arXiv subjects

Jihua Zhang

Publications and source records attributed to Jihua Zhang.

At least 19 recordsLinked to original sources

arXiv2025

Enhanced Tunable Photon Pair Generation from Nonlinear Metasurface with Guided-Mode Cavity

The ability to generate quantum entangled photon pairs through spontaneous parametric down conversion (SPDC) is playing a pivotal role in many applications in quantum technologies, including quantum communications, quantum computation, and quantum imaging. Metasurfaces, two-dimensional arrays of nanostructures with subwavelength thickness, have recently shown extraordinary capability in manipulating classical and quantum states of light and realizing miniaturized SPDC sources. Whereas previous studies have primarily focused on periodic metasurfaces, we uncover the potential of spatially modulated nanopatterns for further SPDC enhancement and state engineering. Specifically, we propose a nonlinear metasurface featuring a lateral guided-mode cavity formed by two distributed Bragg reflectors. With the quasi-normal mode theory, we predict an SPDC rate up to 157 Hz/mW, which represents about 30 times rate enhancement when compared to the metasurface without a cavity. Furthermore, the cavity supports a continuous set of high-Q resonances across a broad bandwidth, allowing the all-optical tuning of the photon-pair emission directions transverse to the cavity by controlling the pump wavelength, which can find applications in quantum imaging.

physics.optics↗

arXiv2025

Broadband bright biphotons from periodically poled triple-resonance metasurface

Biphotons from spontaneous parametric down conversion with broad bandwidth are highly wanted in many quantum technologies. However, achieving broad bandwidth in both frequency and momentum while keeping a high rate remains a challenge for both conventional nonlinear crystals and recently emerging nonlinear metasurfaces. Here, we address this challenge by introducing a periodically poled triple-resonance metasurface (PPTM) incorporating a nano-grating atop a periodically poled LiNbO$_3$ thin film. PPTM supports high-Q guided mode resonances at pump, signal, and idler wavelengths meanwhile enabling quasi-phase matching between three guided modes in a broad frequency/momentum range. The predicted biphoton rate is over 100 MHz/mW with a frequency bandwidth of 165 nm around 1550 nm and a momentum bandwidth of $13^\circ \times 6^\circ$, improving the state-of-the-art by over three orders of magnitude in rate and one order of magnitude in bandwidths. This ultrathin broadband bright biphoton source could stimulate system-level miniaturization of various free-space quantum photonic technologies.

physics.optics↗

arXiv2024

Angle multifunctional dichroism in metasurfaces

We demonstrate metasurfaces with strong polarization dichroism that depends on the angle of incidence. We present original designs obtained through topology optimization that selectively transmit specific linear or circular polarizations at different incident angles, while the orthogonal polarization transmission is suppressed. The designed metasurfaces exceed 95% transmission efficiency and 50x extinction ratio within the target angle ranges. The experimental characterization of fabricated metasurfaces confirms the desired operation with 90% transmission efficiency and 10x extinction ratio. These results provide important insights to non-local and k-space engineering of metasurface response and results reveal new opportunities for future multi-functional and angle-selective polarization devices that can find applications in specialized optical instruments and end-user devices.

physics.optics↗

arXiv2024

Generation of tunable quantum entanglement via nonlinearity symmetry breaking in semiconductor metasurfaces

Tunable biphoton quantum entanglement generated from nonlinear processes is highly desirable for cutting-edge quantum technologies, yet its tunability is substantially constrained by the symmetry of material nonlinear tensors. Here, we overcome this constraint by introducing symmetry-breaking in nonlinear polarization to generate optically tunable biphoton entanglement at picosecond speeds. Asymmetric optical responses have made breakthroughs in classical applications like non-reciprocal light transmission. We now experimentally demonstrate the nonlinear asymmetry response for biphoton entanglement using a semiconductor metasurface incorporating [110] InGaP nano-resonators with structural asymmetry. We realize continuous tuning of polarization entanglement from near-unentangled states to a Bell state. This tunability can also extend to produce tailored hyperentanglement. Furthermore, our nanoscale entanglement source features an ultra-high coincidence-to-accidental ratio of $\approx7\times10^4$, outperforming existing semiconductor flat optics by two orders of magnitude. Introducing asymmetric nonlinear response in quantum metasurfaces opens new directions for tailoring on-demand quantum states and beyond.

physics.optics↗

arXiv2024

Quantum Imaging Using Spatially Entangled Photon Pairs from a Nonlinear Metasurface

