arXiv subjects

Jinkyung Kim

Publications and source records attributed to Jinkyung Kim.

6 recordsLinked to original sources

arXiv2022

An electron-spin qubit platform assembled atom-by-atom on a surface

Creating a quantum-coherent architecture at the atomic scale has long been an ambition in quantum science and nanotechnology. This ultimate length scale requires the use of fundamental quantum properties of atoms, such as the spin of electrons, which naturally occurs in many solid-state environments and allows high-fidelity operations and readout by electromagnetic means. Despite decades of effort, however, it remains a formidable task to realize an atomic-scale quantum architecture where multiple electron spin qubits can be precisely assembled, controllably coupled, and coherently operated. Electron spin qubits created in dopants in semiconductors and color centers in insulators, for example, can be well controlled individually6-8 but are difficult to couple together into a circuit. On the other hand, multiple magnetic atoms and molecules on surfaces can be coupled to each other by building sophisticated atomic structures using a scanning tunneling microscope (STM), but coherent operation has so far been limited to a single qubit in the tunnel junction. Here we demonstrate an atomic-scale qubit platform by showing atom-by-atom construction, coherent operations, and readout of multiple electron-spin qubits on a surface. To enable the coherent control of remote qubits that are outside the tunnel junction, we complement each electron spin with a local magnetic field gradient from a nearby single-atom magnet. To enable readout of remote qubits, we employ a sensor qubit in the tunnel junction and implement pulsed double electron spin resonance. Using these methods, we demonstrate fast single-, two-, and three-qubit operations in an all-electrical fashion. Our work marks the creation of an Angstrom-scale qubit platform, where quantum functionalities using electron spin arrays, built atom-by-atom on a surface, are now within reach.

cond-mat.mes-hall↗

arXiv2022

Anisotropic hyperfine interaction of surface-adsorbed single atoms

Hyperfine interactions between electron and nuclear spins have been widely used in material science, organic chemistry, and structural biology as a sensitive probe to the local chemical environment through spatial identification of nuclear spins. With the nuclear spins identified, the isotropic and anisotropic components of the hyperfine interactions in turn offer unique insight into the electronic ground-state properties of the paramagnetic centers. However, traditional ensemble measurements of hyperfine interactions average over a macroscopic number of spins with different geometrical locations and nuclear isotopes. Here, we use a scanning tunneling microscope (STM) combined with electron spin resonance (ESR) to measure hyperfine spectra of hydrogenated-titanium (Ti) atoms on MgO/Ag(100) and thereby determine the isotropic and anisotropic hyperfine interactions at the single-atom level. By combining vector-field ESR spectroscopy with STM-based atom manipulation, we characterize the full hyperfine tensor of individual Ti-47 and Ti-49 atoms and identify significant spatial anisotropy of hyperfine interaction for both isotopes when they are adsorbed at low-symmetry binding sites. Density functional theory calculations reveal that the large hyperfine anisotropy arises from a highly anisotropic distribution of the ground-state electron spin density. Our work highlights the power of ESR-STM-enabled single-atom hyperfine spectroscopy as a powerful tool in revealing ground-state electronic structures and atomic-scale chemical environments with nano-electronvolt resolution.

cond-mat.mes-hall↗

arXiv2022

Sequential Movie Genre Prediction using Average Transition Probability with Clustering

In recent movie recommendations, predicting the user's sequential behavior and suggesting the next movie to watch is one of the most important issues. However, capturing such sequential behavior is not easy because each user's short-term or long-term behavior must be taken into account. For this reason, many research results show that the performance of recommending a specific movie is not very high in a sequential recommendation. In this paper, we propose a cluster-based method for classifying users with similar movie purchase patterns and a movie genre prediction algorithm rather than the movie itself considering their short-term and long-term behaviors. The movie genre prediction does not recommend a specific movie, but it predicts the genre for the next movie to watch in consideration of each user's preference for the movie genre based on the genre included in the movie. Through this, it is possible to provide appropriate guidelines for recommending movies including the genre to users who tend to prefer a specific genre. In particular, in this paper, users with similar genre preferences are organized into clusters to recommend genres, and in clusters that do not have relatively specific tendencies, genre prediction is performed by appropriately trimming genres that are not necessary for recommendation in order to improve performance. We evaluate our method on well-known movie datasets, and qualitatively that it captures personalized dynamics and is able to make meaningful recommendations.

cs.IR↗

arXiv2021

Atomic Manipulation of In-gap States on the $β$-Bi$_2$Pd Superconductor

Electronic states in the gap of a superconductor inherit intriguing many-body properties from the superconductor. Here, we create these in-gap states by manipulating Cr atomic chains on the $β$-Bi$_2$Pd superconductor. We find that the topological properties of the in-gap states can greatly vary depending on the crafted spin chain. These systems make an ideal platform for non-trivial topological phases because of the large atom-superconductor interactions and the existence of a large Rashba coupling at the Bi-terminated surface. We study two spin chains, one with atoms two-lattice-parameter apart and one with square-root-of-two lattice parameters. Of these, only the second one is in a topologically non-trivial phase, in correspondence with the spin interactions for this geometry.

cond-mat.supr-con↗

arXiv2021

Spin Resonance Amplitude and Frequency of a Single Atom on a Surface in a Vector Magnetic Field

We used electron spin resonance (ESR) combined with scanning tunneling microscopy (STM) to measure hydrogenated Ti (spin-1/2) atoms at low-symmetry binding sites on MgO in vector magnetic fields. We found strongly anisotropic g-values in all three spatial directions. Interestingly, the amplitude and lineshape of the ESR signals are also strongly dependent on the angle of the field. We conclude that the Ti spin is aligned along the magnetic field, while the tip spin follows its strong magnetic anisotropy. Our results show the interplay between the tip and surface spins in determining the ESR signals and highlight the precision of ESR-STM to identify the single atom's spin states.

cond-mat.mes-hall↗

arXiv2013

Shedding new light on the mystery of wetting on soft solids

One of the most questionable issues in wetting is the vertical force balance that is excluded in Young's law. On soft deformable solids, such as biotic materials and synthetic polymers, the vertical force of liquid leads to a microscopic protrusion of the contact line, i.e. a "wetting ridge". The wetting principle that determines the geometry of the ridge-tip is at the heart of the issues over the past half century. Here, we reveal a universal wetting principle by directly visualizing ridge-tips with high spatio-temporal resolution using x-ray microscopy. We find that the tip-geometry is asymmetric and bent, and invariant during ridge growth or by surface softness. This singular geometry is explained by linking the macroscopic and microscopic contact angles to Young's and Neumann's laws, respectively. Our dual-scale model would be applicable to a general framework in wetting and give new clues to various issues in cell-substrate interaction and elasto-capillary problems.

cond-mat.soft↗