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Jihang Zhu

Publications and source records attributed to Jihang Zhu.

At least 19 recordsLinked to original sources

Crystallization in the Fractional Quantum Hall Regime with Disorder-Aware Neural Quantum States

We present the first microscopic demonstration of a disorder-pinned hole Wigner crystal (WC), providing a natural explanation for the reentrant integer quantum Hall effect observed near $ν=2/3$, as well as its analogs in fractional Chern insulators. We further identify a novel crossover regime above filling $ν=2/3$ that connects this hole WC to an electron WC, characterized by a network-like electron density structure. To uncover these phenomena, we use neural-network variational Monte Carlo (NNVMC) with a disorder-aware self-attention neural quantum state that describes both fractional quantum Hall (FQH) liquids and Wigner crystals within a single unbiased variational framework. More broadly, our method establishes a unified phase diagram that exposes a fundamental asymmetry in crystallization across half-filling: near $ν=1/3$, increasing LL mixing and disorder both stabilize an electron WC, whereas near $ν=2/3$, the hole WC dominates at weak LL mixing and ultimately gives way to the electron WC at strong LL mixing.

cond-mat.str-el

Microscopic origin of orbital magnetization in chiral superconductors

Chiral superconductivity is a time-reversal-symmetry-breaking superconducting phase that has attracted broad interest as a potential platform for topological quantum computation. A fundamental consequence of this symmetry breaking is orbital magnetization, yet a clear microscopic formulation of this quantity has remained elusive. This difficulty arises because Bogoliubov quasiparticles do not carry a definite electric charge, precluding a simple interpretation of orbital magnetization in terms of circulating quasiparticle currents. Moreover, superconductivity and ferromagnetism rarely coexist, and in the few materials where they do (e.g. uranium-based compounds), strong spin-orbit coupling obscures the orbital contribution to the magnetization. The recent report of chiral superconductivity in rhombohedral multilayer graphene, which has negligible spin-orbit coupling, therefore provides a unique opportunity to develop and test a microscopic theory of orbital magnetization in chiral superconductors. Here we develop such a theory, unifying the interband coherence effects underlying normal-state orbital magnetization with the intrinsic orbital moments of the Cooper-pair condensate. Applying our theory to rhombohedral tetralayer graphene, we find that the onset of superconductivity can either enhance or suppress the normal-state orbital magnetization, depending on the bandstructure. We further identify a generalized clapping mode with a gap set by the sublattice winding form factor. This collective mode is unique to chiral superconductors and contributes to the orbital magnetization through its role in dressing the photon vertex. Our theory resolves a long-standing conceptual difficulty in defining orbital magnetization in superconducting systems, and measurements of the orbital magnetization relative to the quarter-metal phase would provide a direct experimental test.

cond-mat.supr-con

Superconductivity from phonon-mediated retardation in a single-flavor metal

We study phonon-mediated pairings in a single-flavor metal with a tunable Berry curvature. In the absence of Berry curvature, we discover an unexpected possibility: $p$-wave superconductivity emerging purely from the retardation effect, while the static BCS approximation fails to predict its existence. The gap function exhibits sign-change behavior in frequency (owing to the dynamical structure of the phonon-mediated interaction in the $p$-wave channel), and $T_c$ obeys a BCS-like scaling. We further show that the Berry curvature stabilizes the chiral $p$-wave superconductivity and can induce transitions to higher-angular-momentum pairings. Our results establish that the phonon-mediated mechanism is a viable pairing candidate in single-flavor systems, such as the quarter-metal superconductivity observed in rhombohedral graphene multilayers.

cond-mat.supr-con

Apparent inconsistency between Streda formula and Hall conductivity in reentrant integer quantum anomalous Hall effect in twisted MoTe$_2$