Nonlinear metasurfaces with subwavelength thickness were recently established as versatile platforms for the enhanced and tailorable generation of entangled photon pairs. The small dimensions and inherent stability of integrated metasurface sources are attractive for free-space applications in quantum communications, sensing, and imaging, yet this remarkable potential remained unexplored. Here, we formulate and experimentally demonstrate the unique benefits and practical potential of nonlinear metasurfaces for quantum imaging at infrared wavelengths, facilitating an efficient protocol combining ghost and all-optical scanning imaging. The metasurface incorporates a subwavelength-scale silica metagrating on a lithium niobate thin film. Its distinguishing feature is the capability to all-optically scan the photon emission angle in the direction across the grating simply by tuning the pump beam wavelength. Simultaneously, the photon emission is broad and anti-correlated along the grating direction, allowing for ghost imaging. Thereby, we reconstruct the images of 2D objects using just a 1D detector array in the idler path and a bucket detector in the signal path, by recording the dependencies of photon coincidences on the pump wavelength. Our results reveal new possibilities for quantum imaging with ultra-large field of view and improved imaging resolution as compared to photon pairs from conventional bulky crystals. The demonstrated concept can be extended to multi-wavelength operation and other applications such as quantum object tracking, paving the way for advancements in quantum technologies using ultra-compact nanostructured metasurfaces.

physics.optics↗

arXiv2024

Enhanced infrared vision by nonlinear up-conversion in nonlocal metasurfaces

The ability to detect and image short-wave infrared light has important applications in surveillance, autonomous navigation, and biological imaging. However, the current infrared imaging technologies often pose challenges due to their large footprints, large thermal noise, and the inability to augment infrared and visible imaging. Here, we demonstrate infrared imaging by nonlinear up conversion to the visible on an ultra-compact, high-quality lithium niobate resonant metasurface. Images with high conversion efficiency and resolution quality are obtained despite the strong nonlocality of the metasurface. We further show the possibility of edge-detection image processing augmented with direct-up conversion imaging for advanced night vision applications.

physics.optics↗

arXiv2024

Single-shot characterization of photon indistinguishability with dielectric metasurfaces

Characterizing the indistinguishability of photons is a key task in quantum photonics, underpinning the tuning and stabilization of the photon sources and thereby increasing the accuracy of quantum operations. The protocols for measuring the degree of indistinguishability conventionally require photon-coincidence measurements at several different time or phase delays, which is a fundamental bottleneck towards the fast measurements and real-time monitoring of indistinguishability. Here, we develop a static dielectric metasurface grating without any reconfigurable elements that realizes a tailored multiport transformation in the free-space configuration without the need for phase locking and enables single-shot characterization of the indistinguishability between two photons in multiple degrees of freedom including time, spectrum, spatial modes, and polarization. Topology optimization is employed to design a silicon metasurface with polarization independence, high transmission, and high tolerance to measurement noise. We fabricate the metasurface and experimentally quantify the indistinguishability of photons in the time domain with fidelity over 98.4\%. We anticipate that the developed framework based on ultrathin metasurfaces can be further extended for multi-photon states and additional degrees of freedom associated with spatial modalities.

physics.optics↗

arXiv2024

Inverse Design of Nonlinear Metasurfaces for Sum Frequency Generation

Sum frequency generation (SFG) has multiple applications, from optical sources to imaging, where efficient conversion requires either long interaction distances or large field concentrations in a quadratic nonlinear material. Metasurfaces provide an essential avenue to enhanced SFG due to resonance with extreme field enhancements with an integrated ultrathin platform. In this work, we formulate a general theoretical framework for multi-objective topology optimization of nanopatterned metasurfaces that facilitate high-efficiency SFG and simultaneously select the emitted direction and tailor the metasurface polarization response. Based on this framework, we present novel metasurface designs showcasing ultimate flexibility in transforming the outgoing nonlinearly generated light for applications spanning from imaging to polarimetry. For example, one of our metasurfaces produces highly polarized and directional SFG emission with an efficiency of over 0.2 cm^2/GW in a 10 nm signal operating bandwidth.

physics.optics↗

arXiv2024

Quantum metaphotonics: recent advances and perspective

Quantum metaphotonics has emerged as a cutting-edge subfield of meta-optics employing subwavelength resonators and their planar structures such as metasurfaces to generate, manipulate, and detect quantum states of light. It holds a great potential for the miniaturization of current bulky quantum optical elements by developing a design of on-chip quantum systems for various applications of quantum technologies. Over the past few years, this field has witnessed a surge of intriguing theoretical ideas, groundbreaking experiments, and novel application proposals. This perspective paper aims to summarize the most recent advancements and also provide a perspective on the further progress in this rapidly developing field of research.

