strong optical pulses with sub-gap Terahertz frequencies. A semi-phenomenological formalism is developed to include the damping within the electronic subsystem that arises from effects beyond BCS, such as interactions between Bogoliubov quasiparticles and decay of the Higgs mode. Such processes are conveniently expressed as $T_{1}$ and $T_{2}$ times in the standard pseudospin language for superconductors. Comparing with data on NbN that we report here, we argue that the superconducting dynamics in the picosecond time scale, after the pump is turned off, is governed by the $T_{2}$ process.

cond-mat.supr-con↗

arXiv2015

Beam size and position measurement based on logarithm processing algorithm in HLS II

A logarithm processing algorithm to measure beam transverse size and position is proposed and preliminary experimental results in Hefei Light Source II (HLS II) are given. The algorithm is based on only 4 successive channels of 16 anode channels of multianode photomultiplier tube (MAPMT) R5900U-00-L16 which has typical rise time of 0.6 ns and effective area of 0.8x16 mm for a single anode channel. In the paper, we firstly elaborate the simulation results of the algorithm with and without channel inconsistency. Then we calibrate the channel inconsistency and verify the algorithm using general current signal processor Libera Photon in low-speed scheme. Finally we get turn-by-turn beam size and position and calculate the vertical tune in high-speed scheme. The experimental results show that measured values fit well with simulation results after channel differences are calibrated and the fractional part of the tune in vertical direction is 0.3628 which is very close to the nominal value 0.3621.

physics.acc-ph↗

arXiv2015

Ultrafast terahertz probes of interacting dark excitons in chirality-specific semiconducting single-walled carbon nanotubes

Ultrafast terahertz spectroscopy accesses the {\em dark} excitonic ground state in resonantly-excited (6,5) SWNTs via internal, direct dipole-allowed transitions between lowest lying dark-bright pair state $\sim$6 meV. An analytical model reproduces the response which enables quantitative analysis of transient densities of dark excitons and {\em e-h} plasma, oscillator strength, transition energy renormalization and dynamics. %excitation-induced renormalization. Non-equilibrium, yet stable, quasi-1D quantum states with dark excitonic correlations rapidly emerge even with increasing off-resonance photoexcitation and experience a unique crossover to complex phase-space filling of %a complex distribution between both dark and bright pair states, different from dense 2D/3D excitons influenced by the thermalization, cooling and ionization to free carriers.

cond-mat.mes-hall↗

arXiv2014

Ultrafast Probes of Nonequilibrium Hole Spin Relaxation in Ferromagnetic Semiconductor GaMnAs

We directly measure the hole spin lifetime in ferromagnetic GaMnAs via time- and polarization-resolved spectroscopy. Below the Curie temperature Tc, an ultrafast photoexcitation with linearly-polarized light is shown to create a non-equilibrium hole spin population via the dynamical polarization of holes through p-d exchange scattering with ferromagnetically-ordered Mn spins, and we characterize their relaxation dynamics. The observed relaxation consists of a distinct three-step recovery : (i) femtosecond (fs) hole spin relaxation ~ $160-200 fs, (ii) picosecond (ps) hole energy relaxation ~ 1-2 ps, and (iii) a coherent, damped Mn spin precession with a period of ~ 250 ps. The transient amplitude of the hole spin component diminishes with increasing temperature, directly following the ferromagnetic order, while the hole energy amplitude shows negligible temperature change, consistent with our interpretation. Our results thus establish the hole spin lifetimes in ferromagnetic semiconductors and demonstrate a novel spectroscopy method for studying non-equilibrium hole spins in the presence of correlation and magnetic order.

cond-mat.mtrl-sci↗