Recent experiments in twisted bilayer MoTe$_2$ (tMoTe$_2$) have uncovered a rich landscape of correlated phases. In this work, we investigate the reentrant integer quantum anomalous Hall (RIQAH) states reported by F. Xu, arXiv.2504.06972 which display a notable mismatch between the Hall conductivity measured via transport and that inferred from the Streda formula. We argue that this discrepancy can be explained if the RIQAH state is a quantum Hall bubble or Wigner crystal phase, analogous to similar well-established phenomena in two-dimensional (2D) GaAs quantum wells. While this explains the RIQAH state at filling $ν= -0.63$, F. Xu et al. report that the other RIQAH state at $ν= -0.7$ has a smaller slope, necessitating a different interpretation. We propose and substantiate with analysis of the experimental data that this discrepancy arises due to a nearby resistive peak masking the true slope. Furthermore, we identify this resistive peak as a signature of a phase transition near $ν= -0.75$, possibly driven by a van Hove singularity. The anomalous Hall response and Landau fan evolution across this transition suggest a change in Fermi-surface topology and a metallic phase with a non quantized Hall response. These observations offer new insights into the nature of the RIQAH states and raise the possibility that the nearby superconducting phase may have a valley-imbalanced metal parent state.

cond-mat.str-el

Orbital Magnetization and Streda Formula of Interacting Electrons in the Mean-field Approximation

We study the magnetic-field response of interacting electron systems within mean-field theory using perturbation theory. We show that the linear response of the mean-field density-matrix to a weak magnetic field is purely geometric: it depends only on wavefunction derivatives, the Berry connections linking the occupied and unoccupied subspaces, and does not explicitly depend on the interaction potential and the quasiparticle dispersion. This leads to compact, gauge-invariant projector expressions for both the St\v{r}eda formula and the formula for orbital magnetization. Our calculation explicitly elucidates the role of exchange and self-consistency in defining current vertices for orbital magnetization calculations. Our work establishes a direct connection between mean-field theory, quantum geometry and the non-interacting topological band theory.

cond-mat.mes-hall

2D bilayer electron-hole superfluidity with unequal and anisotropic masses

We investigate the stability of electron-hole superfluidity in two-dimensional bilayers with unequal and anisotropic effective masses. Using a zero-temperature, self-consistent Hartree-Fock approach, we study two experimentally relevant deviations from the ideal equal-mass isotropic case: (i) isotropic but unequal conduction and valence band masses ($m_c^* \neq m_v^*$), and (ii) equal average masses with orthogonal in-plane anisotropies $(m_{c,x}^*, m^*_{c,y}) = (m_1^*, m_2^*)$ and $(m^*_{v,x}, m^*_{v,y}) = (m_2^*, m_1^*)$. For both scenarios, we compute the order parameter and analyze the BEC-BCS crossover as a function of layer separation and mass ratio. We find that both mass imbalance and mass anisotropy reduce the pairing strength and suppress the inferred critical temperature $T_c$ by breaking perfect Fermi surface nesting, and shift the BEC-BCS crossover. Despite these effects, superfluidity remains robust across the full range of densities and interlayer separations considered, with no transition to an unpaired plasma state in the absence of screening. Our results provide a baseline for understanding the interplay of mass mismatch and anisotropy in current and emerging bilayer platforms, including van der Waals heterostructures and anisotropic two-dimensional semiconductors. Our work also establishes that Fermi surface nesting is not a key ingredient for the bilayer superfluidity, which is always the ground state for all electron-hole bilayers although the resultant $T_c$ depends on the parameter details and may very well be unmeasurably low for large interlayer separations.

cond-mat.supr-con

In-plane magnetic field-induced orbital FFLO superconductivity in twisted WSe$_2$ homobilayers

We theoretically predict the in-plane magnetic field-induced orbital Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconducting states in twisted WSe$_2$ homobilayers (tWSe$_2$), focusing on its dependence on layer polarization and Fermi surface geometry. For unpolarized layers, finite-momentum pairing emerges only at low temperatures and above a critical field $B_{c1,\parallel}$. When layer symmetry is broken, finite-momentum pairing is stabilized at any nonzero field, with a critical temperature higher than that of the zero-momentum state. Notably, we identify a phase transition, which separates two distinct FFLO phases, when there are two separate Fermi pockets residing in the two moiré mini-valleys associated with opposite layers. We further discuss the effects of twist angles and applied field directions. Our findings establish tWSe$_2$ as a promising platform for realizing and manipulating FFLO states via twist angle, displacement field, and filling factor.