physics.optics↗

arXiv2024

Directionally Tunable Co- and Counter-Propagating Photon Pairs from a Nonlinear Metasurface

Nonlinear metasurfaces have recently been established as a new platform for generating photon pairs via spontaneous parametric down-conversion. While for classical harmonic generation in metasurfaces a high level of control over all degrees of freedom of light has been reached, this capability is yet to be developed for photon pair generation. In this work, we theoretically and experimentally demonstrate for the first time precise control of the emission angle of photon pairs generated from a nonlinear metasurface. Our measurements show angularly tunable pair-generation with high coincidence-to-accidental ratio for both co- and counter-propagating emission. The underlying principle is the transverse phase-matching of guided-mode resonances with strong angular dispersion in a nonlinear lithium niobate metagrating. We provide a straightforward design strategy for photon pair generation in such a device and find very good agreement between the calculations and experimental results. Here we use all-optical emission angle tuning by means of the pump wavelength, however the principle could be extended to modulation via the electro-optic effect in lithium niobate. In sum, this work provides an important addition to the toolset of sub-wavelength thickness photon pair sources.

physics.optics↗

arXiv2024

Engineering Quantum Light Sources with Flat Optics

Quantum light sources are essential building blocks for many quantum technologies, enabling secure communication, powerful computing, precise sensing and imaging. Recent advancements have witnessed a significant shift towards the utilization of ``flat" optics with thickness at subwavelength scales for the development of quantum light sources. This approach offers notable advantages over conventional bulky counterparts, including compactness, scalability, and improved efficiency, along with added functionalities. This review focuses on the recent advances in leveraging flat optics to generate quantum light sources. Specifically, we explore the generation of entangled photon pairs through spontaneous parametric down-conversion in nonlinear metasurfaces, as well as single photon emission from quantum emitters including quantum dots and color centers in 3D and 2D materials. The review covers theoretical principles, fabrication techniques, and properties of these sources, with particular emphasis on the enhanced generation and engineering of quantum light sources using optical resonances supported by nanostructures. We discuss the diverse application range of these sources and highlight the current challenges and perspectives in the field.

physics.optics↗

arXiv2023

Photon pair generation from lithium niobate metasurface with tunable spatial entanglement

Two-photon state with spatial entanglement is an essential resource for testing fundamental laws of quantum mechanics and various quantum applications. Its creation typically relies on spontaneous parametric down-conversion in bulky nonlinear crystals where the tunability of spatial entanglement is limited. Here, we predict that ultrathin nonlinear lithium niobate metasurfaces can generate and diversely tune spatially entangled photon pairs. The spatial properties of photons including the emission pattern, rate, and degree of spatial entanglement are analysed theoretically with the coupled mode theory and Schmidt decomposition method. We show that by leveraging the strong angular dispersion of the metasurface, the degree of spatial entanglement quantified by the Schmidt number can be decreased or increased by changing the pump laser wavelength and a Gaussian beam size. This flexibility can facilitate diverse quantum applications of entangled photon states generated from nonlinear metasurfaces.

physics.optics↗

arXiv2023

Polarization engineering of entangled photons from a lithium niobate nonlinear metasurface

Complex polarization states of photon pairs are indispensable in various quantum technologies. Conventional methods for preparing desired two-photon polarization states are realized through bulky nonlinear crystals, which can restrict the versatility and tunability of the generated quantum states due to the fixed crystal nonlinear susceptibility. Here we present a solution using a nonlinear metasurface incorporating multiplexed silica metagratings on a lithium niobate film of 300 nanometer thickness. We fabricate two orthogonal metagratings on a single substrate with an identical resonant wavelength, thereby enabling the spectral indistinguishability of the emitted photons, and demonstrate in experiments that the two-photon polarization states can be shaped by the metagrating orientation. Leveraging this essential property, we formulate a theoretical approach for generating arbitrary polarization-entangled qutrit states by combining three metagratings on a single metasurface, allowing the encoding of desired quantum states or information. Our findings enable miniaturized optically controlled quantum devices using ultrathin metasurfaces as polarization-entangled photon sources.

physics.optics↗

arXiv2023

Full conversion of unpolarized to fixed-polarization light with topology optimized metasurfaces

