arXiv subjects

Jingang Li

Publications and source records attributed to Jingang Li.

3 recordsLinked to original sources

arXiv2025

Moire-enabled optical vortex with tunable topological charge in twisted bilayer photonic crystals

The orbital angular momentum (OAM) of light is a versatile degree of freedom with transformative impact across optical communication, imaging, and micromanipulation. These applications have motivated a growing demand for compact, reconfigurable vortex arrays with tunable topological charge, yet integrating these functionalities into nanophotonic platforms remains elusive. Among possible strategies to meet this challenge is exploiting the twist degree of freedom in layered structures, which enables both emerging moire physics and unprecedented reconfigurability of photonic and electronic properties. Here, we harness these capabilities in twisted bilayer moire photonic crystals (TBMPCs) to realize vortex array generation with tunable OAM, demonstrated both analytically and experimentally. Central to this advancement is a new class of quasi-bound state in the continuum: Bessel-type modes emerging from moire-induced interlayer coupling, which generate vortex beams with tailored spiral phase distributions. We experimentally demonstrate vortex beams spanning eight OAM orders, from -3 to 4, and achieve selective excitation of distinct topological charges at a fixed telecommunication wavelength by tuning the interlayer separation and twist angle. Furthermore, localized Bessel-type modes at AA stacking regions can be excited nonlocally across the moire superlattice, enabling vortex array generation. Our work offers new insights into moire physics and introduces an innovative approach for future multiplexing technology integrating OAM, wavelength, and spatial division.

physics.optics↗

arXiv2022

Ultrafast optical nanoscopy of carrier dynamics in silicon nanowires

Carrier distribution and dynamics in semiconductor materials often govern their physical properties that are critical to functionalities and performance in industrial applications. The continued miniaturization of electronic and photonic devices calls for tools to probe carrier behavior in semiconductors simultaneously at the picosecond time and nanometer length scales. Here, we report pump-probe optical nanoscopy in the visible-near-infrared spectral region to characterize the carrier dynamics in silicon nanostructures. By coupling experiments with the point-dipole model, we resolve the size-dependent photoexcited carrier lifetime in individual silicon nanowires. We further demonstrate local carrier decay time mapping in silicon nanostructures with a sub-50 nm spatial resolution. Our study enables the nanoimaging of ultrafast carrier kinetics, which will find promising applications in the future design of a broad range of electronic, photonic, and optoelectronic devices.

cond-mat.mtrl-sci↗

arXiv2022

Light-driven C-H bond activation mediated by 2D transition metal dichalcogenides

C-H bond activation enables the facile synthesis of new chemicals. While C-H activation in short-chain alkanes has been widely investigated, it remains largely unexplored for long-chain organic molecules. Here, we report light-driven C-H activation in complex organic materials mediated by 2D transition metal dichalcogenides (TMDCs) and the resultant solid-state synthesis of luminescent carbon dots in a spatially-resolved fashion. We unravel the efficient H adsorption and a lowered energy barrier of C-C coupling mediated by 2D TMDCs to promote C-H activation. Our results shed light on 2D materials for C-H activation in organic compounds for applications in organic chemistry, environmental remediation, and photonic materials.

cond-mat.mtrl-sci↗