cond-mat.supr-con

Intravalley spin-polarized superconductivity in rhombohedral tetralayer graphene

We study the intravalley spin-polarized superconductivity in rhombohedral tetralayer graphene, which has been discovered experimentally in Han $et$ $al$ arXiv:2408.15233. We construct a minimal model for the intravalley spin-polarized superconductivity, assuming a simplified anisotropic interaction that depends only on the angle between the incoming and outgoing momenta. Despite the absence of \textit{Fermi surface nesting}, we show that superconductivity can emerge near the Van Hove singularity with the maximal $T_c$ near a bifurcation point of the peaks in the density of states. We identify the $p+ip$, $h+ih$, and the nodal $f$-wave pairings as the possible states, which are all pair density wave orders due to the intravalley nature. Furthermore, these pair density wave orders require a finite attractive threshold for superconductivity, resulting in {a narrow stripe shape of superconducting region}, consistent with experimental findings. We point out that the Kohn-Luttinger mechanism is a plausible explanation with a dominant $p+ip$ pairing. The possibility of realizing intravalley spin-polarized superconductivity in other rhombohedral graphene systems is also discussed.

cond-mat.supr-con

Superconductivity in twisted transition metal dichalcogenide homobilayers

For the first time, robust superconductivity has been independently observed in twisted WSe$_2$ bilayers by two separate groups [Y. Xia et al., arXiv:2405.14784; Y. Guo et al., arXiv:2406.03418.]. In light of this, we explore the possibility of a universal superconducting pairing mechanism in twisted WSe$_2$ bilayers. Using a continuum band structure model and a phenomenological boson-mediated effective electron-electron attraction, we find that intervalley intralayer pairing predominates over interlayer pairing. Notably, despite different experimental conditions, both twisted WSe$_2$ samples exhibit a comparable effective attraction strength. This consistency suggests that the dominant pairing glue is likely independent of the twist angle and layer polarization, pointing to a universal underlying boson-induced pairing mechanism.

cond-mat.supr-con

Independently Tunable Flat Bands and Correlations in a Graphene Double Moiré System

We report on a double moiré system consisting of four graphene layers, where the top and bottom pairs form small-twist-angle bilayer graphene, and the middle interface has a large rotational mismatch. This system shows clear signatures of two sets of spatially separated flat bands associated with the top and bottom twisted bilayer graphene (TBG) subsystems, each independently tunable. Thermodynamic analysis reveals weak correlations between layers that allow the chemical potential to be measured as a function of carrier density for each constituent TBG. We find that correlated insulating states at integer number of electrons per moiré unit cell are most robust near magic angle, whereas gapped states at neutrality are more robust at larger twist angles.

cond-mat.mes-hall

Weak Coupling Theory of Magic-Angle Twisted Bilayer Graphene

Strong correlations occur in magic-angle twisted bilayer graphene (MATBG) when the octet of flat moiré minibands centered on charge neutrality (CN) is partially occupied. The octet consists of a single valence band and a single conduction band for each of four degenerate spin-valley flavors. Motivated by the importance of Hartree electrostatic interactions in determining the filling-factor dependent band structure, we use a time-dependent Hartree approximation to gain insight into electronic correlations. We find that the electronic compressibility is dominated by Hartree interactions, that paramagnetic states are stable over a range of density near CN, and that the dependence of energy on flavor polarization is strongly overestimated by mean-field theory.