Conventional polarizers and polarization beam splitters have a fundamental limit of 50\% efficiency when converting unpolarized light into one specific polarization. Here, we overcome this restriction and achieve near-complete conversion of unpolarized light to a single pure polarization state at several outputs of topology-optimized metasurfaces. Our fabricated metasurface achieves an extinction ratio approaching 100, when characterized with laboratory measurements. We further demonstrate that arbitrary power splitting can be achieved between three or more polarized outputs, offering flexibility in target illumination. Our results provide a path toward greatly improving the efficiency of common unpolarized light sources in a variety of applications requiring pure polarizations.

physics.optics↗

arXiv2022

Complex structure and characterization of multi-photon split states in integrated circuits

Multi-photon split states, where each photon is in a different spatial mode, represent an essential resource for various quantum applications, yet their efficient characterization remains an open problem. Here, we formulate the general structure of their reduced spatial density matrices and identify the number of real and complex-valued independent coefficients, which in particular completely determine the distinguishability of all photons. Then, we show that this density matrix can be fully characterized by measuring correlations after photon interference in a static integrated circuit, where the required outputs scale sub-quadratically versus the number of photons. We present optimized circuit designs composed of segmented coupled waveguides, representing a linear optical neural network, which minimize the reconstruction error and facilitate robustness to fabrication deviations.

quant-ph↗

arXiv2022

Spatially entangled photon-pairs from lithium niobate nonlocal metasurfaces

Metasurfaces consisting of nano-scale structures are underpinning new physical principles for the creation and shaping of quantum states of light. Multi-photon states that are entangled in spatial or angular domains are an essential resource for quantum imaging and sensing applications, however their production traditionally relies on bulky nonlinear crystals. We predict and demonstrate experimentally the generation of spatially entangled photon pairs through spontaneous parametric down-conversion from a metasurface incorporating a nonlinear thin film of lithium niobate. This is achieved through nonlocal resonances with tailored angular dispersion mediated by an integrated silica meta-grating, enabling control of the emission pattern and associated quantum states of photon pairs by designing the grating profile and tuning the pump frequency. We measure the correlations of photon positions and identify their spatial anti-bunching through violation of the classical Cauchy-Schwartz inequality, witnessing the presence of multi-mode entanglement. Simultaneously, the photon-pair rate is strongly enhanced by 450 times as compared to unpatterned films due to high-quality-factor metasurface resonances, and the coincidence to accidental ratio reaches 5000. These results pave the way to miniaturization of various quantum devices by incorporating ultra-thin metasurfaces functioning as room-temperature sources of quantum-entangled photons.

physics.optics↗

arXiv2020

Complex-birefringent dielectric metasurfaces for arbitrary polarization-pair transformations

Birefringent materials or nanostructures that introduce phase differences between two linear polarizations underpin the operation of wave plates for polarization control of light. Here we develop metasurfaces realizing a distinct class of complex-birefringent wave plates, which combine polarization transformation with a judiciously tailored polarization-dependent phase retardance and amplitude filtering via diffraction. We prove that the presence of loss enables the mapping from any chosen generally non-orthogonal pair of polarizations to any other pair at the output. We establish an optimal theoretical design-framework based on pairwise nanoresonator structures and experimentally demonstrate unique properties of metasurfaces in the amplification of small polarization differences and polarization coupling with unconventional phase control. Furthermore, we reveal that these metasurfaces can perform arbitrary transformations of biphoton polarization-encoded quantum states, including the modification of the degree of entanglement. Thereby, such flat devices can facilitate novel types of multi-functional polarization optics for classical and quantum applications.

physics.optics↗

arXiv2019

Generalized Brewster-angle effect in thin-film optical absorbers and its application for graphene hydrogen sensing

Generalized Brewster angle (GBA) is the incidence angle at which polarization by reflection for p- and s-polarized light takes place. Realizing s-polarization Brewster effect requires a material with magnetic response which is challenging at optical frequencies since the magnetic response of materials at these frequencies is extremely weak. Here, we experimentally realize GBA effect in the visible using a thin-film absorber system consisting of a dielectric film on an absorbing substrate. Polarization by reflection is realized for both p- and s- polarized light at different angles of incidence and multiple wavelengths. We provide a theoretical framework for the generalized Brewster effect in thin-film light absorbers. We demonstrate hydrogen gas sensing using a single layer graphene film transferred on a thin-film absorber at the GBA with ~1 fg/mm2 aerial mass sensitivity. The ultrahigh sensitivity stems from the strong phase sensitivity near point of darkness, particularly at the GBA, and the strong light-matter interaction in planar nanocavities. These findings depart from the traditional domain of thin-films as mere interference optical coatings and highlight its many potential applications including gas sensing and biosensing.

physics.optics↗