arXiv subjects

Jihong Ma

Publications and source records attributed to Jihong Ma.

8 recordsLinked to original sources

arXiv2026

Tracking thermal transport in colloidal quantum dot films using in-situ time-resolved X-ray diffraction

Colloidal quantum dots (QDs) and their thin-films are increasingly used in electronic and photonic devices replacing traditional bulk semiconductors. However, thermal properties of the QDs are comparatively underexplored relative to device development efforts. This study shows the use of time-resolved X-ray diffraction as a contact-free method to probe the thermal response of QDs in device-like environments, providing in-situ insights for future thermal management strategies. Through the extraction of Debye-Waller Factors on a sub-nanosecond timescale, we use time-resolved X-ray diffraction to directly capture the heating and cooling of core/shell CdSe/CdS QDs following pulsed optical excitation. In a QD thin-film that actively provides optical gain, the thermal conductivity is found to be as low as 0.55 $\mathrm{W\,m^{-1}\,K^{-1}}$, because of the poor heat flow within close-packed QD solids. For QDs dispersed in liquids, interfacial thermal conductance is found to dominate the thermal relaxation with a conductance on the order of 15 $\mathrm{MW\,m^{-2}\,K^{-1}}$.

cond-mat.mes-hall↗

arXiv2024

Ultrafast symmetry control in photoexcited quantum dots

Symmetry control is essential for realizing unconventional properties, such as ferroelectricity, nonlinear optical responses, and complex topological order, thus it holds promise for the design of emerging quantum and photonic systems. Nevertheless, fast and reversible control of symmetry in materials remains a challenge, especially for nanoscale systems. Here, we unveil reversible symmetry changes in colloidal lead chalcogenide quantum dots on picosecond timescales. Using a combination of ultrafast electron diffraction and total X-ray scattering, in conjunction with atomic-scale structural modeling and first-principles calculations, we reveal that symmetry-broken lead sulfide quantum dots restore to a centrosymmetric phase upon photoexcitation. The symmetry restoration is driven by photoexcited electronic carriers, which suppress lead off-centering for about 100 ps. Furthermore, the change in symmetry is closely correlated with the electronic properties as shown by transient optical measurements. Overall, this study elucidates reversible symmetry changes in colloidal quantum dots, and more broadly defines a new methodology to optically control symmetry in nanoscale systems on ultrafast timescales.

cond-mat.mes-hall↗

arXiv2023

Breakdown of Conventional Winding Number Calculation in One-Dimensional Lattices with Interactions Beyond Nearest Neighbors

Topological insulators hold promises to realize exotic quantum phenomena in electronic, photonic, and phononic systems. Conventionally, topological indices, such as winding numbers, have been used to predict the number of topologically protected domain-wall states (TPDWSs) in topological insulators, a signature of the topological phenomenon called bulk-edge correspondence. Here, we demonstrate theoretically and experimentally that the number of TPDWSs in a mechanical Su-Schrieffer-Heeger (SSH) model can be higher than the winding number depending on the strengths of beyond-nearest-neighbor interactions, revealing the breakdown of the winding number prediction. Alternatively, we resort to the Berry connection to accurately characterize the number and spatial features of TPDWSs in SSH systems, further confirmed by the Jackiw-Rebbi theory proving that the multiple TPDWSs correspond to the bulk Dirac cones. Our findings deepen the understanding of complex network dynamics and offer a generalized paradigm for precise TPDWS prediction in potential applications involving localized vibrations, such as drug delivery and quantum computing.

cond-mat.mtrl-sci↗

arXiv2021

Symmetry Effect on the Dynamic Behaviors of Sandwich Beams with Periodic Face Sheets

We investigate theoretically and demonstrate experimentally, the effect of material and geometric periodicity in face sheets on the overall dynamics of sandwich beams. By treating the two face sheets and core as separate entities using the classic sandwich plate theory (CPT), in conjunction with Bloch theorem, and solving the governing equations with the transfer matrix method (TMM) and the generalized differential quadrature method (GDQM), we obtain a low-frequency \textit{total} bandgap in which both transverse and longitudinal waves are blocked in sandwich beams with glide-reflected (GR) face sheets. On the other hand, only \textit{partial} bandgaps blocking either transverse or longitudinal waves are present in the ones with mirror-reflected (MR) face sheets. Furthermore, a combination of full-scale finite element method (FEM) simulations and experimental characterization provide unequivocal evidence of these phenomenal wave features, as well as the accuracy of our theoretical results via defining separate displacement fields in comparison with effective periodic Timoshenko beam models. Our study indicates new mechanisms to suppress low-frequency elastic waves by tuning face sheet symmetry. Our explanation of wave behaviors from a structural symmetry point of view also provides a more comprehensive understanding of the symmetry effect on wave propagation in quasi-one-dimensional structures at large.