cond-mat.str-el

Pseudospin density wave instability in two-dimensional electron bilayers

We investigate the instability of layer pseudospin paramagnetic (PSP) state to the formation of pseudospin density wave (PSDW) in two-dimensional (2D) electron bilayers, analogous to the formation of Overhauser spin density wave (SDW) in a single-layer 2D electron gas (2DEG) with spin 1/2. Our comprehensive study on phase diagrams, based on the self-consistent Hartree-Fock (HF) theory, reveals that the PSDW has a lower energy than both PSP and pseudospin ferromagnetic (PSF) states near the PSP-PSF phase transition boundary. When the two layers are populated by the same number of electrons, the PSDW momentum $Q_c \sim 2k_F$ near the PSP-PSDW boundary, where $k_F= (2πn)^{1/2}$ is the Fermi momentum characterized by the density in one of the two layers, and $Q_c$ decreases as the system transitions to the PSF regime. Extending the HF study to the case of unequal layer densities, the PSP phase is unstable to PSDW for small density imbalances, with momentum $Q_c \sim k_{F,t} + k_{F,b}$, where $k_{F,t}$ and $k_{F,b}$ are Fermi momenta of top and bottom layers, respectively. In PSDW regime, the ground state stability, defined by the energy difference between PSDW and the second lowest-energy state, is one order of magnitude lower than that in PSF regime, and decreases with increasing layer separation $d$. Furthermore, incorporating RPA static screening with the Hubbard-type local field correction leads to disappearance of both SDW and PSDW phases, and pushes the phase boundaries of paramagnetic to ferromagnetic transitions to larger $r_s$ values. Our study on PSDW in 2D electron bilayers is equally applicable to 2D hole bilayers. The idea of pursuing PSDW is, in general, relevant across various 2D bilayer systems, not limited to the parabolic model that we investigate in this paper, and provides a new possibility of exploring novel coherent phases.

cond-mat.mes-hall

Interaction and coherence in 2D bilayers

In bilayer systems, the additional layer pseudospin enables the emergence of interlayer coherence (IC), which is a direct consequence of the interlayer Coulomb interaction. This study presents a comprehensive HF investigation of IC in 2D bilayers, uncovering ground-state behaviors and temperature-dependent phase transitions that are distinct from single-layer 2DEG. This IC signals a spontaneous breaking of the U(1) symmetry in pseudospin. We explore the zero-temperature phase diagrams as a function of the electron density and interlayer separation within the HF formalism. We also calculate the critical temperature ($T_c$) of the interlayer coherence onset by self-consistently solving the HF gap-like equation. We contrast this IC phase in e-e bilayers with the closely related excitonic superfluid phase in e-h bilayers. Though both e-e and e-h bilayers spontaneously break the pseudospin U(1) symmetry, e-h bilayers produce BCS-BEC crossover intrinsic to the excitons acting as effective bosons or Cooper pairs, whereas the symmetry-broken phase in e-e bilayers is akin to the XY or easy-plane pseudospin ferromagnetism. Using the same system parameters and a similar theoretical framework, we find that $T_c$ of the interlayer coherent phase in e-e bilayers is about one-third of that in exciton condensates, suggesting a weaker IC in e-e bilayers. In addition, we examine the effect of a weak interlayer tunneling on the IC order parameter, drawing parallels with the influence of an effective in-plane magnetic field on the XY pseudospin ferromagnetism. Our findings provide a comparative theoretical framework that bridges the gap between the IC physics in e-e and e-h bilayers, contributing to a unified understanding of phase transitions in low-dimensional electron/hole systems and establishing in particular the same universality class for interlayer phase coherence in both e-e and e-h bilayers.

cond-mat.str-el

Layer Hall counterflow as a model probe of magic-angle twisted bilayer graphene

The recent constructions of flat moiré minibands in specifically twisted multilayer graphene and twisted transition metal dichalcogenides (TMDs) have facilitated the observation of strong correlations with a convenient tunability. These correlations in flat bands result in the band dispersion heavily influenced by carrier densities, leading to filling-dependent quasiparticle band renormalizations. Particularly, in magic-angle twisted bilayer graphene (MATBG), the band structure--including the quasiparticle energy and wavefunction--is crucial in understanding the correlated properties. Previous theoretical studies have demonstrated the presence of a time-reversal-even charge Hall counterflow in response to a direct current (DC) electric field in twisted bilayers as chiral structures. In this study, we show that such layer Hall counterflow can serve as a sensitive probe for MATBG model parameters, which are currently ambiguous as a result of unavoidable structural relaxation and twist-angle disorder. We present the layer Hall counterflow and the associated in-plane magnetization for three different MATBG continuum models, based on which many-body interacting models have been widely applied to study strong correlations in MATBG. At the single-particle level, our findings indicate notable differences in layer-projected Hall conductivity, both in magnitude and sign, between different MATBG continuum models. Furthermore, our self-consistent Hartree calculations, performed on each of these single-particle continuum models, reveal renormalized layer-projected Hall conductivity by the self-consistent Hartree field.

cond-mat.mes-hall

Twisted bilayer graphene reveals its flat bands under spin pumping

The salient property of the electronic band structure of twisted bilayer graphene (TBG), at the so-called magic angle (MA), is the emergence of flat bands around the charge neutrality point. These bands are associated with the observed superconducting phases and the correlated insulating states. Scanning tunneling microscopy combined with angle resolved photoemission spectroscopy are usually used to visualize the flatness of the band structure of TBG at the MA. Here, we theoretically argue that spin pumping (SP) provides a direct probe of the flat bands of TBG and an accurate determination of the MA. We consider a junction separating a ferromagnetic insulator and a heterostructure of TBG adjacent to a monolayer of a transition metal dichalcogenide. We show that the Gilbert damping of the ferromagnetic resonance experiment, through this junction, depends on the twist angle of TBG, and exhibits a sharp drop at the MA. We discuss the experimental realization of our results which open the way to a twist switchable spintronics in twisted van der Waals heterostructures.

cond-mat.mes-hall

Observation of the anomalous Hall effect in a layered polar semiconductor

Progress in magnetoelectric materials is hindered by apparently contradictory requirements for time-reversal symmetry broken and polar ferroelectric electronic structure in common ferromagnets and antiferromagnets. Alternative routes could be provided by recent discoveries of a time-reversal symmetry breaking anomalous Hall effect in noncollinear magnets and altermagnets, but hitherto reported bulk materials are not polar. Here, we report the observation of a spontaneous anomalous Hall effect in doped AgCrSe$_2$, a layered polar semiconductor with an antiferromagnetic coupling between Cr spins in adjacent layers. The anomalous Hall resistivity 3 $μΩ$ cm is comparable to the largest observed in compensated magnetic systems to date, and is rapidly switched off when the angle of an applied magnetic field is rotated to $\sim 80^{\circ}$ from the crystalline $c$-axis. Our ionic gating experiments show that the anomalous Hall conductivity magnitude can be enhanced by modulating the $p$-type carrier density. We also present theoretical results that suggest the anomalous Hall effect is driven by Berry curvature due to noncollinear antiferromagnetic correlations among Cr spins, which are consistent with the previously suggested magnetic ordering in AgCrSe$_2$. Our results open the possibility to study the interplay of magnetic and ferroelectric-like responses in this fascinating class of materials.

cond-mat.mtrl-sci

Spontaneous time-reversal symmetry breaking in twisted double bilayer graphene

Twisted double bilayer graphene (tDBG) comprises two Bernal-stacked bilayer graphene sheets with a twist between them. Gate voltages applied to top and back gates of a tDBG device tune both the flatness and topology of the electronic bands, enabling an unusual level of experimental control. Broken spin/valley symmetry metallic states have been observed in tDBG devices with twist angles $\sim $ 1.2-1.3$^\circ$, but the topologies and order parameters of these states have remained unclear. We report the observation of an anomalous Hall effect in the correlated metal state of tDBG, with hysteresis loops spanning 100s of mT in out-of-plane magnetic field ($B_{\perp}$) that demonstrate spontaneously broken time-reversal symmetry. The $B_{\perp}$ hysteresis persists for in-plane fields up to several Tesla, suggesting valley (orbital) ferromagnetism. At the same time, the resistivity is strongly affected by even mT-scale values of in-plane magnetic field, pointing to spin-valley coupling or to a direct orbital coupling between in-plane field and the valley degree of freedom.

cond-mat.mes-hall

Bulk and Edge Properties of Twisted Double-Bilayer Graphene

The emergence of controlled, two-dimensional moiré materials has uncovered a new platform for investigating topological physics. Twisted double bilayer graphene (TDBG) has been predicted to host a topologically non-trivial gapped phase with Chern number equal to two at charge neutrality, when half the flat bands are filled. However, it can be difficult to diagnose topological states using a single measurement because it is ideal to probe the bulk and edge properties at the same time. Here, we report a combination of chemical potential measurements, transport measurements, and theoretical calculations that show that twisted double bilayer graphene can host metallic edge transport while simultaneously being insulating in the bulk. A Landauer-Buttiker analysis of measurements on multi-terminal samples allows us to quantitatively assess edge state scattering. We interpret these results as signatures of the predicted topological phase at charge neutrality.

cond-mat.mes-hall