physics.app-ph↗

arXiv2021

Spatial correlations of entangled polymer dynamics

The spatial correlations of entangled polymer dynamics are examined by molecular dynamics simulations and neutron spin-echo spectroscopy. Due to the soft nature of topological constraints, the initial spatial decays of intermediate scattering functions of entangled chains are, to the first approximation, surprisingly similar to those of an unentangled system in the functional forms. However, entanglements reveal themselves as a long tail in the reciprocal-space correlations, implying a weak but persistent dynamic localization in real space. Comparison with a number of existing theoretical models of entangled polymers suggests that they cannot fully describe the spatial correlations revealed by simulations and experiments. In particular, the strict one-dimensional diffusion idea of the original tube model is shown to be flawed. The dynamic spatial correlation analysis demonstrated in this work provides a useful tool for interrogating the dynamics of entangled polymers. Lastly, the failure of the investigated models to even qualitatively predict the spatial correlations of collective single-chain density fluctuations points to a possible critical role of incompressibility in polymer melt dynamics.

cond-mat.soft↗

arXiv2019

Valley-Hall In-Plane Edge States as Building Blocks for Elastodynamic Logic Circuits

In this work, we investigate theoretically and demonstrate experimentally the existence of valley-Hall edge states in the in-plane dynamics of honeycomb lattices with bi-valued strut thickness. We exploit these states to achieve non-trivial waveguiding of optical modes that is immune to backscattering from sharp corners. We also present how different types of interfaces can be combined into multi-branch junctions to form complex waveguide paths and realize a variety of structural logic designs with unconventional wave transport capabilities. We illustrate this potential with two applications. The first is a direction-selective energy-splitting waveguide tree featuring a pronounced asymmetric wave transport behavior. The second is an internal waveguide loop along which the energy can be temporarily trapped and periodically released, effectively working as a signal delayer. The modal complexity of in-plane elasticity has important consequences on the regime of manifestation of the edge states, as the availability of viable total bandgaps is shifted to higher frequencies compared to the out-of-plane counterpart problem. It also poses additional experimental challenges, associated with proper acquisition and deciphering of the in-plane modes, the solution of which requires a systematic use of in-plane laser vibrometry.

physics.app-ph↗

arXiv2019

Switchable phonon diodes using nonlinear topological Maxwell lattices

Recent progress in topological mechanics have revealed a family of Maxwell lattices that exhibit topologically protected floppy edge modes. These modes lead to a strongly asymmetric elastic wave response. In this paper, we show how topological Maxwell lattices can be used to realize non-reciprocal transmission of elastic waves. Our design leverages the asymmetry associated with the availability of topological floppy edge modes and the geometric nonlinearity built in the mechanical systems response to achieve the desired non-reciprocal behavior, which can be further turned into strongly one-way phonon transport via the addition of on-site pinning potentials. Moreover, we show that the non-reciprocal wave transmission can be switched on and off via topological phase transitions, paving the way to the design of cellular metamaterials that can serve as tunable topologically protected phonon diodes.

cond-mat.soft↗

arXiv2018

Edge Modes and Asymmetric Wave Transport in Topological Lattices: Experimental Characterization at Finite Frequencies

Although topological mechanical metamaterials have been extensively studied from a theoretical perspective, their experimental characterization has been lagging. To address this shortcoming, we present a systematic laser-assisted experimental characterization of topological kagome lattices, aimed at elucidating their in-plane phononic and topological characteristics. We specifically explore the continuum elasticity limit, which is established when the ideal hinges that appear in the theoretical models are replaced by ligaments capable of supporting bending deformation, as observed for instance in realistic physical lattices. We reveal how the zero-energy floppy edge modes predicted for ideal configurations morph into finite-frequency phonon modes that localize at the edges. By probing the lattices with carefully designed excitation signals, we are able to extract and characterize all the features of a complex low-frequency acoustic regime in which bulk modes and topological edge modes overlap and entangle in response. The experiments provide unequivocal evidence of the existence of strong asymmetric wave transport regimes at finite frequencies.

cond-mat.mtrl-sci↗